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Rheological Behaviors of Polymers with Nanoparticles Tethered at Each End

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Chinese Journal of Polymer science 2024年第3期42卷 400-406,I0009页

作者： Song-Qi Zhang Wen-Qing Wang Jia-Ping Lin Li-Quan Wang Shanghai key laboratory of Advanced Polymeric Materials Key Laboratory for Ultrafine Materials of Ministry of EducationSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China

The polymer with nanoparticles tethered at each end is a unique model for unraveling the effect of chain ends on the polymer dynamics. We investigated the rheological behavior of this kind of polymer by using nonequilibrium molecular dynamics simulation. The effect of polymer lengths and nanoparticle radii on the complex moduli and viscosity was examined. The dependence of complex moduli on the frequency becomes less pronounced as the polymer is short or the nanoparticle is large. The shear thinning behavior was revealed for these systems, and the scaling exponent of complex viscosity with respect to the frequency was found to change from-1/2 to-3/4 as the polymer shortens or the nanoparticle enlarges. The rheological behavior was further explained by analyzing the mean square distance of nanoparticles. The simulation results were compared with the existing experimental finding, showing an agreement. The work provides information for understanding the chain end effect on polymer rheology.

关键词： Polymer rheology Modulus Viscosity Molecular dynamics

维普期刊数据库

ASTSDL:predicting the functionality of incomplete programming code via an AST-sequence-based deep learning model

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science China(information sciences) 2024年第1期67卷 86-104页

作者： Yaoshen YU Zhiqiu HUANG Guohua SHEN Weiwei LI Yichao SHAO College of Computer science and technology Nanjing University of Aeronautics and Astronautics Collaborative Innovation Center of Novel Software technology and Industrialization key laboratory of Safety-Critical Software Ministry of Industry and Information Technology

Code recommendation systems have been widely used in helping developers implement unfamiliar programming *** existing code recommenders or code search engines can retrieve relevant code rapidly with high accuracy,however,they cannot recommend any code outside similar *** propose an approach to predict the functionality of incomplete programming code by using syntactical information,and providing a list of potential functionalities to guess what the developers want,in order to increase the diversity of *** this paper,we propose a deep learning model called ASTSDL,which uses a sequencebased representation of source code to predict *** extract syntactical information from the abstract syntax tree(AST) of the source code,apply a deep learning model to capture the syntactic and sequential information,and predict the functionality of the source code *** experimental results demonstrate that ASTSDL can effectively predict the functionality of incomplete code with an accuracy above 84% in the top-10 list,even if there is only half of the complete code.

关键词： functionality prediction incomplete programming code syntactical information code representation model deep learning algorithm

Broadband high-efficiency dielectric metalenses based on quasi-continuous nanostrips

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Opto-Electronic Advances 2024年第5期7卷 43-51页

作者： Xiaohu Zhang Qinmiao Chen Dongliang Tang Kaifeng Liu Haimo Zhang Lintong Shi Mengyao He Yongcai Guo Shumin Xiao key laboratory of optoelectronic technology and Systems of the Education ministry of China Chongqing UniversityChongqing 400044China ministry of Industry and information technology key Lab of Micro-Nano Optoelectronic information System Guangdong Provincial Key Laboratory of Semiconductor Optoelectronic Materials and Intelligent Photonic SystemsHarbin Institute of TechnologyShenzhen 518055China key laboratory for Micro/Nano Optoelectronic Devices of ministry of Education&Hunan Provincial key laboratory of Low-Dimensional Structural Physics and Devices School of Physics and ElectronicsHunan UniversityChangsha 410082China

Benefiting from the abrupt phase changes within subwavelength thicknesses,metasurfaces have been widely applied for lightweight and compact optical *** broadband and high-efficiency characteristics are highly attractive for the practical implementation of ***,current metasurface devices mostly adopt discrete micro/nano structures,which rarely realize both merits *** this paper,dielectric metasurfaces composed of quasi-continuous nanostrips are proposed to overcome this *** quasi-continuous nanostrips metasurface,a normal focusing metalens and a superoscillatory lens overcoming the diffraction limit are designed and experimentally *** quasi-continuous metadevices can operate in a broadband wavelength ranging from 450 nm to 1000nm and keep a high power *** average efficiency of the fabricated metalens reaches 54.24%,showing a significant improvement compared to the previously reported metalenses with the same *** proposed methodology can be easily extended to design other metadevices with the advantages of broadband and high-efficiency in practical optical systems.

