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Protein-activated atomic layer deposition for robust crude-oil-repellent hierarchical nano-armored membranes

Science Bulletin 2024年第2期69卷 218-226页

作者： Xiaobin Yang Pan Sun Yajie Wen Anil U.Mane Jeffrey W.Elam Jun Ma Shaomin Liu Seth B.Darling Lu Shao MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage State Key Laboratory of Urban Water Resource and EnvironmentSchool of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001China Chemical Sciences and engineering Division Argonne National LaboratoryLemont IL 60439USA Applied Materials Division Argonne National LaboratoryLemont IL 60439USA Advanced Materials for Energy-Water Systems Energy Frontier Research Center Argonne National LaboratoryLemont IL 60439USA Pritzker School of Molecular engineering University of ChicagoChicago IL 60637USA department of Physics University of Ilinois at ChicagoChicago IL 60607USA School of Environment Harbin Institute of TechnologyHarbin 150090China WA School of Mines:Minerals Energy and Chemical EngineeringCurtin UniversityPerth WA 6845Australia

Atomic layer deposition(ALD)offers unique capabilities to fabricate atomically engineered porous materials with precise pore tuning and multi-functionalization for diverse applications like advanced membrane separations towards sustainable energy-water ***,current ALD technique is inhibited on most non-polar polymeric membranes due to lack of accessible nucleation ***,we report a facile method to efficiently promote ALD coating on hydrophobic surface of polymeric membranes via novel protein activation/*** a proof of concept,TiO2 ALD-coated membranes activated by bovine serum albumin exhibit remarkable superhydrophilicity,ultralow underwater crude oil adhesion,and robust tolerance to rigorous environments including acid,alkali,saline,and *** importantly,excellent cyclable crude oil-in-water emulsion separation performance can be *** mechanism for activation/sensitization is rooted in reactivity for a particular set of amino ***,the universality of protein-sensitized ALD is demonstrated using common egg white,promising numerous potential usages in biomedical engineering,environmental remediation,lowcarbon manufacturing,catalysis,and beyond.

关键词： Membrane separation Atomic layer deposition Water treatment Antifouling

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A Self-propagating high-temperature synthesis process for the fabrication of Fe（Cr）–Al2O3 nanocomposite

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International Journal of Minerals,Metallurgy and Materials 2019年第6期26卷 775-786页

作者： Seyed Esmaiel Shakib Ramin Raiszadeh Jalil Vahdati-Khaki department of Metallurgy and Materials Science School of EngineeringShahid Bahonar University of KermanKerman ***Iran department of Materials Science and metallurgical engineering Engineering FacultyFerdowsi University of MashhadMashhad ***Iran

Self-propagating high-temperature synthesis(SHS)was used to fabricate a Fe(Cr)–Al2O3 *** composite was fabricated by the reactions between the powders of Fe,Fe2O3,Cr2O3,and *** effect of blending ratio and mechanical activation of the initial powders and the precursor compressing pressure on the microstructure of the final product was studied by optical microscopy,scanning electron microscopy,transmission electron microscopy,and X-ray *** significance of the effect of each of the aforementioned parameters on the quality of the composite(assessed by measuring the compressive strength and wear resistance)was determined using a full-factorial design of experiments *** results showed that the best molar powder ratio that produced the most homogeneous product through a sustainable SHS reaction was Fe:Fe2O3:Cr2O3:Al=10:1:1:4.A lower Fe content caused the Fe(Cr)phase to melt and separate from the rest of the materials.

