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Innovative Mn_(3-x)O_(4-y)@NCA design:Leveraging Mn/O vacancies and amorphous architecture for enhanced sodium-ion storage

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Journal of Energy Chemistry 2024年第10期97卷 747-756,I0015页

作者： Kaijun Xie Xin Liu Kai Xia Lipeng diao Ping Lu Mengmeng Wang Long Fang Yihui Zou dongjiang Yang Xiaodong Zhang College of Chemistry and Chemical Engineering College of Environmental Science and EngineeringState Key Laboratory of Bio-fibers and Eco-textilesShandong Collaborative Innovation Center of Marine Biobased Fibers and Ecological TextilesInstitute of Marine Biobased MaterialsQingdao UniversityQingdao 266071ShandongChina institute of Micro/Nano Materials and devices Ningbo University of TechnologyNingbo 315211ZhejiangChina

Manganese-based oxide electrode materials suffer from severe Jahn-Teller(J-T)distortion,leading to severe cycle instability in sodium ion ***,it is difficult to adjust the electron at d orbitals exactly to a low spin state to eliminate orbital degeneracy and suppress J-T distortion *** article constructed concentration-controllable Mn/O coupled vacancy and amorphous network in Mn_(3)O_(4) and coated it with nitrogen-doped carbon aerogel(Mn_(3-x)O_(4-y)@NCA).The existence of Mn/O vacancies has been confirmed by scanning transmission electron microscopy(STEM)and positron annihilation lifetime spectroscopy(PALS).Atomic absorption spectroscopy(AAS)and X-ray photoelectron spectroscopy(XPS)determine the most optimal ratio of Mn/O vacancies for sodium ion storage is 1:*** functional theory(dFT)calculations prove that Mn/O coupled vacancies with the ratio of 1:2could exactly induce a low spin states and a d~4 electron configuration of Mn,suppressing the J-T distortion *** abundant amorphous regions can shorten the transport distance of sodium ions,increase the electrochemically active sites and improve the pseudocapacitance *** the synergetic effect of Mn/O coupled vacancies and amorphous regions,Mn_(3-x)O_(4-y)@NCA exhibits an energy density of 37.5 W h kg^(-1)and an ultra-high power density of 563 W kg^(-1)in an asymmetric *** sodium-ion batteries,it demonstrates high reversible capacity and exceptional cycling *** research presents a new method to improve the Na^(+)storage performance in manganese-based oxide,which is expected to be generalized to other structural distortion.

关键词： Manganese-based metal oxide Concentration-controllable Mn/O coupled vacancies Amorphous network Sodium ion supercapacitor Sodium ion battery

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Inhibitory effect and mechanism of tannic acid against two starch digestive enzymes

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Food Quality and Safety 2024年第1期8卷 115-123页

作者：钟毓秀倪德让杨玉波李元一王莉田金虎杨帆叶兴乾 department of Food Science and Nutrition Zhejiang Key Laboratory for Agri-Food ProcessingFuli Institute of Food ScienceZhejiang R&D Centre for Food Technology and EquipmentZhejiang UniversityHangzhouChina institute of Science and Technology Moutai GroupZunyiChina Key Laboratory of Industrial Microbial resources development Kweichow Moutai Co.Ltd.RenhuaiChina

Backgrounds:Tannic acid(TA),as a plant-derived phenolic substance,is involved in regulating the activity of starch digestive enzymes,but its underlying mechanism remains *** and results:In the present study,inhibition rate and inhibition kinetics assays were performed and confrmed that TA had a strong inhibitory effect on bothα-amylase andα-glucosidase with IC50 values of 0.1585 mg/mL and 0.00542 mg/mL,respectively,through a mixed inhibition *** secondary structures of both enzymes were confrmed to be modifed by TA through circular dichroism(Cd)*** quenching analysis revealed that the interaction between TA and two enzymes was a static process of pontaneous complex ***,molecular docking revealed that non-covalent bonds were the main interaction forces between TA and both ***:Thus,TA was a promising candidate for the inhibition of starch-digesting enzymes,and the present research provided insight into postprandial glucose regulation through polyphenols.

关键词： Tannic acid α-amylase α-glucosidase inhibition starch digestion.

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Schur Complement Based Preconditioners for Twofold and Block Tridiagonal Saddle Point Problems

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Communications in Mathematical research 2024年第2期40卷 214-244页

作者： Mingchao Cai Guoliang Ju Jingzhi Li department of Mathematics Morgan State UniversityBaltimoreMD 21251USA. Solid state r&d department Shenzhen Tenfong Co.Ltd.Shenzhen 518055P.R.China. department of Mathematics Southern University of Science and TechnologyShenzhen 518055P.R.China.

