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Constructing porous ZnFC-PA/PSF composite spheres for highly efficient Cs^(+) removal

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Journal of Environmental Sciences 2024年第9期143卷 126-137页

作者： Senjian Han Chao Gao Wenfeng Yan Yafei Guo Shiqiang Wang Tianlong Deng college of Marine and Environmental Sciences Tianjin University of Science and TechnologyTianjin 300457China Key Laboratory of Marine Resource Chemistry and Food Technology Ministry of EducationTianjin 300457China

Radioisotope leaking from nuclear waste has become an intractable problem due to its gamma radiation and strong water solubility.In this work,a novel porous ZnFC-PA/PSF composite sphere was fabricated by immobilization of ferrocyanides modified zinc phytate into polysulfone(PSF)substrate for the treatment of Cs-contaminated water.The maximum adsorption capacity of ZnFC-PA/PSF was 305.38 mg/g,and the removal efficiency of Cs+was reached 94.27%within 2 hr.The ZnFC-PA/PSF presented favorable stability with negligible dissolution loss of Zn^(2+)and Fe^(2+)(<2%).The ZnFC-PA/PSF achieved high-selectivity towards Cs+(K_(d)=2.24×10^(4)mL/g)even in actual geothermal water.The adsorption mechanism was inferred to be the ion-exchange between Cs^(+)and K^(+).What’s more,ZnFC-PA/PSF worked well in the fixed-bed adsorption(E=91.92%),indicating the application potential for the hazardous Cs^(+)removal from wastewater.

关键词： Adsorption Cesium Metal ferrocyanide Composite adsorbent

Synthesis of Anti-Pancreatic Cancer Natural Product Majusculamide D and Analogues Reveals a Preliminary Structure-Activity Relationships

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Chinese Journal of Chemistry 2024年第6期42卷 605-610页

作者： Xiuhe Zhao Mengxue Lv Xiaonan Xi Yaxin Lu Liang Wang Yue Chen The State Key Laboratory of Medicinal Chemical Biology College of PharmacyNankai UniversityTianjin300350 China college of Chemistry Nankai UniversityTianjin300071 China

The total synthesis of majusculamide D(1)was achieved from commercially available materials.In addition,we synthesized eight analogues including three stereoisomers of majusculamide D that differ in the fatty acid chain.Six analogues including a simplified analogue 29 exhibited significant nanomolar-level IC50 values against Panc-1 cells in MTT assays.A preliminary SAR analysis indicated that the hydroxyl group at C10 and C2−C3 unsaturated double bond of majusculamide D were essential in maintaining the high activity against Panc-1 cells and the orientation of C40-Me and C42-Me groups was tolerable.

关键词： Majusculamide D Natural products SAR Anti-pancreatic cancer Lipopentapeptide

Electrochemical filtration for drinking water purification:A review on membrane materials,mechanisms and roles

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Journal of Environmental Sciences 2024年第7期141卷 102-128页

作者： Yuying Qi Donghao Li Shixuan Zhang Fengxiang Li Tao Hua college of Environmental Science and Engineering Nankai UniversityTianjin 300350China Key Laboratory of Pollution Process and Environmental Criteria Ministry of EducationTianjin 300350China tianjin Engineering Center of Environmental Diagnosis and Contamination Remediation Tianjin 300350China

Electrochemical filtration can not only enrich low concentrations of pollutants but also produce reactive oxygen species to interact with toxic pollutants with the assistance of a power supply,making it an effective strategy for drinking water purification.In addition,the application of electrochemical filtration facilitates the reduction of pretreatment procedures and the use of chemicals,which has outstanding potential for maximizing process simplicity and reducing operating costs,enabling the production of safe drinking water in smaller installations.In recent years,the research on electrochemical filtration has gradually increased,but there has been a lack of attention on its application in the removal of low concentrations of pollutants from low conductivity water.In this review,membrane substrates and electrocatalysts used to improve the performance of electrochemical membranes are briefly summarized.Meanwhile,the application prospects of emerging single-atom catalysts in electrochemical filtration are also presented.Thereafter,several electrochemical advanced oxidation processes coupled with membrane filtration are described,and the related working mechanisms and their advantages and shortcomings used in drinking water purification are illustrated.Finally,the roles of electrochemical filtration in drinking water purification are presented,and the main problems and future perspectives of electrochemical filtration in the removal of low concentration pollutants are discussed.

