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Hydrogen-bonded organic framework modified separator for simultaneously enhancing the safety and electrochemical performance of Ni-rich lithium-ion battery

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Journal of Energy Chemistry 2024年第9期96卷 72-78页

作者： Chengyu Han Yu Cao Ming Yang Yuhan Wang Di Tang Shaojie Zhang Yiran Jia Yiming Zhang Hern Kim Fusheng Pan Zhongyi Jiang Jie Sun Key Laboratory for Green Chemical Technology of Ministry of education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Science and Technology on Power Sources Laboratory Tianjin Institute of Power SourcesTianjin 300384China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China Quzhou Institute for Innovation in Resource Chemical Engineering Quzhou 324000ZhejiangChina Department of Energy Science and Technology director Environmental Waste Recycle InstituteYongin 17058Republic of Korea School of Chemistry and Chemical Engineering Hainan UniversityHaikou 570228HainanChina

Nickel-rich layered oxide cathode(LiNi_(x)Co_(y)Mn_(1−x−y)O_(2),x>0.5,NCM)shows substantial potential for applications in longer-range electrical ***,the rapid capacity decay and serious safety concerns impede its practical *** work provides a hydrogen-bonded organic framework(HOF)modification strategy to simultaneously improve the electrochemical performance,thermal stability and incombustibility of *** cyanurate(MCA),as a low-cost and reliable flame-retardant HOF,was implemented in the separator modification layer,which can prevent the battery short circuit even at a high *** addition,the supermolecule properties of MCA provide unique physical and chemical microenvironment for regulating ion-transport behavior in *** MCA coating layer enabled the nickel-rich layered oxide cathode with a high-capacity retention of 90.3%after 300 cycles at 1.0 ***,the usage of MCA in lithium-ion batteries(LIBs)affords a simple,low-cost and efficient strategy to improve the security and service life of nickel-rich layered cathodes.

关键词： Hydrogen-bonded organic framework Modified separator Ni-richlayered oxide cathode Thermal runaway Li^(+)transference number

Rattling-like behavior and band convergence induced ultra-low lattice thermal conductivity in MgAl_(2)Te_(4) monolayer

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Journal of Materiomics 2024年第5期10卷 1004-1016页

作者： Da Wan Shulin Bai Xiaodong Li Jingyi Zhang Peng Ai Wanrong Guo Shuwei Tang College of Materials Science and Engineering Liaoning Technical UniversityFuxinLiaoning123000China Faculty of Chemistry Northeast Normal UniversityChangchunJilin130024China

Inspired by the excellent stability exhibited by experimentally synthesized two-dimensional(2D)MoSi_(2)N_(4) layered material,the thermal and electronic transport,and thermoelectric(TE)properties of MgAl2Te4 monolayer are systematically investigated using the First-principles calculations and Boltzmann transport *** mechanical stability,dynamic stability,and thermal stability(900 K)of the MgAl_(2)Te_(4) monolayer are demonstrated,*** MgAl_(2)Te_(4) monolayer exhibits a bandgap of 1.35 eV using the HSE06 functional in combination with spin-orbit coupling(SOC)*** convergence in the valence band is favorable to improve the thermoelectric *** rattling thermal damping effect caused by the weak bonding of Mgsingle bondTe bonds in MgAl2Te4 monolayer leads to ultra-low lattice thermal conductivity(0.95/0.38 W/(m·K)@300 K along the x-/y-direction),which is further demonstrated by the phonon group velocities,phonon relaxation time,Grüneisen parameters,and scattering *** optimal zT of 3.28 at 900 K is achieved for the p-type MgAl_(2)Te_(4) monolayer,showing the great promising prospect for the excellent p-type thermoelectric *** current work not only reveals the underlying mechanisms responsible for the excellent TE properties,but also elaborates on the promising thermoelectric application of MgAl_(2)Te_(4) monolayer material at high temperature.

