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The contribution of solid-state chemistry in the determination of multicomponent phase diagrams

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Rare Metals 2006年第5期25卷 576-581页

作者： Jean Claude Tedenac Franck Gascoin Didier Ravot université montpellier 2 LPMC-UMR-CNRS-5617 MontpellierFrance

For a long period of time, the determination of phase diagrams was only supported by experiments related to thermal effects or thermodynamic measurements： thermal analysis, calorimetric measurements, vapor pressures, and EMF measurements. As a matter of fact, solid-solid transformations were not so accurately determined and could not be taken into account in the system＇s analysis. First, X-ray diffraction methods were used as a support for the thermal analysis. Second, the implementation of novel tools in structural analysis （for example, the Rietveld method） has permitted to increase the knowledge of phase stability. Finally, modeling the phases using a Calphad method needed increasingly more structural results to determine and better understand the phase diagrams. On the other hand, the Calphad method has been widely developed for metallic systems, for oxide systems, and in the past 10 years, for some semi-conductor systems, for example, gallium arsenide, cadmium telluride, and lead telluride systems. In such applications, it is very important to bring point defects in the modeling of the phases to map the defects as a function of the chemical composition. Owing to its complexity, this characteristic, the knowledge of which is crucial for the understanding and the control of potential physical applications, was ignored in the previous assessment of semi-conductor systems.

关键词： thermodynamic modeling solid-state chemistry phase diagram

Fusion of spatiotemporal and thematic features of textual data for animal disease surveillance

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Information Processing in Agriculture 2023年第3期10卷 347-360页

作者： Sarah Valentin Renaud Lancelot Mathieu Roche CIRAD F-34398 MontpellierFrance ASTRE Univ MontpellierCIRADINRAEMontpellierFrance TETIS Univ MontpellierAgroParisTechCIRADCNRSINRAEMontpellierFrance Departement de Biologie Universite de SherbrookeSherbrookeQuebecCanada

Several internet-based surveillance systems have been created to monitor the web for animal health *** systems collect a large amount of news dealing with outbreaks related to animal *** identifying news articles that describe the same outbreak event is a key step to quickly detect relevant epidemiological information while alleviating manual curation of news *** paper addresses the task of retrieving news articles that are related in epidemiological *** tackle this issue using text mining and feature fusion *** main objective of this paper is to identify a textual representation in which two articles that share the same epidemiological content are *** compared two types of representations(i.e.,features)to represent the documents:(i)morphosyntactic features(i.e.,selection and transformation of all terms from the news,based on classical textual processing steps)and(ii)lexicosemantic features(i.e.,selection,transformation and fusion of epidemiological terms including diseases,hosts,locations and dates).We compared two types of term weighing(i.e.,Boolean and TF-IDF)for both *** combine and transform lexicosemantic features,we compared two data fusion techniques(i.e.,early fusion and late fusion)and the effect of features generalisation,while evaluating the relative importance of each type of *** conducted our analysis using a corpus composed of a subset of news articles in English related to animal disease *** results showed that the combination of relevant lexicosemantic(epidemiological)features using fusion methods improves classical morphosyntactic representation in the context of disease-related news *** lexicosemantic representation based on TF-IDF and feature generalisation(F-measure=0.92,r-precision=0.58)outperformed the morphosyntactic representation(F-measure=0.89,r-precision=0.45),while reducing the features *** the features into lower granular

关键词： Animal disease surveillance Text mining Ranking Fusion

Prussian Blue Analogue‑Templated Nanocomposites for Alkali‑Ion Batteries:Progress and Perspective

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Nano-Micro Letters 2025年第1期17卷 216-261页

作者： Jian‑En Zhou Yilin Li Xiaoming Lin Jiaye Ye Key Laboratory of Theoretical Chemistry of Environment Ministry of EducationSchool of ChemistrySouth China Normal UniversityGuangzhou 510006People’s Republic of China School of Chemistry and Physics Faculty of ScienceQueensland University of Technology2 George StreetBrisbaneQLD 4000Australia Centre for Materials Science Queensland University of Technology2 George StreetBrisbaneQLD 4000Australia

