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Interfacial engineering of the layered oxide cathode materials for sodium-ion battery

Nano research 2024年第3期17卷 1441-1464页

作者： Quanqing Zhao Ruru Wang Ming Gao Faheem KButt Jianfeng Jia Haishun Wu Youqi Zhu Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education School of Chemistry and Materials ScienceShanxi Normal UniversityTaiyuan 030032China Metals and Chemistry research Institute China Academy of Railway Sciences Corporation LimitedBeijing 100081China Department of Physics Division of Science and TechnologyUniversity of EducationLahore 54770Pakistan research Center of Materials Science Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green ApplicationsBeijing Institute of TechnologyBeijing 100081China

The layered metal oxides are reviewed as the hopeful cathode materials for high-performance sodium-ion batteries(SIBs)due to their large theoretical capacity,favorable two-dimensional(2D)ion diffusion channel,and simple ***,their cycling stability,rate capability,and thermal stability are still significantly concerned and highlighted before further practical *** chemical,mechanical and electrochemical stability of the cathode–electrolyte interfaces upon cycling is of great ***,the unique structural and electrochemical properties of the layered oxide cathode materials for SIB are *** mechanism of bulk/surface degradation induced by oxygen evolution,phase transition,microcrack,and electrolyte decomposition is thoroughly ***,the interfacial engineering to construct stable interface through various effective methods is fully *** future outlook and challenges for interfacial engineering in this filed are also *** review should shed light on the rational design and construct of robust interface for applications of superior layered oxide cathodes in SIB and may suggest future research directions.

关键词： interfacial engineering sodium-ion battery layered oxide electrolyte interface

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Modeling mass transfer of CO_2 in brine at high pressures by chemical potential gradient

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Science China Chemistry 2013年第6期56卷 821-830页

作者： JI YuanHui JI XiaoYan LU XiaoHua TU YongMing division of Energy Science Lule University of Technology State Key Laboratory of Materials-Oriented Chemical engineering Nanjing University of Technology Key Laboratory of Concrete and Prestressed Concrete Structures of Ministry of Education Southeast University division of structural engineering and bridges Royal Institute of Technology (KTH)

To investigate long-term CO2 behavior in geological formations and quantification of possible CO2 leaks, it is crucial to inves- tigate the potential mobility of CO2 dissolved in brines over a wide range of spatial and temporal scales and density distribu- tions in geological media. In this work, the mass transfer of aqueous CO2 in brines has been investigated by means of a chemi- cal potential gradient model based on non-equilibrium thermodynamics in which the statistical associating fluid theory equa- tion of state was used to calculate the fugacity coefficient of CO2 in brine. The investigation shows that the interracial concen- tration of aqueous CO2 and the corresponding density both increase with increasing pressure and decreasing temperature; the effective diffusion coefficients decrease initially and then increase with increasing pressure; and the density of the CO2-disolved brines increases with decreasing CO2 pressure in the CO2 dissolution process. The aqueous CO2 concentration profiles obtained by the chemical potential gradient model are considerably different from those obtained by the concentration gradient model, which shows the importance of considering non-ideality, especially when the pressure is high.

关键词： C02 geological sequestration dissolution non-equilibrium thermodynamics mass transport diffusion density SAFTEoS

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Study on gust alleviation control and wind tunnel test

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Science China Technological Sciences 2013年第3期56卷 762-771页

作者： WU ZhiGang CHEN Lei YANG Chao School of Aeronautic Science and engineering Beijing University of Aeronautics and Astronautics division of structural Strength Shanghai Aircraft Design and Research Institute

Aircraft are inevitably affected by gust during flight,which disturbs the regular operations of pilots and worsens the ride *** more grievous cases,flight mission cannot be completed and the flight safety may be *** order to improve the ride quality and the fatigue life of the plane structure under the affect of gust,it is necessary to explore and validate the gust alleviation *** the low-speed wind tunnel test,the gust alleviation active control technology applied to elastic aircraft is *** a large-type passenger plane configuration with high aspect ratio wing,a test system was designed and three gust alleviation control schemes with PID controllers were *** the gust alleviation control low-speed wind tunnel test was carried out in the FD-09 wind *** results showed that at certain speed and gust frequency,all of the 3 control schemes can alleviate the acceleration at fuselage and wing-tip to a certain extent,as well as the bending moment of *** gust alleviation control scheme,which uses aileron,elevator and canard as control surfaces synthetically,gives the most satisfying gust alleviation effect.

