Short-Term and Long-Term Effects of Natural and Artificial Carbonaceous Substrates on Greenhouse Gas Fluxes

作     者：Jürgen Kern Judy Libra Christian Ammon York Neubauer Wenceslau Teixeira 

作者机构：Leibniz Institute for Agricultural Engineering and Bioeconomy e.V.(ATB)Potsdam14469Germany TCKON Engineering Services Dr.-Ing.York NeubauerBerlin13088Germany Embrapa SoilsRio de Janeiro24600-000Brazil 

出 版 物：《Journal of Renewable Materials》 (可再生材料杂志（英文）)

年 卷 期：2022年第10卷第7期

页      面：1773-1786页

核心收录：

学科分类：0830[工学-环境科学与工程（可授工学、理学、农学学位）] 09[农学] 0903[农学-农业资源与环境] 0805[工学-材料科学与工程（可授工学、理学学位）] 0706[理学-大气科学] 090301[农学-土壤学] 

主　　题：Biochar HTC char incubation experiment GHG carbon stability 

摘      要：The emissions of two greenhouse gases(GHG),carbon dioxide(CO_(2))and nitrous oxide(N2O),from six substrates with different carbonaceous content were compared in short and long-term incubation *** natural soils and three artificial chars were mixed with carbon(C)poor soil(Cambisol)to simulate real conditions after application of char to *** natural soils were a Cambisol,an Anthrosol and a Histosol with C contents of 1.3%,4.4%and 13.2%,*** three chars produced through thermal conversion of wood chips by hydrothermal carbonisation(HTC),fluidized bed gasification and pyrolysis had C contents of 56.9%,75.4%and 79.9%,*** rates of CO_(2)and N2O from the rewetted substrates were measured by gas chromatography over a short time of 72 h and over a long period of nearly two *** short-term CO_(2)emissions from the natural soils showed a clear relationship to their C *** emission rate for the Histosol/Cambisol mixture was three times higher than that for the pure Cambisol,77.1 vs.23.5 mg CO_(2)-C kg^(-1)organic matter(OM)per *** C emission rates for the char/Cambisol mixtures were much lower,ranging between 3.0 and 9.1 mg CO_(2)-C kg OM^(-1)h^(-1),and did not correspond to their total C *** between the two incubation lengths showed that the long-term CO_(2)emission rates were generally one order of magnitude lower than the short-term *** final emission rates for natural substrates over a period of two years were still twice those for artificial char substrates,between 2.2–3.5 mg CO_(2)-C kg OM^(-1)h^(-1)and 1.3–1.8 mg CO_(2)-C kg OM^(-1)h^(-1),*** the contents of total nitrogen(Ntot)and extractable nitrogen(Nmin)were considerable in the chars under study,enhanced N2O release was not observed in the incubation ***,N2O emission rates in the three mixtures of chars and Cambisol were lower by one to two orders of magnitude compared to the pure Cambisol in