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Energy & Environmental Materials 2024年第4期7卷 163-174页

作者： Hao Li Rui Wang Jiangping Song Dan Liu Hongyang Gao Yimin Chao Haolin Tang A State Key laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Department of Chemistry Chemical Engineering and Life Science Wuhan University of Technology Foshan Xianhu laboratory of the Advanced Energy science and Technology Guangdong laboratory School of Chemistry University of East Anglia

As the persistent concerns regarding sluggish reaction kinetics and insufficient conductivities of sulfur cathodes in all-solid-state Li-S batteries(ASSLSBs),numerous carbon additives and solid-state electrolytes (SSEs) have been incorporated into the cathode to facilitate ion/electron pathways around ***,this has resulted in a reduced capacity and decomposition of SSEs.

关键词： all-solid-state lithium–sulfur batteries conversion/intercalation high-loading and long-life low carbon content mixed ionic/electronic conductivities

Nonlinear metamaterial enabled aeroelastic vibration reduction of a supersonic cantilever wing plate

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Applied Mathematics and Mechanics(English Edition) 2024年第10期45卷 1749-1772页

作者： Peng SHENG Xin FANG Dianlong YU Jihong WEN laboratory of science and Technology on Integrated Logistics Support College of Intelligence Science and TechnologyNational University of Defense TechnologyChangsha 410073China

The violent vibration of supersonic wings threatens aircraft *** paper proposes the strongly nonlinear acoustic metamaterial(NAM)method to mitigate aeroelastic vibration in supersonic wing *** employ the cantilever plate to simulate the practical behavior of a *** aeroelastic vibration model of the NAM cantilever plate is established based on the mode superposition method and a modified third-order piston *** aerodynamic properties are systematically studied using both the timedomain integration and frequency-domain harmonic balance *** presenting the flutter and post-flutter behaviors of the NAM wing,we emphasize more on the preflutter broadband vibration that is prevalent in *** results show that the NAM method can reduce the low-frequency and broadband pre-flutter steady vibration by 50%-90%,while the post-flutter vibration is reduced by over 95%,and the critical flutter velocity is also slightly *** clarified,the significant reduction arises from the bandgap,chaotic band,and nonlinear resonances of the NAM *** reduction effect is robust across a broad range of parameters,with optimal performance achieved with only 10%attached *** work offers a novel approach for reducing aeroelastic vibration in aircraft,and it expands the study of nonlinear acoustic/elastic metamaterials.

关键词： nonlinear acoustic metamaterial(NAM) hypersonic aeroelastic vibration vibration reduction fluid-structure interaction

Polymer: Non-fullerene acceptor heterojunction-based phototransistor for short-wave infrared photodetection

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Nano Research 2024年第4期17卷 3087-3095页

作者： Jing Li Weigang Zhu Yang Han Yanhou Geng Wenping Hu Key laboratory of Organic Integrated Circuits of Ministry of Education&Key laboratory of Molecular Optoelectronic sciences School of Science&Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)Tianjin UniversityTianjin 300072China Key laboratory of Organic Integrated Circuits of Ministry of Education&Key laboratory of Molecular Optoelectronic sciences School of Materials Science and EngineeringTianjin UniversityTianjin 300072China

It remains full of challenge for extending short-wave infrared(SWIR)spectral response and weak-light detection in the context of broad spectral responses for *** this work,a novel poly(2,5-bis(4-hexyldodecyl)-2,5-dihydro-3,6-di-2-thienyl-pyrrolo[3,4-c]pyrrole-1,4-dione-alt-thiophene)(PDPPT3-HDO):COTIC-4F organic bulk-heterojunction is prepared as active layer for bulk heterojunction ***3-HDO serves as a hole transport material,while COTIC-4F enhances the absorption of SWIR light to 1020 *** a result,smooth and connected PDPPT3-HDO film is fabricated by blade coating method and exhibits high hole mobility up to 2.34 cm^(2)·V^(-1)·s^(-1) with a current on/off ratio of 4.72×10^(5) in organic thin film ***3-HDO:COTIC-4F heterojunction phototransistors exhibit high responsivity of 2680 A·W^(-1) to 900 nm and 815 A·W^(-1) to 1020 nm,with fast response time(rise time~20 ms and fall time~100 ms).The photosensitivity of the heterojunction phototransistor improves as the mass ratio of non-fullerene acceptors increases,resulting in an approximately two orders of magnitude enhancement compared to the bare polymer ***,the phototransistor exhibits decent responsivity even under ultra-weak light power of 43μW·cm^(-2) to 1020 *** work represents a highly effective and general strategy for fabricating efficient and sensitive SWIR light photodetectors.

