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Constructing electron-blocking grain boundaries in garnet to suppress lithium dendrite growth

Journal of Advanced Ceramics 2024年第2期13卷 166-175页

作者： Xing Xiang Zecheng Fang Congkun Du Zhenzhen Zhao Jiajia Chen Yanhua Zhang Huihu Wang Chenhuinan Wei Fei Chen Qiang Shen Hubei Provincial Key Laboratory of green Materials for Light industry Hubei University of TechnologyWuhan 430068China Hubei Longzhong Laboratory Wuhan University of Technology Xiangyang Demonstration ZoneXiangyang 441000China Collaborative Innovation center of green Light-weight Materials and Processing Hubei University of TechnologyWuhan 430068China New Materials and green manufacturing Talent Introduction and Innovation Demonstration Base Hubei University of TechnologyWuhan 430068China State Key Lab of Advanced technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Li_(7)La_(3)Zr_(2)O_(12)(LLZO)is considered as a promising solid-state electrolyte due to its high ionic conductivity,wide electrochemical window,and excellent electrochemical ***,its application in solid-state lithium metal batteries(SSLMBs)is impeded by the growth of lithium dendrites in LLZO due to some reasons such as its high electronic *** this study,lithium fluoride(LiF)was introduced into Ta-doped LLZO(LLZTO)to modify its grain boundaries to enhance the performance of SSLMBs.A nanoscale LiF layer was uniformly coated on the LLZTO grains,creating a threedimensional continuous electron-blocking network at the grain *** from the electronic insulator LiF and the special structure of the modified LLZTO,the symmetric cells based on LLZO achieved a high critical current density(CCD)of 1.1 mA·cm^(-2)(in capacity-constant mode)and maintained stability over 2000 h at 0.3 mA·cm^(-2).Moreover,the full cells combined with a LiFePO_(4)(LFP)cathode,demonstrated excellent cycling performance,retaining 97.1% of capacity retention after 500 cycles at 0.5 ***,this work provides a facile and effective approach for preparing a modified electrolyte suitable for high-performance SSLMBs.

关键词： solid electrolyte garnet lithium dendrite microstructure solid-state batteries

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Simultaneous determination of typical toxic aldehydes formed during food frying and digestion using isotope dilution UHPLC-QqQ-MS/MS

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Grain & Oil Science and technology 2024年第1期7卷 42-49页

作者： Feng Wang Yun Cui Dongjie Liu Charles Brennan Soottawat Benjakul Weiwei Cheng Gengsheng Xiao Lukai Ma Key Laboratory of green Processing and intelligent manufacturing of Lingnan Specialty Food of Ministry and Rural Affairs College of Light Industry and FoodZhongkai University of Agriculture and EngineeringGuangzhou 510225China School of Science Royal Melbourne Institute of Technology UniversityMelbourneAustralia International center of Excellence in Seafood Science and Innovation Faculty of Agro-IndustryPrince of Songkla UniversitySongkhla 90110Thailand College of Food Science and technology Zhejiang University of TechnologyHangzhou 310014China

An isotope dilution ultra-performance liquid chromatography-triple quadrupole mass spectrometry method was developed to simultaneously detect two typical kinds ofα,β-unsaturated aldehydes,namely 4-hydroxy-2-hexenal(4-HHE)and 4-hydroxy-2-nonenal(4-HNE),in *** proposed method exhibited a linear range of 10-1000 ng/mL with a limit of detection of 0.1-2.0 ng/g and a limit of quantification of 0.3-5.0 ng/*** recovery rates of these typical toxic aldehydes(i.e.,4-HHE,4-HNE)and their d3-labeled analogues were 91.54%-105.12%with a low matrix ***,this proposed method was successfully applied to a real frying system and a simulated digestion system,wherein the contents of 4-HHE and 4-HNE were determined for ***,the obtained results provide strong support for further research into the production of 4-HHE and 4-HNE resulting from foods during oil digestion and frying.

