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Transforming waste particles into valuable adsorbents via amyloid-mediated molecular engineering

Science China Chemistry 2025年第01期 317-328页

作者： Qingmin Yang Jian Zhao Yujia Zhang Xingyu Zhou Hao Ren Bowen Hu Zhongli Lei Lixin Chen Peng Yang School of Material and Chemical Engineering Bengbu University Anhui Provincial Engineering Laboratory of Silicon-Based Materials School of Chemistry and Chemical Engineering Northwestern Polytechnical University Key Laboratory of Applied Surface and Colloid Chemistry Ministry of Education School of Chemistry and Chemical EngineeringShaanxi Normal University Xi'an Key Laboratory of Polymeric Soft Matter School of Chemistry and Chemical Engineering Shaanxi Normal University international Joint Research center on Functional Fiber and Soft Smart Textile School of Chemistry and Chemical EngineeringShaanxi Normal University

The high-value utilization of industrial solid waste using a facile and eco-friendly process is of great interest and significance in reducing environmental pollution and developing a green circular economy. Herein, we propose an amyloid-mediated molecular engineering strategy to transform particulate waste into valuable adsorbents for metal ions. Our method has the advantage of aqueous solution fabrication under mild conditions without the use of high-temperature hydrothermal methods and toxic chemical reagents. Amyloid-mediated molecular engineering manipulates the phase transition of bovine serum albumin(BSA)on particulate waste surfaces, resulting in a remarkable ～3.1 times improvement in the adsorption capacity of fly ash, a typical industrial solid waste for gold ions after modification with the phase-transitioned BSA(PTB). The resultant adsorption ability was 69–1,980 times higher than those of conventional and emerging adsorbent materials such as ion exchange resins, activated carbon(AC), covalent organic frameworks(COFs), and metal-organic frameworks(MOFs). We further demonstrated the application of our PTB-modified materials in the recovery of precious metals from low-grade gold ore and electronic waste leachates. Consequently, this strategy could increase the value of waste materials nearly 27 times. In addition, this method is generally extendable to other conventional industrial adsorbents such as resin, clay, and Al2O3, and enhances their adsorption capabilities at least twofold. Overall, this work provides a simple and green approach for improving the adsorption performance of solid particles, and is expected to develop into a universal strategy for transforming waste particles into high-value-added products.

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Neuroprotective effects of neural stem cells pretreated with neuregulin1β on PC12 cells exposed to oxygen-glucose deprivation/reoxygenation

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Neural Regeneration Research 2023年第3期18卷 618-625页

作者： Qiu-Yue Zhai Yuan-Hua Ye Yu-Qian Ren Zhen-Hua Song Ke-Li Ge Bao-He Cheng Yun-Liang Guo Institute of Cerebrovascular Diseases Medical Research CenterThe Affiliated Hospital of Qingdao UniversityTaishan Scholars Construction Project Excellent Innovative Team of Shandong ProvinceQingdaoShandong ProvinceChina Department of Obstetrics The Affiliated Hospital of Qingdao UniversityQingdaoShandong ProvinceChina Research center of Stem Cells Shandong Haoyun International Hospital of Stem CellsJinanShandong ProvinceChina

Studies on ischemia/reperfusion(I/R)injury suggest that exogenous neural stem cells(NSCs)are ideal candidates for stem cell therapy reperfusion ***,NSCs are difficult to obtain owing to ethical *** addition,the survival,differentiation,and proliferation rates of transplanted exogenous NSCs are low,which limit their clinical *** previous study showed that neuregulin1β(NRG1β)alleviated cerebral I/R injury in *** this study,we aimed to induce human umbilical cord mesenchymal stem cells into NSCs and investigate the improvement effect and mechanism of NSCs pretreated with 10 nM NRG1βon PC12 cells injured by oxygen-glucose deprivation/reoxygenation(OGD/R).Our results found that 5 and 10 nM NRG1βpromoted the generation and proliferation of ***-culture of NSCs and PC12 cells under condition of OGD/R showed that pretreatment of NSCs with NRG1βimproved the level of reactive oxygen species,malondialdehyde,glutathione,superoxide dismutase,nicotinamide adenine dinucleotide phosphate,and nuclear factor erythroid 2-related factor 2(Nrf2)and mitochondrial damage in injured PC12 cells;these indexes are related to *** has reported that p53 and solute carrier family 7 member 11(SLC7A11)play vital roles in ferroptosis caused by cerebral I/R *** data show that the expression of p53 was increased and the level of glutathione peroxidase 4(GPX4)was decreased after RNA interference-mediated knockdown of SLC7A11 in PC12 cells,but this change was alleviated after co-culturing NSCs with damaged PC12 *** findings suggest that NSCs pretreated with NRG1βexhibited neuroprotective effects on PC12 cells subjected to OGD/R through influencing the level of ferroptosis regulated by p53/SLC7A11/GPX4 pathway.

