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Enhancing Photocatalytic Hydrogen Evolution through Electronic Structure and Wettability Adjustment of ZnIn2S4/Bi2O3 S-Scheme Heterojunction

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物理化学学报 2024年第8期40卷 50-63页

作者： Linfeng Xiao Wanlu Ren Shishi Shen Mengshan Chen Runhua Liao Yingtang Zhou Xibao Li School of Materials Science and engineering Jingdezhen Ceramic UniversityJingdezhen 333403Jiangxi ProvinceChina zhejiang key laboratory of Petrochemical Environmental Pollution Control National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316022Zhejiang ProvinceChina School of Materials Science and engineering Nanchang Hangkong UniversityNanchang 330063China

The production of renewable fuels through water splitting via photocatalytic hydrogen production holds significant ***,the sluggish kinetics of hydrogen evolution and the inadequate water adsorption on photocatalysts present notable *** this study,we have devised a straightforward hydrothermal method to synthesize Bi_(2)O_(3)(BO)derived from metal‐organic frameworks(MOFs),loaded with flower-like ZnIn_(2)S_(4)(ZIS).This approach substantially enhances water adsorption and surface catalytic reactions,resulting in a remarkable enhancement of photocatalytic *** employing triethanolamine(TEOA)as a sacrificial agent,the hydrogen evolution rate achieved with 15%(mass fraction)ZIS loading on BO reached an impressive value of 1610μmol∙h^(−1)∙g^(−1),marking a 6.34-fold increase compared to that observed for bare ***,through density functional theory(DFT)and ab initio molecular dynamics(AIMD)calculations,we have identified the reactions occurring at the ZIS/BO S-scheme heterojunction interface,including the identification of active sites for water adsorption and catalytic *** study provides valuable insights into the development of high-performance composite photocatalytic materials with tailored electronic properties and wettability.

关键词： S-scheme Hydrogen evolution Wettability Photocatalysis Electronic structure

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New perspectives on the genetic structure of dotted gizzard shad(Konosirus punctatus)based on RAD-seq

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marine Life Science & technology 2024年第1期6卷 50-67页

作者： Ying Peng Yifan Liu Jiasheng Li Kun Zhang Xun Jin Sixu Zheng Yunpeng Wang Zhenming Lu Liqin Liu Li Gong Bingjian Liu National engineering laboratory of marine Germplasm Resources Exploration and Utilization Zhejiang Ocean UniversityZhoushan 316022China National engineering Research Center for facilitated marine aquaculture Marine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316022China

To maintain,develop and rationally utilize marine organisms,understanding their genetic structure and habitat adaptation pattern is *** punctatus,which is a commercial fish species inhabiting the Indo-west Pacific Ocean,has shown an obvious annual global capture and aquaculture production decline due to climate changes and human *** the present study,restriction-site associated DNA sequencing(RAD-seq)was used to describe its genome-wide single nucleotide polymorphisms panel(SNPs).Among 146 individuals collected at nine locations scattered in China,Korea and Japan,a set of 632,090 SNPs were *** genetic analysis showed that *** individuals were divided into two significant genetic ***,potential genetic differentiation between northern and southern population of *** was *** results indicated that gene flow existed among sampling locations of ***,especially from southern Japan to ***,candidate genes associated with habitat adaptations of *** were identified,which are involved in diverse physiological processes of *** including growth and development(e.g.,KIDINS220,PAN3),substance metabolism(e.g.,PGM5)and immune response(e.g.,VAV3,CCT7,HSPA12B).Our findings may aid in understanding the possible mechanisms for the population genetic structure and local adaptation of ***,which is beneficial to establish the management and conservation units of ***,guiding the rational use of resources,with reference significance for a profound understanding of the adaptative mechanisms of other marine organisms to the environment.

关键词： Population structure Konosirus punctatus SNP RAD-seq Local adaptation

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In-situ growth of MIL-53(Fe) on charcoal sponge as a highly efficient and recyclable photocatalyst for removal of Cr(Ⅵ)

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Rare Metals 2024年第9期43卷 4344-4355页

作者： Zhuo-Fan Yu Ye Yang Hai-Feng Zhuang Sheng-Dao Shan Mihail-Simion Beldean-Galea Qing-Quan Xue Xiao-Feng Shen Shi-Jie Li key laboratory of Recycling and Eco-Treatment of Waste Biomass of zhejiang Province School of Environmental and Natural Resources Zhejiang University of Science and Technology Faculty of Environmental Science and engineering Babes-Bolyai University key laboratory of Pollution Exposure and Health Intervention of zhejiang Province Interdisciplinary Research Academy (IRA) Zhejiang Shuren University National engineering Research Center for marine aquaculture Institute of Innovation & Application Zhejiang Ocean University

