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Wetland and habitat dynamics in the evolving landscape of the Middle Yangtze River Basin

Journal of Geographical sciences 2025年第1期35卷 88-111页

作者： YANG Peng SUN Kaiya ZHU Yanchao XIA Jun HUANG Heqing SONG Jingxia SHI Xiaorui LU Xixi Hubei key laboratory of Regional Ecology and Environmental Change School of Geography and Information Engineering China University of Geosciences Department of Geography National University of Singapore state key laboratory of water resources and hydropower engineering science Wuhan University

Wetlands play a critical role in the global environment. The Middle Yangtze River Basin(MYRB), known for its abundant wetland resources, has experienced notable changes resulting from the complex interplay of environmental factors. Therefore, we investigated the spatiotemporal characteristics of wetland ecological quality in the MYRB from 2001 to *** the random forest(RF) regression algorithm and patch-generated land-use simulation(PLUS) model, we forecasted variations in wetland habitat quality and their determinants under the Shared Socioeconomic Pathway-Representative Concentration Pathway(SSPRCP) framework from 2035 to 2095. The main findings are as follows:(1) The RF algorithm was optimal for land-use and land-cover(LULC) classification in the MYRB from 2001 to 2020,when notable changes were observed in water bodies and buildings. However, the forested area exhibited an increase and decrease of 3.9% and 1.2% under the SSP1-2.6 and SSP5-8.5 scenarios, respectively, whereas farmland exhibited a diminishing trend.(2) Wetlands were primarily concentrated in the central and eastern MYRB, with counties in the southwest exhibiting superior ecological-environmental quality from 2001 to 2020. Notably,wetland coverage revealed significantly high level, significant changes, frequent but relatively minor changes under the SSP1-2.6, SSP2-4.5, and SSP 5-8.5 scenarios, respectively.(3)Regions with lower habitat quality were primarily concentrated in urbanized areas characterized by frequent human activities, indicating a clear degradation in habitat quality across different scenarios. In conclusion, we established a foundational framework for future investigations into the eco-hydrological processes and ecosystem quality of watersheds.

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Evapotranspiration and its components partitioning based on an improved hydrological model: historical attributions and future projections

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Journal of Earth science 2025年

作者： Hong Du Sidong Zeng Yongyue Ji Jun Xia College of resources and Environmental science， South-Central Minzu university Chongqing Institute of Green and Intelligent Technology， Chinese Academy of sciences Chongqing School， university of Chinese Academy of sciences state key laboratory of water resources and hydropower engineering science， wuhan university

Estimation and attribution of evapotranspiration （ET） and its components under changing environment is still a challenge but is essential for understanding the mechanisms of water and energy transfer subsequently regional water resources management. In this study， an improved hydrological model is developed to estimate evapotranspiration and its components i.e.， evaporation （E） and transpiration （T） by integrated the advantages of hydrological modeling constrained by water balance and the water-carbon close relationships. Results show that the improved hydrological model could captures ET and its components well in the study region. During the past years， annual ET and E increase obviously about 2.40mm/a and 1.42mm/a， particularly in spring and summer accounting for 90%. T shows less increasement and mainly increases in spring while it decreases in summer. Precipitation is the dominant factor and contributes 74.1% and 90.0% increases of annual ET and E， while the attribution of T changes is more complex by coupling of the positive effects of precipitation， rising temperature and interactive influences， the negative effects of solar diming and elevated CO2. In the future， ET and its components tend to increase under most of the Shared Socioeconomic Pathways （SSP） scenarios except for T decreases under the very high emissions scenario （SSP5-8.5） based on the projections. From seasonal perspective， the changes of ET and the components are mainly in spring and summer accounting for 75%， while more slightly changes are found in autumn and winter. This study highlights the effectiveness of estimating ET and its components by improving hydrological model within water-carbon coupling relationships， and more complex mechanisms of transpiration changes than evapotranspiration and evaporation changes under the interactive effects of climate variability and vegetation dynamics. Besides， decision makers should pay attention to the more increases in the undesirable E than desirab

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Small modifications of endo-functionalized cavities lead to large changes in molecular interaction in water

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science China Chemistry 2025年第1期68卷 369-376页