关键词： ferroptosis p53 SLC7A11 GPX4 human umbilical cord-mesenchymal stem cells neural stem cells neuregulin1β neuroprotection oxygen-glucose deprivation/reoxygenation PC12 cell

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Usage and method of "cauterization" in Khitans people medicine based on the contents of the valuable text of medical exchanges between Iran and China called "Tanksuq-nāmeh"

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History & Philosophy of Medicine 2022年第4期4卷 16-19页

作者： Gholam Reza Bateni Persian and Arabic Language and Literature Unit International Research Center for Iranian Biomedical Scholars(IRIBS)Gorgan ***Iran

Cauterization(Perian:Dāgh/Arabic:Al-Kayy or Al-Wasm)is one of the oldest methods of treatment in most ancient cultures and medical schools;the history of these methods,with archaeological studies,is estimated to be more than a few thousand years,and this issue can determine the reason for the spread of cauterizing methods in the traditional medicine of ancient civilizations,including Iran and *** present research,as a descriptive/historical research,tries to examine the text of the manuscript of Tanksuq-nāmeh;and identify the theoretical foundations and practical methods of cauterization in Chinese and Khitans medicine,based on one of the key texts of the Ilkhanid period.(Text translated from Chinese to Persian in the 14th century AD)The results of the present study show that cauterization has a long history among the Chinese and Khitans peoples and has been performed in different ways and for different diseases.

关键词： cauterizing Khitans traditional medicine Iranian traditional medicine Chinese traditional medicine The Ilkhanid Tanksuq-nāmeh

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The power of the public purse: financing of global health partnerships and acienda setting for sustainability

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Chinese Journal of Population,Resources and Environment 2018年第3期16卷 186-196页

作者： Liliana B.Andonova Department of international Relations and Political Science Center for International Environmental Studies Graduate Institute of International and Development Studies

Public-private partnerships(PPPs) have reshaped the institutional structure of global *** have advanced collaboration on core issues such as health, clean energy, the rights of women and children, and access to infrastructure, among others. But which actors create and finance public-private partnerships in global governance to advance such objectives? What are the implications of the agency behind such collaboration for influencing the global agenda on sustainable development? While some scholars and advocacy groups see the growing role of private actors as a powershift away from public institutions, others argue that such arrangements tend to be complementary to public mandates and indeed may provide a new means for international institutions to pursue such mandates. The article probes this debate by analyzing the type of actors that finance global health partnerships, an area in which the influence of hybrid initiatives is particularly prominent. It reveals that public financing remains a core and necessary condition for the emergence and functioning of PPPs. The growing share of private financing,nonetheless, has important implications for shaping partnerships agendas and steering global health and sustainability governance. Rather than a powershift or abdication of responsibilities by the state, there is rather a tendency of deliberate diffusion of power by donors toward hybrid structures.

关键词： Public-private partnerships power global governance health sustainable development SDGs donor financing public financing global public goods club governance

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Construction of 3D porous Cu_(1.81)S/nitrogen-doped carbon frameworks for ultrafast and long-cycle life sodium-ion storage

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international Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 191-200页

作者： Chen Chen Hongyu Xue Qilin Hu Mengfan Wang Pan Shang Ziyan Liu Tao Peng Deyang Zhang Yongsong Luo Key Laboratory of Microelectronics and Energy of Henan Province Henan Joint International Research Laboratory of New Energy Storage TechnologyCollege of Physics and Electronic EngineeringXinyang Normal UniversityXinyang 464000China School of Physics and Electronic Engineering Nanyang Normal UniversityNanyang 473061China