The application of metalDorganic frameworks(MOFs) is hindered by several crucial factors, including low photocatalytic efficiency, poor stability and challenges in recycling. In this study, MIL-53(Fe) was grown in situ on a charcoal sponge(CS) with a large surface area,excellent mechanical properties, and high photocatalytic efficiency using a solvothermal method, thus addressing the above-mentioned shortcomings of MOF ***, CS/MIL-53(Fe) has an amazing light-harvesting capacity in the visible range, leading to a significant improvement in the utilization of light. The results of the experiments indicate that CS/MIL-53(Fe) displays a higher photocatalytic activity(87% Cr(VI)) when exposed to visible light than CS(58%) or MIL-53(Fe)(27%),attributing to the increased separation of photogenerated carriers. e-is the main reactive radical and dominates the photocatalytic reduction process, rooting from that e-can reduce Cr(VI) to low-toxicity Cr(III). This study presents a novel method for constructing photocatalysts with large surface areas, superior mechanical characteristics, and enhanced photocatalytic performance. Additionally, it achieves the resource utilization of agricultural and forestry waste.

关键词： Charcoal sponge Cr(VI) Light absorption MIL-53(Fe) Photocatalysis

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Transcriptome profiling and RXR gene family identification reveals the molecular mechanism of rapid aging after spawning of cuttlefish Sepiella japonica

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Journal of Oceanology and Limnology 2024年第3期42卷 865-880页

作者： Zhenyu DONG Jiemei ZHAO Feng GUO Shuangrui LIN Huai YANG Yingying YE Changfei CHI Hongfei LI Baoying GUO College of marine Science and technology Zhejiang Ocean UniversityZhoushan 316022China National engineering Research Center for marine aquaculture Zhejiang Ocean UniversityZhoushan 316022China Donghai laboratory Zhoushan 316021China

Sepiella japonica is a worldwide marine cuttlefish species of high economic *** routinely modifying behaviors in reproductive life,such as rapid aging until death after spawning,has been recognized in artificial ***,reproductive behavior at the level of genes is rarely reported,thus,the research on the genetic basis of behavior,reproduction,and artificial breeding was *** applied RNA-seq in different stages of reproduction to investigate the reason of rapid aging after spawning,pre-maturity,pre-spawning after maturity,and *** retinoid X receptor(RXR)gene family in *** was identified,and 1343–1452 differentially expressed genes(DEGs)in all 3 stages of reproductive life were identified from pairwise m RNA ***,through the GO term and KEGG analysis,*** could handle neuronal development and network formation before maturity and have a functional degradation of neural communication,signal transduction,vision,and gene expression after *** Sj RXRαs have been identified and they played different roles in growth development or ***,the regulation of several channels and receptors is the intrinsic molecular mechanism of rapid aging after spawning in *** study revealed the survival strategy and provided fundamental data on the level of genes for understanding the reproductive behavior and the reproduction of ***.

关键词： Sepiella japonica RAN-seq retinoid X receptor(RXR)gene family rapid aging intrinsic molecular mechanism

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Photoelectrocatalytic hydrogen evolution and synchronous degradation of organic pollutants by pg-C_(3)N_(4)/β-FeOOH S-scheme heterojunction

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Science China(Technological Sciences) 2024年第4期67卷 1238-1252页

作者： LI XiBao HAN Tao ZHOU YingTang XIE Yu LUO YiDan HUANG JunTong CHEN Zhi DENG Fang School of Materials Science and engineering Nanchang Hangkong UniversityNanchang 330063China National-Local Joint engineering Research Center of Heavy Metal Pollutants Control and Resource Utilization Nanchang Hangkong UniversityNanchang 330063China zhejiang key laboratory of Petrochemical Environmental Pollution Control National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316022China

Crafting photoelectrocatalytic materials with robust oxidation-reduction properties for simultaneous hydrogen evolution and pollutant degradation poses a formidable *** this study,a pg-C_(3)N_(4)/β-FeOOH S-scheme heterostructure with a special energy band structure was developed by anchoring porous pg-C_(3)N_(4)on needle shapedβ-*** as a hole extraction layer,needle-leaf-likeβ-FeOOH can facilitate efficient hole migration and enhance charge ***,the optimized 0.2-pg-C_(3)N_(4)/β-FeOOH could degrade 78%of ofloxacin(OFLO)in 90 *** organic pollutants could absorb a large number of holes,which prompted a greater proportion of photogenerated electrons to actively participate in the hydrogen evolution reaction at the ***,the hydrogen production of 0.2-pg-C_(3)N_(4)/β-FeOOH reached 1452.88μmol cm^(-2)h^(-1),exhibiting a notable increase of 61.81-165.12μmol cm^(-2)h^(-1)compared with that in the absence of *** and theoretical calculation results underscore that this investigation is grounded in a distinctive electron and hole dual channel transfer *** findings offer novel insights for the future development of S-scheme heterojunction photoelectrocatalytic materials capable of concurrently degrading pollutants and promoting hydrogen evolution.