作者： Song-Meng Wang Hao Nian Yan-Fang Wang Li-Shuo Zheng Yu-Tao Zheng Yi-Wei Dong Liping Huang Xiaoping Wang Wei Jiang Liu-Pan Yang Department of Chemistry Southern University of Science and Technology School of Chemistry and Pharmaceutical sciences State Key Laboratory for Chemistry and Molecular Engineering of Medicinal ResourcesGuangxi Normal University School of Pharmaceutical science Hengyang Medical School University of South China

Studying molecular recognition in aqueous environments is crucial for understanding biological processes. Herein, we present a series of N-doped endo-functionalized anthracene-based cavities by introducing inward-directed pyridine units. The subtle modifications can significantly affect the binding properties of these receptors, which is similar to the mutations in biological systems. Combining theoretical calculations and molecular recognition experiments demonstrated that these “mutations” have an impact on the hydrophobicity and charge distribution of the hosts, consequently significantly influencing molecular *** is crucial for understanding the intricate mechanisms of molecular-level interactions in biological receptors.

关键词： host-guest interaction hydrophobic effect endo-functionalized cavity mutation pyridine

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Merging polymers of intrinsic microporosity and porous carbon-based zinc oxide composites in novel mixed matrix membranes for efficient gas separation

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Green Energy & Environment 2025年第1期10卷 203-213页

作者： Muning Chen Jiemei Zhou Jing Ma Weigang Zheng Guanying Dong Xin Li Zhihong Tian Yatao Zhang Jing Wang Yong Wang School of Chemical engineering Zhengzhou UniversityZhengzhou450001HenanChina state key laboratory of Materials-Oriented Chemical engineering and College of Chemical engineering Nanjing Tech UniversityNanjing211816JiangsuChina Singapore Membrane Technology Centre Nanyang Environment and Water Research InstituteNanyang Technological UniversitySingapore637141Singapore engineering Research Center for Nanomaterials Henan UniversityKaifeng475004HenanChina state key laboratory of Coking Coal resources Green Exploitation Zhengzhou UniversityZhengzhou 450001China School of Energy and Environment Southeast UniversityNanjing210096JiangsuChina

Mixed matrix membranes(MMMs)have demonstrated significant promise in energy-intensive gas separations by amalgamating the unique properties of fillers with the facile processability of ***,achieving a simultaneous enhancement of permeability and selectivity remains a formidable challenge,due to the difficulty of achieving an optimal match between polymers and *** this study,we incorporate a porous carbon-based zinc oxide composite(C@ZnO)into high-permeability polymers of intrinsic microporosity(PIMs)to fabricate *** dipole–dipole interaction between C@ZnO and PIMs ensures their exceptional compatibility,mitigating the formation of non-selective voids in the resulting ***,C@ZnO with abundant interconnected pores can provide additional low-resistance pathways for gas transport in *** a result,the CO_(2) permeability of the optimized C@ZnO/PIM-1 MMMs is elevated to 13,215 barrer,while the CO_(2)/N_(2) and CO_(2)/CH4 selectivity reached 21.5 and 14.4,respectively,substantially surpassing the 2008 Robeson upper ***,molecular simulation results further corroborate that the augmented membrane gas selectivity is attributed to the superior CO_(2) affinity of C@*** summary,we believe that this work not only expands the application of MMMs for gas separation but also heralds a paradigm shift in the application of porous carbon materials.

关键词： Mixed matrix membranes Polymers of intrinsic microporosity CO_(2)separation Porous carbon materials

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Innovative dual-mode device integrating capacitive desalination and solar vapor generation for high-efficiency seawater desalination

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Journal of Energy Chemistry 2025年第1期100卷 171-179页

作者： Jiacheng Wang Zhaoyu Chen Ruduan Yuan Jiaxin Luo Ben Zhang Keju Ji Meng Li Juanxiu Xiao Kuan Sun National Innovation Center for Industry-Education Integration of Energy Storage Technology MOE Key Laboratory of Low-grade Energy Utilization Technologies and SystemsCollege of Energy & Power Engineering Chongqing University Xuefeng Mountain Energy Equipment Safety National Observation and Research Station CQU-NUS Renewable Energy Materials & Devices Joint Laboratory Chongqing University Southwest Technology and engineering Research Institute Jiangsu Provincial key laboratory of Bionic Functional Materials College of Mechanical and Electrical Engineering Nanjing University of Aeronautics and Astronautics state key laboratory of Marine resources Utilization in South China Sea Collaborative Innovation Center of Marine Science and Technology School of Marine Science and Engineering Hainan University

