Engineering membrane electrode assembly for advanced polymer electrolyte water electrolyzer

作     者：Heming Liu Xin Kang Taifeng Zhao Zhiyuan Zhang Shiyu Ge Shuqi Hu Yuting Luo Fengning Yang Shao-Hai Li Chenghua Sun Qiangmin Yu Hui-Ming Cheng Bilu Liu 刘鹤鸣;康馨;赵泰沣;张致远;葛诗玉;胡书萁;罗雨婷;杨丰宁;李少海;孙成华;余强敏;成会明;刘碧录

作者机构：Shenzhen Geim Graphene CenterTsinghua-Berkeley Shenzhen Institute&Institute of Materials ResearchShenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Department of Electrical and Computer EngineeringUniversity of Toronto35 St.George St.TorontoOntario M5S 1A4Canada Department of PhysicsUniversity of OxfordClarendon LaboratoryParks RoadOxfordOX13PUUK Department of Chemistry and Biotechnologyand Center for Translational AtomaterialsSwinburne University of TechnologyHawthornVIC 3122Australia Shenyang National Laboratory for Materials ScienceInstitute of Metal ResearchChinese Academy of SciencesShenyang 110016China Faculty of Materials Science and EngineeringInstitute of Technology for Carbon NeutralityShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China 

出 版 物：《Science China Materials》 (中国科学（材料科学（英文版）)

年 卷 期：2022年第65卷第12期

页      面：3243-3272页

核心收录：

学科分类：081702[工学-化学工艺] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：the National Natural Science Foundation of China(52188101) the National Science Fund for Distinguished Young Scholars(52125309) Guangdong Basic and Applied Basic Research Foundation(2021A1515110829) Guangdong Innovative and Entrepreneurial Research Team Program(2017ZT07C341) Shenzhen Basic Research Project(JCYJ20200109144620815) 

主　　题：water electrolysis polymer electrolyte water electrolyser membrane electrolyte assembly electrocatalyst 

摘      要：As an important energy carrier in terms of carbon neutrality,green hydrogen produced by water electrolysis using renewable electricity has attracted worldwide *** polymer electrolyte water electrolyzer(PEWE)has the potential to be a mainstay in the green hydrogen market in the future because of its superior ***,the development of PEWE is constrained by the slow progress of the membrane electrode assembly(MEA),which is an essential component of PEWE and largely determines the cost and performance of the ***,the MEA must be optimized from the aspects of reducing cost and improving performance to promote the development of *** this review,we first discuss the recent progress of the materials and design strategies of MEA,including the cost,activity,and stability of catalysts,distribution and thickness of ionomers,and ion transport efficiency of ion exchange membranes(IEMs).Then,the effects of all components and interlayer interfaces on the ions,electrons,and mass transfer in MEA and,consequently,the performance of PEWE are ***,we propose perspectives on developing MEA by optimizing the catalyst activity and stability of IEM,interface contact between adjacent components,and evaluation methods of performance.