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Mechanistic insight into the synergy between nickel single atoms and nanoparticles on N-doped carbon for electroreduction of CO2

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Journal of energy Chemistry 2025年第1期100卷 327-336页

作者： Mingdong Sun Wenwen Guan Cailing Chen Chao Wu Xiaoling Liu Biao Meng Tao Chen Yu Han Jun Wang Shibo Xi Yu Zhou State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Advanced Membranes and Porous Materials Center Physical Sciences and Engineering Division King Abdullah University of Science and Technology institute of Sustainability for Chemicals Energy and Environment A*STAR (Agency for Science Technology and Research) College of Materials Science and Engineering Sichuan University

The synergy of single atoms （SAs） and nanoparticles （NPs） has demonstrated great potential in promoting the electrocatalytic carbon dioxide reduction reaction （CO2RR）;however,the rationalization of the SAs/NPs proportion remains one challenge for the catalyst ***,a Ni2+-loaded porous poly（ionic liquids）(PIL) precursor synthesized through the free radical self-polymerization of the ionic liquid monomer,1-allyl-3-vinylimidazolium chloride,was pyrolyzed to prepare the Ni,N co-doped carbon materials,in which the proportion of Ni SAs and NPs could be facilely modulated by controlling the annealing *** catalyst Ni-NC-1000 with a moderate proportion of Ni SAs and NPs exhibited high efficiency in the electrocatalytic conversion of CO2into *** Ni K-edge X-ray absorption near-edge structure （XANES） spectra and theoretical calculations were conducted to gain insight into the synergy of Ni SAs and *** charge transfer from Ni NPs to the surrounding carbon layer and then to the Ni SAs resulted in the electron-enriched Ni SAs active *** the electroreduction of CO2,the coexistence of Ni SAs and NPs strengthened the CO2activation and the affinity towards the key intermediate of*COOH,lowering the free energy for the potential-determining*CO2→*COOH step,and therefore promoted the catalysis efficiency.

关键词： Single atom catalyst Synergy effect Carbon catalyst Electrocatalysis

A modular parallelization framework for power flow transfer analysis of large-scale power systems

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Journal of Modern Power Systems and Clean energy 2018年第4期6卷 679-690页

作者： Chuntian CHENG Bin LUO Jianjian SHEN Shengli LIAO institute of Hydropower System and Hydroinformatics Dalian University of Technology tsinghua sichuan energy internet research institute

Power flow transfer(PFT) analysis under various anticipated faults in advance is important for securing power system operations. In China, PSD-BPA software is the most widely used tool for power system analysis, but its input/output interface is easily adapted for PFT analysis,which is also difficult due to its computationally *** solve this issue, and achieve a fast and accurate PFT analysis, a modular parallelization framework is developed in this paper. Two major contributions are included. One is several integrated PFT analysis modules, including parameter initialization, fault setting, network integrity detection, reasonableness identification and result *** other is a parallelization technique for enhancing computation efficiency using a Fork/Join framework. The proposed framework has been tested and validated by the IEEE 39 bus reference power system. Furthermore, it has been applied to a practical power network with 11052 buses and 12487 branches in the Yunnan Power Grid ofChina, providing decision support for large-scale power system analysis.

关键词： Power flow transfer Modular Parallelization Fork/Join framework PSD-BPA

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Record-breaking bifunctional oxygen electrocatalyst accomplished by a data-driven approach for zinc-air batteries

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Journal of energy Chemistry 2025年第1期100卷 144-145页

作者： Deviprasath Chinnadurai Zhi Wei Seh institute of Materials research and Engineering (IMRE) Agency for Science Technology and Research (A*STAR)

Rechargeable zinc-air batteries(ZABs) have recently drawn great attention in energy research due to their high theoretical capacity,low costs, and inherently safe nature [1–3]. However, the sluggish cathode reactions necessitate the development of bifunctional oxygen electrocatalysts with lower ΔE indicator values. The ΔE indicator is commonly employed to quantitatively evaluate the electrocatalytic activity of a bifunctional oxygen electrocatalyst,representing the overall overpotential from oxygen reduction reaction(ORR) to oxygen evolution reaction(OER).

