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Life cycle assessment of homogeneous Fenton process as pretreatment for refractory pharmaceutical wastewater

Frontiers of Chemical Science and engineering 2024年第5期18卷 1-11页

作者： Maojun Zou Jie Wei Yuanyuan Qian Yanjing Xu Zhihuang Fang Xuejing Yang Zhiyuan Wang School of Energy and Power engineering University of Shanghai for Science and TechnologyShanghai 200093China Shanghai engineering Laboratory of Lean Operational Technologies for Full Water System East China University of Science and TechnologyShanghai 200237China Mcwong Environmental Technology Company limited Shanghai 200135China National engineering Laboratory of High Concentration and Refractory Organic Wastewater Treatment Technology East China University of Science and TechnologyShanghai 200237China

The applicability of the life cycle assessment(LCA)to the Fenton process should be considered not only at the laboratory-scale but also at the *** this study,the LCA process was applied to evaluate the homo-geneous Fenton process for the treatment of high salinity pharmaceutical *** potential environmental impacts were calculated using Simapro software implemen-ting the CML 2001 methodology with normalization factors of 1995 *** data obtained directly from the full-scale wastewater treatment plant and labora-tory were used to conduct a life cycle inventory analysis,ensuring highly accurate *** normalized results,the Fenton process reveals sensitive indicators,primarily toxi-city indicators(human toxicity,freshwater aquatic toxicity,and marine aquatic toxicity),as well as acidification and eutrophication impacts,contributed by hydrogen peroxide and iron sludge incineration,***,hydrogen peroxide and iron sludge incineration contribute significantly,accounting for at least 78%of these *** sludge treatment phase,treatment of iron mud and infrastructure of hazardous waste incineration plants were the key contributors of environmental impacts,adding up to more than 95%.This study suggests the need to develop efficient oxidation processes and effective iron sludge treatment methods to reduce resource utilization and improve environmental benefits.

关键词： advanced oxidation processes full-scale life cycle assessment Fenton process pharmaceutical high-salinity wastewater

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Reducing Operation Emissions and Improving Work Efficiency Using a Pure Electric Wheel Drive Tractor

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engineering 2024年第6期37卷 230-245页

作者： Chang-Kai Wen Wen Ren Qing-Zhen Zhu Chun-Jiang Zhao Zhen-Hao Luo Sheng-Li Zhang Bin Xie Zhi-Jun Meng Research Center of Intelligent Equipment Beijing Academy of Agriculture and Forestry SciencesBeijing 100097China State Key Laboratory of Intelligent Agricultural Power Equipment Beijing 100097China BYD Company limited Shenzhen 518118China College of Agricultural engineering Jiangsu UniversityZhenjiang 212013China College of engineering China Agricultural UniversityBeijing 100083China

In response to the problems of excessive greenhouse-gas and particulate emissions and the low traction efficiency of conventional diesel tractors in the field,a purely electric wheel-side drive tractor was studied,including an electric motor drive system,a battery ballast system,and an electro–hydraulic suspension *** paper develops a dynamics model of an electric tractor-ploughing unit under complex soil conditions,leading to the proposal of an active control method for drive wheel torque and a joint control method for the traction force of the suspension system and the front-and rear-axle loads of a ***,the tractor is prototyped and assembled,and ploughing tests are carried *** ploughing results show that the active torque-distribution control method proposed in this study reduces the tractor slip by 14.83%and increases the traction efficiency by 10.28%compared with the average torquedistribution *** with the conventional traction control mode,the joint control method for traction and ballast proposed in this paper results in a 3.7%increase in traction efficiency,a 15.05%decrease in slip,and a 4.9%reduction in total drive motor energy *** study will help to improve the operation quality and traction efficiency of electric tractors in complex soil conditions.

