Biomimetic asymmetric catalysis
作者机构：State Key Laboratory of Organometallic ChemistryCenter for Excellence in Molecular SynthesisShanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China The Education Ministry Key Laboratory of Resource ChemistryShanghai Key Laboratory of Rare Earth Functional Materialsand Shanghai Frontiers Science Center of Biomimetic CatalysisShanghai Normal UniversityShanghai 200234China Center of Basic Molecular ScienceDepartment of ChemistryTsinghua UniversityBeijing 100084China Beijing National Laboratory for Molecular SciencesCAS Key Laboratory of Molecular Recognition and FunctionInstitute of ChemistryChinese Academy of SciencesBeijing 100190China University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of CatalysisDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China State Key Laboratory for Oxo Synthesis and Selective OxidationLanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China State Key Laboratory and Institute of Elemento-Organic ChemistryCollege of ChemistryNankai UniversityTianjin 300071China Key Laboratory of Coal to Ethylene Glycol and Its Related TechnologyState Key Laboratory of Structural ChemistryCenter for Excellence in Molecular SynthesisFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China
出 版 物：《Science China Chemistry》 (中国科学（化学英文版）)
年 卷 期：2023年第66卷第6期
页 面：1553-1633页
核心收录：
学科分类：081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）]
基 金：supported by the National Natural Science Foundation of China(22231011,22221002,22031006,21831008,22271192,92256301,92256303,91956116) the NSFC Distinguished Young Scholars(22225107) the Major Program of the Lanzhou Institute of Chemical Physics,Chinese Academy of Sciences(ZYFZFX-9)
主 题：biomimetic catalysis amine catalysis carbene catalysis vitamin Br carbonyl catalysis vitamin Bo NAD(P)H flavin biomimetic oxidation dinuclear/multinuclear metal catalysis asymmetric hydrogenation
摘 要：Enzymes are the core for biological transformations in *** structures and functions have drawn enormous attention from biologists as well as chemists since last *** large demand of bioactive molecules and the pursuit of efficiency and greenness of synthesis have spurred the rapid development of biomimetic chemistry in the past several *** asymmetric catalysis,mimicking the structures and functions of enzymes,has been recognized as one of the most promising synthetic strategies for the synthesis of valuable chiral *** review summarizes the evolution of asymmetric catalysis inspired by aldolases,vitamin B_(1)/B_(6)-dependent enzymes,NAD(P)H,flavin,hydrogenases,heme oxygenases,nonheme oxygenases,and dinuclear/multinuclear metalloenzymes in aspects of biomimetic design,catalyst development and related catalytic *** well-established synthetic approaches originating from biological reactions have demonstrated the unique prowess of biomimetic asymmetric catalysis in bridging the gap between bio-catalysis and chemical synthesis.
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