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Efficient and Stable Inverted Perovskite Solar Modules Enabled by Solid-Liquid Two-Step Film Formation

Nano-Micro Letters 2024年第9期16卷 571-582页

作者： Juan Zhang Xiaofei Ji Xiaoting Wang Liujiang Zhang Leyu Bi Zhenhuang Su Xingyu Gao Wenjun Zhang Lei Shi Guoqing Guan Abuliti Abudula Xiaogang Hao Liyou Yang Qiang Fu Alex K.‑Y.Jen Linfeng Lu graduate School of Science and Technology Hirosaki University3‑BunkyochoHirosaki 036‑8561Japan Department of Materials Science and Engineering Department of ChemistryHong Kong Institute for Clean EnergyCity University of Hong Kong KowloonHong Kong 999077People’s Republic of China The Interdisciplinary Research Center Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201210People’s Republic of China Shanghai Synchrotron Radiation Facility(SSRF) Zhangjiang LabShanghai Advanced Research InstituteChinese Academy of SciencesShanghai201204People’s Republic of China JINNENG Clean Energy Technology Ltd. Jinzhong 030300ShanxiPeople’s Republic of China Hangzhou Zhongneng Photoelectricity Technology Co. Ltd.Hangzhou 310018People’s Republic of China College of Chemical Engineering and Technology Taiyuan University of TechnologyTaiyuan 030024People’s Republic of China Institute of Regional Innovation Hirosaki University3‑BunkyochoHirosaki 036‑8561Japan

A considerable efficiency gap exists between large-area perovskite solar modules and small-area perovskite solar *** control of forming uniform and large-area film and perovskite crystallization is still the main obstacle restricting the efficiency of *** this work,we adopted a solid-liquid two-step film formation technique,which involved the evaporation of a lead iodide film and blade coating of an organic ammonium halide solution to prepare perovskite *** method possesses the advantages of integrating vapor deposition and solution methods,which could apply to substrates with different roughness and avoid using toxic solvents to achieve a more uniform,large-area perovskite ***,modification of the NiO_(x)/perovskite buried interface and introduction of Urea additives were utilized to reduce interface recombination and regulate perovskite *** a result,a large-area perovskite film possessing larger grains,fewer pinholes,and reduced defects could be *** inverted PSM with an active area of 61.56 cm^(2)(10×10 cm^(2)substrate)achieved a champion power conversion efficiency of 20.56%and significantly improved *** method suggests an innovative approach to resolving the uniformity issue associated with large-area film fabrication.

关键词： Inverted perovskite solar cells Perovskite solar modules Two-step film formation Crystallization Defect passivation

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Decomposition of dynamic transcriptomic responses during effector-triggered immunity reveals conserved responses in two distinct plant cell populations

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Plant Communications 2024年第8期5卷 1-17页

作者： Xiaotong Liu Daisuke Igarashi Rachel A.Hillmer Thomas Stoddard You Lu Kenichi Tsuda Chad L.Myers Fumiaki Katagiri Department of Plant and Microbial Biology University of Minnesota-Twin CitiesSt PaulMN 55108USA Department of Computer Science and Engineering University of Minnesota-Twin CitiesMinneapolisMN 55455USA Bioinformatics and Computational Biology graduate Program University of Minnesota-Twin CitiesMinneapolisMN 55455USA Institute for Innovation Ajinomoto Co.Inc.KawasakiJapan State Key laboratory of Agricultural Microbiology Hubei Hongshan LaboratoryHubei Key Lab of Plant PathologyCollege of Plant Science and TechnologyHuazhong Agricultural UniversityWuhan 430070China Present address:225 S 6th St MinneapolisMN 55402USA Present address:Biotalys Inc.2520 Meridian Parkway Suite 480DurhamNC 27713USA Present address:Life Sciences Institute and Department of Cell and Developmental Biology University of Michigan Medical SchoolAnn ArborMI 48109USA

Rapid plant immune responses in the appropriate cells are needed for effective defense against *** transcriptome analysis is often used to describe overall immune responses,collection of transcriptome data with sufficient resolution in both space and time is *** reanalyzed public Arabidopsis time-course transcriptome data obtained after low-dose inoculation with a Pseudomonas syringae strain expressing the effector AvrRpt2,which induces effector-triggered immunity in ***-peak time-course patterns are prevalent among thousands of upregulated *** implemented a multicompartment modeling approach to decompose the double-peak pattern into two single-peak patterns for each *** decomposed peaks reveal an“echoing”pattern:the peak times of the first and second peaks correlate well across most upregulated *** demonstrated that the two peaks likely represent responses of two distinct cell populations that respond either cell autonomously or indirectly to ***,the peak decomposition has extracted spatial information from the time-course *** echoing pattern also indicates a conserved transcriptome response with different initiation times between the two cell populations despite different elicitor types.A gene set highly overlapping with the conserved gene set is also upregulated with similar kinetics during pattern-triggered *** of a WRKY network via different entry-point WRKYs can explain the similar but not identical transcriptome responses elicited by different elicitor *** discuss potential benefits of the properties of the WRKY activation network as an immune signaling network in light of pressure from rapidly evolving pathogens.

