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Pressure-Induced Distinct Self-Trapped Exciton Emission in Sb^(3+)-Doped Cs_(2)NaInCl_(6)Double Perovskite

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Chinese physics Letters 2024年第6期41卷 18-43页

作者：冯友佳陈亚平王乐瑶王家祥常断华袁亦方武敏付瑞净张丽丽王庆林王凯郭海中王玲瑞 Key laboratory of Materials physics(Ministry of Education) School of PhysicsZhengzhou UniversityZhengzhou 450001China Shandong Key laboratory of optical Communication Science and Technology School of Physics Science and Information TechnologyLiaocheng UniversityLiaocheng 252059China College of Applied physics and Materials Wuyi UniversityJiangmen 529020China

The Cs_(2)NaInCl_(6) double perovskite is one of the most promising lead-free perovskites due to its exceptional stability and straightforward ***,it faces challenges related to inefficient *** and high pressure are employed to tailor the optical properties of Cs_(2)NaInCl_(6).Herein,Sb^(3+)doped Cs_(2)NaInCl_(6)(Sb^(3+):Cs_(2)NaInCl_(6)) was synthesized and it exhibits blue emission with a photoluminescence quantum yield of up to 37.3%.Further,by employing pressure tuning,a blue stable emission under a very wide range from 2.7 GPa to 9.8 GPa is realized in Sb^(3+):Cs_(2)NaInCl_(6).Subsequently,the emission intensity of Sb^(3+):Cs_(2)NaInCl_(6) experiences a significant increase(3.3 times)at 19.0 *** is revealed that the pressure-induced distinct emissions can be attributed to the carrier self-trapping and detrapping between Cs_(2)NaInCl_(6) and Sb^(3+).Notably,the lattice compression in the cubic phase inevitably modifies the band gap of Sb^(3+):Cs_(2)NaInCl_(6).Our findings provide valuable insights into effects of the high pressure in further boosting unique emission characteristics but also offer promising opportunities for development of doped double perovskites with enhanced optical functionalities.

关键词： synthesis perovskite trapping

Road map for, and technical challenges of, carbon-nanotube integrated circuit technology

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National Science Review 2024年第3期11卷 14-16页

作者： Jia Si Panpan Zhang Zhiyong Zhang Key laboratory for the physics and Chemistry of Nanodevices and Center for Carbon-based Electronics School of Electronics Peking University State Key laboratory of Information Photonics and optical Communications Beijing University of Posts and Telecommunications

The past decade has witnessed an explosion of research on carbon-nanotube(CNT) electronics due to their outstanding properties, including an ultrathin body, a high carrier mobility and a high saturation velocity.

关键词： TRANSISTORS

Controllable transitions among phase-matching conditions in a single nonlinear crystal

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Chinese Optics Letters 2024年第2期22卷 141-147页

作者：曾梓琦尤世欣杨子祥袁晨智由成龙金锐博 Hubei Key laboratory of optical Information and Pattern Recognition Wuhan Institute of TechnologyWuhan 430205China Quantum Photonics laboratory Department of Physics and AstronomyLouisiana State UniversityBaton RougeLouisiana 70803USA

Entangled photon pairs are crucial resources for quantum information processing *** the process of spontaneous parametric downconversion(SPDC),we can generate these photon pairs using bulk nonlinear ***,the crystal is designed to satisfy a specific type of phase-matching ***,we report controllable transitions among different types of phase matching in a single periodically poled potassium titanyl phosphate *** carefully selecting pump conditions,we can satisfy different phase-matching *** allows us to observe first-order Type-II,fifth-order Type-I,third-order Type-0,and fifth-order Type-II *** temperature-dependent spectra of our source were also analyzed in ***,we discussed the possibility of observing more than nine SPDCs in this *** work not only deepens the understanding of the physics behind phase-matching conditions,but also offers the potential for a highly versatile entangled biphoton source for quantum information research.