关键词： Thermoelectric material Mg atomic rattling Band convergence Ultra-low lattice thermal conductivity

A comprehensive review on the development of data-driven methods for wind power prediction and AGC performance evaluation in wind–thermal bundled power systems

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Energy and AI 2024年第2期16卷 450-463页

作者： Shuai Wang Bin Li Guanzheng Li Botong Li Hongbo Li Kui Jiao Chengshan Wang National Industry-education Platform for Energy Storage Tianjin UniversityTianjin300350China Key Laboratory of Smart Grid of Ministry of education Tianjin UniversityTianjin300072China Power Dispatching and Control Center Inner Mongolia Power(Group)Co.LtdHohhot010020China

The wind–thermal bundled power system achieves energy complementarity and optimized scheduling, which is an important way to build a new type of energy system. For the safe and stable operation of the wind–thermal bundled power system, accurate data-driven analysis is necessary to maintain real-time balance between electricity supply and demand. By summarizing the development and characteristics of wind–thermal bundled power system in China and different countries, current research in this field can be clearly defined in two aspects: short-term wind power prediction for wind farms and performance evaluation of automatic generation control (AGC) for thermal power generation units. For short-term wind power prediction, it is recommended to focus on historical data preprocessing and artificial intelligence methods. The technical characteristics of different data-driven wind power prediction methods have been compared in detail. For performance evaluation of AGC units, a comprehensive analysis was conducted on current evaluation methods, including the “permitted-band” and “regulation mileage” methods, as well as the issue of evaluation failure in traditional evaluation methods in practical engineering. Finally, the relative optimal dynamic performance of AGC units was discussed and the future trend of data-driven research in wind–thermal bundled power system was summarized.

关键词： Wind power prediction Automatic generation control Performance evaluation Data-driven Feature analysis

Tailoring chaotic motion of microcavity photons in ray and wave dynamics by tuning the curvature of space

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 107-112页

作者： Wei Lin Yechun Ding Yongsheng Wang Peng Li Yanpeng Zhang Feng Yun Feng Li Key Laboratory for Physical Electronics and Devices of the Ministry of education Shaanxi Key Lab of Information Photonic TechniqueSchool of Electronic Science and EngineeringFaculty of Electronic and Information EngineeringXi’an Jiaotong UniversityXi’an 710049China Department of Electrical and Photonics Engineering Technical University of DenmarkKgs.Lyngby 2800Denmark Center for Regenerative and Reconstructive Medicine Med-X InstituteThe First Affiliated Hospital of Xi’an Jiaotong UniversityXi’an 710061China Solid-State Lighting Engineering Research Center Xi’an Jiaotong UniversityXi’an 710049China

Microcavity photon dynamics in curved space is an emerging interesting area at the crossing point of nanophotonics,chaotic science,and non-Euclidean *** report the sharp difference between the regular and chaotic motions of cavity photons subjected to the varying space *** the island modes of regular motion rise in the phase diagram in the curved space,the chaotic modes show special mechanisms to adapt to the space curvature,including the fast diffusion of ray dynamics,and the localization and hybridization of the Husimi wavepackets among different periodic *** observations are unique effects enabled by the combination of the chaotic trajectory,the wave nature of light,and the non-Euclidean orbital motion,and therefore make the system a versatile optical simulator for chaotic science under quantum mechanics in curved space-time.

关键词： microcavity chaotic motion curved space

Analyze the Performance of Electroactive Anticorrosion Coating of Medical Magnesium Alloy Using Deep Learning

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Computers, Materials & Continua 2024年第4期79卷 263-278页

作者： Yashan Feng Yafang Tian Yongxin Yang Yufang Zhang Haiwei Guo Jing’an Li Advanced Functional Materials Laboratory Zhengzhou Railway Vocational and Technical CollegeZhengzhou450000China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou450000China

Electroactive anticorrosion coatings are specialized surface treatments that prevent or minimize corrosion. Thestudy employs strategic thermodynamic equilibriumcalculations to pioneer a novel factor in corrosion protection.A first-time proposal, the total acidity (TA) potential of the hydrogen (pH) concept significantly shapes medicalmagnesium alloys. These coatings are meticulously designed for robust corrosion resistance, blending theoreticalinsights and practical applications to enhance our grasp of corrosion prevention mechanisms and establisha systematic approach to coating design. The groundbreaking significance of this study lies in its innovativeintegration of the TA/pH concept,which encompasses the TA/pH ratio of the chemical environment. This approachsurpasses convention by acknowledging the intricate interplay between the acidity and pH levels within thecoating formulation, thereby optimizing metal-phosphate-based conversion coatings and transforming corrosionmitigation strategies. To authenticate the TA/pH concept, the study comprehensively compares its findings withexisting research, rigorously validating the theoretical framework and reinforcing the correlates among TA/pHvalues and observed corrosion resistance in the coatings. The influence of mutations that occur naturally inthe detergent solution on persistent phosphorus changes is shown by empirical confirmation, which improvescorrosion resistance. This realization advances the field ofmaterials and the field’s knowledge of coated generation,particularly anticorrosion converter layers.