关键词： Electrochemical filtration Drinking water Conductive membrane Low concentration Electrocatalyst

Flat Band and η-Pairing States in a One-Dimensional MoiréHubbard Model

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Chinese Physics Letters 2024年第4期41卷 69-76页

作者：王冉宋智 college of Physics and Materials Science Tianjin Normal UniversityTianjin 300387China School of Physics Nankai UniversityTianjin 300071China

A Moirésystem is formed when two periodic structures have a slightly mismatched period,resulting in unusual strongly correlated states in the presence of particle-particle interactions.The periodic structures can arise from the intrinsic crystalline order and periodic external field.We investigate a one-dimensional Hubbard model with periodic on-site potential of period n_(0),which is commensurate to the lattice constant.For large n_(0),the exact solution demonstrates that there is a midgap flat band with zero energy in the absence of Hubbard interaction.Each Moiréunit cell contributes two zero energy levels to the flat band.In the presence of Hubbard interaction,the midgap physics is demonstrated to be well described by a uniform Hubbard chain in which the effective hopping and on-site interaction strength can be controlled by the amplitude and period of the external field.Numerical simulations are performed to demonstrate the correlated behaviors in the finite-sized Moiré Hubbard system,including the existence of an η-pairing state and bound pair oscillation.This finding provides a method to enhance the correlated effect by a spatially periodic external field.

关键词： oscillation interaction field

Assessing Dietary Consumption of Sodium and Potassium in China through Wastewater Analysis

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Biomedical and Environmental Sciences 2024年第1期37卷 127-131页

作者： TAN Dong Qin LIANG Yi GUO Ting LI Yan Ying SONG Yong Xin WANG De Gao college of Environmental Science and Engineering Dalian Maritime UniversityDalian 116026LiaoningChina college of Marine Engineering Dalian Maritime UniversityDalian 116026LiaoningChina

A causal relationship has been reported between the average population salt(sodium chloride)intake and the increased risk of stroke and cardiovascular and cerebrovascular diseases in some epidemiological and clinical studies.The World Health Organization has recommended that a sodium intake of<2 g/day is preventive against cardiovascular disease,although the current intake is in excess in most countries.

关键词： Wastewater intake Potassium

The impact of supply chain resilience on customer satisfaction and financial performance:A combination of contingency and configuration approaches

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Journal of Management Science and Engineering 2024年第1期9卷 38-52页

作者： Baofeng Huo Dan Li Minhao Gu college of Management and Economics Tianjin UniversityTianjin300072China

Supply chain resilience(SCR)refers to a supply chain's(SC's)ability to recover from disruptions timely and effectively.This study uses a combination of contingency and configuration approaches to examine the direct and contingent relationships between SCR dimensions(i.e.,internal,supplier,and customer resilience)and performance.It analyzes survey data collected from 206 Chinese manufacturers.The results show that the three SCR dimensions are positively related to customer satisfaction,whereas customer resilience has no direct contribution to financial performance.Internal resilience moderates the relationship between supplier resilience and performance(negative for customer satisfaction and positive for financial performance).A taxonomy for SCR was developed based on internal,supplier,and customer resilience,providing a holistic perspective for examining the performance discrepancies among four different SCR patterns:high externalleaning,high uniform,medium uniform,and low uniform.These findings offer insights for managers in building SCR from the crisis-management process.

关键词： Supply chain resilience Risk management Taxonomy Performance China

A preliminary study on life history of marine red alga Stylonema alsidii(Zandardini)Drew f.ramosum Zheng et Li

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Journal of Oceanology and Limnology 2024年第3期42卷 915-922页

作者： Bingxin HUANG Yao ZHANG Yue CHU Youxuan GUO Junxia LIANG Jianan QIN Lanping DING tianjin Key Laboratory of Animal and Plant Resistance College of Life SciencesTianjin Normal UniversityTianjin 300387China

Stylonema alsidii(Zandardini)Drew f.ramosum Zheng et Li is a common species in the genus Stylonema,but there are limited reports on morphological taxonomy and a lack of studies on life history and the regulation of early development.The early development,discoid formation,and erect thallus growth of Stylonema alsidii f.ramosum were observed under laboratory conditions.In addition,the influence of main environmental factors such as temperature and light intensity on its development was briefly studied,and various stages of its life history were observed.The result shows:(1)there are two reproductive modes:asexual reproduction and sexual reproduction;(2)the morphology of this species varies in different degrees under laboratory culture conditions;(3)sexual reproduction and asexual reproduction can coexist under suitable conditions.Five pathways of life history were inferred from experimental phenomena.Mature sporophytes form mature gametophytes by producing initially isolated or initially attached monospore,and mature gametophytes form mature sporophytes by fertilization of eggs and sperms.The sexual and asexual reproduction processes of Stylonema alsidii f.ramosum were reported for the first time,and this is also the first report on sexual reproduction in the genus Stylonema.