Lithium-ion batteries(LIBs)have dominated the portable electronic and electrochemical energy markets since their commercialisation,whose high cost and lithium scarcity have prompted the development of other alkali-ion batteries(AIBs)including sodium-ion batteries(SIBs)and potassium-ion batteries(PIBs).Owing to larger ion sizes of Na^(+)and K^(+)compared with Li^(+),nanocomposites with excellent crystallinity orientation and well-developed porosity show unprecedented potential for advanced lithium/sodium/potassium *** enticing open rigid framework structures,Prussian blue analogues(PBAs)remain promising self-sacrificial templates for the preparation of various nanocomposites,whose appeal originates from the well-retained porous structures and exceptional electrochemical activities after thermal *** review focuses on the recent progress of PBA-derived nanocomposites from their fabrication,lithium/sodium/potassium storage mechanism,and applications in AIBs(LIBs,SIBs,and PIBs).To distinguish various PBA derivatives,the working mechanism and applications of PBA-templated metal oxides,metal chalcogenides,metal phosphides,and other nanocomposites are systematically evaluated,facilitating the establishment of a structure–activity correlation for these *** on the fruitful achievements of PBA-derived nanocomposites,perspectives for their future development are envisioned,aiming to narrow down the gap between laboratory study and industrial reality.

关键词： Prussian blue analogues Self-sacrificial template Lithium-ion batteries Sodium-ion batteries Potassium-ion batteries

The productivity of two serial chemostats

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International Journal of Biomathematics 2023年第6期16卷 57-111页

作者： Manel Dali-Youcef Tewfik Sari MISTEA L'institut Agro Montpellier INRAEUniversite Montpellier2 Place Pierra Viala F-34060 Montpellier Cedec 2France ITAP L'Institut Agro MontpellierINRAE UniversitéMontpellier361 rue Jean-Francois Breton BP 5095F-34196 Montpellier Cedea 5France

This paper considers the production of biomass of two interconnected chemostats in series with biomass mortality and a growth kinetic of the biomass described by an increasing function.A comparison is made with the productivity of a single chemostat with the same mortality rate and with volume equal to the sum of the volumes of the two *** determine the operating conditions under which the productivity of the serial configuration is greater than the productivity of the single ***,the differences and similarities in the results corresponding to the case with mortality and the one without mortality,are *** mortality leads to surprising results where the productivity of a steady state where the bacteria are washed out in the first chemostat is greater than the one where the bacteria are present in both chemostats.

关键词： Chemostat gradostat mortality bifurcations global stability operating diagram biomass productivity

Sigma-1 receptor: culprit and rescuer in motor neuron diseases

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Neural Regeneration Research 2021年第1期16卷 106-107页

作者： Jean-Charles Liévens Tangui Maurice MMDN Univ MontpellierINSERMEPHEMontpellierFrance

Initially,the Sigma-1 receptor(S1R)was incorrectly categorized as one of the opioid *** it has since become clear that S1R is a non-opioid non-phencyclidine receptor with molecular chaperone activity.S1R is a 223 amino-acid long protein that shares no clear homology with any other known mammalian proteins,its closest homolog being the fungal ERG2 sterol *** its pharmacological counterpart,the Sigma-2 receptor that was only recently cloned,is genetically distinct.S1R is more likely considered as an atypical ligand-modulated chaperone protein.S1R is widely expressed in many organs including brain where its function has mainly been explored.

关键词： organs opioid Sigma

Dust pollen distribution on a continental scale and its relation to present-day vegetation along north-south transects in east China

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Science China Earth Sciences 2007年第2期50卷 236-246页

作者： P. COUR D. DUZER G. ROBERT M. CALLEJA C. BEAUDOUIN Ecole Nationale Supérieure Agronomique de montpellier 34000 Montpellier France UMR CNRS 5554 ISEM Université Montpellier 2 34000 Montpellier France Department of Earth Sciences Sun Yat-sen University

A series of dust pollen samples was collected along N-S transects in east China (18°N to 53°N latitudes). Sample sites extend from the cold-temperate zone in the north to the tropical region in the south. Pollen taxa characterize each region and reflect the natural and devastated vegetation as well as corre- sponding climatic zones. The quantitative pollen data can be used to estimate the spatial distribution of planted and introduced species. Valuable information of human disturbance of the natural forest is evaluated by quantitative comparison between dust pollen and in-situ pollen of protected forest. In addition, percentages of grass pollen vary regularly from north to south that is consistent with spatial distribution of net primary productivity in east China. Among all grasses, Artemisia and the Gramineae carry the clearest signal: their ratio increases northwards and therefore represent a suitable and con- venient tool for palaeoclimate reconstructions.