关键词： aeroelasticity aeroservoelasticity gust response gust alleviation active control wind tunnel test

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Chloride Penetration Capacity in NPP Structures caused by Crack

Chloride Penetration Capacity in NPP Structures caused by Cr...

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2011 First International Conference on High Performance Structures and Materials engineering (ICHPSM 2011)

作者： Ki-Beom Kim Do-Gyeum Kim Jang-Hwa Lee structural engineering ＆ bridges research division Korea Institute of Construction Technology

The speed of chloride penetration caused by cracking at the concrete surface is determined by the crack *** this study,the impact of the cracks that can occur on the concrete surface（occurring from the contraction during concrete curing） on the chloride penetration speed was revealed through *** accuracy of the established model was also verified through laboratory *** definition of the minimum crack width that affects the chloride penetration speed was established,based on testing and consideration of *** comparison of crack widths（20,85,125um） based on the chloride profile and model prediction showed that there is virtually no chloride penetration at 20 μm,while the chloride penetration speed increased sharply at crack widths of 85 μm and 125 μm.

关键词： Chloride penetration Concrete crack Chloride ion diffusion Chloride profile

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High-silica faujasite zeolite-tailored metal encapsulation for the low-temperature production of pentanoic biofuels

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Journal of Energy Chemistry 2024年第1期88卷 552-560,I0012页

作者： Wenhao Cui Yuanshuai Liu Pengfei Guo Zhijie Wu Liqun Kang Huawei Geng Shengqi Chu Linying Wang Dong Fan Zhenghao Jia Haifeng Qi Wenhao Luo Peng Tian Zhongmin Liu National engineering research Center of Lower-Carbon Catalysis Technology Dalian National Laboratory for Clean EnergyDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina University of Chinese Academy of Sciences Beijing 100049China Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of SciencesQingdao 266101ShandongChina College of Chemistry and Chemical engineering Inner Mongolia UniversityHohhot 010021Inner MongoliaChina State Key Laboratory of Heavy Oil Processing and Key Laboratory of Catalysis of CNPC China University of PetroleumBeijing 102249China Department of Inorganic Spectroscopy Max Planck Institute for Chemical Energy ConversionMülheim an der Ruhr 45470Germany Beijing Synchrotron Radiation Facility Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China division of Energy research Resources Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina Leibniz-Institut für Katalyse Albert-Einstein-Straβe 29aRostock 18059Germany

Zeolite-encapsulated metal nanoclusters are at the heart of bifunctional catalysts,which hold great potential for petrochemical conversion and the emerging sustainable ***,efficient encapsulation of metal nanoclusters into a high-silica zeolite Y in particular with good structural integrity still remains a significant ***,we have constructed Ru nanoclusters(~1 nm)encapsulated inside a high-silica zeolite Y(SY)with a SiO_(2)/Al_(2)O_(3) ratio(SAR)of 10 via a cooperative strategy for direct zeolite synthesis and a consecutive impregnation for metal *** with the benchmark Ru/H-USY and other analogues,the as-prepared Ru/H-SY markedly boosts the yields of pentanoic biofuels and stability in the direct hydrodeoxygenation of biomass-derived levulinate even at a mild temperature of 180℃,which are attributed to the notable stabilization of transition states by the enhanced acid accessibility and properly sized constraints of zeolite cavities owing to the good structural integrity.