关键词： Stylonema alsidii(Zandardini)Drew f.ramosum Zheng et Li life history environmental factor asexual reproduction sexual reproduction

Risk of cardiovascular death in patients with hepatocellular carcinoma based on the Fine-Gray model

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World Journal of Gastrointestinal Oncology 2024年第3期16卷 844-856页

作者： Yu-Liang Zhang Zi-Rong Liu Zhi Liu Yi Bai Hao Chi Da-Peng Chen Ya-Min Zhang Zi-Lin Cui First Central Clinical college Tianjin Medical UniversityTianjin 300070China Department of Hepatobiliary Surgery Tianjin First Central HospitalSchool of MedicineNankai UniversityTianjin 300192China

BACKGROUND Hepatocellular carcinoma(HCC)is one of the most common types of cancers worldwide,ranking fifth among men and seventh among women,resulting in more than 7 million deaths annually.With the development of medical tech-nology,the 5-year survival rate of HCC patients can be increased to 70%.How-ever,HCC patients are often at increased risk of cardiovascular disease(CVD)death due to exposure to potentially cardiotoxic treatments compared with non-HCC patients.Moreover,CVD and cancer have become major disease burdens worldwide.Thus,further research is needed to lessen the risk of CVD death in HCC patient survivors.METHODS This study was conducted on the basis of the Surveillance,Epidemiology,and End Results database and included HCC patients with a diagnosis period from 2010 to 2015.The independent risk factors were identified using the Fine-Gray model.A nomograph was constructed to predict the CVM in HCC patients.The nomograph performance was measured using Harrell’s concordance index(C-index),calibration curve,receiver operating characteristic(ROC)curve,and area under the ROC curve(AUC)value.Moreover,the net benefit was estimated via decision curve analysis(DCA).RESULTS The study included 21545 HCC patients,of whom 619 died of CVD.Age(5 cm:2.090(1.543-2.830),P<0.001],surgery(no)[0.376(0.297-0.476),P<0.001],and chemotherapy(none/unknown)[0.578(0.472-0.709),P<0.001]were independent risk factors for CVD death in HCC patients.The discrimination and calibration of the nomograph were better.The C-index values for the training and validation sets were 0.736 and 0.665,respectively.The AUC values of the ROC curves at 2,4,and 6 years were 0.702,0.725,0.740 in the training set and 0.697,0.710,0.744 in the validation set,respectively.The calibration curves showed that the predicted probab-ilities of the CVM prediction

关键词： Hepatocellular carcinoma Cardiovascular disease deaths Fine-Gray model Risk factor Nomograph Predict

Energy-saving design and optimization of pressure-swing-assisted ternary heterogenous azeotropic distillations

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Chinese Journal of Chemical Engineering 2024年第4期68卷 1-7页

作者： Lianjie Wu Kun Lu Qirui Li Lianghua Xu Yiqing Luo Xigang Yuan tianjin Key Laboratory of Organic Solar Cells and Photochemical Conversion College of Chemical and Chemical EngineeringTianjin University of TechnologyTianjin 300384China State Key Laboratory of Chemical Engineering Tianjin UniversityTianjin 300072China

A huge amount of energy is always consumed to separate the ternary azeotropic mixtures by distillations.The heterogeneous azeotropic distillation and the pressure-swing distillation are two kinds of effective technologies to separate heterogeneous azeotropes without entrainer addition.To give better play to the synergistic energy-saving effect of these two processes,a novel pressure-swing-assisted ternary heterogeneous azeotropic distillation(THAD)process is proposed firstly.In this process,the ternary heterogeneous azeotrope is decanted into two liquid phases before being refluxed into the azeotropic distillation column to avoid the aqueous phase remixing,and three columns'pressures are modified to decrease the flowrates of the recycle streams.Then the dividing wall column and heat integration technologies are introduced to further reduce its energy consumption,and the pressureswing-assisted ternary heterogeneous azeotropic dividing-wall column and its heat integration structure are achieved.A genetic algorithm procedure is used to optimize the proposed processes.The design results show that the proposed processes have higher energy efficiencies and lower CO_(2)emissions than the published THAD process.

关键词： Distillation Separation Process control Process systems