关键词： dust pollen vegetation east China human impact climate zones

NRF2 signaling cascade in amyotrophic lateral sclerosis:bridging the gap between promise and reality

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Neural Regeneration Research 2024年第5期19卷 1006-1012页

作者： Pauline Tarot Christelle Lasbleiz Jean-Charles Liévens MMDN Univ MontpellierEPHEINSERMMontpellierFrance CNRS ParisFranceEPHEINSERMMontpellierFrance

Amyotrophic lateral sclerosis is a very disabling disease due to the degeneration of motor *** include muscle weakness and atrophy,spasticity,and progressive ***,there is no treatment to reverse damage to motor neurons and cure amyotrophic lateral *** only two treatments actually approved,riluzole and edaravone,have shown mitigated beneficial *** difficulty to find a cure lies in the complexity and multifaceted pattern of amyotrophic lateral sclerosis *** mechanisms,abnormal RNA metabolism,nucleocytoplasmic transport defects,accumulation of unfolded protein,and mitochondrial dysfunction would in fine induce oxidative damage and vice versa.A potent therapeutic strategy will be to find molecules that break this vicious *** the nuclear factor erythroid-2 related factor 2 signaling may fulfill this objective since nuclear factor erythroid-2 related factor 2 has a multitarget profile controlling antioxidant defense,mitochondrial functioning,and *** here discuss the interest of developing nuclear factor erythroid-2 related factor 2-based therapy in regard to the pathophysiological mechanisms and we provide a general overview of the attempted clinical assays in amyotrophic lateral sclerosis.

关键词： amyotrophic lateral sclerosis C9orf72 NRF2 oxidative defense oxidative stress sulforaphane superoxide dismutase 1 TDP43

Mechanics of granular column collapse in fluid at varying slope angles

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Journal of Hydrodynamics 2017年第4期29卷 529-541页

作者： K.Kumar J.-Y.Delenne K.Soga Computational Geomechanics Research Group Department of Engineering University of Cambridge IATE UMR 1208 INRA-CIRAD-Montpellier Supagro-UM2 University of Montpellier 2 Department of Civil and Environmental Engineering University of California

This paper investigates the effect of initial volume fraction on the runout characteristics of collapse of granular columns on slopes in fluid. 2-D sub-grain scale numerical simulations are performed to understand the flow dynamics of granular collapse in fluid. The discrete element method（DEM） technique is coupled with the lattice Boltzmann method（LBM）, for fluid-grain interactions, to understand the evolution of submerged granular flows. The fluid phase is simulated using multiple-relaxation-time LBM（LBM-MRT） for numerical stability. In order to simulate interconnected pore space in 2-D, a reduction in the radius of the grains（hydrodynamic radius） is assumed during LBM computations. The collapse of granular column in fluid is compared with the dry cases to understand the effect of fluid on the runout behaviour. A parametric analysis is performed to assess the influence of the granular characteristics（initial packing） on the evolution of flow and run-out distances for slope angles of 0 °, 2.5°, 5 ° and 7.5 °. The granular flow dynamics is investigated by analysing the effect of hydroplaning, water entrainment and viscous drag on the granular mass. The mechanism of energy dissipation, shape of the flow front, water entrainment and evolution of packing density is used to explain the difference in the flow characteristics of loose and dense granular column collapse in fluid.

关键词： Lattice Boltzmann method(LBM) discrete element method(DEM) granular column collapse granular flows hydroplaning water entrainment viscous drag

X-ray diffraction investigation of amorphous calcium phosphate and hydroxyapatite under ultra-high hydrostatic pressure

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International Journal of Minerals,Metallurgy and Materials 2015年第11期22卷 1225-1231页

作者： Elisa Lam Qinfen Gu Peter J.Swedlund Sylvie Marchesseau Yacine Hemar School of Chemical Sciences The University of Auckland Australian Synchrotron université montpellier 2 UMR IATE Pl.E Bataillon34095 Montpellier cedex 5 France

The changes in the crystal structures of synthetically prepared amorphous calcium phosphate（ACP） and hydroxyapatite（HAP） in water（1：1 mass ratio） were studied by synchrotron X-ray diffraction（XRD） under ultra-high hydrostatic pressures as high as 2.34 GPa for ACP and 4 GPa for HAP. At ambient pressure, the XRD patterns of the ACP and HAP samples in capillary tubes and their environmental scanning electron micrographs indicated amorphous and crystalline characteristics for ACP and HAP, respectively. At pressures greater than 0.25 GPa, an additional broad peak was observed in the XRD pattern of the ACP phase, indicating a partial phase transition from an amorphous phase to a new high-pressure amorphous phase. The peak areas and positions of the ACP phase, as obtained through fitting of the experimental data, indicated that the ACP exhibited increased pseudo-crystalline behavior at pressures greater than 0.96 GPa. Conversely, no structural changes were observed for the HAP phase up to the highest applied pressure of 4 GPa. For HAP, a unit-cell reduction during compression was evidenced by a reduction in both refined lattice parameters a and c. Both ACP and HAP reverted to their original structures when the pressure was fully released to ambient pressure.

关键词： calcium phosphate hydroxyapatite high hydrostatic pressure X-ray diffraction