关键词： photodetection phototransistor organic semiconductor heterojunction non-fullerene acceptor

Lens-free wavefront shaping method for a diffuse non-lineof-sight link in visible light communication

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Chinese Optics Letters 2024年第2期22卷 81-87页

作者：陈超旭周晓萌李子薇沈超张俊文施剑阳迟楠 Key laboratory for Information science of Electromagnetic Waves(MoE) Fudan UniversityShanghai 200433China Peng Cheng laboratory Shenzhen 518038China

In this Letter,we propose and experimentally demonstrate a lens-free wavefront shaping method that utilizes synchronized signal block beam alignment and a genetic algorithm(SSBGA)for a diffuse non-line-of-sight(NLOS)visible light communication(VLC)*** proposed method effectively controls the position and mobility of visible light beams by partitioning spatial light modulator pixels and manipulating beams to converge at distinct spatial positions,thereby enhancing wavefront shaping efficiency,which achieves a significant 23.9 dB optical power enhancement at+2 mm offset,surpassing the lens-based continuous sequence(CS)scheme by 21.7 ***+40°angle,the improvement reaches up to 11.8 dB and 16.8 dB compared to the results with and without lens-based CS,respectively.A maximum rate of 5.16 Gbps is successfully achieved using bit-power loading discrete multi-tone(DMT)modulation and the proposed SSBGA in an NLOS VLC system,which outperforms the lens-based CS by 1.07 Gbps and obtains a power saving of 55.6%during the transmission at4 *** the best of our knowledge,this is the first time that high-speed communication has been realized in an NLOS VLC system without a lens.

关键词： non-line-of-sight lens-free wavefront shaping visible light communication

Atomically precise Ru-O-Ru clusters for enhanced water dissociation in alkaline hydrogen evolution

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Nano Research 2024年第8期17卷 6993-7000页

作者： Dong Liu Li Xu Sicheng Li Airong Xu Yuanhua Sun Tong Liu Mengyuan Liu Huijuan Wang Xiaokang Liu Tao Yao Tao Ding Hefei National Research Center for Physical sciences at the Microscale School of Nuclear Science and TechnologyKey Laboratory of Precision and Intelligent ChemistryNational Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029China Experimental Center of Engineering and Materials science University of Science and Technology of ChinaHefei 230026China

Atomic clusters typically exhibit distinctive electronic structures and physicochemical ***,as the size decreases,their ability to adsorb and dissociate water also diminishes,thereby affecting chemical reactions involving water *** the adsorption and dissociation capabilities of atomic clusters towards water molecules and elucidating the mechanisms underlying their performance enhancement have become important research ***,employing the carrier-anchored strategy,Ru-O-Ru atomic clusters were prepared and displayed excellent activity and durability in the hydrogen evolution ***,the Ru-O-Ru atomic clusters exhibited only 86 mV overpotential at 100 mA·cm−^(2) and superior membrane-electrode-assembly activity than commercial Ru/C *** radiation-based Fourier transform infrared spectroscopic measurements revealed that the modification of oxygen in Ru-O-Ru units promoted the reorientation of water molecules from a H-up orientation to H-down,therefore,enhanced the formation of strong hydrogen-bond network of interfacial water on the surface of Ru-O-Ru clusters,leading to enhanced adsorption and dissociation of water and accelerated Volmer *** findings provide a potential strategy and deep insights for the development of atomic clusters in electrocatalysts.

