Comparative architecture in monolithic perovskite/silicon tandem solar cells

作     者：Sayantan Mazumdar Ying Zhao Xiaodan Zhang 

作者机构：Institute of Photoelectronic Thin Film Devices and TechnologyRenewable Energy Conversion and Storage CenterSolar Energy Conversion CenterNankaiUniversityTianjin 300350China Key Laboratory of Photoelectronic Thin Film Devices and Technology of TianjinTianjin 300350China Haihe Laboratory of Sustainable Chemical TransformationsTianjin 300192China Engineering Research Center of Thin Film Photoelectronic Technology of Ministry of EducationTianjin 300350China Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)Tianjin 300072China 

出 版 物：《Science China(Physics,Mechanics & Astronomy)》 (中国科学：物理学、力学、天文学（英文版）)

年 卷 期：2023年第66卷第1期

页      面：60-84页

核心收录：

学科分类：08[工学] 0805[工学-材料科学与工程（可授工学、理学学位）] 080502[工学-材料学] 0704[理学-天文学] 

基　　金：supported by the National Key Research and Development Program of China(Grant No.2018YFB1500103) the Joint Funds of the National Natural Science Foundation of China(Grant No.U21A2072) the Natural Science Foundation of Tianjin(Grant No.20JCQNJC02070) China Postdoctoral Science Foundation(Grant No.2020T130317) the Overseas Expertise Introduction Project for Discipline Innovation of Higher Education of China(Grant No.B16027) Tianjin Science and Technology Project(Grant No.18ZXJMTG00220) the Key R&D Program of Hebei Province(Grant No.19214301D) the Haihe Laboratory of Sustainable Chemical Transformations the Fundamental Research Funds for the Central Universities Nankai University 

主　　题：tandem solar cell silicon solar cell perovskite perovskite solar cell solar cell architecture polarity of tandem solar cell photoelectrochemical cells photoconduction and photovoltaic effects solar cells and arrays 

摘      要：Inorganic-organic metal halide perovskite light harvester-based perovskite solar cells(PSCs)with widely tunable bandgap have achieved rapid growth in power conversion efficiency,which exceeds 25%*** is deliberated that if a semitransparent solar cell made of wider bandgap materials was placed on top of a narrow bandgap materials-based solar cell such as a silicon solar cell,with proper optical and electrical arrangements,the resultant tandem device consisting of two subcells could more effectively utilize the solar spectrum than a single junction solar *** a perovskite/silicon tandem solar cell(PSTSC),a semitransparent PSC with a wider bandgap is placed on top of a narrow bandgap silicon solar *** PSC efficiently harvests the higher energy photons in the ultraviolet and visible regions of the solar spectrum while the silicon solar cell can convert the photons of the infrared region to *** PSTSC is proposed as a potential candidate to overcome the Shockley-Queisser limit of single-junction silicon solar *** the theoretical limit of a PSTSC is calculated as~42%,its actual efficiency achieved until now is less than 30%.Therefore,a great scope of research exists in improving the efficiency of *** issues of stability and upscaling of the device in PSCs are also a matter of concern for PSTSCs.A tandem device consists of multiple parts,and different configurations can be applied,thus tuning the architecture of the *** various parts may result in significant changes in the efficiency of the *** this review,competing architectures of otherwise comparable devices are compared in terms of photovoltaic ***,future directions to improve the efficiency of the device based on architecture design are proposed *** particular,the influence of the polarity of PSCs and the surface morphology of silicon solar cells(both front and rear)on determining the properties of the PSTSC are discussed.