Vertically aligned two-dimensional materials-based thick electrodes for scalable energy storage systems

作     者：Zhengyu Ju Xiao Zhang Jingyi Wu Guihua Yu Zhengyu Ju;Xiao Zhang;Jingyi Wu;Guihua Yu

作者机构：Materials Science and Engineering ProgramTexas Materials InstituteThe University of Texas at AustinAustinTexas 78712USA 

出 版 物：《Nano Research》 (纳米研究（英文版）)

年 卷 期：2021年第14卷第10期

页      面：3562-3575页

核心收录：

学科分类：08[工学] 0805[工学-材料科学与工程（可授工学、理学学位）] 080502[工学-材料学] 

基　　金：G.H.Y.acknowledges the funding support from the Center for Mesoscale Transport Properties an Energy Frontier Research Center supported by the DOE-BES(No.DE-SC0012673) 

主　　题：two-dimensional materials energy storage alignment assembly high energy/power 

摘      要：Together with the blooming of portable smart devices and electric vehicles in the last decade,electrochemical energy storage(EES)devices capable of high-energy and high-power storage are urgently ***-dimensional(2D)materials,benefiting from the short solid-state diffusion distance,are well recognized to possess excellent electrochemical ***,liquid diffusion,the rate-determining process in thick electrodes,is notably slow in 2D materials-based electrodes stemming from their stacking during electrode processing,which considerably limits their applications for high energy *** fully exploit intrinsic advantages of 2D materials for scalable energy storage devices,this review summarizes several important strategies,ranging from assembly to template methods,to fabricate vertically aligned 2D materials-based *** further discuss the advantages and challenges of these methods in terms of key features of thick electrodes and illustrate the design principles for high-energy/power devices.