关键词： hydrogen evolution in-situ Fourier transform infrared(FTIR) Ru catalysts electrocatalysis atomic clusters

Ultra-broadband microwave absorber and high-performance pressure sensor based on aramid nanofiber,polypyrrole and nickel porous aerogel

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International Journal of Minerals,Metallurgy and Materials 2024年第8期31卷 1912-1921页

作者： Leyi Zhang Hongyu Jin Hanxin Liao Rao Zhang Bochong Wang Jianyong Xiang Congpu Mu Kun Zhai Tianyu Xue Fusheng Wen State Key laboratory of Metastable Materials science&Technology Yanshan UniversityQinhuangdao 066004China Key laboratory for Microstructural Material Physics of Hebei Province School of ScienceYanshan UniversityQinhuangdao 066004China

Electronic devices have become ubiquitous in our daily lives,leading to a surge in the use of microwave absorbers and wearable sensor devices across various sectors.A prime example of this trend is the aramid nanofibers/polypyrrole/nickel(APN)aerogels,which serve dual roles as both microwave absorbers and pressure *** this work,we focused on the preparation of aramid nanofibers/polypyrrole(AP15)aerogels,where the mass ratio of aramid nanofibers to pyrrole was 1:*** employed the oxidative polymerization method for the preparation *** this,nickel was thermally evaporated onto the surface of the AP15 aerogels,resulting in the creation of an ultralight(9.35 mg·cm^(-3)).This aerogel exhibited a porous *** introduction of nickel into the aerogel aimed to enhance magnetic loss and adjust impedance matching,thereby improving electromagnetic wave absorption *** minimum reflection loss value achieved was-48.7 dB,and the maximum effective absorption bandwidth spanned 8.42 GHz with a thickness of 2.9 *** impressive metrics can be attributed to the three-dimensional network porous structure of the aerogel and perfect impedance ***,the use of aramid nanofibers and a three-dimensional hole structure endowed the APN aerogels with good insulation,flame-retardant properties,and compression *** under a compression strain of 50%,the aerogel maintained its resilience over 500 *** incorporation of polypyrrole and nickel particles further enhanced the conductivity of the ***,the final APN aerogel sensor demonstrated high sensitivity(10.78 kPa-1)and thermal *** conclusion,the APN aerogels hold significant promise as ultra-broadband microwave absorbers and pressure sensors.

关键词： porous aerogel aramid nanofibers microwave absorbers pressure sensor porous structure

Multiplayer Reach-Avoid Differential Games in 3D Space Inspired by Harris'Hawks'Cooperative Hunting Tactics

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Research 2024年第2期2023卷 41-54页

作者： Wanying Ruan Haibin Duan Yongbin Sun Wanmai Yuan Jie Xia State Key laboratory of Virtual Reality Technology and Systems School of Automation Science and Electrical EngineeringBeihang UniversityBeijingChina Peng Cheng laboratory ShenzhenChina Information science Academy of CETC BeijingChina

This paper investigates a multiplayer reach-avoid differential game in 3-dimensional(3D)space,which involves multiple pursuers,multiple evaders,and a designated target *** evaders aim to reach the target region,while the pursuers attempt to guard the target region by capturing the *** class of research holds significant practical ***,the complexity of the problem escalates substantially with the growing number of players,rendering its solution extremely *** this paper,the multiplayer game is divided into many subgames considering the cooperation among pursuers,reducing the computational burden,and obtaining numerically tractable strategies for ***,the Apollonius sphere,a fundamental geometric tool for analyzing the 3D differential game,is formulated,and its properties are *** on this,the optimal interception point for the pursuer to capture the evader is derived and the winning conditions for the pursuer and evader are ***,based on the Apollonius sphere,the optimal state feedback strategies of players are designed,and simultaneously,the optimal one-to-one pairings are ***,the Value function of the multiplayer reach-avoid differential game is explicitly given and is proved to satisfy Hamilton-Jacobi-Isaacs(HJI)***,the matching algorithm for the case with pursuers outnumbered evaders is provided through constructing a weighted bipartite graph,and the cooperative tactics for multiple pursuers are proposed,inspired by the Harris'Hawks intelligent cooperative hunting ***,numerical simulations are conducted to illustrate the effectiveness of the theoretical results for both cases where the number of adversary players is equal and unequal between the 2 groups.