关键词： Arabidopsis Pseudomonas syringae plant immune response multi-compartment model WRKY transcription factors resilient immune signaling network

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Heterointerface engineering of rhombic Rh nanosheets confined on MXene for efficient methanol oxidation

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Journal of Energy Chemistry 2024年第6期93卷 419-428,I0011页

作者： Qi Zhang Quanguo Jiang Xiang Yang Chi Zhang Jian Zhang Lu Yang Haiyan He Guobing Ying Huajie Huang College of Materials Science and Engineering Hohai UniversityNanjing 210098JiangsuChina New Energy Technology Engineering lab of Jiangsu Province College of ScienceNanjing University of Posts&Telecommunications(NUPT)Nanjing 210023JiangsuChina School of Materials Science and Engineering Southeast UniversityNanjing 211100JiangsuChina

Although metallic rhodium(Rh)is regarded as a promising platinum-alternative anode catalyst of direct methanol fuel cell(DMFC),the conventional"particle-to-face"contact model between Rh and matrix largely limits the overall electrocatalytic performance due to their insufficient cooperative ***,we report a controllable and robust heterointerface engineering strategy for the bottom-up fabrication of rhombic Rh nanosheets in situ confined on Ti_3C_(2)T_x MXene nanolamellas(Rh NS/MXene)via a convenient stereoassembly *** unique design concept gives the resulting 2D/2D Rh NS/MXene heterostructure intriguing textural features,including large accessible surface areas,strong"face-toface"interfacial interactions,homogeneous Rh nanosheet distribution,ameliorative electronic structure,and high electronic *** a consequence,the as-prepared Rh NS/MXene nanoarchitectures exhibit exceptional electrocatalytic methanol oxidation properties in terms of a large electrochemically active surface area of 126.2 m~2 g_(Rh)~(-1),a high mass activity of 1056.9 mA mg_(Rh)-~1,and a long service life,which significantly outperform those of conventional particle-shaped Rh catalysts supported by carbon black,carbon nanotubes,reduced graphene oxide,and MXene matrixes as well as the commercial Pt nanoparticle/carbon black and Pd nanoparticle/carbon black catalysts with the same noble metal loading *** functional theory calculations further demonstrate that the direct electronic interaction at the well-contacted 2D/2D heterointerfaces effectively enhances the adsorption energy of Rh nanosheets and induces a left shift of the d-band center,thereby making the Rh NS/MXene configuration suffer less from CO *** work highlights the importance of rational heterointerface design in the construction of advanced noble metal/MXene electrocatalysts,which may provide new avenues for developing the next-generation DMFC devices.

关键词： Rhodium nanosheet Ti_(3)C_(2)T_(x)MXene Heterointerface Electrocatalyst Fuel cell

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INFLUENCE OF DIALKYLZINC IN RARE-EARTH TERNARY CATALYST ONTHE COPOLYMERIZATION OF CARBON DIOXIDE AND PROPYLENE OXIDE

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Chinese Journal of Polymer Science 2005年第6期23卷 671-674页

作者： Dong Xie Xian-hong Wang Xiao-jiang Zhao and Fo-song Wang Polymer Material Engineering lab,Changchun Institute of Applied Chemistry,graduate School of Chinese Academy of Sciences,Changchun 130022,China Polymer Material Engineering lab Changchun Institute of Applied Chemistry Graduate School of Chinese Academy of Sciences Changchun 130022 China

Rare-earth ternary catalysts Y（CCl3COO）3-ZnR2-glycerin were prepared for the copolymerization of carbon dioxide and propylene oxide （PO）, where dialkylzincs （ZnR2） were diethylzinc, di（n-propyl）zinc, di（n-butyl）zinc, di（i-propyl）zinc, di（i-butyl）zinc, di（s-butyl）zinc,respectively. The Y（CCl3COO）3-ZnR2-glycerin catalysts displayed the highest catalytic activity at the molar ratio of Y（CCl3COO）3：ZnR2：glycerin = 1：20：10. In the same copolymerization condition, catalysts containing dialkylzincs with branched alkyl group showed lower catalytic activity than that with primary alkyl group. For those catalysts including dialkylzincs with primary alkyl group, their catalytic activity decreases with increasing number of carbon atom in the alkyl group with the following sequence： Y（CCl3COO）3-ZnEt2-glycerin 〉 Y（CCl3COO）3-Zn（n- Pr）2-glycerin〉Y（CCl3COO）3-Zn（n-Bu）2-glycerin. However, the alkyl group in the dialkylzinc does not influence the insertion of PO into the propagation chain end.