关键词： self-propagating high temperature synthesis phase separation mechanical activation iron-chrome nanocomposite

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Legendre-Weighted Residual Methods for System of Fractional Order Differential Equations

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Journal of Applied Mathematics and Physics 2024年第9期12卷 3163-3184页

作者： Umme Ruman Md. Shafiqul Islam department of Computer Science & engineering Green University of Bangladesh Dhaka Bangladesh department of Applied Mathematics University of Dhaka Dhaka Bangladesh

The numerical approach for finding the solution of fractional order systems of boundary value problems (BPVs) is derived in this paper. The implementation of the weighted residuals such as Galerkin, Least Square, and Collocation methods are included for solving fractional order differential equations, which is broadened to acquire the approximate solutions of fractional order systems with differentiable polynomials, namely Legendre polynomials, as basis functions. The algorithm of the residual formulations of matrix form can be coded efficiently. The interpretation of Caputo fractional derivatives is employed here. We have demonstrated these methods numerically through a few examples of linear and nonlinear BVPs. The results in absolute errors show that the present method efficiently finds the numerical solutions of fractional order systems of differential equations.

关键词： Fractional Differential Equations System of Fractional Order BVPs Weighted Residual Methods Modified Legendre Polynomials

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Analytical Solution for the Reissner-Sagoci Problem of a Piezoelectric Half-Space

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Acta Mechanica Solida Sinica 2024年第3期37卷 363-370页

作者： Keqiang Hu Cun-Fa Gao Zengtao Chen Zheng Zhong State Key Laboratory of Mechanics and Control of Mechanical Structures Nanjing University of Aeronautics and AstronauticsNanjing210016China department of Mechanical engineering University of AlbertaEdmontonABT6G 1H9Canada School of Science Harbin Institute of TechnologyShenzhen518055China

In this paper,a transversely isotropic piezoelectric half-space with the isotropy axis parallel to the z-axis is considered under rotation on a rigid circular disk bonded to the surface of the piezoelectric *** is a type of Reissner-Sagoci mixed boundary value *** utilizing the Hankel transform,the mixed boundary value problem is simplified into solving a pair of dual integral ***-field analytical expressions for displacement,stresses,and electric displacement inside the half-space are *** shear stresses and electric displacement on the surface are found to be singular at the edge of the rigid circular disk,and the stress intensity factors and electric displacement intensity factor are *** results show that material properties and geometric size have significant effects on displacement,shear stresses,and electric displacement.

关键词： Piezoelectric half-space Circular disk Reissner-Sagoci problem Stress intensity factor Electric displacement intensity factor

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Recent advances in vacancy engineering for reliable lithiumsulfur batteries

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Rare Metals 2024年第2期43卷 455-477页

作者： Wen-Dong Liu Xiao Tang Jun-An Feng Chao-Yue Zhang Hao Liu Chuan Shi Xiao-Xian Zhao Jian-Jun Song College of Physics School of Chemistry and Chemical EngineeringQingdao UniversityQingdao266071China Faculty of Science Centre for Clean Energy TechnologySchool of Mathematical and Physical SciencesUniversity of Technology SydneySydneyNSW2007Australia department of Chemistry College of ScienceHebei Agricultural UniversityBaoding071001China

The high-energy-density and low-cost features endow lithium-sulfur batteries with broad application ***,many drawbacks,especially the detrimental shuttle effect,have hindered the further development of *** response,a lot of new structures have been applied to suppress the shuttle effect and promote the development of ***,vacancy engineering has gained the attention of researchers due to its unique electronic *** review aims to analyze the application of vacancy engineering in ***,the electrochemistry of LSBs has been systematically discussed and the existing challenges as well as improvement tactics of LSBs have also been ***,the preparation methods and characterization technologies of various vacancies are summarized,including oxygen vacancies,sulfur vacancies,selenium vacancies,other anion vacancies,cation vacancies,*** latest applications of vacancy engineering in LSBs are also summarized in this ***,some prospects and insights for further investigation and practical application of vacancy engineering in LSBs are put forward.