关键词： broadband high-efficiency metalens sub-diffraction quasi-continuous

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Artificial intelligence-assisted design of new chemical materials: a perspective

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science China(information sciences) 2024年第8期67卷 334-336页

作者： Feng QIAN Wenli DU Weimin ZHONG Yang TANG Jingyi LU key laboratory of Smart Manufacturing in Energy Chemical Process Ministry of EducationEast China University of Science and Technology

New chemical materials are a fresh category of substances created through chemical reactions or by refining existing materials through secondary processes. By using creative methods, advanced technologies, innovative techniques, and state-of-the-art equipment, these materials(e.g., high-end polyolefin, nano materials) [1] are carefully designed and developed to showcase outstanding performance and unique capabilities beyond what traditional chemical materials can offer [2].

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A Comprehensive Overview of CFN From a Commonsense Perspective

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Machine Intelligence Research 2024年第2期21卷 239-256页

作者： Ru Li Yunxiao Zhao Zhiqiang Wang Xuefeng Su Shaoru Guo Yong Guan Xiaoqi Han Hongyan Zhao key laboratory of Computational Intelligence and Chinese information Processing of ministry of Education School of Computer and Information TechnologyShanxi UniversityTaiyuan 030006China

Chinese FrameNet(CFN)is a scenario commonsense knowledge base(CKB)that plays an important role in research on Chinese language *** is based on the theory of frame semantics and English FrameNet(FN).The CFN knowledge base contains a wealth of scenario commonsense knowledge,including frames,frame elements,and frame relations,as well as annotated instances with rich scenario-related labels on Chinese sentences and *** this paper,we conduct a comprehensive overview of CFN from a commonsense perspective,covering topics such as scenario commonsense representation,CFN resources,and its *** also summarize recent breakthroughs and identify future research ***,we introduce the concept of scenario commonsense,including its definitions,examples,and representation methods,with a focus on the relationship between scenario commonsense and the frame concept in *** addition,we provide a comprehensive overview of CFN resources and their applications,highlighting the newly proposed frame-based discourse representation and a human-machine collaboration framework for expanding the CFN ***,we explore emerging topics such as expanding the CFN resource,improving the interpretability of machine reading comprehension,and using scenario CKBs for text generation.

关键词： Chinese FrameNet(CFN) commonsense scenario commonsense frame knowledge

Enhancing thermoelectric performance in P-type Mg_(3)Sb_(2)-based Zintls through optimization of band gap structure and nanostructuring

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Journal of Materials science & technology 2024年第3期170卷 25-32页

作者： Yi-bo Zhang Ji-Sheng Liang Chengyan Liu Qi Zhou Zhe Xu Hong-bo Chen Fu-cong Li Ying Peng Lei Miao Guangxi key laboratory of information Material Engineering Research Center of Electronic Information Materials and DevicesMinistry of EducationSchool of Material Science and EngineeringGuilin University of Electronic TechnologyGuilin 541004China Guangxi key laboratory for Relativity Astrophysics Center on Nanoenergy ResearchGuangxi Key Laboratory of Processing for Nonferrous Metal and Featured MaterialsSchool of Physical Science&TechnologyGuangxi UniversityNanning 530004China Guangxi key laboratory of Precision Navigation technology and Application Guilin University of Electronic TechnologySchool of Information and CommunicationGuilin 541004China

P-type Mg_(3)Sb_(2)-based Zintls have attracted considerable interest in the thermoelectric(TE)field due to their environmental friendliness and low ***,compared to their n-type counterparts,they show relatively low TE performance,limiting their application in TE *** this work,we simultaneously introduce Bi alloying at Sb sites and Ag doping at Mg sites into the Mg_(3)Sb_(2)to coopera-tively optimize the electrical and thermal properties for the first time,acquiring the highest ZT value of∼0.85 at 723 K and a high average ZT of 0.39 in the temperature range of 323-723 K in sample Mg_(2.94)Ag_(0.06)Sb_(1.9)Bi_(0.1).The first-principle calculations show that the codoping of Ag and Bi can shift the Fermi level into the valence band and narrow the band gap,resulting in the increased carrier concentration from 3.50×10^(17)cm^(-3)in the reference Mg 3 Sb 0.9 Bi 0.1 to∼7.88×10^(19)cm^(-3)in sample Mg 2.94 Ag 0.06 Sb 0.9 Bi *** a result,a remarkable power factor of∼778.9μW m^(-1)K^(-2)at 723 K is achieved in sample Mg 2.94 Ag 0.06 Sb 0.9 Bi ***,a low lattice thermal conductivity of∼0.48 W m^(-1)K^(-1)at 723 K is also obtained with the help of phonon scattering at the distorted lattice,point defects,and nano-precipitates in sample Mg 2.94 Ag 0.06 Sb 0.9 Bi *** synergistic effect of using the multi-element co-doping/-alloying to optimize electrical properties in Mg_(3)Sb_(2)holds promise for further improving the TE performance of Zintl phase materials or even others.