关键词： Carbon dioxide Propylene oxide Copolymerization Dialkylzinc

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Debonding Patch Detection in FRP-Strengthened Materials with Fiber-Optic Interferometer

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Transactions of Nanjing University of Aeronautics and Astronautics 2017年第3期34卷 255-264页

作者： Xu Ying Wang Dexiang Tang Tianyou Lu Miaomiao Shenzhen Key lab of Urban & Civil Engineering Disaster Prevention & Reduction Harbin Institute of Technology Shenzhen Graduate School

The interfacial debonding in fiber-reinforced plastic(FRP)strengthened repair material will affect the bonding strength and lead to failure of the repair without *** the interfacial damage is normally invisible and often in the form of a patch rather than a through-width ***,a debonding patch detection technique based on fiber optic interferometry is proposed.A quasi-impulse loading is applied with a rubberhead hammer and the total elongation of a surface-mounted optical fiber along the length of the repair material is measured as a function of load *** a debonding patch is present,the induced sudden slope or sign change on the plot of fiber integral strain *** position will reveal the extent and the location of the debonded *** results of the study indicate that the proposed technique is applicable for debonding patch detection in repaired members under various support conditions.

关键词： patch Patch repair hammer interfacial sudden impulse elongation optic interferometry

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Electrical stimulation with polypyrrole-coated polycaprolactone/silk fibroin scaffold promotes sacral nerve regeneration by modulating macrophage polarisation

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Biomaterials Translational 2024年第2期5卷 157-174页

作者： Haofeng Cheng Jun Bai Xingyu Zhou Nantian Chen Qingyu Jiang Zhiqi Ren Xiangling Li Tianqi Su Lijing Liang Wenli Jiang Yu Wang Jiang Peng Aijia Shang School of Medicine Nankai UniversityTianjinChina Department of Neurosurgery Chinese PLA General HospitalBeijingChina Institute of Orthopedics Chinese PLA General HospitalBeijing Key Lab of Regenerative Medicine in OrthopedicsKey Laboratory of Musculoskeletal Trauma&War Injuries PLABeijingChina Co-innovation Center of Neuroregeneration Nantong UniversityNantongJiangsu ProvinceChina graduate School of Chinese PLA General Hospital BeijingChina Department of Ultrasound Chinese PLA General HospitalBeijingChina

Peripheral nerve injury poses a great threat to neurosurgery and limits the regenerative potential of sacral nerves in the neurogenic *** remains unknown whether electrical stimulation can facilitate sacral nerve regeneration in addition to modulate bladder *** objective of this study was to utilise electrical stimulation in sacra nerve crush injury with newly constructed electroconductive scaffold and explore the role of macrophages in electrical stimulation with crushed *** a result,we generated a polypyrrole-coated polycaprolactone/silk fibroin scaffold through which we applied electrical *** electrical stimulation boosted nerve regeneration and polarised the macrophages towards the M2 *** in vitro test using bone marrow derived macrophages revealed that the pro-regenerative polarisation of M2 were significantly enhanced by electrical *** analysis showed that the expression of signal transducer and activator of transcriptions(STATs)was differentially regulated in a way that promoted M2-related genes *** work indicated the feasibility of electricals stimulation used for sacral nerve regeneration and provided a firm demonstration of a pivotal role which macrophages played in electrical stimulation.