关键词： Data-driven approach Bifunctional oxygen electrocatalyst Record breaking performance Zinc-air batteries

Three-dimensional fracture of UO2 ceramic pellets by phase field modeling

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 169-180页

作者： Wei Xiong Xuan Ye Hongzhang Cheng Xiaoming Liu institute of Nuclear and New energy Technology Collaborative Innovation Center of Advanced Nuclear Energy Technology Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education Tsinghua University State Key Laboratory of Nonlinear Mechanics Institute of Mechanics Chinese Academy of Sciences School of Engineering Science University of Chinese Academy of Sciences

Fracture is the primary failure type for the UO2ceramic pellets,which are operated under irradiation and thermal processes,and physically confined by the *** this work,by combining closely coupled physical processes of heat conduction,heat transfer,and mechanical deformation with the cohesive phase field framework,we proposed a high-precision modeling of quasistatic cracking of three-dimensional （3D） UO2ceramic fuel pellets under high temperature and *** simulation results agree well with the experimental results,indicating that the proposed method has the potential to capture 3D crack modes in the interested time ***,we studied the relation of the 3D fracture patterns of fuel pellets with the peak power *** was found that the power level plays a critical role in determining the competition between radial and circumferential cracks,as well as transverse penetrating cracks.

关键词： phase field method nuclear fuel pellet coupled thermo-mechanical model thermal fracture

Value Evaluation Method for Pumped Storage in the New Power System

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Chinese Journal of Electrical Engineering 2023年第3期9卷 26-38页

作者： Yumin Peng Ying Yang Man Chen Xuelin Wang Yijun Xiong Mu Wang Yikai Li Bushi Zhao CSG PGC Power Storage research institute Guangzhou 510635China sichuan energy internet research institute Tsinghua UniversityChengdu 610213China

When integrating the generation of large-scale renewable energy,such as wind and solar energy,the supply and demand sides of the new power system will exhibit high *** storage power stations can improve flexible resource supply regulation in the power system,which is the key support and important guarantee for building low-carbon,safe,and efficient new power *** by the current operation mode and electricity price mechanism,the pumped storage power station cost cannot be effectively recovered,and the value cannot be reasonably compensated,resulting in difficult return on investment,single investment subjects,and notable industry development *** to the operational requirements of the new power system,combined with the various functions of pumped storage power stations,the value of pumped storage power stations in the new power system was *** on the equivalent value substitution principle and system operation simulation,a pumped storage value evaluation method for the new power system was *** new power system operation was simulated considering the dispatching model of wind and photovoltaic power abandonment *** the same dispatching objectives,the output of various power sources and power generation operating costs with and without pumped storage power stations in the system were *** economic,safety,social,and environmental benefit perspectives,a quantitative model of the pumped storage power station value was established,covering seven dimensions:asset investment savings,power generation operating cost reduction,flexible adjustment capability improvement,system resilience enhancement,power outage loss reduction,renewable energy consumption,and emission reduction *** on the new power system operation and planning data for southern China,the value of typical pumped storage power stations was analyzed,and the results showed that with new power system’s construction and dev

关键词： Pumped storage new power system evaluation method value substitution operation simulation

Multi-layer multi-pass friction rolling additive manufacturing of Al alloy:Toward complex large-scale high-performance components

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 425-438页

作者： Haibin Liu Run Hou Chenghao Wu Ruishan Xie Shujun Chen College of Mechanical&energy Engineering Beijing University of TechnologyBeijing 100124China Chongqing research institute of Beijing University of Technology Chongqing 401121China

At present,the emerging solid-phase friction-based additive manufacturing technology,including friction rolling additive man-ufacturing(FRAM),can only manufacture simple single-pass *** this study,multi-layer multi-pass FRAM-deposited alumin-um alloy samples were successfully prepared using a non-shoulder tool *** material flow behavior and microstructure of the over-lapped zone between adjacent layers and passes during multi-layer multi-pass FRAM deposition were studied using the hybrid 6061 and 5052 aluminum *** results showed that a mechanical interlocking structure was formed between the adjacent layers and the adja-cent passes in the overlapped center *** friction and rolling of the tool head led to different degrees of lateral flow and plastic deformation of the materials in the overlapped zone,which made the recrystallization degree in the left and right edge zones of the over-lapped zone the highest,followed by the overlapped center zone and the non-overlapped *** tensile strength of the overlapped zone exceeded 90%of that of the single-pass deposition *** is proved that although there are uneven grooves on the surface of the over-lapping area during multi-layer and multi-pass deposition,they can be filled by the flow of materials during the deposition of the next lay-er,thus ensuring the dense microstructure and excellent mechanical properties of the overlapping *** multi-layer multi-pass FRAM deposition overcomes the limitation of deposition width and lays the foundation for the future deposition of large-scale high-performance components.