In this paper,we consider using Schur complements to design preconditioners for twofold and block tridiagonal saddle point *** type of the preconditioners are based on the nested(or recursive)Schur complement,the other is based on an additive type Schur complement after permuting the original saddle point *** analyze different preconditioners incorporating the exact Schur *** show that some of them will lead to positively stable preconditioned systems if proper signs are selected in front of the Schur *** positive-stable preconditioners outperform other preconditioners if the Schur complements are further approximated *** experiments for a 3-field formulation of the Biot model are provided to verify our predictions.

关键词： Schur complement block tridiagonal systems positively stable preconditioners routh-Hurwitz stability criterion.

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Microstructure and Shear Properties Evolution of Minor Fe-doped SAC/Cu Substrate Solder Joint under Isothermal Aging

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Acta Metallurgica Sinica(English Letters) 2024年第7期37卷 1279-1290页

作者： Quanzhen Li Chengming Li Xiaojing Wang Shanshan Cai Jubo Peng Shujin Chen Jiajun Wang Xiaohong Yuan Jiangsu University of Science and Technology Zhenjiang212003China r&d Center Yunnan Tin Group(Holding)Co.LtdKunming650000China The 58 Research Institute of China Electronics Technology Group CorporationWuxi214100China Yunnan Precious Metals Lab Sino-Platinum Metals Co.LtdKunming650156China

different amounts of Fe(0.005,0.01,0.03,0.05,and 0.07 wt%)were added to SAC305 to study the shear behavior damage of Fe-doped SAC solder joints under thermal loading(170℃,holding time of 0,250,500,and 750 h).The results show that during isothermal aging at 170℃,the average shear force of all solder joints decreases with increasing aging time,while the average fracture energy first increases and then decreases,reaching a maximum at 500 *** Fe doping could both increase shear forces and related fracture energy,with the optimum Fe doping amount being 0.03 wt%within the entire aging *** is because the doping Fe reduces the undercooling of the SAC305 alloy,resulting in the microstructure refining of solder *** in turn causes the microstructure changing from network structure(SAC305 joint:eutectic network+β-Sn)to a single matrix structure(0.03Fe-doped SAC305 joint:β-Sn matrix+small compound particles).Specifically,Fe atoms can replace some Cu in Cu_(6)Sn_(5)(both inside the solder joint and at the interface),and then form(Cu,Fe)_(6)Sn_(5) compounds,resulting in an increase in the elastic modulus and nanohardness of the ***,the growth of Cu_(6)Sn_(5) and Cu_(3)Sn intermetallic compounds(IMC)layer are inhibited by Fe doping even after the aging time prolonging,and Fe aggregates near the interface compound to form FeSn_(2).This study is of great significance for controlling the growth of interfacial compounds,stabilizing the microstructures,and providing strengthening strategy for solder joint alloy design.

关键词： SAC305 solder Fe doping Shear mechanical behavior Isothermal aging Interfacial intermetallic compounds(IMC)

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Multi-Channel Based on Attention Network for Infrared Small Target detection

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Journal of Shanghai Jiaotong university(Science) 2024年第3期29卷 414-427页

作者：张彦军王碧云蔡云泽 department of Automation Shanghai Jiao Tong UniversityShanghai 200240China Shanghai institute of Aerospace Control Technology Shanghai 201109China Infrared detection Technology r&d Center of China Aerospace Science and Technology Corporation Shanghai 201109China Key Laboratory of System Control and Information Processing Ministry of Education of ChinaShanghai 200240China Shanghai Engineering research Center of Intelligent Control and Management Shanghai 200240China Key Laboratory of marine Intelligent Equipment and System of Ministry of Education Shanghai Jiao Tong UniversityShanghai 200240China institute of marine Equipment Shanghai Jiao Tong UniversityShanghai 200240China

Infrared detection technology has the advantages of all-weather detection and good concealment,which is widely used in long-distance target detection and tracking ***,the complex background,the strong noise,and the characteristics of small scale and weak intensity of targets bring great difficulties to the detection of infrared small targets.A multi-channel based on attention network is proposed in this paper,aimed at the problem of high missed detection rate and false alarm rate of traditional algorithms and the problem of large model,high complexity and poor detection performance of deep learning ***,given the difficulty in extracting the features of infrared multiscale and small dim targets,the multiple channels are designed based on dilated convolution to capture multiscale target ***,the coordinate attention block is incorporated in each channel to suppress background clutters adaptively and enhance target *** addition,the fusion of shallow detail features and deep abstract semantic features is realized by synthesizing the contextual attention fusion ***,it is verified that,compared with other state-of-the-art methods based on the datasets SIrST and MdFA,the proposed algorithm further improves the detection effect,and the model size and computational complexity are smaller.