关键词： Lithium-sulfur batteries(LSBs) Defects Vacancy engineering Electronic structure Shuttle effect

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Advancements on metal oxide semiconductor photocatalysts in photo-electrochemical conversion of carbon dioxide into fuels and other useful products

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Frontiers in Energy 2024年第2期18卷 187-205页

作者： Jai PRAKASH Zhangsen CHEN Shakshi SAINI Gaixia ZHANG Shuhui SUN department of Chemistry National Institute of Technology HamirpurHamirpur 177005India Institut National de la Recherche Scientifique(INRS) Centre Énergie Matériaux TélécommunicationsVarennes J3X 1P7Canada department of Chemistry Indian Institute of Technology MandiHimachal PradeshIndia department of Electrical engineering École de Technologie SupérieureMontréal H3C 1K3Canada

Due to its fascinating and tunable optoelectronic properties,semiconductor nanomaterials are the best choices for multidisciplinary ***,the use of semiconductor photocatalysts is one of the promising ways to harness solar energy for useful applications in the field of energy and *** recent years,metal oxide-based tailored semiconductor photocatalysts have extensively been used for photocatalytic conversion of carbon dioxide(CO_(2))into fuels and other useful products utilizing solar *** is very significant not only from renewable energy consumption but also from reducing global warming point of *** current research activities are promising for a better future of *** present mini-review is focused on recent developments(2–3 years)in metal oxide semiconductor hybrid photocatalysts-based photo-electrochemical conversion of CO_(2)into fuels and other useful ***,general mechanism of photo-electrochemical conversion of CO_(2)into fuels or other useful products has been ***,various metal oxide-based emerging hybrid photocatalysts including tailoring of their morphological,compositional,and optoelectronic properties have been discussed with emphasis on their role in enhancing photoelectrochemical ***,mechanism of their photo-electrochemical reactions and applications in CO_(2)conversion into fuels/other useful products have been ***,challenges and future prospects have been discussed followed by a summary.

关键词： metal-oxide semiconductors nanohybrid photocatalysts photo-electrochemical CO_(2)conversion tailoring morphology fuels challenges and future prospects

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Power Quality Disturbance Identification Basing on Adaptive Kalman Filter andMulti-Scale Channel Attention Fusion Convolutional Network

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Energy engineering 2024年第7期121卷 1865-1882页

作者： Feng Zhao Guangdi Liu Xiaoqiang Chen Ying Wang School of Automation and Electrical engineering Lanzhou Jiaotong UniversityLanzhou730070China

In light of the prevailing issue that the existing convolutional neural network(CNN)power quality disturbance identification method can only extract single-scale features,which leads to a lack of feature information and weak anti-noise performance,a new approach for identifying power quality disturbances based on an adaptive Kalman filter(KF)and multi-scale channel attention(MS-CAM)fused convolutional neural network is *** and composite-disruption signals are generated through *** adaptive maximum likelihood Kalman filter is employed for noise reduction in the initial disturbance signal,and subsequent integration of multi-scale features into the conventional CNN architecture is *** multi-scale features of the signal are captured by convolution kernels of different sizes so that the model can obtain diverse feature *** attention mechanism(ATT)is introduced to adaptively allocate the extracted features,and the features are fused and selected to obtain the new main *** Softmax classifier is employed for the classification of power quality ***,by comparing the recognition accuracy of the convolutional neural network(CNN),the model using the attention mechanism,the bidirectional long-term and short-term memory network(MS-Bi-LSTM),and the multi-scale convolutional neural network(MSCNN)with the attention mechanism with the proposed *** simulation results demonstrate that the proposed method is higher than CNN,MS-Bi-LSTM,and MSCNN,and the overall recognition rate exceeds 99%,and the proposed method has significant classification accuracy and robust classification *** achievement provides a new perspective for further exploration in the field of power quality disturbance classification.

关键词： Power quality disturbance kalman filtering convolutional neural network attention mechanism

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Low-Carbon Dispatching for Virtual Power Plant with Aggregated Distributed Energy Storage Considering Spatiotemporal Distribution of Cleanness Value

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Journal of Modern Power Systems and Clean Energy 2024年第2期12卷 346-358页

作者： Hongchao Gao Tai Jin Guanxiong Wang Qixin Chen Chongqing Kang Jingkai Zhu State Key Laboratory of Power System Operation and Control Department of Electrical EngineeringTsinghua UniversityBeijing 100084China Sichuan Energy Internet Research Institute Tsinghua University Chengdu 200016China Power Dispatching and Control Center of Shanghai Municipal Electric Power Company Shanghai 200122China IEEE

