Metal-organic frameworks enable broad strategies for lithium-sulfur batteries

作     者：Cheng Zhou Zhaohuai Li Xu Xu Liqiang Mai Cheng Zhou;Zhaohuai Li;Xu Xu;Liqiang Mai

作者机构：State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of Technology International Schoo of Materials Science and EngineeringWuhan University of Technology Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory 

出 版 物：《National Science Review》 (国家科学评论(英文版))

年 卷 期：2021年第8卷第12期

页      面：104-121页

核心收录：

学科分类：0808[工学-电气工程] 08[工学] 0805[工学-材料科学与工程（可授工学、理学学位）] 080502[工学-材料学] 

基　　金：supported by the National Key Research and Development Program of China (2020YFA0715000,2016YFA0202603 and 2018YFB0104200) the National Natural Science Foundation of China (51702247 and 51832004) the Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory (XHT2020-003) the Fundamental Research Funds for the Central Universities(WUT:2019III174, 2020III023 and 2020III050) 

主　　题：metal-organic frameworks lithium-sulfur batteries cathode separator electrolyte 

摘      要：The lithium-sulfur(Li-S) battery is considered to be a potential next-generation power battery system,however, it is urgent that suitable materials are found in order to solve a series of challenges, such as the shuttle effect and lithium dendrite growth. As a multifunctional porous material, metal-organic frameworks(MOFs) can be used in different parts of Li-S batteries. In recent years, the application of MOFs in Li-S batteries has been developed rapidly. This review summarizes the milestone works and recent advances of MOFs in various aspects of Li-S batteries, including cathode, separator and electrolyte. The factors affecting the performance of MOFs and the working mechanisms of MOFs in these different parts are also discussed in detail. Finally, the opportunities and challenges for the application of MOFs in Li-S batteries are proposed. We also put forward feasible solutions to related problems. This review will provide better guidance for the rational design of novel MOF-based materials for Li-S batteries.