Solar-driven interface evaporation with high solar-to-steam conversion efficiency has shown great potential in seawater ***,due to the influence of latent heat and condensation efficiency,the water yield from solar-driven interface evaporation remains insufficient,posing a significant challenge that requires *** this work,we designed a dual-mode high-flux seawater desalination device that combines solar-driven interface evaporation and capacitive *** utilizing coupled desalination materials exhibiting both photothermal conversion and capacitance activity,the device demonstrated photothermal evaporation rates of 1.41 and 0.97 kg m-2h-1for condensate water yield under one-sun ***,the device exhibited a salt adsorption capacity of up to48 mg g-1and a salt adsorption rate of 2.1 mg *** addition,the salt adsorption capacity increased by approximately 32% under one-sun ***,photo-enhanced capacitive desalination performance was explored through numerical simulations and theoretical *** calculations and characterizations confirmed that the defect energy levels formed by the introduction of sulfur vacancies can effectively widen the light absorption range,improve photothermal conversion performance,and stimulate more photoelectrons to participate in capacitive ***,the electron distribution state of molybdenum disulfide with sulfur vacancies and surface defect sites contributes to ion/electron transport at the solid-liquid *** work provides a novel pathway for integrating solar vapor generation with other low-energy desalination technologies.

关键词： Desalination

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Deciphering water Oxidation Catalysts:The Dominant Role of Surface Chemistry over Reconstruction Degree in Activity Promotion

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Nano-Micro Letters 2025年第3期17卷 340-354页

作者： Li An Jianyi Li Yuanmiao Sun Jiamin Zhu Justin Zhu Yeow Seow Hong Zhang Nan Zhang Pinxian Xi * Zhichuan JXu Chun‑Hua Yan state key laboratory of Applied Organic Chemistry Key Laboratory of Nonferrous Metal Chemistry and Resources Utilization of Gansu ProvinceFrontiers Science Center for Rare IsotopesCollege of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou 730000People’s Republic of China School of Materials science and engineering Nanyang Technological UniversitySingapore 639798Singapore Faculty of Materials science and Energy engineering Institute of Technology for Carbon NeutralityShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055People’s Republic of China key laboratory of Electromagnetic Materials and Devices National Center for International Research On Photoelectric and Energy MaterialsSchool of Materials and EnergyElectron Microscopy CenterYunnan UniversityKunming 650091People’s Republic of China state key laboratory of Baiyunobo Rare Earth Resource Researches and Comprehensive Utilization Baotou Research Institute of Rare EarthsBaotou 014030People’s Republic of China Beijing National laboratory for Molecular sciences State Key Laboratory of Rare Earth Materials Chemistry and ApplicationsPKU‑HKU Joint Laboratory in Rare Earth Materials and Bioinorganic ChemistryPeking UniversityBeijing 100871People’s Republic of China

water splitting hinges crucially on the availability of electrocatalysts for the oxygen evolution *** surface reconstruction has been widely observed in perovskite catalysts,and the reconstruction degree has been often correlated with the activity ***,a systematic study on the roles of Fe substitution in activation of perovskite LaNiO_(3)is *** substituting Fe content influences both current change tendency and surface reconstruction ***_(0.9)Fe_(0.1)O_(3)is found exhibiting a volcano-peak intrinsic activity in both pristine and reconstructed among all substituted perovskites in the LaNi_(1-x)Fe_(x)O_(3)(x=0.00,0.10,0.25,0.50,0.75,1.00)*** reconstructed LaNi_(0.9)Fe_(0.1)O_(3)shows a higher intrinsic activity than most reported NiFe-based ***,density functional theory calculations reveal that Fe substitution can lower the O 2p level,which thus stabilize lattice oxygen in LaNi0.9Fe0.1O3 and ensure its long-term ***,it is vital interesting that activity of the reconstructed catalysts relied more on the surface chemistry rather than the reconstruction *** effect of Fe on the degree of surface reconstruction of the perovskite is decoupled from that on its activity enhancement after surface *** finding showcases the importance to customize the surface chemistry of reconstructed catalysts for water oxidation.