关键词： spontaneous parametric downconversion nonlinear crystals phase-matching condition

Dynamical nonlinear excitations induced by interaction quench in a two-dimensional box-trapped Bose-Einstein condensate

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Chinese physics B 2024年第2期33卷 209-215页

作者：牛真霞高超 Department of physics Zhejiang Normal UniversityJinhua 321004China Key laboratory of optical Information Detection and Display Technology of Zhejiang Zhejiang Normal UniversityJinhua 321004China

Manipulating nonlinear excitations,including solitons and vortices,is an essential topic in quantum many-body physics.A new progress in this direction is a protocol proposed in[***.2043256(2020)]to produce dark solitons in a one-dimensional atomic Bose–Einstein condensate(BEC)by quenching inter-atomic *** by this work,we generalize the protocol to a two-dimensional BEC and investigate the generic scenario of its post-quench *** an isotropic disk trap with a hard-wall boundary,we find that successive inward-moving ring dark solitons(RDSs)can be induced from the edge,and the number of RDSs can be controlled by tuning the ratio of the after-and before-quench interaction strength across different critical *** role of the quench played on the profiles of the density,phase,and sound velocity is also *** to the snake instability,the RDSs then become vortex–antivortex pairs with peculiar dynamics managed by the initial density and the after-quench *** tuning the geometry of the box traps,demonstrated as polygonal ones,more subtle dynamics of solitons and vortices are *** proposed protocol and the discovered rich dynamical effects on nonlinear excitations can be realized in near future cold-atom experiments.

关键词： Bose-Einstein condensate quench interaction soliton vortex

λ/20-Thick cavity for mimicking electromagnetically induced transparency at telecommunication wavelengths

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Advanced Photonics 2024年第3期6卷 42-50页

作者： Hua Lu Shouhao Shi Dikun Li Shuwen Bo Jianxu Zhao Dong Mao Jianlin Zhao Northwestern Polytechnical University School of Physical Science and Technology MOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions Key Laboratory of Light-Field Manipulation and Information Acquisition Ministry of Industry and Information TechnologyShaanxi Key Laboratory of Optical Information Technology

optical cavities play crucial roles in enhanced light–matter interaction, light control, and optical communications, but their dimensions are limited by the material property and operating *** planar cavities are urgently in demand for large-area and integrated optical devices. However,extremely reducing the planar cavity dimension is a critical challenge, especially at telecommunication wavelengths. Herein, we demonstrate a type of ultrathin cavities based on large-area grown Bi2Te3topological insulator（TI） nanofilms, which present distinct optical resonance in the near-infrared region. The result shows that the Bi2Te3TI material presents ultrahigh refractive indices of >6 at telecommunication wavelengths. The cavity thickness can approach 1/20 of the resonance wavelength, superior to those of planar cavities based on conventional Si and Ge high refractive index materials. Moreover, we observed an analog of the electromagnetically induced transparency（EIT） effect at telecommunication wavelengths by depositing the cavity on a photonic crystal. The EIT-like behavior is derived from the destructive interference coupling between the nanocavity resonance and Tamm plasmons. The spectral response depends on the nanocavity thickness, whose adjustment enables the generation of obvious Fano *** experiments agree well with the simulations. This work will open a new door for ultrathin cavities and applications of TI materials in light control and devices.

关键词： Bismuth Tellurium Refractive index Nanofilms Photonic crystals Transparency Silver Telecommunications Crystals Plasmons

optical free induction decay emission carrying orbit angular momentum from ionic nitrogen enabled by multiple-photon resonance

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Chinese Optics Letters 2024年第6期22卷 177-181页

作者： Kailu Wang Haicheng Mei Jingsong Gao Liang Xu Hongbing Jiang Yi Liu Shanghai Key laboratory of Modern optical System University of Shanghai for Science and TechnologyShanghai 200093China State Key laboratory for Mesoscopic physics School of PhysicsPeking UniversityBeijing 100871China CAS Center for Excellence in Ultra-intense Laser Science Shanghai 201800China

Coherent optical emission of free induction decay (FID) excited by the multiple-photon resonance has been recently observed in nitrogen ions produced by intense femtosecond laser *** we report that orbit angular momentum (OAM) of the pump laser pulses can be transferred to the much longer pulsed free induction decay emission with the OAM *** was found that when the pump laser frequency approaches the fraction of the 391.4 nm emission (ν_(0)/5),an FID emission is emitted whereas its topological charge was identified to be 5 times of the pump *** to the reduced laser intensity with a vortex pump compared to the conventional Gaussian beam,the resonant pump laser wavelength presents a redshift,and the FID signal is significantly weaker.