关键词： aluminum alloy additive manufacturing solid-state friction stir welding multi-layer multi-pass

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research of simulation and experiment on arc characteristics of gas mechanical switch

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High Voltage 2024年第3期9卷 626-635页

作者： Cheng Jiang Lu Qu Zhangqing Yu Zhizheng Gan Xin yan Rong Zeng Yulong Huang Shaofu Li Department of Electrical Engineering Tsinghua UniversityBeijingChina School of Information Engineering Southwest University of Science and TechnologyMianyangChina sichuan energy internet research institute Tsinghua UniversityChengduChina

An arc is the high-temperature discharge plasma produced in the opening process of mechanical switches,which directly affects the breaking capability of a hybrid DC circuit *** to the physical mechanism of an electric arc,the construction of an arc model for simulation analysis is an important technical means in the electrical *** this study,based on the theory of magneto hydrodynamics(MHD),a gas mechanical switch model of a natural commutation DC circuit breaker with a compound gap is *** arc motion process under different conditions is simulated and *** influence of different initial pressures,different opening speeds,and different striking currents on the arc voltage characteristics is *** results show that the larger the gas pressure,the smaller the arc volume and the higher the arc *** faster the opening speed,the longer the arc and the higher the arc voltage;with the increase of the current,the arc voltage increases rapidly at a low current,while the arc voltage increases slowly at a high current.

关键词： characteristics striking slowly

Investigation of sensitivity of the ultra-high frequency partial-discharge detection technology for micro-crack in epoxy insulator in GIS

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High Voltage 2020年第6期5卷 697-703页

作者： Jiangrong Cheng Yang Xu Dengwei Ding Weidong Liu Department of Electrical Engineering Tsinghua UniversityBeijingPeople's Republic of China sichuan energy internet research institute Tsinghua UniversityChengduPeople's Republic of China

The ultra-high frequency(UHF)method has been widely used in a gas-insulated system(GIS)for partial-discharge detection,and many achievements have been *** addition,many studies based on artificial defects have been made to confirm its ***,the UHF method is generally believed to be sufficiently effective for GIS ***,in practical application,the authors find that for some micro-crack discharge in GIS insulator,the UHF method has low *** fully study the characteristics of the micro-crack discharge in the GIS insulator,an experiment is conducted in this study using an actual post insulator with a micro-crack *** current signal based on IEC 60270 standard and the radio-frequency electromagnetic signal is simultaneously measured for thorough *** results show that some submillimetre crack defects may occur in the GIS *** discharge is mainly presented as glow discharge,and the discharge signal frequency usually cannot reach the UHF band;thus,it cannot be effectively detected by the UHF *** study provides complementary information to the applicability of the UHF method and inspires further study of the GIS insulator and its monitoring technology.

关键词： insulator crack high

A surface engineering strategy for the stabilization of zinc metal anodes with montmorillonite layers toward long-life rechargeable aqueous zinc ion batteries

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Journal of energy Chemistry 2025年第1期100卷 94-105页

作者： Wenbo Wang Ruifeng Xu Xu Zhang Peiyu Wang Bao Yang Bingjun Yang Juan Yang Kailimai Su Pengjun Ma Yanan Deng Xianfeng Fan Wanjun Chen Key Laboratory for Electronic Materials College of Electrical Engineering Northwest Minzu University Resource Chemistry and energy Materials research Center State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical Physics Chinese Academy of Sciences University of Chinese Academy of Sciences institute for Materials and Processes School of Engineering University of Edinburgh

Rechargeable aqueous zinc-ion batteries （AZIBs） exhibit appreciable potential in the domain of electrochemical energy ***,there are serious challenges for AZIBs,for instance zinc dendrite growth,hydrogen evolution reaction （HER）,and corrosion side ***,we propose a surface engineering modification strategy for coating the montmorillonite （MMT） layer onto the surface of the Zn anode to tackle these issues,thereby achieving high cycling stability for rechargeable *** results reveal that the MMT layer on the surface of the Zn anode is able to provide ordered zincophilic channels for zinc ions migration,facilitating the reaction kinetics of zinc *** functional theory（DFT） calculations and water contact angle （CA） tests prove that MMT@Zn anode exhibits superior adsorption capacity for Zn2+and better hydrophobicity than the bare Zn anode,thereby achieving excellent cycling ***,the MMT@Zn||MMT@Zn symmetric cell holds the stable cycling over 5600 h at 0.5 mA cm-2and 0.125 m A h cm-2,even exceeding 1800 h long cycling under harsh conditions of 5 m A cm-2and 1.25 m A h *** MMT@Zn||V2O5full cell reaches over 3000 cycles at 2 A g-1with excellent rate ***,this surface engineering modification strategy for enhancing the electrochemical performance of AZIBs represents a promising application.

关键词： Surface engineering strategy Montmorillonite layer Protection mechanism of Zn anode Cycling stability Aqueous zinc ion batteries