关键词： UHPLC-QqQ-MS/MS 4-Hydroxy-2-hexenal 4-Hydroxy-2-nonenal Frying Simulated digestion

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Advances in sodium-ion batteries at low-temperature: Challenges and strategies

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Journal of Energy Chemistry 2024年第3期90卷 518-539,I0012页

作者： Haoran Bai Xiaohui Zhu Huaisheng Ao Guangyu He Hai Xiao Yinjuan Chen Key Laboratory of Advanced Catalytic Materials and technology Advanced Catalysis and Green Manufacturing Collaborative Innovation CenterChangzhou UniversityChangzhou 213164JiangsuChina Department of Chemistry Tsinghua UniversityBeijing 100084China

With the continuing boost in the demand for energy storage,there is an increasing requirement for batteries to be capable of operation in extreme environmental ***-ion batteries(SIBs) have emerged as a highly promising energy storage solution due to their promising performance over a wide range of temperatures and the abundance of sodium resources in the earth's *** to lithiumion batteries(LIBs),although sodium ions possess a larger ionic radius,they are more easily desolvated than lithium *** rthermore,SIBs have a smaller Stokes radius than lithium ions,resulting in improved sodium-ion mobility in the ***,SIBs demonstrate a significant decrease in performance at low temperatures(LT),which constrains their operation in harsh weather *** the increasing interest in SIBs,there is a notable scarcity of research focusing specifically on their mechanism under LT *** review explores recent research that considers the thermal tolerance of SIBs from an inner chemistry process perspective,spanning a wide temperature spectrum(-70 to100℃),particularly at LT *** addition,the enhancement of electrochemical performance in LT SIBs is based on improvements in reaction kinetics and cycling stability achieved through the utilization of effective electrode materials and electrolyte ***,the safety concerns associated with SIBs are addressed and effective strategies are proposed for mitigating these ***,prospects conducted to extend the environmental frontiers of commercial SIBs are discussed mainly from three viewpoints including innovations in materials,development and research of relevant theoretical mechanisms,and intelligent safety management system establishment for larger-scale energy storage SIBs.

关键词： Low-temperature Sodium-ion batteries Reaction kinetics Cycle stability Safety concerns of Sodium-ion batteries

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Multifunctional polyeugenol-based nanoparticles with antioxidant and antibacterial properties

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Particuology 2024年第4期87卷 194-204页

作者： Qiaoqiao Lan Xuying Zhang Jiaming Liang Wei Wang Leili Lv Jiamin He Zefeng Wang Chunsheng Qu The People's Hospital of Lishui Lishui323000China College of Ecology Lishui UniversityLishui32300China R&D center of green manufacturing New Materials and technology of Synthetic Leather Sichuan University-Lishui University Lishui323000China

Over the past few decades,extensive scientific has been dedicated to polymer synthesis employing renewable *** this study,we devised and synthesized multifunctional polyeugenol-based nanoparticles,exhibiting remarkable antioxidant and antibacterial *** grafting of eugenol onto the nanoparticle surface was achieved via a thiol-ene chemical reaction with a grafting rate of 3.5%.To comprehend the properties of the synthesized nanoparticles,we employed Fourier transform infrared spectroscopy,X-ray photoelectron spectroscopy and pyrolysis-gas chromatography mass *** scanning electron microscopic and transmission electron microscopic analyses revealed the presence of a crosslinked structure within the polyeugenol-based nanoparticles,as well as a heteroge-neous microsphere structure on the *** to the inherent crosslinking structure,the polyeugenol-based nanoparticles demonstrated robust the resistance to solvents,as ascertained through thermog-ravimetric analysis and solvent resistance ***,nitrogen adsorption/desorption studies confirmed the adsorption capacity of the polyeugenol-based nanoparticles,rendering them potentially suitable for drug transport ***,the assays for assessing cytocompatibility and reactive oxygen species scavenging activities demonstrated better performance of the eugenol-based nano-particles compared to ***,the polyeugenol-based nanoparticles exhibited certain bactericidal activities against Escherichia coli,Staphylococcus aureus,and Fusobacterium ***,these observations indicated the nontoxic nature and expansive application prospects of the polyeugenol-based nanoparticles in the domains of medicine and food *** work presented a pioneering concept for the development of antioxidant and antibacterial multifunctional polymer materials derived from eugenol.

