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Frontiers of Environmental Science & engineering 2024年第5期18卷 73-83页

作者： Marvin Yeung Lan Tian Yuhong Liu Hairong Wang Jinying Xi Environmental simulation and Pollution Control state key Joint laboratory School of EnvironmentTsinghua UniversityBeijing100084China Graduate School at Shenzhen Tsinghua UniversityShenzhen518055China

Electrochemical disinfection(ECD)is a promising disinfection technique for wastewater reclamation;however,the impacts of ECD on the microbiome in secondary effluent wastewater remain *** this study,Propidium monoazide-qPCR(PMA-qPCR)and the plate count method were used to evaluate the inactivation performance,and the PMA-16S rRNA gene sequences of living cells were targeted to study the microbiome.A discrepancy was found between PMA-qPCR and the plate count method in the evaluation of cell count,with increases of 1.5 to 2.2 orders of magnitude in the disinfection rate after 150 s of ***,the cell count recovered and occasionally exceeded original levels within 3 d after *** was suppressed after ECD,but the microbiome after 150 s disinfection retained a higher level of evenness and stability in the community with a median Shannon index(>3.7).Pathogenic bacteria remained high in relative abundance even after 150 s of 25 V disinfection,but the biofilm-forming population was effectively suppressed by *** co-occurrence network revealed a centralized and fragile network as disinfection persisted,demonstrating the destabilizing effects of ECD on the *** pathways for cell membrane synthesis and organic compound degradation were enriched after *** reaction of the microbiome after ECD was similar to other disinfection techniques in terms of community structure.

关键词： Electrochemical disinfection Secondary effluent Microbiome

Analytical solutions of turbulent boundary layer beneath forward-leaning waves

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Applied Mathematics and Mechanics(English Edition) 2024年第4期45卷 695-710页

作者： Yiqin XIE Jifu ZHOU Xu WANG Jinlong DUAN Yongjun LU Shouqian LI laboratory for Mechanics in Fluid Solid Coupling Systems Institute of MechanicsChinese Academy of SciencesBeijing 100190China state key laboratory of simulation and Regulation of Water Cycle in River Basin China Institute of Water Resources and Hydropower ResearchBeijing 100038China School of engineering Sciences University of Chinese Academy of SciencesBeijing 100049China state key laboratory of Hydrology-Water Resources and Hydraulic engineering Nanjing Hydraulic Research InstituteNanjing 210024China

As a typical nonlinear wave,forward-leaning waves can be frequently encountered in the near-shore areas,which can impact coastal sediment transport ***,it is of significance to describe the characteristics of the boundary layer beneath forward-leaning waves accurately,especially for the turbulent boundary *** this work,the linearized turbulent boundary layer model with a linear turbulent viscosity coefficient is applied,and the novel expression of the near-bed orbital velocity that has been worked out by the authors for forward-leaning waves of arbitrary forward-leaning degrees is further used to specify the free stream boundary condition of the bottom boundary ***,a variable transformation is found so as to make the equation of the turbulent boundary layer model be solved analytically through a modified Bessel ***,an explicit analytical solution of the turbulent boundary layer beneath forward-leaning waves is derived by means of variable separation and variable *** analytical solutions of the velocity profile and bottom shear stress of the turbulent boundary layer beneath forward-leaning waves are verified by comparing the present analytical results with typical experimental data available in the previous literature.

关键词： forward-leaning wave turbulent boundary layer velocity profile bottom shear stress

Highly active copper-intercalated weakly crystallized δ-MnO_(2) for low-temperature oxidation of CO in dry and humid air

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Frontiers of Environmental Science & engineering 2024年第5期18卷 127-136页

作者： Hao Zhang Huinan Li Pengyi Zhang Tingxia Hu Xianjie Wang state key Joint laboratory of Environment simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Beijing key laboratory for Indoor Air Quality Evaluation and Control Beijing100084China Midea Corporate Research Center Foshan528311China

Copper intercalated birnessite MnO_(2)(δ-MnO_(2))with weak crystallinity and high specific surface area(421 m^(2)/g)was synthesized by a one-pot redox method and investigated for low-temperature CO *** molar ratio of Cu/Mn was as high as 0.37,which greatly weakened the Mn-O bond and created a lot of low-temperature active oxygen *** situ DRIFTS revealed strong bonding of copper ions with ***-synthesized MnO_(2)-150Cu achieved 100%conversion of 250 ppm CO in normal air(3.1 ppm H_(2)O)even at−10°C under the weight-hourly space velocity(WHSV)of 150 L/(g·h).In addition,it showed high oxygen storage capacity to oxidize CO in inert *** the concurrent moisture in air significantly inhibited CO adsorption and its conversion at ambient temperature,MnO_(2)-150Cu could stably convert CO in 1.3%moisture air at 70°C owing to its great low-temperature activity and reduced competitive adsorption of water with increased *** study discovers the excellent low-temperature activity of weakly crystallized δ-MnO_(2) induced by high content intercalated copper ions.