关键词： Electric tractor Ploughing unit Torque distribution Active ballast Traction performance

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Investigation of pore structure alteration and permeability enhancement of shale matrix by supercritical water treatment after hydraulic fracturing

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Petroleum 2024年第2期10卷 265-274页

作者： Yili Kang Peisong Li Wangkun Cao Mingjun Chen Lijun You Jiang Liu Zhehan Lai State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu610500China Institute of engineering Technology Petro China Coalbed Methane Company LimitedXi'an710082China Chemical and Petroleum engineering University of CalgaryCalgaryT2N 1N4Canada

Shale gas reservoirs are unconventional tight gas reservoirs,in which horizontal wells and hydraulic fracturing are required to achieve commercial *** fracture networks created by hydraulic fracturing can increase the drainage area extensively to enhance shale gas ***,large volumes of fracturing fluid that is difficult to flow back to the surface and remained in the shale formation,will inevitably lead to damages of the shale formations and limit the effectiveness of *** water(SCW)treatment after hydraulic fracturing is a new method to enhance shale gas recovery by using appropriate heat treatment methods to the specific formation to convert the retained fracturing fluid into a supercritical state(at temperatures in excess of 373.946°C and pressures in excess of 22.064 MPa).An experiment was conducted to simulate the reaction between shale and SCW,and the capacity of SCW treatment to enhance the permeability of the shale was evaluated by measuring the response of the shale porosity and permeability on SCW *** experimental results show that the shale porosity and permeability increase by 213.43%and 2198.37%,*** pore structure alteration and permeability enhancement of the shale matrix were determined by analyzing the changes in pore structure and mineral composition after SCW *** mechanisms that affect pore structure and mineral composition include oxidative catalysis decomposition of organic matters and reducing minerals,acid-catalyzed decomposition of carbonate minerals and feldspar minerals,hydrothermal catalysis induced fracture extension and cementation weakening induced fracture *** treatment converts harm into a benefit by reducing the intrusion of harmful substances into the shale formation,which will broaden the scope and scale of shale formation stimulation.

关键词： Shale gas Formation damage control Formation heat treatment Supercritical water

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Analysis of Electricity Consumption Pattern Clustering and Electricity Consumption Behavior

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Energy engineering 2024年第9期121卷 2639-2653页

作者： Liang Zhu Junyang Liu Chen Hu Yanli Zhi Yupeng Liu Power Supply Service Management Center State Grid Jiangxi Electric Power Corporation LimitedNanchang330077China State Grid Jiangxi Electric Power Corporation limited Nanchang330077China College of Electrical and Information engineering Hunan UniversityChangsha410082China

Studying user electricity consumption behavior is crucial for understanding their power usage ***,the traditional clustering methods fail to identify emerging types of electricity consumption *** address this issue,this paper introduces a statistical analysis of clusters and evaluates the set of indicators for power usage *** fuzzy C-means clustering algorithm is then used to analyze 6 months of electricity consumption data in 2017 from energy storage equipment,agricultural drainage irrigation,port shore power,and electric ***,the proposed method is validated through experiments,where the Davies-Bouldin index and profile coefficient are calculated and *** showed that the optimal number of clusters is *** study demonstrates the potential of using a fuzzy C-means clustering algorithmin identifying emerging types of electricity consumption behavior,which can help power system operators and policymakers to make informed decisions and improve energy efficiency.

关键词： Electricity consumption clustering consumption behavior fuzzy C-means

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Effect of fracture fluid flowback on shale microfractures using CT scanning

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Journal of Rock Mechanics and Geotechnical engineering 2024年第2期16卷 426-436页

作者： Jiale He Zhihong Zhao Yiran Geng Yuping Chen Jianchun Guo Cong Lu Shouyi Wang Xueliang Han Jun Zhang State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu610500China Key Laboratory of Thermo-Fluid Science and engineering of Ministry of Education School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an710049China Drilling Test engineering Department of Longdong Oil and Gas Development Company Changqing OilfieldPetroChina Company LimitedQingyang745000China Tight Oil and Gas Exploration and Development Project Department PetroChina Southwest Oil and Gas Field CompanyChengdu610056China No.11 Oil Production Plant Changqing Oilfield CompanyPetroChina Company LimitedQingyang745000China

The field data of shale fracturing demonstrate that the flowback performance of fracturing fluid is different from that of conventional reservoirs,where the flowback rate of shale fracturing fluid is lower than that of conventional *** the early stage of flowback,there is no single-phase flow of the liquid phase in shale,but rather a gas-water two-phase flow,such that the single-phase flow model for tight oil and gas reservoirs is not *** this study,pores and microfractures are extracted based on the experimental results of computed tomography(CT)scanning,and a spatial model of microfractures is ***,the influence of rough microfracture surfaces on the flow is corrected using the modified cubic law,which was modified by introducing the average deviation of the microfracture height as a roughness factor to consider the influence of microfracture surface *** flow in the fracture network is simulated using the modified cubic law and the lattice Boltzmann method(LBM).The results obtained demonstrate that most of the fracturing fluid is retained in the shale microfractures,which explains the low fracturing fluid flowback rate in shale hydraulic fracturing.