Transition metal sulfides have great potential as anode mterials for sodium-ion batteries(SIBs)due to their high theoretical specific ***,the inferior intrinsic conductivity and large volume variation during sodiation-desodiation processes seriously affect its high-rate and long-cyde performance,unbeneficial for the application as fast-charging and long-cycling SIBs ***,the three-dimensional porous Cu_(1.81)S/nitrogen-doped carbon frameworks(Cu_(1.81)S/NC)are synthesized by the simple and facile sol-gel and annealing processes,which can accommodate the volumetric expansion of Cu_(1.81)S nanoparticles and accelerate the transmission of ions and electrons during Na^(+)insertion/extraction processes,exhibiting the excellent rate capability(250.6 mA·g^(-1)at 20.0 A·g^(-1))and outstanding cycling stability(70% capacity retention for 6000 cycles at 10.0 A·g^(-1))for ***,the Na-ion full cells coupled with Na_(3)V_(2)(PO_(4))_(3)/C cathode also demonstrate the satisfactory reversible specific capacity of 330.5 mAh·g^(-1)at 5.0 A·g^(-1)and long-cycle performance with the 86.9% capacity retention at 2.0 A·g^(-1)after 750 *** work proposes a promising way for the conversionbased metal sulfides for the applications as fast-charging sodium-ion battery anode.

关键词： copper sulfide nanoparticles porous carbon framework fast charging long-cycle performance sodium-ion full batteries

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***:A Platform for Mainstreaming Citizen Science and Open Science in Europe

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Data Intelligence 2021年第1期3卷 136-149页

作者： Katherin Wagenknecht Tim Woods Francisco García Sanz Margaret Gold Anne Bowser Simone Rüfenacht Luigi Ceccaroni Jaume Piera Technische Hochschule Wildau Hochschulring 115745 WildauGermany European Citizen Science Association Invalidenstraße 41Berlin 10115Germany Ibercivis Foundation Campus Río EbroC/Mariano Esquillor s/n Edificio I+DZaragoza 50018Spain Leiden University Rapenburg 702311 EZ LeidenThe Netherlands woodrow wilson international center for scholars 1300 Pennsylvania Ave.WashingtonDCDistrict of Columbia 20004United States Earthwatch Mayfield House256 Banbury RoadOxfordOxfordshire OX27DEUK Institut de Ciències del Mar Consejo Superior de Investigaciones CientíficasPasseig Marítim de la Barceloneta37-49Barcelona 08003Spain

Citizen Science(CS)is a prominent field of application for Open Science(OS),and the two have strong synergies,such as:advocating for the data and metadata generated through science to be made publicly available[1];supporting more equitable collaboration between different types of scientists and citizens;and facilitating knowledge transfer to a wider range of audiences[2].While primarily targeted at CS,the *** platform can also support *** of its key functions is to act as a knowledge hub to aggregate,disseminate and promote experience and know-how;for example,by profiling CS projects and collecting tools,resources and training materials relevant to both *** do this,the platform has developed an information architecture that incorporates the public participation in scientific research(PPSR)-Common Conceptual Model.This model consists of the Project Metadata Model,the Dataset Metadata Model and the Observation Data Model,which were specifically developed for CS *** implementing these,the platform will strengthen the interoperating arrangements that exist between other,similar platforms(e.g.,BioCollect and SciStarter)to ensure that CS and OS continue to grow globally in terms of participants,impact and fields of application.

关键词： Citizen Science Metadata Open Science Public participation in scientific research(PPSR)

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1000 Wh L-1 lithium-ion batteries enabled by crosslink-shrunk tough carbon encapsulated silicon microparticle anodes

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National Science Review 2021年第9期8卷 77-87页

作者： Fanqi Chen Junwei Han Debin Kong Yifei Yuan Jing Xiao Shichao Wu Dai-Ming Tang Yaqian Deng Wei Lv Jun Lu Feiyu Kang Quan-Hong Yang Nanoyang Group State Key Laboratory of Chemical Engineering School of Chemical Engineering and Technology Tianjin University Shenzhen Geim Graphene center Tsinghua Shenzhen International Graduate School Tsinghua University CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in Nanoscience National Center for Nanoscience and Technology Chemical Sciences and Engineering Division Argonne National Laboratory international center for Materials Nanoarchitectonics(WPI-MANA) National Institute for Materials Science(NIMS) Joint School of National University of Singapore and Tianjin University International Campus of Tianjin University

Microparticulate silicon（Si）, normally shelled with carbons, features higher tap density and less interfacial side reactions compared to its nanosized counterpart, showing great potential to be applied as high-energy lithium-ion battery anodes. However, localized high stress generated during fabrication and particularly,under operating, could induce cracking of carbon shells and release pulverized nanoparticles, significantly deteriorating its electrochemical performance. Here we design a strong yet ductile carbon cage from an easily processing capillary shrinkage of graphene hydrogel followed by precise tailoring of inner *** a structure, analog to the stable structure of plant cells, presents ‘imperfection-tolerance' to volume variation of irregular Si microparticles, maintaining the electrode integrity over 1000 cycles with Coulombic efficiency over 99.5%. This design enables the use of a dense and thick(3 m Ah cm–2) microparticulate Si anode with an ultra-high volumetric energy density of 1048 Wh L–1 achieved at pouch full-cell level coupled with a Li Ni0.8Co0.1Mn0.1O2cathode.