关键词： CO oxidation Birnessite Interlayer copper Low-temperature Oxygen storage capacity

A review of rock macro-indentation:Theories,experiments,simulations,and applications

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Journal of Rock Mechanics and Geotechnical engineering 2024年第6期16卷 2351-2374页

作者： Weiqiang Xie Xiaoli Liu Xiaoping Zhang Xinmei Yang Xiaoxiong Zhou state key laboratory of Hydroscience and engineering Tsinghua UniversityBeijing100084China Yunlong Lake laboratory of Deep Underground Science and engineering Xuzhou221116China state key laboratory of Water Resources and Hydropower engineering Science Wuhan UniversityWuhan430072China

Rock macro-indentation plays a fundamental role in mechanical rock breaking for various rock engineering application,such as drilling,tunneling,cutting,and *** the past decades,extensive research has been conducted to understand the indentation mechanisms and responses through various *** review aims to provide an overview of the current status and recent advancements in theories,experiments,numerical simulations,and applications of macro-indentation in rock *** starts with elaborating on the mechanisms of macro-indentation,followed by a discussion of the merits and limitations of commonly used *** factors and their effects on indentation test results are then *** numerical simulation methods for rock macro-indentation are highlighted,along with their advantages and ***,the applications of indentation tests and indentation indices in characterizing rock properties are *** reveals that compression-tension,compression-shear,and composite models are widely employed in rock *** the compression-tension model is straightforward to use,it may overlook the anisotropic properties of *** the other hand,the composite model provides a more comprehensive description of rock indentation but requires complex ***,factors,such as indentation rate,indenter geometry,rock type,specimen size,and confining pressure,can significantly influence the indentation *** methods for macro-indentation encompass continuous medium,discontinuous medium,and continuous-discontinuous medium methods,with selection based on their differences in ***,rock macro-indentation can be practically applied to mining engineering,tunneling engineering,and petroleum drilling *** indices serve as valuable tools for characterizing rock strength,brittleness,and *** review sheds light on the development of rock macro-inde

关键词： Rock macro-indentation Indentation test Indentation indices Mechanism Rock breaking

A novel box-counting method for quantitative fractal analysis of threedimensional pore characteristics in sandstone

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International Journal of Mining Science and Technology 2024年第4期34卷 479-489页

作者： Huiqing Liu Heping Xie Fei Wu Cunbao Li Renbo Gao state key laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400030China School of Resources and safety engineering Chongqing UniversityChongqing 400030China Guangdong Provincial key laboratory of Deep Earth Sciences and Geothermal Energy Exploitation and Utilization Shenzhen UniversityShenzhen 518060China Shenzhen key laboratory of Deep Underground engineering Sciences and Green Energy College of Civil and Transportation EngineeringShenzhen UniversityShenzhen 518060China

Fractal theory offers a powerful tool for the precise description and quantification of the complex pore structures in reservoir rocks,crucial for understanding the storage and migration characteristics of media within these *** with the challenge of calculating the three-dimensional fractal dimensions of rock porosity,this study proposes an innovative computational process that directly calculates the three-dimensional fractal dimensions from a geometric *** employing a composite denoising approach that integrates Fourier transform(FT)and wavelet transform(WT),coupled with multimodal pore extraction techniques such as threshold segmentation,top-hat transformation,and membrane enhancement,we successfully crafted accurate digital rock *** improved box-counting method was then applied to analyze the voxel data of these digital rocks,accurately calculating the fractal dimensions of the rock pore *** numerical simulations of permeability experiments were conducted to explore the physical correlations between the rock pore fractal dimensions,porosity,and absolute *** results reveal that rocks with higher fractal dimensions exhibit more complex pore connectivity pathways and a wider,more uneven pore distribution,suggesting that the ideal rock samples should possess lower fractal dimensions and higher effective porosity rates to achieve optimal fluid transmission *** methodology and conclusions of this study provide new tools and insights for the quantitative analysis of complex pores in rocks and contribute to the exploration of the fractal transport properties of media within rocks.