关键词： holds satisfy rendering

Low-Volatile Binder Enables Thermal Shock-Resistant Thin-Film Cathodes for Thermal Batteries

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Energy & Environmental Materials 2024年第4期7卷 126-134页

作者： Yong Xie Yong Cao Xu Zhang Liangping Dong Xiaojiang Liu Yixiu Cui Chao Wang Yanhua Cui Xuyong Feng Hongfa Xiang Long Qie laboratory of Electrochemical Power Sources Institute of Electronic Engineering China Academy of Engineering Physics School of Materials science and Engineering Hefei University of Technology State Key laboratory of Material Processing and Die & Mold Technology School of Materials Science and Engineering Huazhong University of Science and Technology

Manufacturing thin-film components is crucial for achieving high-efficiency and high-power thermal batteries (TBs).However,developing binders with low-gas production at the operating temperature range of TBs (400-550℃)has proven to be a significant ***,we report the use of acrylic acid derivative terpolymer (LA136D) as a low-volatile binder for thin-film cathode fabrication and studied the chain scission and chemical bondbreaking mechanisms in pyrolysis.

关键词： gas production high-power low-volatile binder thermal battery thin-film cathode

Seasonal variation of mesoscale eddy intensity in the global ocean

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Acta Oceanologica Sinica 2024年第1期43卷 48-58页

作者： Yongcan Zu Yue Fang Shuangwen Sun Libao Gao Yang Yang Guijun Guo First Institute of Oceanography/Key laboratory of Marine science and Numerical Modeling Ministry of Natural ResourcesQingdao 266061China laboratory for Regional Oceanography and Numerical Modeling Laoshan LaboratoryQingdao 266237China Shandong Key laboratory of Marine science and Numerical Modeling Qingdao 266061China

Mesoscale eddies are a prominent oceanic phenomenon that plays an important role in oceanic mass transport and energy *** by rotational speed,the eddy intensity is one of the most fundamental properties of an ***,the seasonal spatiotemporal variation in eddy intensity has not been examined from a global ocean *** this study,we unveil the seasonal spatiotemporal characteristics of eddy intensity in the global ocean by using the latest satellite-altimetry-derived eddy trajectory data *** results suggest that the eddy intensity has a distinct seasonal variation,reaching a peak in spring while attaining a minimum in autumn in the Northern Hemisphere and the opposite in the Southern *** seasonal variation of eddy intensity is more intense in the tropical-subtropical transition zones within latitudinal bands between 15°and 30°in the western Pacific Ocean,the northwestern Atlantic Ocean,and the eastern Indian Ocean because baroclinic instability in these areas changes *** analysis found that the seasonal variation of baroclinic instability precedes the eddy intensity by a phase of 2–3 months due to the initial perturbations needing time to grow into mesoscale eddies.

关键词： seasonal variation mesoscale eddy intensity baroclinic instability global ocean

A Distributed Self-Tallying Electronic Voting System Using the Smart Contract

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Chinese Journal of Electronics 2024年第4期33卷 1063-1076页

作者： Jingyu YAO Bo YANG Tao WANG Wenzheng ZHANG School of Computer science Shaanxi Normal University State Key laboratory of Integrated Services Networks Xidian University science and Technology on Communication Security laboratory

For electronic voting(e-voting) with a trusted authority, the ballots may be discarded or tampered, so it is attractive to eliminate the dependence on the trusted party. An e-voting protocol, where the final voting result can be calculated by any entity, is known as self-tallying e-voting protocol. To the best of our knowledge, addressing both abortive issue and adaptive issue simultaneously is still an open problem in self-tallying e-voting *** Ethereum blockchain with cryptographic technologies, we present a decentralized self-tallying e-voting protocol. We solve the above problem efficiently by utilizing optimized Group Encryption Scheme and standard Exponential El Gamal Cryptosystem. We use zero-knowledge proof and homomorphic encryption to protect votes' secrecy and achieve self-tallying. All ballots can be verified by anyone and the final voting result can be calculated by any entity. In addition, using the paradigm of score voting and “1-out-of-k” proof, our e-voting system is suitable for a wide range of application scenarios. Experiments show that our protocol is more competitive and more suitable for large-scale voting.

关键词： Electronic voting systems Smart contracts Blockchains Cryptocurrency Electronic voting Homomorphic encryption Standards