The scale of distributed energy resources is increasing,but imperfect business models and value transmission mechanisms lead to low utilization ratio and poor *** address this issue,the concept of cleanness value of distributed energy storage(DES)is proposed,and the spatiotemporal distribution mechanism is discussed from the perspectives of electrical energy and *** on this,an evaluation system for the environmental benefits of DES is constructed to balance the interests between the aggregator and the power system ***,an optimal low-carbon dispatching for a virtual power plant(VPP)with aggregated DES is constructed,where-in energy value and cleanness value are both *** achieve the goal,a green attribute labeling method is used to establish a correlation constraint between the nodal carbon potential of the distribution network(DN)and DES behavior,but as a cost,it brings multiple nonlinear ***,a solution method based on the convex envelope(CE)linear re-construction method is proposed for the multivariate nonlinear programming problem,thereby improving solution efficiency and ***,the simulation verification based on the IEEE 33-bus DN is *** simulation results show that the multidimensional value recognition of DES motivates the willingness of resource users to ***,resolving the impact of DES on the nodal carbon potential can effectively alleviate overcompensation of the cleanness value.

关键词： Distributed energy storage virtual power plant(VPP) spatiotemporal distribution low-carbon dispatching

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Recent advances in biomimetic aggregation-induced emission photosensitizers for photodynamic therapy and immunotherapy

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BMEMat(BioMedical engineering Materials) 2024年第3期2卷 74-91页

作者： Shuai Guo Hui Tang Yahui Zhang Zhouyu Wang Swee Ching Tan department of Materials Science and engineering National University of SingaporeSingapore department of Chemistry School of ScienceXihua UniversityChengduChina

The development of novel photosensitizers(PSs)with aggregation-induced emission(AIE)properties has emerged as a crucial advancement in the field of photodynamic therapy(PDT).However,the versatile applications of AIE PSs are limited by low encapsulation efficiency and inadequate target tissue *** technology stands out as a promising strategy to overcome these challenges,aiming to enhance AIE PSs tumor penetration efficacy,and their association with antitumor immune *** this review,recent advancements in biomimetic AIE PSs for PDT and immunotherapy are *** start with introducing strategies involving biomimetic AIE PSs based on cell membranes and extracellular vesicles for the combined application of PDT and *** then discuss the preparation of biomimetic AIE PSs ***,we briefly outline the challenges and prospects associated with biomimetic AIE PSs.

关键词： aggregation induced emission biomimetic immunotherapy photodynamic therapy photosensitizers

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Weak interaction-steered evolution of polyoxovanadate-based metal-organic polyhedra from transformation via interlock to packing

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Chinese Chemical Letters 2024年第2期35卷 527-533页

作者： Yan-Hu Wang Ke-Wei Tong Chao-Qin Chen Jing Du Peng Yang College of Chemistry and Chemical engineering Advanced Catalytic Engineering Research Center of the Ministry of EducationHunan UniversityChangsha 410082China College of Chemistry and Materials Science Testing and Analysis CenterHebei Normal UniversityShijiazhuang 050024China

A bottleneck in biomimetic synthesis consists in the full copy of,for example,the hierarchical structure of proteins directed by weak *** contrast with covalent bonds bearing definite orientation and high stability,weak intermolecular forces within a continuous dynamic equilibrium can be hardly tamed for molecular *** this endeavor,a ligand-dominated strategy that embodies tunable electrostatic repulsion andπ···πstacking was first employed to shape polyoxovanadate-based metal-organic polyhedra(VMOPs).Structural evolution involving transformation,interlock,and discovery of an unprecedented prototype of the Star of David was hence *** only as a handy tool for the primary structural control over VMOPs,these weak forces allow for an advanced management on the spatial distribution of such manmade macromolecules as well as the associated physicochemical behaviors,representing an ideal model for simulating and interpreting the conformation-function relationship of proteins.

关键词： Polyoxometalates Polyoxovanadates Metal-organic polyhedron Interlock Weak intermolecular forces

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