关键词： Polyeugenol-based nanoparticles Bactericidal activities Cytocompatibility

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PSMFNet: Lightweight Partial Separation andMultiscale Fusion Network for Image Super-Resolution

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Computers, Materials and Continua 2024年第1期81卷 1491-1509页

作者： Cao, Shuai Liang, Jianan Cao, Yongjun Huang, Jinglun Yang, Zhishu Institute of intelligent manufacturing GDAS Guangdong Key Laboratory of Modern Control Technology Guangzhou 510030 China School of Mechanical & Automotive Engineering South China University of Technology Guangzhou 511442 China Faculty of Information Engineering and Automation Kunming University of Science and Technology Kunming 650500 China School of Faculty of intelligent manufacturing Wuyi University Jiangmen 529020 China

The employment of deep convolutional neural networks has recently contributed to significant progress in single image super-resolution (SISR) research. However, the high computational demands of most SR techniques hinder their applicability to edge devices, despite their satisfactory reconstruction performance. Thesemethods commonly use standard convolutions,which increase the convolutional operation cost of the model. In this paper, a lightweight Partial Separation and Multi scale Fusion Network (PSMFNet) is proposed to alleviate this problem. Specifically, this paper introduces partial convolution (PConv), which reduces the redundant convolution operations throughout the model by separating some of the features of an image while retaining features useful for image reconstruction. Additionally, it is worth noting that the existing methods have not fully utilized the rich feature information, leading to information loss, which reduces the ability to learn feature representations. Inspired by self-attention, this paper develops a multi scale feature fusion block (MFFB), which can better utilize the non-local features of an image. MFFB can learn long-range dependencies from the spatial dimension and extract features fromthe channel dimension, thereby obtaining more comprehensive and rich feature information. As the role of the MFFB is to capture rich global features, this paper further introduces an efficient inverted residual block (EIRB) to supplement the local feature extraction ability of PSMFNet. A comprehensive analysis of the experimental results shows that PSMFNet maintains a better performance with fewer parameters than the state-of-the-art models. © 2024 The Authors. Published by Tech Science Press.

关键词： Convolution

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UAV-Assisted Dynamic Avatar Task Migration for Vehicular Metaverse Services: A Multi-Agent Deep Reinforcement Learning Approach

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 430-445页

作者： Jiawen Kang Junlong Chen Minrui Xu Zehui Xiong Yutao Jiao Luchao Han Dusit Niyato Yongju Tong Shengli Xie IEEE School of Automation Guangdong University of TechnologyGuangzhou 510006China 111 center for intelligent Batch manufacturing based on IoT technology Guangzhou 510006China Key Laboratory of intelligent Information Processing and System Integration of IoT Ministry of EducationGuangzhou 510006China School of Computer Science and Engineering Nanyang Technological UniversitySingaporeSingapore Pillar of Information Systems technology and Design Singapore University of Technology and DesignSingaporeSingapore College of Communication Engineering Army Engineering University of PLANanjing 210007China National Natural Science Foundation of China Beijing 100085China Key Laboratory of intelligent Detection and IoT in manufacturing Ministry of EducationGuangzhou 510006China Guangdong Key Laboratory of IoT Information technology Guangzhou 510006China