关键词： infrared image small target detection deep learning attention mechanism feature fusion

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Analysis of quality-related proteins in golden pompano(Trachinotus ovatus)fillets with modified atmosphere packaging under superchilling storage

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Food Science and Human Wellness 2024年第4期13卷 2253-2265页

作者： Chuang Pan Xiaofan Zhang Shengjun Chen Yong Xue Yanyan Wu Yueqi Wang di Wang South China Sea Fisheries research institute Chinese Academy of Fishery SciencesKey Laboratory of Aquatic Product ProcessingMinistry of Agriculture and Rural AffairsNational R&D Centre for Aquatic Product ProcessingGuangzhou 510300China Co-Innovation Center of Jiangsu marine Bio-industry Technology Jiangsu Ocean UniversityLianyungang 222005China Collaborative Innovation Center of Seafood deep Processing Dalian Polytechnic UniversityDalian 116034China Key Laboratory of Efficient Utilization and Processing of marine Fishery resources of Hainan Province Sanya Tropical Fisheries Research InstituteSanya 572018China College of Food Science and Engineering Ocean University of ChinaQingdao 266003China

Here,we aimed to study the changes in proteome of golden pompano fillets during post-mortem *** mass tags(TMT)-labeled quantitative proteomic strategy was applied to investigate the relationships between protein changes and quality characteristics of modified atmosphere packaging(MAP)fillets during superchilling(-3°C)*** electron microscopy was used to show that the muscle histology microstructure of fillets was damaged to varying degrees,and low-field nuclear magnetic resonance was used to find that the immobilized water and free water in the muscle of fillets changed *** sulfhydryl content,TCA-soluble peptides and Ca2+-ATPase activity also showed that the fillet protein had a deterioration by oxidation and *** Fresh(FS),MAP,and air packaging(AP)groups were *** of 150 proteins were identified as differential abundant proteins(dAPs)in MAP/FS,while 209 dAPs were in AP/FS *** KEGG pathway analysis indicated that most dAPs were involved in binding proteins and protein *** analysis found that 52 dAPs were correlated with quality *** them,8 highly correlated dAPs are expected to be used as potential quality markers for protein oxidation and water-holding *** results provide a further understanding of the muscle deterioration mechanism of packaging golden pompano fillets during superchilling.

关键词： Tandem mass tags(TMT)proteomics Trachinotus ovatus Modified atmosphere packaging Superchilling storage Low-field nuclear magnetic resonance Protein deterioration

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The environmental analysis and site selection of mussel and large yellow croaker aquaculture areas based on high resolution remote sensing

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Acta Oceanologica Sinica 2024年第3期43卷 66-86页

作者： Lina Cai Jie Yin Xiaojun Yan Yongdong Zhou rong Tang Menghan Yu marine Science and Technology College Zhejiang Ocean UniversityZhoushan 316022China Zhejiang marine Fisheries research institute Zhejiang Ocean UniversityZhoushan 316004China

Mussel aquaculture and large yellow croaker aquaculture areas and their environmental characteristics in Zhoushan were analyzed using satellite data and in-situ surveys.A new two-step remote sensing method was proposed and applied to determine the basic environmental characteristics of the best mussel and large yellow croaker aquaculture *** methodology includes the first step of extraction of the location distribution and the second step of the extraction of internal environmental *** fishery ranching index(FrI1,FrI2)was established to extract the mussel and the large yellow croaker aquaculture area in Zhoushan,using Gaofen-1(GF-1)and Gaofen-6(GF-6)satellite data with a special resolution of 2 *** the second step,the environmental factors such as sea surface temperature(SST),chlorophyll a(Chl-a)concentration,current and tide,suspended sediment concentration(SSC)in mussel aquaculture area and large yellow croaker aquaculture area were extracted and analyzed in *** results show the following three points.(1)For the extraction of the mussel aquaculture area,FrI1 and FrI2 are complementary,and the combination of FrI1 and FrI2 is suitable to extract the mussel aquaculture *** for the large yellow croaker aquaculture area extraction,FrI2 is suitable.(2)Mussel aquaculture and the large yellow croaker aquaculture area in Zhoushan are mainly located on the side near the islands that are away from the eastern open *** water environment factor template suitable for mussel and large yellow croaker aquaculture was determined.(3)This two-step remote sensing method can be used for the preliminary screening of potential site selection for the mussels and large yellow croaker aquaculture area in the *** fishery ranching index(FrI1,FrI2)in this paper can be applied to extract the mussel and large yellow croaker aquaculture areas in coastal waters around the world.

