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Bimetallic Single‑Atom Catalysts for Water Splitting

Nano-Micro Letters 2025年第1期17卷 1-45页

作者： Megha A.Deshmukh Aristides Bakandritsos Radek Zbořil Nanotechnology Centre Centre for Energy and Environmental TechnologiesVŠB–Technical University of Ostrava17.listopadu 2172/1570800 Ostrava‑PorubaCzech Republic Regional Centre of Advanced technologies and Materials Czech Advanced Technology and Research Institute(CATRIN)Palacky University OlomoucŠlechtitelů241/2778371 Olomouc–HoliceCzech Republic

Green hydrogen from water splitting has emerged as a critical energy vector with the potential to spearhead the global transition to a fossil fuel-independent *** field of catalysis has been revolutionized by single-atom catalysts(SACs),which exhibit unique and intricate interactions between atomically dispersed metal atoms and their ***,bimetallic SACs(bimSACs)have garnered significant attention for leveraging the synergistic functions of two metal ions coordinated on appropriately designed *** offer an avenue for rich metal–metal and metal–support cooperativity,potentially addressing current limitations of SACs in effectively furnishing transformations which involve synchronous proton–electron exchanges,substrate activation with reversible redox cycles,simultaneous multi-electron transfer,regulation of spin states,tuning of electronic properties,and cyclic transition states with low activation *** review aims to encapsulate the growing advancements in bimSACs,with an emphasis on their pivotal role in hydrogen generation via water *** subsequently delve into advanced experimental methodologies for the elaborate characterization of SACs,elucidate their electronic properties,and discuss their local coordination ***,we present comprehensive discussion on the deployment of bimSACs in both hydrogen evolution reaction and oxygen evolution reaction,the two half-reactions of the water electrolysis process.

关键词： Single-atom catalysts Single-atom dimers Hydrogen evolution Oxygen evolution Water splitting

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Electrochemical conversion of methane to bridge the gap in the artificial carbon cycle

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Journal of energy Chemistry 2025年第1期100卷 286-308页

作者： Yuhao Peng Yuefeng Song Ihar Razanau Juanxiu Xiao Wei Xiao Di Hu Guoxiong Wang College of Chemistry and Molecular Sciences Hubei Key Laboratory of Electrochemical Power Sources Wuhan University State Key Laboratory of Catalysis Dalian National Laboratory for Clean Energy iChEM (Collaborative Innovation Center of Chemistry for Energy Materials) Dalian Institute of Chemical Physics Chinese Academy of Sciences Laboratory of Physical-Chemical technologies SSPA Scientific and Practical Materials Research Centre of NAS of Belarus State Key Laboratory of Marine Resources Utilization in South China Sea Collaborative Innovation Center of Marine Science and Technology School of Marine Science and Engineering Hainan University Department of Chemical and Environmental Engineering University of Nottingham Ningbo China

Methane, an abundant one-carbon（C1） resource, is extensively used in the industrial production of vital fuels and value-added chemicals. However, current industrial methane conversion technologies are energy-and carbon-intensive, mainly due to the high activation energy required to break the inert C–H bond, low selectivity, and problematic side reactions, including CO2emissions and coke deposition. Electrochemical conversion of methane（ECM） using intermittent renewable energy offers an attractive solution, due to its modular reactor design and operational flexibility across a broad spectrum of temperatures and pressures. This review emphasizes conversion pathways of methane in various reaction systems, highlighting the significance and advantages of ECM in facilitating a sustainable artificial carbon cycle. This work provides a comprehensive overview of conventional methane activation mechanisms and delineates the complete pathways of methane conversion in electrolysis contexts. Based on surface/interface chemistry, this work systematically analyzes proposed reaction pathways and corresponding strategies to enhance ECM efficiency towards various target products, including syngas, hydrocarbons, oxygenates, and advanced carbon materials. The discussion also encompasses opportunities and challenges for the ECM process, including insights into ECM pathways, rational electrocatalyst design, establishment of benchmarking protocols, electrolyte engineering, enhancement of CH4conversion rates, and minimization of CO2emission.