关键词： High-silica zeolite Y Metal encapsulation Bifunctional catalysis Hydrodeoxygenation Biofuels

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Biomimicking synovial joints trans-scale structured AgQDs/MXene/SiOC achieving macroscale high lubrication and superior wear resistance

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Journal of Materials Science & Technology 2024年第7期174卷 63-73页

作者： Yu Zhao Hui Mei Peng Chang Yubo Yang Laifei Cheng Litong Zhang Science and Technology on Thermostructural Composite Materials Laboratory School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an710072China School of Textile Science and engineering Xi’an Polytechnic UniversityXi’an710048China

Naturally optimized successful synovial joints with lightweight,high load-carrying,ultra-low friction and wear have attracted tribological communities to constantly imitate and *** impressive advances in cartilage lubrication,extending such extraordinary performance advantages to macroscale solid lubrication remains a ***,inspired by the fascinating interplay of synovial joints,a novel kind of trans-scale hierarchical structured ceramic-based composite was ***-ducing microscale Ag microspheres(AgMs)“cartilage”layer and nanoscale Ag quantum dots/MXene(AgQDs/MXene)“synovial fluid”into the interior and exterior of printed macroscale SiOC“hard bone”realistically restores the gradient structure of synovial joint *** resulted composite with ideal compressive strength(70.44 MPa)can achieve a 60.53%friction reduction and a low wear rate(2.05×10^(−6)mm 3 N^(−1)m^(−1))in dry tribo-contact for 3600 sliding cycles,while also maintaining considerable low friction(∼0.11)over 10,000 sliding cycles and long-term stable lubrication(∼0.13)for up to 50,000 re-ciprocating *** extraordinary performance can be explained by the division of macro contacts,full loading of AgMs and AgQDs/MXene,abrasive debris capture and removal,as well as the shear rolling effect induced by friction *** work opens a new avenue to develop structural lubricating mate-rials for complex engineering applications.

关键词： 3D printing Synovial joints trans-scale structure AgQDs/MXene/SiOC High lubrication Superior wear resistance

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Fatigue Crack Propagation Law of Corroded Steel Box Girders in Long Span bridges

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Computer Modeling in engineering & Sciences 2024年第7期140卷 201-227页

作者： Ying Wang Longxiao Chao Jun Chen Songbai Jiang Key Laboratory of Concrete and Prestressed Concrete Structures of Ministry of Education School of Civil EngineeringSoutheast UniversityNanjing211189China Jiangsu Provincial engineering Construction Standard Station Nanjing210036China

In order to investigate the fatigue performance of orthotropic anisotropic steel bridge decks,this study realizes the simulation of the welding process through elastic-plastic finite element theory,thermal-structural sequential coupling,and the birth-death element *** simulated welding residual stresses are introduced into the multiscale finite element model of the bridge as the initial ***,the study explores the impact of residual stress on crack propagation in the fatigue-vulnerable components of the corroded steel box *** results indicate that fatigue cracks at the weld toe of the top deck,the weld root of the top deck,and the opening of the transverse diaphragm will not propagate under the action of a standard vehicle ***,the inclusion of residual stress leads to the propagation of these *** considering residual stress,the fatigue crack propagation paths at the weld toe of the transverse diaphragm and the U-rib weld toe align with those observed in actual *** the absence of residual stress,the cracks at the toe of the transverse diaphragm with a 15%mass loss rate are categorized as type I ***,when residual stress is considered,these cracks become I-II composite *** stress significantly alters the cumulative energy release rate of the three ***,incorporating the influence of residual stress is essential when assessing the fatigue performance of corroded steel box girders in long-span bridges.

关键词： Residual stress crack propagation corroded steel box girder cumulative energy release rate

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Data-driven approach to predict the fatigue properties of ferrous metal materials using the cGAN and machine-learning algorithms

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Advances in Manufacturing 2024年第3期12卷 447-464页

作者： Si-Geng Li Qiu-Ren Chen Li Huang Min Chen Chen-Di Wei Zhong-Jie Yue Ru-Xue Liu Chao Tong Qing Liu School of Advanced Technology Xi’an Jiaotong-Liverpool UniversitySuzhou215123JiangsuPeople’s Republic of China Key Laboratory for Light-weight Materials Nanjing Tech UniversityNanjing210009People’s Republic of China Materials Bigdata and Application division Material Academy JitriSuzhou215131JiangsuPeople’s Republic of China School of Mechanical engineering Shanghai Jiao Tong UniversityShanghai200240People’s Republic of China