关键词： Shale Flowback of fracturing fluid Microfracture Lattice Boltzmann method(LBM)

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Simulation of gas-solids heat transfer in cyclone pyrolyzer using CFD-DEM model

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Particuology 2024年第2期85卷 155-166页

作者： Nan Zhang Xueer Pan Jingxuan Yang Qian Liu Wenhao Lian Xiao Du Zhonglin Zhang Xiaogang Hao Guoqing Guan College of Chemical engineering and Technology Taiyuan University of TechnologyTaiyuan030024China School of Chemistry and Chemical engineering North University of ChinaTaiyuan030051China Shanxi Jinke Technology Service Company limited Taiyuan030000China Labraory of Eey onveron Engineerng Institute f Rgional Innvation(RI)Hosaki Univerty3-BunkychoHiroak036-8561Japan

Fast heat transfer in the pyrolyzer can increase the yield of pyrolysis gas and tar,and improve the quality of *** with the downer pyrolyzer,the cyclone pyrolyzer can simultaneously achieve high solids holdup and violent turbulence,and correspondingly faster heat *** this work,the heat transfer behavior in the cyclone pyrolyzer is specifically studied using the computational fluid dynamics-discrete element *** simulation results reveal that the gas-solids heat convection contributes mainly to the heat transfer process,and the heat radiation and conduction are relatively small and almost negligible,*** with the downer pyrolyzer under the same operating conditions,the heating rate is significantly increased in the cyclone *** analyzing the flow characteristics in the cyclone pyrolyzer,it is found that the region of high convective heat transfer rate coincides with that of natural cyclone ***,the final coal temperature increases with the increase of gas velocity and exists a maximum *** results can offer some qualitative understanding of the heat transfer behavior in the cyclone pyrolyzer.

关键词： Cyclone pyrolyzer Rapidly heating Heat convection Natural cyclone length CFD-DEM

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A novel nano-grade organosilicon polymer:Improving airtightness of compressed air energy storage in hard rock formations

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International Journal of Mining Science and Technology 2024年第3期34卷 305-321页

作者： Zhuyan Zheng Guibin Wang Chunhe Yang Hongling Ma Liming Yin Youqiang Liao Kai Zhao Zhen Zeng Hang Li Yue Han Institute of Rock and Soil Mechanics Chinese Academy of SciencesWuhan 430071China University of Chinese Academy of Sciences Beijing 100049China State Key Laboratory of Geomechanics and Geotechnical engineering Wuhan 430071China State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400044China PowerChina Huadong engineering Corporation limited Hangzhou 310014China

Enhancing cavern sealing is crucial for improving the efficiency of compressed air energy storage(CAES)in hard rock *** study introduced a novel approach using a nano-grade organosilicon polymer(NOSP)as a sealant,coupled with an air seepage evaluation model that incorporates Knudsen ***,the initial coating application methods were outlined,and the advantages of using NOSP compared to other sealing materials,particularly regarding cost and construction techniques,were also examined and *** results indicated a significant reduction in permeability of rock specimens coated with a 7–10μm thick NOSP ***,under a 0.5 MPa pulse pressure,the permeability decreased to less than 1 n D,and under a 4 MPa pulse pressure,it ranged between4.5×10^(-6)–5.5×10^(-6)m D,marking a 75%–80%decrease in granite *** sealing efficacy of NOSP surpasses concrete and is comparable to rubber *** optimal viscosity for application lies between 95 and 105 KU,and the coating thickness should ideally range from 7 to 10μm,applied to substrates with less than 3%*** study provides new insights into air transport and sealing mechanisms at the pore level,proposing NOSP as a cost-effective and simplified solution for CAES applications.