Avatars, as promising digital representations and service assistants of users in Metaverses, can enable drivers and passengers to immerse themselves in 3D virtual services and spaces of UAV-assisted vehicular Metaverses. However, avatar tasks include a multitude of human-to-avatar and avatar-to-avatar interactive applications, e.g., augmented reality navigation,which consumes intensive computing resources. It is inefficient and impractical for vehicles to process avatar tasks locally. Fortunately, migrating avatar tasks to the nearest roadside units(RSU)or unmanned aerial vehicles(UAV) for execution is a promising solution to decrease computation overhead and reduce task processing latency, while the high mobility of vehicles brings challenges for vehicles to independently perform avatar migration decisions depending on current and future vehicle status. To address these challenges, in this paper, we propose a novel avatar task migration system based on multi-agent deep reinforcement learning(MADRL) to execute immersive vehicular avatar tasks dynamically. Specifically, we first formulate the problem of avatar task migration from vehicles to RSUs/UAVs as a partially observable Markov decision process that can be solved by MADRL algorithms. We then design the multi-agent proximal policy optimization(MAPPO) approach as the MADRL algorithm for the avatar task migration problem. To overcome slow convergence resulting from the curse of dimensionality and non-stationary issues caused by shared parameters in MAPPO, we further propose a transformer-based MAPPO approach via sequential decision-making models for the efficient representation of relationships among agents. Finally, to motivate terrestrial or non-terrestrial edge servers(e.g., RSUs or UAVs) to share computation resources and ensure traceability of the sharing records, we apply smart contracts and blockchain technologies to achieve secure sharing management. Numerical results demonstrate that the proposed approach

关键词： Avatar blockchain metaverses multi-agent deep reinforcement learning transformer UAVs

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Data Driven Vibration Control:A Review

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IEEE/CAA Journal of Automatica Sinica 2024年第9期11卷 1898-1917页

作者： Weiyi Yang Shuai Li Xin Luo Chongqing Institute of green and intelligent technology Chinese Academy of SciencesChongqing 400714 Chongqing School University of Chinese Academy of SciencesChongqing 400714China Faculty of Information technology and Electrical Engineering University of OuluOulu 90570 VTT-technology Research center of Finland Oulu 90570Finlan College of Computer and Information Science Southwest UniversityChongqing 400715China

With the ongoing advancements in sensor networks and data acquisition technologies across various systems like manufacturing,aviation,and healthcare,the data driven vibration control(DDVC)has attracted broad interests from both the industrial and academic *** shaping(IS),as a simple and effective feedforward method,is greatly demanded in DDVC *** convolves the desired input command with impulse sequence without requiring parametric dynamics and the closed-loop system structure,thereby suppressing the residual vibration *** on a thorough investigation into the state-of-the-art DDVC methods,this survey has made the following efforts:1)Introducing the IS theory and typical input shapers;2)Categorizing recent progress of DDVC methods;3)Summarizing commonly adopted metrics for DDVC;and 4)Discussing the engineering applications and future trends of *** doing so,this study provides a systematic and comprehensive overview of existing DDVC methods from designing to optimizing perspectives,aiming at promoting future research regarding this emerging and vital issue.

关键词： Data driven vibration control(DDVC) data science designing method feedforward control industrial robot input shaping optimizing method residual vibration

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Multi-functional photonic spin Hall effect sensor controlled by phase transition

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Chinese Physics B 2024年第7期33卷 336-342页

作者：程杰李瑞昭程骋张亚林刘胜利董鹏 School of Science Jiangsu Province Engineering Research Center of Low Dimensional Physics and New EnergyNanjing University of Posts and TelecommunicationsNanjing 210023China College of Electronic and Optical Engineering Nanjing University of Posts and TelecommunicationsNanjing 210023China School of Electrical Engineering Research Center of Intelligent Sensor and Network Engineering Technology of Jiangsu ProvinceNanjing Vocational University of Industry TechnologyNanjing 210023China

