Design of B/N Co-doped micro/meso porous carbon electrodes from CNF/BNNS/ZIF-8 nanocomposites for advanced supercapacitors

作     者：Zhen Shang Xingye An Shuangxi Nie Na Li Haibing Cao Zhengbai Cheng Hongbin Liu Yonghao Ni Liqin Liu Zhen Shang;Xingye An;Shuangxi Nie;Na Li;Haibing Cao;Zhengbai Cheng;Hongbin Liu;Yonghao Ni;Liqin Liu

作者机构：Tianjin Key Laboratory of Pulp and PaperTianjin University of Science and TechnologyTianjin 300457China Guangxi Key Laboratory of Clean Pulp&Papermaking and Pollution ControlCollege of Light Industry and Food EngineeringGuangxi UniversityNanning 530004China Department of Chemical EngineeringUniversity of New BrunswickFredericton NB E3B 5A3Canada Institute of Nuclear and New Energy TechnologyTsinghua UniversityBeijing 100084China Zhejiang Jingxing Paper Co.Ltd.Pinghu 314214China 

出 版 物：《Journal of Bioresources and Bioproducts》 (生物质资源与工程（英文）)

年 卷 期：2023年第8卷第3期

页      面：292-305页

核心收录：

学科分类：080801[工学-电机与电器] 0808[工学-电气工程] 08[工学] 0805[工学-材料科学与工程（可授工学、理学学位）] 080502[工学-材料学] 

基　　金：support from the Natural Science Foundation of China (No.32101470) Foundation of Tianjin Key Laboratory of Pulp&Paper of Tianjin University of Science&Technology (No.202003,No.202106) China Postdoctoral Science Foundation (No.2022M712379,No.2021M692401) National Key Research and Development Plan (No.2022YFC2900031) Foundation of Guangxi Key Laboratory of Clean Pulp&Papermaking and Pollution Control,College of Light Industry and Food Engineering,Guangxi University (No.2021KF37) the support from Zhejiang Jingxing Paper Co.Ltd.,and University of New Brunswick 

主　　题：Cellulose nanofiber Zeolitic imidazolate framework Hexagonal boron nitride nanosheets B/N co-dopants Hierarchical structure Supercapacitor 

摘      要：Boron(B)and nitrogen(N)co-doped 3D hierarchical micro/meso porous carbon(BNPC)were successfully fabricated from cellulose nanofiber(CNF)/boron nitride nanosheets(BNNS)/zinc-methylimidazolate framework-8(ZIF-8)nanocomposites prepared by 2D BNNS,ZIF-8 nanoparticles,and wheat straw based ***,CNF/ZIF-8 acts as versatile skeleton and imparts partial N dopant into porous carbon structure,while the introduced BNNS can help strengthen the hierarchical porous superstructure and endow abundant B/N co-dopants within BNPC *** obtained BNPC electrode possesses a high specific surface area of 505.4 m2/g,high B/N co-doping content,and desirable *** assembled with BNPC-2(B/N co-doped porous carbon with a CNF/BNNS mass ratio of 1꞉2)electrodes exhibited exceptional electrochemical performance,demonstrating high capacitance stability even after 5000 charge-discharge *** devices exhibited outstanding energy density and power density,as well as the highest specific capacitance of 433.4 F/g at 1.0 A/g,when compared with other similar *** study proposes a facile and sustainable strategy for efficiently fabrication of rich B/N co-doped hierarchical micro/meso porous carbon electrodes from agricultural waste biomass for advanced supercapacitor performance.