关键词： lithium-ion batteries anode silicon microparticles volumetric capacity mechanical stability

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Interface effect on structural and electronic properties of graphdiyne adsorbed on SiO_2 and h-BN substrates:A first-principles study

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Chinese Physics B 2015年第9期24卷 419-423页

作者：董宝娟杨腾王吉章张志东 Shenyang National Laboratory for Materials Science Institute of Metal Research and International Center for Materials PhysicsChinese Academy of Sciences

We use the first-principles calculation method to study the interface effect on the structure and electronic properties of graphdiyne adsorbed on the conventional substrates of rough SiO2 and flat h-BN. For the SiO2 substrate, we consider all possible surface terminations, including Si termination with dangling bond, Si terminations with full and partial hydrogenation, and oxygen terminations with dimerization and hydrogenation. We find that graphdiyne can maintain a flat geometry when absorbed on both h-BN and SiO2 substrates except for the Si termination with partial hydrogenation（Si-H） SiO2 substrate. A lack of surface corrugation in graphdiyne on the substrates, which may help maintain its electronic band character, is due to the weak Van der Waals interaction between graphdiyne and the substrate. Si-H SiO2 should be avoided in applications since a covalent type bonding between graphdiyne and SiO2 will totally vary the band structure of ***, the oxygen termination with dimerization SiO2 substrate has spontaneous p-type doping on graphdiyne via interlayer charge transfer even in the absence of extrinsic impurities in the substrate. Our result may provide a stimulus for future experiments to unveil its potential in electronic device applications.

关键词： graphdiyne electronics applications interface effect spontaneous doping

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Theoretical study of thermoelectric properties of MoS_2

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Chinese Physics B 2014年第1期23卷 367-373页

作者：郭怀红杨腾陶鹏张志东 Shenyang National Laboratory for Materials Science Institute of Metal Research and International Center for Materials Physics Chinese Academy of Sciences Shenyang 110016 China

We systematically studied the thermoelectric properties of MoS2 with doping based on the Boltzmann transport theory and first-principles calculations. We obtained an optimal doping region(around 1019cm 3) for thermoelectric properties along in-plane and cross-plane directions. MoS2in the optimal doping region has a vanishingly small anisotropy of thermopower possibly due to the decoupling of in-plane and cross-plane conduction channels, but big anisotropies of electrical conductivity σ and electronic thermal conductivity κearising from the anisotropic electronic scattering time. The κeis comparable to the lattice counterpart κlin the plane, while κldominates over κeacross the plane. The figure of merit ZT can reach 0.1 at around 700 K with in-plane direction preferred by doping.

关键词： THERMOELECTRICITY MOLYBDENUM disulfide TRANSPORT theory (Mathematics) BOLTZMANN'S equation ANISOTROPY

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A zero-sum hybrid stochastic differential game with impulse controls

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Science China(Information Sciences) 2024年第11期67卷 285-299页

作者： Siyu LV Zhen WU Jie XIONG School of Mathematics Southeast University School of Mathematics Shandong University Department of Mathematics and SUSTech international center for Mathematics Southern University of Science and Technology

In this paper, we study a zero-sum stochastic differential game with the following salient features:(i) the system state is dictated by a hybrid diffusion,(ii) both players use impulse controls, and(iii) the game takes place on an infinite time horizon. First, the dynamic programming principle for the problem is ***, the lower and upper value functions of the game are characterized as the unique viscosity solution of the associated Hamilton-Jacobi-Bellman-Isaacs(HJBI) equation, which turns out to be a coupled system of variational inequalities with bilateral obstacles. Moreover, a verification theorem as a sufficient condition to identify a Nash equilibrium is established. The Nash equilibrium strategies for the two players, indicating when and how it is optimal to intervene, are given in terms of the obstacle part of the HJBI equation.

关键词： stochastic differential game Markov chain impulse control HJBI equation viscosity solution verification theorem

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