Photonic spin Hall effect(PSHE), as a novel physical effect in light–matter interaction, provides an effective metrological method for characterizing the tiny variation in refractive index(RI). In this work, we propose a multi-functional PSHE sensor based on VO_(2), a material that can reveal the phase transition behavior. By applying thermal control, the mutual transformation into different phase states of VO_(2) can be realized, which contributes to the flexible switching between multiple RI sensing tasks. When VO_(2) is insulating, the ultrasensitive detection of glucose concentrations in human blood is achieved. When VO_(2) is in a mixed phase, the structure can be designed to distinguish between the normal cells and cancer cells through no-label and real-time monitoring. When VO_(2) is metallic, the proposed PSHE sensor can act as an RI indicator for gas analytes. Compared with other multi-functional sensing devices with the complex structures, our design consists of only one analyte and two VO_(2) layers, which is very simple and elegant. Therefore, the proposed VO_(2)-based PSHE sensor has outstanding advantages such as small size, high sensitivity, no-label, and real-time detection, providing a new approach for investigating tunable multi-functional sensors.

关键词： photonic spin Hall effect multi-functional sensors phase transition sensing performance

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Salt reduction in cured meat products: A review on strategies and mechanisms

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Food Science and Human Wellness 2024年

作者： Qi Chen Jinxuan Cao Wenhai She Weidong Bai Xiaofang Zeng Hao Dong School of Food and Health， Beijing technology and Business University Guangzhou Luxu Food Ltd. Guangdong Provincial Key Laboratory of Lingnan Specialty Food Science and technology， Key Laboratory of green Processing and intelligent manufacturing of Lingnan Specialty Food， Ministry of Agriculture， College of Light industry and Food Sciences， Academy of Contemporary Agricultural Engineering Innovations， Zhongkai University of Agriculture and Engineering

Sodium chloride is one of the most widely used additives in meat curing. However， cured meat products contribute to a portion of the total sodium dietary intake. Consumers and researchers’ concern about excessive sodium intake has prompted the food industry to consider ways to reduce salt content of cured meat products. The aim of this review is to provide a broad but comprehensive understanding of salt reduction strategies for cured meat products. The impact and limitations of each approach were discussed. green technologies treatments， such as ultrasonic technology， high-pressure processing， seem to be potential to ensure microbiological safety in low-sodium cured meat products. However， these novel technologies can cause protein and fat oxidization in meat products. A combination of multiple treatments could give the desired effect. In addition， different parameter conditions need to be set according to the specific meat to achieve better salt reduction effect.

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Surface phonon resonance:A new mechanism for enhancing photonic spin Hall effect and refractive index sensor

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Chinese Physics B 2024年第8期33卷 254-261页

作者：程杰汪承龙李一铭张亚林刘胜利董鹏 School of Science Jiangsu Province Engineering Research Center of Low Dimensional Physics and New EnergyNanjing University of Posts and TelecommunicationsNanjing 210023China College of Electronic and Optical Engineering Nanjing University of Posts and TelecommunicationsNanjing 210023China School of Electrical Engineering Research Center of Intelligent Sensor and Network Engineering Technology of Jiangsu ProvinceNanjing Vocational University of Industry TechnologyNanjing 210023China

Metal-based surface plasmon resonance(SPR)plays an important role in enhancing the photonic spin Hall effect(SHE)and developing sensitive optical ***,the very large negative permittivities of metals limit their applications beyond the near-infrared *** this work,we theoretically present a new mechanism to enhance the photonic SHE by taking advantage of SiC-supported surface phonon resonance(SPhR)in the mid-infrared *** transverse displacement of photonic SHE is very sensitive to the wavelength of incident light and the thickness of SiC *** the optimal parameter setup,the calculated largest transverse displacement of SiC-based SPhR structure reaches up to 163.8 ym,which is much larger than the condition of ***,an NO_(2) gas sensor based on the SPhR-enhanced photonic SHE is theoretically proposed with the superior sensing *** the intensity and angle sensitivity of this sensor can be effectively manipulated by varying the damping rate of *** results may provide a promising paradigm to enhance the photonic SHE in the mid-infrared region and open up new opportunity of highly sensitive refractive index sensors.

关键词： photonic spin Hall effect refractive index sensor surface phonon resonance SiC

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