Advances in photothermal conversion of carbon dioxide to solar fuels

作     者：Wa Gao Yinwen Li Dequan Xiao Ding Ma Wa Gao;Yinwen Li;Dequan Xiao;Ding Ma

作者机构：College of Bioscience and Resources EnvironmentBeijing University of AgricultureBeijing 102206China College of Chemistry and Molecular Engineering and College of EngineeringPeking UniversityBeijing 100871China Center for Integrative Materials DiscoveryDepartment of Chemistry and Chemical and Biomedical EngineeringUniversity of New HavenWest HavenCT 06516USA 

出 版 物：《Journal of Energy Chemistry》 (能源化学（英文版）)

年 卷 期：2023年第83卷第8期

页      面：62-78,I0004页

核心收录：

学科分类：083002[工学-环境工程] 0830[工学-环境科学与工程（可授工学、理学、农学学位）] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：financially supported by the Natural Science Foundation of Beijing,China (2204079) the Science and Technology General Project of Beijing Municipal Education Commission(KM202010020001) support from the endowed Jacob F. Buckman Chair fund 

主　　题：Solarenergy Photothermal catalysis CO_(2)reduction Catalyst design Performance improvement 

摘      要：Converting carbon dioxide(CO_(2)) into useful fuels or chemical feedstocks is important for achieving peak carbon emission and carbon ***,photothermal catalysis has been extensively studied and applied due to its advantages over traditional heat-driven *** this review,we focus on photothermal catalysis of thermodynamically uphill reactions that convert CO_(2)into value-added *** first introduce the fundamentals of photothermal catalysis for CO_(2)reduction,including the definition and classification of photothermal catalysis,followed by their photothermal conversion *** structure design of different types of photothermal catalysts is *** superior performance of photothermal catalytic conversion of CO_(2)is illustrated and discussed,including improved CO_(2)activation,tunable selectivity towards different solar fuel products,and resistance to sintering and ***,the perspectives and challenges in this cutting-edge field are presented with the aim of advancing understanding of the underlying mechanisms and inspiring rational design of photothermal catalysts for highly efficient solar-to-fuel conversion.