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Enhanced electrocatalytic activity of carbon cloth by synergetic effect of plasma and acid treatment

Enhanced electrocatalytic activity of carbon cloth by synergetic effect of plasma and acid treatment

作     者:Tingting MEI Ming GAO Danni LIU Yu WANG Yifan HUANG 梅婷婷;高明;刘丹妮;王裕;黄逸凡

作者机构:Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055People's Republic of China University of Chinese Academy of SciencesBeijing 100049People's Republic of China 

出 版 物:《Plasma Science and Technology》 (等离子体科学和技术(英文版))

年 卷 期:2021年第23卷第2期

页      面:57-63页

核心收录:

学科分类:081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程(可授工学、理学学位)] 

基  金:by Shenzhen Science and Technology Innovation Committee(No.JCYJ20180507182200750) 

主  题:carbon cloth electrocatalytic activity plasma treatment acid oxidation 

摘      要:Commercial carbon cloth(CC)is an ideal electrocatalysis material to produce oxygen evolution reaction(OER)due to its high conductive and 3D flexible structure,but the lacked active sites limit its *** improving its OER performance,the present study proposed an effective method combining plasma and acid treatment to introduce oxygen-containing functional groups and produce more active sites on its *** to the pristine CC,the plasma and acid treated carbon cloth(PN-CC)delivers a reduced overpotential by 34.6%to achieve current density of 10 mA cm^(−2).The Tafel slope declines from 97.5 mV dec^(–1)(pristine CC)to 55.9 mV dec–1(PN-CC),showing an increased OER ***,PN-CC electrocatalyst shows outstanding stability after 5000 cycles or 25000 *** combination of plasma and acid treatment shows a significant potential in surface modification for electrocatalysts.

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