关键词： air lasing orbital angular momentum free induction decay femtosecond pulses photoionization

Revisiting the spin effects induced by thermal vorticity

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Chinese physics C 2024年第5期48卷 194-208页

作者：高建华杨诗正 Shandong Key laboratory of optical Astronomy and Solar-Terrestrial Environment School of Space Science and PhysicsShandong UniversityWeihai 264209China Institute of Frontier and Interdisciplinary Science Key Laboratory of Particle Physics and Particle Irradiation(MOE)Shandong UniversityQingdao 266237China

We revisit the spin effects induced by thermal vorticity by calculating them directly from the spin-dependent distribution *** spin-1/2 particles,we provide the polarization up to the first order of thermal vorticity and compare it with the usual results calculated from the spin *** spin-1 particles,we show that all the non-diagonal elements vanish and there is no spin alignment up to the first order of thermal *** present the spin alignment at second-order contribution from thermal *** also show that the spin effects for both Dirac and vector particles receive an extra contribution when the spin direction is associated with the momentum of the particle.

关键词： relativistic heavy ion collisions global polarization quark gluon plasma

Realization of one-dimensional 2^(n)-root topological states in photonic lattices

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Science China(Technological Sciences) 2024年第1期67卷 98-104页

作者： WEI RuiShan ZHANG QingLong YANG DanDan HUANG XiongJian PAN QiWen KANG Juan QIU JianRong YANG ZhongMin DONG GuoPing State Key laboratory of Luminescent Materials and Devices and Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied TechniquesGuangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and DevicesSchool of Materials Science and EngineeringSouth China University of TechnologyGuangzhou 510640China School of physics and Optoelectronics South China University of TechnologyGuangzhou 510640China State Key laboratory of Modern optical Instrumentation College of Optical Science and EngineeringZhejiang UniversityHangzhou 310027China

Square-root topological insulators recently discovered are intriguing topological *** possess topological properties inherited from the squared Hamiltonian and exhibit double-band *** mechanism of the square root was generalized to 2^(n)-root topological insulators,giving rise to more band *** this study,we describe the experimental realization of onedimensional 2^(n)-root topological insulators in photonic waveguide arrays using the archetypical Su-Schrieffer-Heeger(SSH)*** edge states with tunable numbers are clearly observed under visible *** particular,we visualized the dynamic evolutions of the light propagation by varying the sample lengths,which further proved the localization and multiple numbers of edge states in 2^(n)-root topological *** experiment,which involves constructing 2^(n)-root topological photonic lattices in various geometric arrangements,provides a stable platform for studying topological states that exhibit a remarkable degree of flexibility and control.

关键词： 2^(n)-root topological insulators multiple edge states photonic waveguide arrays light dynamics

Designing simple non-fused terthiophene-based electron acceptors for efficient organic solar cells

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Journal of Energy Chemistry 2024年第9期96卷 501-508页

作者： Jiayu Li Kun Li Zhe Mei Yu Chen Qian Xie Chenxu Yu Xuefeng Liu Yanqi Wang Yishi Wu Qing Liao Cunbin An Hongbing Fu Beijing Key laboratory for optical Materials and Photonic Devices Department of ChemistryCapital Normal UniversityBeijing 100048China Beijing Synchrotron Radiation laboratory Institute of High Energy PhysicsChinese Academy of Sciences(CAS)Beijing 100049China

Low-cost photovoltaic materials are essential for realizing large-scale commercial applications of organic solar cells(OSCs).However,highly efficient OSCs based on low-cost photovoltaic materials are scarce due to a deficiency in understanding the structure-property ***,we investigated two low-cost terthiophene-based electron acceptors,namely,3TC8 and 3TEH,with 3,4-bis(octan-3-yloxy)thiophene,differing only in the alkylated *** acceptors exhibit low optical gaps(∼1.43 eV)and possess deep highest occupied molecular orbital(HOMO)levels(∼−5.8 eV).Notably,the single-crystal structure of 3TEH demonstrates highly planar conjugated backbone and strongπ-πstacking between intermolecular terminal groups,attributed to the presence of the bulky alkylated noncovalently conformational *** utilizing both acceptors to fabricate OSCs,the 3TC8-based device exhibited a power conversion efficiency(PCE)of 11.1%,while the 3TEH-based OSC demonstrated an excellent PCE of 14.4%.This PCE is the highest among OSCs based on terthiophene-containing electron *** results offer a new strategy for designing low-cost electron acceptors for highly efficient OSCs.

关键词： Organic solarcells Low cost Terthiophene Non-fused electron acceptor