关键词： Methane Electrochemical conversion Reaction mechanism Catalyst design Electrode Electrocatalysis

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An Overview to the Concept of Smart Coupling and Battery Management for Grid Connected Photovoltaic Battery system

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Journal of Electronic Science and Technology 2015年第4期13卷 367-372页

作者： Deepranjan Dongol Elmar Bollin Thomas Feldmann the institute of energy system(INES) Offenburg University of Applied Science the institute of energy system(INES) Offenburg University of Applied Science

The paper gives an overview on the need for smart coupling for battery management in grid integrated renewable energy system （RES）. Grid integrated photovoltaic （PV） battery system, as being popular and extensively used has been discussed in the paper. Smart coupling refers to intelligent grid integration such that it can foresee local network conditions and issue battery power flow management strategy accordingly to shave the peak PV and peak load. Therefore, a need for predictive energy management arises for smart integration to the grid and supervision of the power flow in accordance to the grid conditions. This is also a running project at the institute of energy systems （INES）, Offenburg University of Applied Science, Germany since January, 2015. The paper should provide insights to the motivation, need and gives an outlook to the features of desired predictive energy management system （PEMS）.

关键词： Battery management optimization,predictive energy management smart coupling

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THE HYDRODYNAMIC CHARACTERISTICS OF FREE VARIABLE-PITCH VERTICAL AXIS TIDAL TURBIN

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Journal of Hydrodynamics 2012年第6期24卷 834-839页

作者： ZHANG Xue-weii WANG Shu-qi WANG Feng ZHANG Liang SHENG Qi-hu institute of Ocean Renewable energy system Harbin Engineering University

The hydrodynamic characteristics of free variable-pitch vertical axis tidal turbine are investigated by combining experimental and numerical simulations. The variations of hydrodynamics are obtained based on testing the kinematics and the dynamics of the turbine under different flow and structural conditions. Through analyzing the movement of the turbine and the characteristics of the flow field by numerical simulations, it is shown how the turbine＇s performance is improved.

关键词： tidal current energy vertical axis variable-pitch turbine hydrodynamic characteristics experiments

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From waste to wealth:Coal tar residue derived carbon materials as low-cost anodes for potassium-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 464-475页

作者： Zhonghua Lu Jun Shen Xin Zhang Lingcong Chao Liang Chen Ding Zhang Tao Wei Shoudong Xu College of Chemical Engineering and Technology Taiyuan University of TechnologyTaiyuan 030024China College of Chemistry Taiyuan University of TechnologyTaiyuan 030024China School of Chemical Engineering and Pharmacy Wuhan Institute of TechnologyWuhan 430205China School of energy and Power Jiangsu University of Science and TechnologyZhenjiang 212003China

Carbon materials are widely recognized as highly promising electrode materials for various energy storage system *** tar residues(CTR),as a type of carbon-rich solid waste with high value-added utilization,are crucially important for the development of a more sustainable *** this study,we employed a straightforward direct carbonization method within the temperature range of 700-1000℃to convert the worthless solid waste CTR into economically valuable carbon materials as anodes for potassium-ion batteries(PIBs).The effect of carbonization temperature on the microstructure and the potassium ions storage properties of CTR-derived carbons(CTRCs)were systematically explored by structural and morphological characterization,alongside electrochemical performances *** on the co-regulation between the turbine layers,crystal structure,pore structure,functional groups,and electrical conductivity of CTR-derived carbon carbonized at 900℃(CTRC-900H),the electrode material with high reversible capacity of 265.6m Ah·g^(-1)at 50 m A·g^(-1),a desirable cycling stability with 93.8%capacity retention even after 100 cycles,and the remarkable rate performance for PIBs were ***,cyclic voltammetry(CV)at different scan rates and galvanostatic intermittent titration technique(GITT)have been employed to explore the potassium ions storage mechanism and electrochemical kinetics of *** indicate that the electrode behavior is predominantly governed by surface-induced capacitive processes,particularly under high current densities,with the potassium storage mechanism characterized by an“adsorption-weak intercalation”*** work highlights the potential of CTR-based carbon as a promising electrode material category suitable for high-performance PIBs electrodes,while also provides valuable insights into the new avenues for the high value-added utilization of CTR.