关键词： Medical magnesium alloys hydrogen gas anticorrosion total acidity potential of the hydrogen(pH)

System Strength Assessment Based on Multi-task Learning

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 41-50页

作者： Baoluo Li Shiyun Xu Huadong Sun Zonghan Li Lin Yu Key Laboratory of Power System Intelligent Dispatch and Control of Ministry of education Shandong UniversityJinan 250014China China Electric Power Research Institute Beijing 100192China

Increase in permeability of renewable energy sources(RESs)leads to the prominent problem of voltage stability in power system,so it is urgent to have a system strength evaluation method with both accuracy and practicability to control its access scale within a reasonable ***,a hybrid intelligence enhancement method is proposed by combining the advantages of mechanism method and data driven ***,calculation of critical short circuit ratio(CSCR)is set as the direction of intelligent enhancement by taking the multiple renewable energy station short circuit ratio as the quantitative ***,the construction process of CSCR dataset is proposed,and a batch simulation program of samples is developed accordingly,which provides a data basis for subsequent ***,a multi-task learning model based on progressive layered extraction is used to simultaneously predict CSCR of each RESs connection point,which significantly reduces evaluation error caused by weak *** performance and anti-noise performance of the proposed method are verified on the CEPRI-FS-102 bus system,which provides strong technical support for real-time monitoring of system strength.

关键词： Critical short circuit ratio hybrid intelligence enhancement multi-task learning system strength

Adoption of green finance and green innovation for achieving circularity:An exploratory review and future directions

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Geoscience Frontiers 2024年第4期15卷 333-346页

作者： Rohit Agrawal Shruti Agrawal Ashutosh Samadhiya Anil Kumar Sunil Luthra Vranda Jain Operations Management and Quantitative Techniques Indian Institute of ManagementBodhgaya 824234BiharIndia Department of Humanities and Social Sciences Malaviya National Institute of Technology Jaipur RajasthanIndia Jindal Global Business School OP Jindal Global UniversitySonipatIndia Guildhall School of Business and Law London Metropolitan UniversityLondonUK AICTE Training and Learning(ATAL) All India Council for Technical EducationDelhiIndia Economics and International Business Jaipuria Institute of ManagementNoidaIndia

There is growing attention from governments and regulators towards crucial matters such as climate change and global warming,resulting in a pressing need to investigate the factors that make it possible for businesses to engage in green finance(GF).The externality of environmental pollution prioritizes the need of green innovation(GI)in public *** distributes financial resources to the research and development(R&D)of clean energy and environmentally friendly goods and processes;it is complementary to the GI process for environmental *** policies help to alleviate the impacts of financial constraints and GI impaired industries involving new products,processes,services and the global *** better understand how GF and GI have functioned as a catalyst for circular economy practices,this paper seeks to present a historical and contemporary overview of these *** research is thoroughly dissected by a systematic literature evaluation of articles from 2016 to 2023 that appear in peer-reviewed journals and are indexed in the SCOPUS *** attain supply chain circularity,this article encompasses four major research themes concerning the adoption of GF and green *** research also includes a network analysis of shortlisted articles to examine the overall citation *** is shown that several institutional theories are associated with the investigated *** a final step,a framework is provided to illustrate how GF and GIs might be used to achieve supply chain *** research findings provide a novel concept related to GF within the context of GI which are significant for environmentalists,policymakers,green investors,and *** its findings,the study provides a conceptual framework that promotes sustainable strategies to effectively balance financial considerations and environmental *** helps to leverage the potential of green research and practice to create value for businesses and to benefi

关键词： Green finance Green innovation Systematic literature review Environmental protection Climate change

Graphene enables equiatomic FeNiCrCoCu high-entropy alloy with improved TWIP and TRIP effects under shock compression