关键词： photoelectrocatalysis hydrogen evolution degradation synchronous S-scheme heterojunction

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Effect of Active–Passive Deformation on the Thrust by the Pectoral Fins of Bionic Manta Robot

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Journal of Bionic engineering 2024年第2期21卷 718-728页

作者： Yang Lu Shaomin Meng Cheng Xing Yiwei Hao Yonghui Cao Guang Pan Yong Cao School of marine Science and technology Northwestern Polytechnical UniversityXi’an710072China Unmanned Vehicle Innovation Center Ningbo Institute of NPUNingbo315103China State key lab of Fluid Power and Mechatronic Systems School of Mechanical EngineeringZhejiang UniversityHangzhou310027China zhejiang key laboratory of Advanced Manufacturing technology School of Mechanical EngineeringZhejiang UniversityHangzhou310027China

Bionic manta underwater vehicles will play an essential role in future oceans and can perform tasks,such as long-duration reconnaissance and exploration,due to their efficient *** manta wings’deformation is evident during the swimming *** improve the propulsion performance of the unmanned submersible,the study of the deformation into the bionic pectoral fin is *** this research,we designed and fabricated a flexible bionic pectoral fin,which is based on the Fin Ray®effect with active and passive deformation(APD)*** APD fin was actively controlled by two servo motors and could be passively deformed to variable *** APD fin was moved at 0.5 Hz beat frequency,and the propulsive performance was experimentally verified of the bionic pectoral fins equipped with different extents of *** results showed that the pectoral fin with active–passive deformed capabilities could achieve similar natural biological deformation in the wingspan *** average thrust(T)under the optimal wingspan deformation is 61.5%higher than the traditional passive deformed pectoral *** obtained results shed light on the design and optimization of the bionic pectoral fins to improve the propulsive performance of unmanned underwater vehicles(UUV).

关键词： Manta ray Bionic pectoral fin Fin Ray®effect Active-passive deformation(APD)

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Construction of ZnO@CDs@Co_(3)O_(4) sandwich heterostructure with multi-interfacial electron-transfer toward enhanced photocatalytic CO_(2) reduction

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Chinese Chemical Letters 2024年第4期35卷 147-152页

作者： Xiuzheng Deng Yi Ke Jiawen Ding Yingtang Zhou Hui Huang Qian Liang Zhenhui Kang Advanced Catalysis and Green Manufacturing Collaborative Innovation Center CNPC-CZU Innovation AllianceSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China zhejiang key laboratory of Petrochemical Environmental Pollution Control National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316004China

Photocatalytic conversion of CO_(2) into small-molecule chemical feedstocks can meet the growing demand for energy and alleviate the global warming. Herein, a p-n ZnO@CDs@Co_(3)O_(4) heterojunction with sandwich structure was constructed by calcination method of self-assembled ZIF-8@CDs@ZIF-67. The ZnO@CDs@Co_(3)O_(4) with well-defined interfacial structure exhibited the significantly enhanced photocatalytic CO_(2) reduction activity, and the optimal catalyst indicated the(CO + CH_(4)) evolution rate of 214.53μmol g^(-1)h^(-1) under simulated solar light, which was superior to ZnO, Co_(3)O_(4) and binary ZnO@Co_(3)O_(4).The internal cavity, exposed active sites, multiple interfaces and constructed p-n heterojunction can facilitate the light harvesting and photoexcited electron transfer. Besides, after introduction of CDs placed in the middle layer between ZnO and Co_(3)O_(4), CDs with excellent photoelectric property further promoted charge separation and migration. This work represents an appealing strategy to construct well-defined photocatalysts for boosting CO_(2) photoreduction.

关键词： Metal-organic framework Photocatalytic CO_(2) reduction Carbon dots p-n heterojunction Sandwich heterostructure

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Effects of nutrient limitations on the sinking velocity of Thalassiosira weissflogii

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Acta Oceanologica Sinica 2024年第6期43卷 163-172页

作者： Jie Zhu Qiang Hao Wei Zhang Yingying Ma Jiangning Zeng Ocean College Zhejiang UniversityZhoushan 316000China Second Institute of Oceanography Ministry of Natural ResourcesHangzhou 310012China key laboratory of marine Ecosystem Dynamics Ministry of Natural ResourcesHangzhou 310012China zhejiang key laboratory of Nearshore engineering Environment and Ecological Security Hangzhou 310012China Tianjin key lab of Aqua-Ecology and aquaculture College of FisheriesTianjin Agricultural UniversityTianjin 300384China