The stress-life curve(S–N)and low-cycle strain-life curve(E–N)are the two primary representations used to characterize the fatigue behavior of a *** material fatigue curves are essential for structural fatigue ***,conducting material fatigue tests is expensive and *** address the challenge of data limitations on ferrous metal materials,we propose a novel method that utilizes the Random Forest Algorithm and transfer learning to predict the S–N and E–N curves of ferrous *** addition,a data-augmentation framework is introduced using a conditional generative adversarial network(cGAN)to overcome data *** incorporating the cGAN-generated data,the accuracy(R2)of the Random Forest Algorithm-trained model is improved by 0.3–*** is proven that the cGAN can significantly enhance the prediction accuracy of the machine-learning model and balance the cost of obtaining fatigue data from the experiment.

关键词： Fatigue life curve Machine learning Transfer learning Conditional generative adversarial network(cGAN)

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Chloride binding and time-dependent surface chloride content models for fly ash concrete

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Frontiers of structural and Civil engineering 2016年第1期10卷 112-120页

作者： S. MUTHULINGAM B. N. RAO Department of Civil engineering SSN College of Engineering Kalavakkam 603 110 India structural engineering division Department of Civil Engineering Indian Institute of Technology Madras Chennai 600 036 India

Corrosion of embedded rebars is a classical deterioration mechanism of reinforced concrete structures exposed to chloride environments. Such environments can be attributed to the presence of seawater, deicing or sea-salts, which have high concentrations of chloride ion. Chloride ingress into concrete, essential for inducing rebar corrosion, is a complex interaction between many physical and chemical processes. The current study proposes two chloride ingress parameter models for fly ash concrete, namely： 1） surface chloride content under tidal exposure condition; and 2） chloride binding. First, inconsistencies in surface chloride content and chloride binding models reported in literature, due to them not being in line with past research studies, are pointed out. Secondly, to avoid such inconsistencies, surface chloride content and chloride binding models for fly ash concrete are proposed based upon the experimental work done by other researchers. It is observed that, proposed models are simple, consistent and in line with past research studies reported in literature.

关键词： binding isotherms chloride ingress concrete fly ash surface chloride content

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Rethinking development and major research plans of Industrial Internet in China

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Fundamental research 2024年第1期4卷 3-7页

作者： Chunxiao Jiang Yang Cong Jiming Chen Chenghong Wang Guozheng Wu Ruizhen Zhao Zhiheng Wang Bin Xiao Ting Chen Beijing National research Center for Information Science and Technology Tsinghua UniversityBeijing 100084China Tsinghua Space Center Tsinghua UniversityBeijing 100084China State Key Laboratory of Robotics Shenyang Institute of AutomationChinese Academy of SciencesShenyang 110016China College of Control Science and engineering Zhejiang UniversityHangzhou 310027China division III Department of Information SciencesNational Natural Science Foundation of ChinaBeijing 100085China division II Department of Information SciencesNational Natural Science Foundation of ChinaBeijing 100085China Chongqing Key Laboratory of Image Cognition School of Computer Science and TechnologyChongqing University of Posts and TelecommunicationsChongqing 400065China University of Electronic Science and Technology of China Chengdu 611731China

This paper gives a definition of the Industrial Internet and expounds on the academic connotation of the future Industrial *** this foundation,we outline the development and current status of the Industrial Internet in China and ***,we detail the avant-garde paradigms encompassed within the National Natural Science Foundation of China(NSFC)’s“Future Industrial Internet Fundamental Theory and Key Technologies”research plan and its corresponding management *** research initiative endeavors to enhance interdisciplinary collaborations,aiming for a synergistic alignment of industry,academia,research,and practical *** primary focus of the research plan is on the pivotal scientific challenges inherent to the future industrial *** is poised to traverse the“first mile”,encompassing foundational research and pioneering innovations specific to the industrial internet,and seamlessly bridges to the“last mile”,ensuring the effective commercialization of scientific and technological breakthroughs into tangible industrial market *** anticipated contributions from this initiative are projected to solidify both the theoretical and practical scaffolding essential for the cultivation of a globally competitive industrial internet infrastructure in China.

关键词： Industrial Internet Academic connotation Major research plan Scientific problem Policy advice

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