关键词： electrical stimulation JAK-STAT signalling pathway macrophage polarisation peripheral nerve regeneration polypyrrole sacral nerve injury

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Effect of water vapor on NH_3–NO/NO_2 SCR performance of fresh and aged MnO_x–NbO_x–CeO_2 catalysts

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Journal of Environmental Sciences 2015年第5期27卷 240-247页

作者： Lei Chen Zhichun Si Xiaodong Wu Duan Weng Zhenwei Wu State Key lab of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University graduate School at Shenzhen Tsinghua University

A MnOx-NbOx-CeO2 catalyst for low temperature selective catalytic reduction（SCR） of NOx with NH3 was prepared by a sol-gel method, and characterized by NH3-NO/NO2 SCR catalytic activity, NO/NH3 oxidation activity, NOx/NH3 TPD, XRD, BET, H2-TPR and in-situ Diffuse Reflectance Infrared Fourier Transform Spectroscopy（DRIFTS）. The results indicate that the Mn Ox-Nb Ox-CeO2 catalyst shows excellent low temperature NH3-SCR activity in the temperature range of 150-300℃. Water vapor inhibits the low temperature activity of the catalyst in standard SCR due to the inhibition of NOx adsorption. As the NO2 content increases in the feed, water vapor does not affect the activity in NO2 SCR. Meanwhile, water vapor significantly enhances the N2 selectivity of the fresh and the aged catalysts due to its inhibition of the decomposition of NH4NO3 into N2O.

关键词： Water effect MnOx-NbOx-CeO2 catalysts Acid sites Fast SCR reaction NO/NO2 ratio

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Existence of 3-round zero-knowledge proof systems for NP

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Science in China(Series F) 2008年第3期51卷 273-282页

作者： LI HongDat LI Bao State Key lab of Information Security Graduate University of Chinese Academy of Sciences Beijing 100049China

This paper considers the existence of 3-round zero-knowledge proof systems for NP. Whether there exist 3-round non-black-box zero-knowledge proof systems for NP language is an open problem. By introducing a new interactive proof model, we construct a 3-round zero-knowledge proof system for graph 3-coloring under standard assumptions. Our protocol is a non-black-box zero-knowledge proof because we adopt a special strategy to prove the zero-knowledge property. Consequently, our construction shows the existence of 3-round non-black-box zero-knowledge proof for all languages in NP under the DDH assumption.

关键词： interactive proof zero-knowledge proof non-black-box simulation DDH assumption

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High-sensitivity formaldehyde gas sensor based on Ce-doped urchin-like SnO_(2) nanowires derived from calcination of Sn-MOFs

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Frontiers of Materials Science 2024年第1期18卷 29-43页

作者： Wei Xiao Wei Yang Shantang Liu Hubei Key lab of Novel Reactor&Green Chemical Technology School of Chemistry and Environmental EngineeringWuhan Institute of TechnologyWuhan 430073China Hubei Key laboratory of Wudang Local Chinese Medicine Research Department of ChemistrySchool of Pharmaceutical SciencesHubei University of MedicineShiyan 442000China

Metal-organic frameworks(MOFs)have attracted widespread attention due to their regular structures,multiple material centers,and various *** are always considered as one kind of ideal templates for developing highly sensitive and selective gas *** this study,the advantages of MOFs with the high specific surface area(71.9891 m^(2)·g^(-1))and uniform morphology were fully utilized,and urchin-like SnO_(2) nanowires were obtained by the hydrothermal method followed by the calcination using Sn-MOFs consisting of the ligand of C_(9)H_(6)O_(6)(H_(3)BTC)and Sn/Ce center ions as sacrificial *** unique urchin-like nanowire structure facilitated gas diffusion and adsorption,resulting in superior gas sensitivity.A series of Ce-doped SnO_(2) nanowires with different doping ratios were synthesized,and their gas sensing properties towards formaldehyde were *** resulted Ce-SnO_(2) was revealed to have high sensitivity(201.2 at 250℃),rapid response(4 s),long-term stability,and good repeatability for formaldehyde sensing,and the gas sensing mechanism of Ce-SnO_(2) exposed to formaldehyde was also systematically discussed.

关键词： Ce-SnO_(2) SnO_(2) gas sensor formaldehyde Sn-MOF

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PRECISE SYNTHESIS OF OLEFIN BLOCK COPOLYMERS USING A SYNDIOSPECIFIC LIVING POLYMERIZATION SYSTEM

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Chinese Journal of Polymer Science 2013年第4期31卷 541-549页

作者：蔡正国 Hai-hui Su Takeshi Shiono State Key lab for Modification of Chemical Fibers and Polymer Materials College of Material Science and EngineeringDonghua University graduate School of Engineering Hiroshima University

This feature article summarizes the synthesis of novel olefin block copolymers using fast syndiospecific living homo- and copolymerization of propylene, higher 1-alkene, and norbornene with ansa-fluorenylamidodimethyltitanium- based catalyst according to the authors＇ recent results. The catalytic synthesis of monodisperse polyolefin and olefin block copolymer was also described using this living system.

关键词： Single-site catalyst Propylene Norbomene Living polymerization Block copolymer.

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