关键词： Compressed air energy storage Lining Permeability Transient pulse method Hard rock cavern Nano-grade organosilicon polymer coating

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Geotechnical behavior of uranium mill tailings from Saskatchewan,Canada

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International Journal of Mining Science and Technology 2016年第3期26卷 369-375页

作者： Bhuiyan Imteaz Azam Shahid Khaled Shifullah Landine Patrick Environmental Systems engineering University of Regina thurber engineering limited Cameco Corporation

This paper investigates the geotechnical behavior of uranium mill tailings from Saskatchewan, *** 4% tailings were well-graded with 29% fines whereas the 5% and 6% tailings were gap-graded with 49% fines. All samples exhibited a negligible strength(0.4 k Pa) up to 60% solids, followed by a rapid increase. The 4% tailings exhibited a lower rate and amount of settlement than 5% and 6% tailings. The kidecreased from 10^(-2)to 10^(-4)m/s with a decrease in eifrom 16 to 4 and a decrease in ef from 8 to 4 such that 4% tailings showed one order of magnitude lower values than the 5% and 6%tailings. The settling potential decreased ten times(50%–5%) for 4% tailings and four times(60%–15%)for 5% and 6% tailings. The effective stress increased from 80 to 260 Pa in the settling tests. The 4%tailings were less prone to segregation when compared with 5% and 6% tailings. The average solids content after settling was 35% for 4% tailings, 40% for 5% tailings and 39% for 6% tailings with a solids content deviation of ±3%, ±8%, ±6%, respectively. All materials were essentially non-segregating at 40%initial solids.

关键词： Uranium mill tailings Rheology Settling Segregation

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LATP-coated LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)cathode with compatible interface with ultrathin PVDF-reinforced PEO-LLZTO electrolyte for stable solid-state lithium batteries

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Journal of Materiomics 2024年第3期10卷 682-693页

作者： Xiao Chen Yinda Li Yunhao Lu Jian Xie Cheng Huang Xiongwen Xu Jian Tu Xinbing Zhao Tiejun Zhu State Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and EngineeringZhejiang UniversityHangzhou310058China Department of Physics Zhejiang UniversityHangzhou310058China LI-FUN Technology Corporation limited Zhuzhou412000China

LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)is considered as a promising cathode for high-energy-density solid-sate Li metal battery for its high theoretical ***,the high oxidizability and structural instability during charge limit its practical *** this work,1%(in mass)of nanosized Li_(1.3)Al_(0.3)Ti_(1.7)(PO_(4))_(3)(LATP)was coated on NCM811 to enhance its electrochemical stability with a ceramic/polymer com-posite electrolyte.A robust,ultrathin(11 mm)composite electrolyte film was prepared by combining poly(vinylidene fluoride)(PVDF)with polyethylene oxide(PEO)-Li_(6.5)La_(3)Zr_(1.5)Ta_(0.5)O_(12)(LLZTO).An in-situ polymerization process was used to enhance the interface between the PVDF/PEO-LLZTO(PPL)com-posite electrolyte and the LATP-coated NCM811(LATP-NCM811).Coin-type Li|LATP-NCM811 cell with the PPL electrolyte exhibits stable cycling with an 81%capacity retention after 100 cycles at 0.5 ***-type cell was also fabricated,which can be stably cycled for 70 cycles at 0.5 C/1.0 C(80%retention),and withstand abuse tests of bending,cutting and nail *** work provides an applicable method to fabricate solid-state Li metal batteries with high performance.

关键词： Ultrathin electrolyte film LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2) Li_(1.3)Al_(0.3)Ti_(1.7)(PO_(4))_(3)coating In-situ polymerization Li metal battery

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Improving mathematical model of burden distribution and correcting chute angle to cope with fluctuation of stock line

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Journal of Iron and Steel Research International 2024年第2期31卷 342-356页

作者： Jian-sheng Chen Wen-guo Liu Hao Guo Wang Ding Qing-guo Xue Jing-song Wang Hai-bin Zuo State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing100083China MCC Capital engineering&Research Incorporation limited Beijing100176China Hunan Valin Xiangtan Iron and Steel Co. Ltd.Xiangtan411101HunanChina

Accurate evaluations of the burden distribution are of critical importance to stabilize the operation of blast *** mathematical model and discrete element method(DEM)are two attractive methods for predicting burden *** on DEM,the initial velocities of the pellet,sinter,and coke were calculated,and the velocity attenuations of the above three particles between the burden and the chute were *** initial velocity and velocity attenuation were applied to a mathematical model for improving the ***,based on the improved model,a scheme for rectifying the chute angles was proposed to address the fluctuation of the stock line and maintain a stable burden *** validity of the scheme was confirmed via a stable burden distribution under different stock *** mathematical model has been successfully applied to evaluate the online burden distribution and cope with the fluctuation of the stock line.

关键词： Burden distribution Mathematical model Discrete element method Velocity attenuation Stock line fluctuation

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