关键词： 3D fractal analysis Fractal dimension Rock pore structure Box-counting method Permeability simulation Computational geosciences

A systematic review of the inequality of health burdens related to climate change

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Frontiers of Environmental Science & engineering 2024年第5期18卷 137-153页

作者： Xinke Song Shihui Zhang Hai Huang Qun Ding Fang Guo Yaxin Zhang Jin Li Mingyu Li Wenjia Cai Can Wang state key Joint laboratory of Environment simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Department of Earth System Science Tsinghua UniversityBeijing100084China

Climate change significantly impacts human health,exacerbating existing health inequalities and creating new *** study addresses the lack of systematic review in this area by analyzing 2440 publications,focusing on four key terms:health,disparities,environmental factors,and climate *** inclusion criteria limited the selection to English-language,peer-reviewed articles related to climate health hazards,ensuring the relevance and rigor of the synthesized *** process synthesized 65 relevant *** investigation revealed that recent research,predominantly from developed countries,has broadened its scope beyond temperature-related impacts to encompass diverse climate hazards,including droughts,extreme weather,floods,mental health issues,and the intersecting effects of Coronavirus Disease *** has highlighted exposure as the most studied element in the causal chain of climate change-related health inequalities,followed by adaptive capability and inherent *** most significant vulnerabilities were observed among populations with low socioeconomic status,ethnic minorities,and *** study further reveals research biases and methodological limitations,such as the paucity of attention to underdeveloped regions,a narrow focus on non-temperature-related hazards,challenges in attributing climate change effects,and a deficit of large-scale empirical *** findings call for more innovative research approaches and a holistic integration of physical,socio-political,and economic dimensions to enrich climate-health discourse and inform equitable policy-making.

关键词： Climate change Health impact Human well-being Inequality Vulnerability

A robust triaxial localization method of AE source using refraction path

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International Journal of Mining Science and Technology 2024年第4期34卷 521-530页

作者： Yichao Rui Jie Chen Jiongkun Chen Jiadong Qiu Zilong Zhou Wenzhong Wang Jinyang Fan state key laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400044China School of Resources and safety engineering Chongqing UniversityChongqing 400044China School of Resources Environment and safety engineering University of South ChinaHengyang 421001China School of Resources and safety engineering Central South UniversityChangsha 410083China Coal Geological Exploration Institute of Gansu Lanzhou 730030China

Acoustic emission(AE)localization algorithms based on homogeneous media or single-velocity are less accurate when applied to the triaxial localization *** the end,a robust triaxial localization method of AE source using refraction path is ***,the control equation of the refraction path is established according to the sensor coordinates and arrival ***,considering the influence of time-difference-of-arrival(TDOA)errors,the residual of the governing equation is calculated to estimate the equation ***,the refraction points in different directions are solved using Snell’s law and orthogonal ***,the source coordinates are iteratively solved by weighted correction *** feasibility and accuracy of the proposed method are verified by pencil-lead breaking *** simulation results show that the new method is almost unaffected by the refraction ratio,and always holds more stable and accurate positioning performance than the traditional method under different ratios and scales of TDOA outliers.

关键词： Acoustic emission(AE) Source localization Robust method Refraction paths Weight estimations

Evolution hydrothermal aging resistance mechanism study of zirconium and manganese doped CeO_(2)catalysts in soot catalytic combustion based on low Miller indices crystal surface effect

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Journal of Rare Earths 2024年第7期42卷 1272-1281,I0003页

作者： Zonglin Li Pan Wang Hong Ni Chengcheng Ao Lidong Zhang Hefeng Zhang Kai Li School of Automotive and Traffic engineering Jiangsu UniversityZhenjiang212013China state Environmental Protection key laboratory of Vehicle Emission Control and simulation Chinese Research Academy of Environmental ScienceBeijing100012China National Synchrotron Radiation laboratory University of Science and Technology of ChinaHefei230026China