关键词： mussel aquaculture area large yellow croaker aquaculture area high resolution satellite site selection environmental analysis

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Tracing nitrate sources in one of the world's largest eutrophicated bays(Hangzhou Bay):insights from nitrogen and oxygen isotopes

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Acta Oceanologica Sinica 2024年第6期43卷 86-95页

作者： Zhi Yang Jianfang Chen Haiyan Jin Hongliang Li Zhongqiang Ji Yangjie Li Bin Wang Zhenyi Cao Qianna Chen Key Laboratory of marine Ecosystem dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China state Key Laboratory of Satellite Ocean Environment dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China

Eutrophication caused by inputs of excess nitrogen(N) has become a serious environmental problem in Hangzhou Bay(China),but the sources of this nitrogen are not well *** this study,the August 2019 distributions of salinity,nutrients [nitrate(NO_(3)^(-)),nitrite,ammonium,and phosphate],and the stable isotopic composition of NO_(3)^(-)(δ^(15)N and δ^(18)O) were used to investigate sources of dissolved inorganic nitrogen(dIN) to Hangzhou B *** distributions of nitrate,salinity,and nitrate δ^(18)O indicate that the Qiantang river,the Changjiang river,and nearshore coastal waters may all contribute nitrate to the *** on the isotopic compositions of nitrate in these potential source waters and conservative mixing of nitrate in our study area,we suggest that the NO_(3)^(- )in Hangzhou B ay was likely derived mainly from soils,synthetic N fertilizer,and manure and ***-member modeling indicates that in the upper half of the bay,the Qiantang river was a very important dIN source,possibly contributing more than 50% of dIN in the bay head *** the lower half of the bay,dIN was sourced mainly from strongly intruding coastal *** coming directly from the Changjiang river made a relatively small contribution to Hangzhou Bay dIN in August 2019.

关键词： nitrogen isotopes oxygen isotopes nitrogen cycle nitrate sources Hangzhou Bay

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Global intensification of weak tropical cyclones in the past 30 years

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Science China Earth Sciences 2024年第2期67卷 639-640页

作者： dake CHEN state Key Laboratory of Satellite Ocean Environment dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China Southern marine Science and Engineering Guangdong Laboratory(Zhuhai) Zhuhai 519000Chin

The response of tropical cyclones(TCs)to climate change is a hot topic in ocean and atmosphere *** theoretical analysis and numerical experiments indicated that the intensity of TCs may increase with global warming(Emanuel,1987;Knutson and Tuleya,2004),which however has not been convincingly validated by presently available observations(Landsea,2005;Pielke,2005).Using a huge amount of global ocean surface drifter data,Wang et al.

关键词： tropical ocean cyclones

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A novel TNKS/USP25 inhibitor blocks the Wnt pathway to overcome multi-drug resistance in TNKS-overexpressing colorectal cancer

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Acta Pharmaceutica Sinica B 2024年第1期14卷 207-222页

作者： Hongrui Zhu Yamin Gao Liyun Liu Mengyu Tao Xiao Lin Yijia Cheng Yaoyao Shen Haitao Xue Li Guan Huimin Zhao Li Liu Shuping Wang Fan Yang Yongjun Zhou Hongze Liao Fan Sun Houwen Lin research Center for marine drugs Department of PharmacyRen Ji HospitalShanghai Jiao Tong University School of MedicineShanghai 200127China department of Oncology Shanghai General HospitalShanghai Jiao Tong University School of MedicineShanghai 200080China institute of marine drugs Guangxi University of Chinese MedicineNanning 530200China state Key Laboratory of New drug and Pharmaceutical Process Shanghai Professional and Technical Ser-vice Center for Biological Material Drug-ability EvaluationShanghai Institute of Pharmaceutical IndustryChina State Institute of Pharmaceutical IndustryShanghai 200437China institute of marine Biomedicine Shenzhen PolytechnicShenzhen 518055China

Modulating Tankyrases(TNKS),interactions with USP25 to promote TNKS degradation,rather than inhibiting their enzymatic activities,is emerging as an alternative/specific approach to inhibit the Wnt/β-catenin ***,we identified UAT-B,a novel neoantimycin analog isolated from Streptomyces conglobatus,as a small-molecule inhibitor of TNKS-USP25 protein-protein interaction(PPI)to overcome multi-drug resistance in colorectal cancer(CrC).The disruption of TNKS-USP25 complex formation by UAT-B led to a significant decrease in TNKS levels,triggering cell apoptosis through modulation of the Wnt/β-catenin ***,UAT-B successfully inhibited the CrC cells growth that harbored high TNKS levels,as demonstrated in various in vitro and in vivo studies utilizing cell line-based and patient-derived xenografts,as well as APC^(min/+)spontaneous CrC ***,these findings suggest that targeting the TNKS-USP25 PPI using a small-molecule inhibitor represents a compelling therapeutic strategy for CrC treatment,and UAT-B emerges as a promising candidate for further preclinical and clinical investigations.

关键词： Colorectal cancer TNKSeUSP25 interaction Multi-drug resistance TNKS overexpression Wnt pathway Apoptosis Neoantimycin analog

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