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Journal of Materials Science & Technology 2024年第3期170卷 186-199页

作者： Hongcai Xie Zhichao Ma Wei Zhang Hongwei Zhao Luquan Ren School of Mechanical and Aerospace Engineering Jilin UniversityChangchun 130025China Key Laboratory of CNC Equipment Reliability Ministry of education Jilin UniversityChangchun 130025China Key Laboratory of Bionic Engineering Ministry of education Jilin UniversityChangchun 130025China Weihai Institute for Bionics-Jilin University Weihai 264400China Institute of Structured and Architected Materials Liaoning Academy of MaterialsShenyang 110167China

Graphene(Gr)reinforced high-entropy alloy(HEA)matrix composites are expected as potential candidates for next-generation structural applications in light of outstanding mechanical properties.A deep comprehension of the underlying deformation mechanisms under extreme shock loading is of paramount importance,however,remains lacking due to experimentally technical limitations in *** the present study,by means of nonequilibrium molecular dynamics simulations,dynamic deformation behaviors and corresponding mechanisms in equiatomic FeNiCrCoCu HEA/Gr composite systems were investigated in terms of various shock *** resistance to dislocation propagation imparted by Gr was corroborated to encourage the elevated local stress level by increasing the likelihood of dislocation interplays,which facilitated the onset of twins and hexagonal close-packed(HCP)martensite ***,the advent of Gr was demonstrated to endow the HEA with an additional twinning pathway that induced a structural conversion from HCP to parent face-centered cubic(FCC)inside HCP martensite laths,different from the classical one that necessitated undergoing the intermediate procedure of extrinsic stacking fault(ESF)*** than that,by virtue of an increase in flow stress,the transformation-induced plasticity(TRIP)effect was validated to be additionally evoked as the predominant strain accommodation mechanism at higher strains on the one hand,but which only assisted plasticity in pure systems,and on the other hand,can also act as an auxiliary regulation mode together with the twinning-induced plasticity(TWIP)effect under intermediate strains,but with enhanced contributions relative to pure *** may expect that TRIP and TWIP effects promoted by introducing Gr would considerably inspire a synergistic effect between strength and ductility,contributing to the exceptional shock-resistant performance of FeNiCrCoCu HEAs under extreme regimes.

关键词： Molecular dynamics High-entropy alloy Graphene TRIP TWIP Shock

Bioinspired Double-stranded Yarn with Alternating Hydrophobic/Hydrophilic Patterns for High-efficiency Fog Collection

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Chinese Journal of Polymer Science 2024年第7期42卷 968-975,I0008页

作者： Lan-Lan Hou Meng-Na Qiu Ya-Qiong Wang Tong-Hua Bai Zhi-Min Cui Jing-Chong Liu Ying-Qun Qi Nü Wang Yong Li Yong Zhao Beijing Institute of Graphic Communication Beijing102600China Key Laboratory of Bioinspired Smart Interfacial Science and Technology of Ministry of education Beijing Key Laboratory of Bioinspired Energy Materials and DevicesSchool of ChemistryBeijing Advanced Innovation Center for Biomedical EngineeringBeihang UniversityBeijing100191China Key Laboratory of Cryogenics Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing100190China Beijing Key Laboratory for Bioengineering and Sensing TechnologyDaxing Research InstituteSchool of Chemistry and Biological EngineeringUniversity of Science and Technology BeijingBeijing100083China

Efforts to develop innovative water harvesting strategies offer powerful solutions to alleviate the water crisis,especially in remote and arid *** by the hydrophobic/hydrophilic pattern of desert beetles and water self-propulsion property of spider silks,a double-strand hydrophobic PVDF-HFP/hydrophilic PAN nanofibers yarn is proposed by electrospinning and twisting *** double-strand cooperation approach allows for water deposition on hydrophobic PVDF-HFP segment and transport under the asymmetric capillary driving force of hydrophilic PAN segment,thus speeded up the aggregation and growth of *** effects of the composition and the diameter ratio of the two primary yarns were studied and optimized for boosting fog collection *** double-strand anisotropic yarn not only provide an effective method for water harvesting,but also hold the potential to inspire innovative design concepts for fog collection materials in challenging environments.

关键词： Fog collection Wettability Electrospinning Nanofibers Spider silk