The sinking of diatoms is critic al to the formation of oceanic biological pumps and coastal hypoxic ***,little is known about the effects of different nutrient restrictions on diatom *** this study,we measured the sinking velocity(SV) of Thalassiosira weissflogii using a new phytoplankton video observation instrument and analyzed major biochemical components under varying nutrient *** results showed that the SV of *** under different nutrient limitation conditions varied *** highest SV of(1.77±0.02) m/d was obtained under nitrate limitation,signific antly surpassing that under phosphate limitation at(0.98±0.13) m/*** the nutrient limitation was released,the SV steadily decreased to(0.32±0.03) m/d and(0.15±0.05) m/d,***;under conditions with limited nitrate and phosphate concentrations,the SV values of *** significantly positively correlated with the lipid content(P marine nutrient structure.

关键词： nutrient limitation Thalassiosira weissflogii sinking velocity biochemical component lipid content

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Accurate Source-Receiver Positioning Method for a High-Resolution Deep-Towed Multichannel Seismic Exploration System

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Journal of Ocean University of China 2024年第2期23卷 415-426页

作者： LI Jing LIU Kai WEI Zhengrong ZHANG Liancheng LIU Yangting PEI Yanliang LIU Chenguang LIU Baohua key laboratory of marine Geology and Metallogeny First Institute of OceanographyMNRQingdao 266061China laboratory for marine Geology Laoshan LaboratoryQingdao 266061China College of Ocean Science and engineering Shandong University of Science and TechnologyQingdao 266590China key laboratory of Fluid Transmission technology of zhejiang Province Zhejiang Sci-Tech UniversityHangzhou 310018China

The near-seabed multichannel seismic exploration systems have yielded remarkable successes in marine geological disaster assessment,marine gas hydrate investigation,and deep-sea mineral exploration owing to their high vertical and horizontal ***,the quality of deep-towed seismic imaging hinges on accurate source-receiver positioning *** light of existing technical problems,we propose a novel array geometry inversion method tailored for high-resolution deep-towed multichannel seismic exploration *** method is independent of the attitude and depth sensors along a deep-towed seismic streamer,accounting for variations in seawater velocity and seabed slope *** approach decomposes the towed line array into multiline segments and characterizes its geometric shape using the line segment distance and pitch *** optimization parameters for seawater velocity and seabed slope angle,we establish an objective function based on the model,yielding results that align with objective *** the particle swarm optimization algorithm enables synchronous acquisition of optimized inversion results for array geometry and seawater *** validation using theoretical models and practical data verifies that our approach effectively enhances source and receiver positioning inversion *** algorithm exhibits robust stability and reliability,addressing uncertainties in seismic traveltime picking and complex seabed topography conditions.

关键词： high-resolution deep-towed multichannel seismic exploration source-receiver positioning array geometry inversion seawater heterogeneity seabed slope angle

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Toughened (Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))B_(2)–SiC composites fabricated by one-step reactive sintering with a unique SiB_(6) additive

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Journal of Advanced Ceramics 2024年第1期13卷 86-100页

作者： Wei Hao Xinzhe Lu Ling Li Tao Wang Guoliang Ren Huangyue Cai Xiaofeng Zhao Dongyun Wang Na Ni zhejiang Provincial key laboratory of Urban Rail Transit Intelligent Operation and Maintenance technology&Equipment Zhejiang Normal UniversityZhejiang 321004China key lab of Education Ministry for Power Machinery and engineering School of Mechanical EngineeringShanghai Jiao Tong UniversityShanghai 200240China School of Materials Science and engineering Shanghai Jiao Tong UniversityShanghai 200240China

High-entropy diboride has been arousing considerable interest in recent ***,the low toughness and damage tolerance limit its applications as ultra-high-temperature structural *** we report that a unique SiB_(6) additive has been first incorporated as boron and silicon sources to fabricate a high-entropy boride(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))B_(2)–SiC composite though one-step boro/carbothermal reduction reactive sintering.A synergetic effect of high-entropy sluggish diffusion and SiC secondary phase retarded the grain growth of the(Ti_(0.2)Zr_(0.2)Hf_(0.2)Nb_(0.2)Ta_(0.2))B_(2)–51SiC *** small grain size was beneficial to shorten the diffusion path for mass transport,thereby enhancing the relative density to~99.3%.These results in an increase of fracture toughness from~5.2 in HEBS-1900 to~7.7 MPa·m^(1/2) in HEBS-2000,which corresponded to a large improvement of 48%.The improvement was attributed to a mixed mode of intergranular and transgranular cracking for offering effective pinning in crack propagation,resulting from balanced grain boundary strength collectively affected by improved densification,solid solution strengthening,and incorporation of SiC secondary phase.

关键词： high-entropy diboride silicon hexaboride boro/carbothermal reduction reactive sintering fracture toughness

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