The thermogravimetric analysis(TGA)experiments were carried out to reveal the mechanism of Zr and Mn doping on catalytic activity of CeO_(2)catalyst both fresh and after hydrothermal aging,and the lattice morphology and valence changes were characterized by means of Brunauer-Emmett-Teller(BET)method,X-ray diffraction(XRD),X-ray photoelectron spectroscopy(XPS),and H_(2)-temperature programmed reduction(H_(2)-TPR).Density functional theory(DFT)and molecular thermodynamics calculations were applied to investigate the change in catalytic activity,crystal surface energy and crystal morphology caused by hydrothermal *** maximum reaction rate temperature of fresh Mn/CeO_(2)(389℃)is similar to that of CeO_(2)(371℃)and lower than that of Zr/CeO_(2)(447℃),but the catalytic performance of CeO_(2)decreases more severely after hydrothermal *** catalyst crystals show different degrees of crystal surface migration after hydrothermal aging,which leads to the reduction of Ce^(3+)/Ce^(4+) ratio and the active sites *** calculations indicate that the doping of Zr and Mn reduces the surface energy of the low Miller indices surface and increases the oxygen vacancy formation energy,leading to better thermal stability and lower catalytic *** Zr and Mn doping also changes the adsorption energy and Gibbs free energy of H_(2)O,which dominates the migration of(111)to(110)and(100)in the vapor *** crystal surface migration mechanism of CeO_(2)catalysts doped with Zr and Mn induced by H_(2)O molecules at high temperature obtained in this study can provide a valuable addition to the regeneration of CeO_(2)catalysts in the after-treatment systems of diesel engines.

关键词： Soot CeO_(2)-based catalyst CDPF Rare earth metal oxides DFT calculations

Automated Identification of Ordered Phases for simulation Studies of Block Copolymers

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Chinese Journal of Polymer Science 2024年第5期42卷 683-692,I0011页

作者： Yu-Chen Zhang Wei-Ling Huang Yi-Xin Liu state key laboratory of Molecule engineering of Polymers Department of Macromolecular ScienceFudan UniversityShanghai200433China

In unit cell simulations,identification of ordered phases in block copolymers(BCPs)is a tedious and time-consuming task,impeding the advancement of more streamlined and potentially automated research *** this study,we propose a scattering-based automated identification strategy(SAIS)for characterization and identification of ordered phases of BCPs based on their computed scattering *** approach leverages the scattering theory of perfect crystals to efficiently compute the scattering patterns of periodic morphologies in a unit *** the first stage of the SAIS,phases are identified by comparing reflection conditions at a sequence of Miller *** confirm or refine the identification results of the first stage,the second stage of the SAIS introduces a tailored residual between the test phase and each of the known candidate ***,our strategy incorporates a variance-like criterion to distinguish background species,enabling its extension to multi-species BCP *** has been demonstrated that our strategy achieves exceptional accuracy and robustness while requiring minimal computational ***,the approach allows for real-time expansion and improvement to the candidate phase library,facilitating the development of automated research workflows for designing specific ordered structures and discovering new ordered phases in BCPs.

关键词： Block copolymer Phase identification Scattering function

Analysis of multi-objective optimisation method for main insulation structure configuration scheme of valve-side winding of ultra-high voltage converter transformer considering multi-field coupling

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High Voltage 2024年第2期9卷 296-308页

作者： Lijun Yang Zhidong Cheng Li Cheng Ruijin Liao state key laboratory of Power Transmission Equipment Technology School of Electrical EngineeringChongqing UniversityChongqingChina

Because DC conductivities of oil-paper materials can be easily affected by electric field and temperature,the electrical properties under electro-thermal coupling of oil-paper materials should be considered when optimising the insulation structure of valve-side winding of the converter *** on the finite element multi-physical field coupling simulation,the multi-objective optimisation of main insulation structure of valve-side winding is carried *** view of the high time consuming of multi-physical field calculation and the actual needs of an insulation structure optimisation,the Kriging method and technique for order preference by similarity to the ideal solution(TOPSIS)method are introduced,and combines them with NSGA-II to obtain a joint algorithm that can be used for the optimisation of insulation structure of the converter *** using the joint algorithm of multi-objective optimisation,the insulation structure configuration scheme of valve-side winding is *** can be seen from the experiment result that,on the one hand,the joint algorithm adopted can obtain the insulation structure configuration scheme that meets the design *** the other hand,when facing the configuration scheme optimisation under multi-field coupling,the computational time required by this method is only 0.15%of that required by original genetic algorithm.

关键词： converter insulation coupling