关键词： Thermoelectric materials Band engineering Nanostructuring P-type Mg_(3)Sb_(2) Ag and Bi Co-doping

Single-shot probing of sub-picosecond solid-tooverdense-plasma dynamics

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Light(science & Applications) 2024年第8期13卷 1448-1450页

作者： Kunjian Dai Qingzhe Cui Jinwei Zhang School of Optical and Electronic information and Wuhan National laboratory for optoelectronics Huazhong University of Science and TechnologyWuhan 430074China

A single-shot near-infrared probing method has been developed to characterize the formation and evolution of the pre-plasma dynamics over sub-picosecond timescales,which is essential for the societal applications of l... 详细信息

关键词： dynamics picosecond technologies

OsNAC120 balances plant growth and drought tolerance by integrating GA and ABA signaling in rice

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Plant Communications 2024年第3期5卷 197-215页

作者： Zizhao Xie Liang Jin Ying Sun Chenghang Zhan Siqi Tang Tian Qin Nian Liu Junli Huang key laboratory of Biorheological science and technology of ministry of Education Bioengineering College of Chongqing UniversityChongqingChina

The crosstalk between gibberellin(GA)and abscisic acid(ABA)signaling is crucial for balancing plant growth and adaption to environmental ***,the molecular mechanism of their mutual antagonism still remains to be fully *** this study,we found that knockout of the rice NAC(NAM,ATAF1/2,CUC2)tran-scription factor gene OsNAC120 inhibits plant growth but enhances drought tolerance,whereas OsNAC120 overexpression produces the opposite *** GA can rescue the semi-dwarf phenotype of osnac120 mutants,and further study showed that OsNAC120 promotes GA biosynthesis by transcriptionally activating the GA biosynthetic genes OsGA20ox1 and *** DELLA protein SLENDER RICE1(SLR1)interacts with OsNAC120 and impedes its transactivation ability,and GA treatment can remove the inhi-bition of transactivation activity caused by *** the other hand,OsNAC120 negatively regulates rice drought tolerance by repressing ABA-induced stomatal *** investigation revealed that OsNAC120 inhibits ABA biosynthesis via transcriptional repression of the ABA biosynthetic genes OsNCED3 and *** OSMOTIC STRESS/ABA-ACTIVATED PROTEIN KINASE 9(OsSAPK9)physically interacts with OsNAC120 and mediates its phosphorylation,which results in OsNAC120 *** treatment ac-celerates OsNAC120 degradation and reduces its transactivation ***,ourndings provide evi-dencethatOsNAC120playscriticalrolesinbalancingGA-mediatedgrowthandABA-induceddroughttolerance in *** research will help us to understand the mechanisms underlying the trade-off between plant growth and stress tolerance and to engineer stress-resistant,high-yielding crops.

关键词： abscisic acid ABA drought stress gibberellin GA OsNAC120 OsSAPK9 rice Oryza sativa L. SLR1

Influence of tungsten particle size on microstructure and mechanical properties of high strength and tough tungsten particle-reinforced nickel-based composites by laser-direct energy deposition

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Journal of Materials science & technology 2024年第5期172卷 213-227页

作者： Wenji Song Dengzhi Wang Congwen Tang Pengfei Sun Jiaxing Yang Zhidong Xu Tao Lai Jianqiang Gong Qianwu Hu Xiaoyan Zeng Wuhan National laboratory for optoelectronics Huazhong University of Science and TechnologyWuhan 430000China

Tungsten(W)particle-reinforced nickel(Ni)-based composites were fabricated via laser-direct energy de-position(L-DED).The influence of the W particle size on the microstructure and mechanical properties of the deposited samples was systematically *** results indicate that refining the W particle size could refine theγ-Ni grains and subgrains,thin the(Ni,Cr)_(4)W interface layer,and increase the disloca-tion density of the intergranular matrix,thus improving the tensile strength and elongation of the L-DED *** W particle size decreased from 75 to 150μm to 6.5-12μm,the tensile strength and elonga-tion of the deposited samples increased by 150 MPa and 2.9 times to 1347.6±15.7 MPa and 17.5±0.4%,*** on the properties of the interface(Ni,Cr)_(4)W,a load-transfer efficiency factor suitable for this composite was proposed and the load-transfer strengthening formula was optimized.A quanti-tative analysis of the strengthening mechanisms was established considering load-transfer strengthening,Hall-Petch strengthening,thermal-mismatch strengthening,and solid-solution *** calcu-lated contribution of each strengthening mechanism to the yield strength and theoretical calculations were in good agreement with the experimental *** article breaks the bottleneck of poor plasticity of W particle-reinforced Ni-based composites prepared by L-DED and provides a theoretical basis for the construction design of W particle-reinforced Ni-based composites with excellent mechanical properties.

关键词： Laser-direct energy deposition(L-DED) Tungsten particle reinforcements Mechanical property Strengthening mechanism