关键词： coal tar residue carbon materials anode potassium-ion batteries high value-added

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Multiperspective Analysis of Microscale Trigeneration systems and Their Role in the Crowd energy Concept

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Journal of Electronic Science and Technology 2015年第3期13卷 206-211页

作者： Parantapa Sawant Naim Meftah Jens Pfafferott the institute of energy system technologies Offenburg University of Applies Sciences the Department of Mechanical and Process Engineering Offenburg University of Applied Sciences

The energy system of the future will transform from the current centralised fossil based to a decentralised, clean, highly efficient, and intelligent network. This transformation will require innovative technologies and ideas like trigeneration and the crowd energy concept to pave the way ahead. Even though trigeneration systems are extremely energy efficient and can play a vital role in the energy system, turning around their deployment is hindered by various barriers. These barriers are theoretically analysed in a multiperspective approach and the role decentralised trigeneration systems can play in the crowd energy concept is highlighted. It is derived from an initial literature research that a multiperspective （technological, energy-economic, and user） analysis is necessary for realising the potential of trigeneration systems in a decentralised grid. And to experimentally quantify these issues we are setting up a microseale trigeneration lab at our institute and the motivation for this lab is also briefly introduced.

关键词： Adsorption cooling decentralisation,energy efficiency energy system analysis trigeneration.

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Metal-organic frameworks with dinuclear metal centers for synergistically boosting CO2 photoreduction

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Science China Chemistry 2025年第1期 201-208页

作者： Hui-Feng Wang Wen-Jie Shi Yu-Xin Yang Bao-Xia Dong Tong-Bu Lu Di-Chang Zhong School of Chemistry and Chemical Engineering Yangzhou University institute for New energy Materials and Low Carbon technologies School of Materials Science and Engineering Tianjin University of Technology

Dinuclear metal synergistic catalysis （DMSC） has been proved powerful in boosting CO2reduction,while this has not been achieved in heterogeneous catalysts with long-range order *** this study,we,by introduction of metal catalytic centers into an indium-based metal-organic framework （MOF）,obtained a series of isostructural In-MOFs,including three MOFs with mononuclear metal catalytic center （M-In）,three MOFs with dinuclear homometallic catalytic centers （MM-In）,and three MOFs with dinuclear heterometallic catalytic centers (MM’-In,M/M’=Co（II）,Ni（II）,Zn（II）).It was found that all these MOFs can serve as catalysts for photochemical CO2reduction to *** with M-In,the catalytic activities of MM-In were obviously enhanced,and that of MM’-In was further significantly *** example,the CO yield of Co Zn-In reaches a record value of 12,700μmol g-1h-1,which is 4.0,8.1,9.4,and 18.6-fold higher than that of Co Co-In,Zn Zn-In,Co-In,and Zn-In,***,the catalytic activities of Co Ni-In and Ni Zn-In also show different fold increase than those of corresponding dinuclear homometallic and mononuclear metallic *** results of control experiments and theoretical calculation reveal that the higher catalytic activities of MM-In over M-In can be ascribed to the DMSC effect,and the higher catalytic activity of MM’-In over MM-In can be ascribed to the strengthened DMSC *** work reveals the relationship between DMSC effect and bimetal centers in CO2reduction,which provides new insights into the DMSC and paves a new way to design highly active catalysts for photochemical CO2reduction.

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Co-production of hydrogen, oxygen, and electricity via an integrated solar-driven system with decoupled water electrolyzer and Na-Zn ion battery

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Journal of energy Chemistry 2025年第1期100卷 621-627页

作者： Fei Lv Longjie Liu Jiazhe Wu Pengfei Wang Lixia Pan Dengwei Jing Yubin Chen International Research Center for Renewable energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

Combining water electrolysis and rechargeable battery technologies into a single system holds great promise for the co-production of hydrogen （H2） and ***,the design and development of such systems is still in its ***,an integrated hydrogen-oxygen （O2）-electricity co-production system featuring a bipolar membrane-assisted decoupled electrolyzer and a Na-Zn ion battery was established with sodium nickelhexacyanoferrate （NaNiHCF） and Zn2+/Zn as dual redox *** decoupled electrolyzer enables to produce H2and O2in different time and space with almost 100%Faradaic efficiency at 100 mA ***,the charged NaNiHCF and Zn electrodes after the electrolysis processes formed a Na-Zn ion battery,which can generate electricity with an average cell voltage of 1.75 V at 10 m A *** connecting Si photovoltaics with the modular electrochemical device,a well-matched solar driven system was built to convert the intermittent solar energy into hydrogen and electric energy with a solar to hydrogen-electricity efficiency of 16.7%,demonstrating the flexible storage and conversion of renewables.

关键词： Hydrogen Electricity Decoupled water electrolyzer Na-Zn ion battery Solar energy

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Evaluation of Electricity Generating system's Technology Mix Using 3E Indicator

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Journal of Thermal Science 2019年第2期28卷 218-224页

作者： GRKOVIC Vojin Steinbeis energy technologies

For the purpose of the research, the technologies for electricity generation are classified in four categories: CO_2-free-desspatchable(hydro, nuclear, and biomass fired), CO_2-free-non-desspatchable(wind generators and photo voltaic), CO_2-dependent-despatchable and CO_2-dependent-non-despatchable ones. 3E indicator is introduced purposely to enable quantitative evaluation of the considered complex technology structures, as well as to provide support for decision making during the design and operation procedures of electricity generating systems. The application of the indicator is demonstrated with appropriate model numerical simulations for the general European conditions. In the model calculations are analyzed simplified technology mixes with CO_2 free, non-despatchable technologies in overall load, two technologies in base part of the residual load(lignite fired and nuclear), one technology in intermediate part of the residual load and one in the pick part of the residual load both CO_2 dependent, despatchable ones. The results show that the introduced 3E indicator is suitable for analysis of the technological combinations for electricity generation within considered countries. The results also show that increase participation of nuclear power plants in residual load domain contribute to better(lower) value of 3E indicator. The results obtained for technology structures in nine analyzed European countries(Germany, France, Austria, Greece, Serbia, Hungary, Bulgaria, Belgium and Netherlands) point out that the country with higher participation of CO_2 free despatchable and lower participation of CO_2 free non-despatchable technologies in electricity generation has tendency toward better i.e. lower value of 3E indicator. On the other hand the country with the higher participation of CO_2 free non-despatchable and lower to moderate participation of CO_2 free despatchable technologies has tendency toward the higher value of 3E indicator. These results are in accorda

关键词： 3E indicator technology matrix energy technologies carbon-free despatchable

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A modular parallelization framework for power flow transfer analysis of large-scale power systems

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Journal of Modern Power systems and Clean energy 2018年第4期6卷 679-690页

作者： Chuntian CHENG Bin LUO Jianjian SHEN Shengli LIAO institute of Hydropower system and Hydroinformatics Dalian University of Technology Tsinghua Sichuan energy Internet Research institute

Power flow transfer(PFT) analysis under various anticipated faults in advance is important for securing power system operations. In China, PSD-BPA software is the most widely used tool for power system analysis, but its input/output interface is easily adapted for PFT analysis,which is also difficult due to its computationally *** solve this issue, and achieve a fast and accurate PFT analysis, a modular parallelization framework is developed in this paper. Two major contributions are included. One is several integrated PFT analysis modules, including parameter initialization, fault setting, network integrity detection, reasonableness identification and result *** other is a parallelization technique for enhancing computation efficiency using a Fork/Join framework. The proposed framework has been tested and validated by the IEEE 39 bus reference power system. Furthermore, it has been applied to a practical power network with 11052 buses and 12487 branches in the Yunnan Power Grid ofChina, providing decision support for large-scale power system analysis.

关键词： Power flow transfer Modular Parallelization Fork/Join framework PSD-BPA

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