关键词： Oxygen evolution reaction Perovskite oxides Doping Activation and reconstruction

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Three-dimensional prediction of reservoir water temperature by the lattice Boltzmann method: Validation

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Journal of Hydrodynamics 2015年第2期27卷 248-256页

作者：刁伟程永光张春泽吴家阳 state key laboratory of water resources and hydropower engineering science Wuhan University

The water temperature stratification in large reservoirs might have serious ecological and environmental consequences. The modeling of the temperature distribution and its history is of great importance both for studying the underlying mechanisms and for controlling the adverse effects. To develop an effective and efficient method for simulation of temporal and spatial temperature variations, a lattice Boltzmann method（LBM） model for 3-D thermal buoyancy flows is proposed and validated by the temperature data measured in a model reservoir. This paper discusses important aspects of the LBM and its turbulence model, analyzes the gravity sinking mechanism of cold currents, and demonstrates the complexity of the temperature redistribution process. Good agreement between the simulated and measured results shows that the newly developed method is feasible and powerful, and it will be used for the water temperature prediction in actual reservoirs in a near future.

关键词： lattice Boltzmann method(LBM) thermal buoyancy reservoir water temperature multi-dimensional simulation

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The mechanical energy equation for total flow in open channels

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Journal of Hydrodynamics 2014年第3期26卷 416-423页

作者：刘士和范敏薛娇 state key laboratory of water resources and hydropower engineering science Wuhan University

The mechanical energy equation is a fundamental equation of a 1-D mathematical model in Hydraulics and engineering Fluid Mechanics. This equation for the total flow used to be deduced by extending the Bernoulli＇s equation for the ideal fluid in the streamline to a stream tube, and then revised by considering the viscous effect and integrated on the cross section. This derivation is not rigorous and the effect of turbulence is not considered. In this paper, the energy equation for the total flow is derived by using the Navier-Stokes equations in Fluid Mechanics, the results are as follows：（1） A new energy equation for steady channel flows of incompressible homogeneous liquid is obtained, which includes the variation of the turbulent kinetic energy along the channel, the formula for the mechanical energy loss of the total flow can be determined directly in the deduction process.（2） The theoretical solution of the velocity field for laminar flows in a rectangular open channel is obtained and the mechanical energy loss in the energy equation is calculated. The variations of the coefficient of the mechanical energy loss against the Reynolds number and the width-depth ratio are obtained.（3） The turbulent flow in a rectangular open channel is simulated using 3-D Reynolds averaged equations closed by the Reynolds stress model（RSM）, and the variations of the coefficient of the mechanical energy loss against the Reynolds number and the width-depth ratio are discussed.

关键词： open channel mechanical energy equation steady flow turbulent flow

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Flow characteristics of rectangular open channels with compound vegetation roughness

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Applied Mathematics and Mechanics(English Edition) 2016年第3期37卷 341-348页

作者： Yuhong ZENG Wenxin HUAI Mingdeng ZHAO state key laboratory of water resources and hydropower engineering science Wuhan University

An idealized parallel flow caused by a lateral bed roughness difference due to the partial vegetation across a channel is investigated. Similar to the flow in a compound channel, there are mixing layers adjacent to the interface between the vegetation and the non-vegetation lanes, and a lateral momentum exchange occurs between the slow- moving water in the former lane and the fast-moving water in the latter lane. Under a uniform flow condition, the three-dimensional with different discharges and water depths are （3D） instantaneous velocities of two cases measured with a 16 MHz acoustic Doppler velocimeter （micro ADV）. The longitudinal variation of the streamwise velocity and the vertical variation of the Reynolds stress are analyzed. A quadrant analysis is carried out to investigate the outward and inward interaction, ejection, and sweep phenomenon caused by the vegetation variation across the channel. The results show that the flow characteristics in the vegetation lane are similar to those in an open channel fully covered with submerged vegetation, and the flow characteristics in the smooth non-vegetation lane are similar to those in a free open channel. For the cases studied here, the width of the mixing region is about 10~ of the channel width, and the mixing region is mainly on the non-vegetation half.

关键词： vegetated flow lateral momentum exchange acoustic Doppler velocimeter(ADV) mixing layer quadrant analysis

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Effect of vegetation on flow structure and dispersion in strongly curved channels

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Journal of Hydrodynamics 2015年第2期27卷 286-291页

作者：李成光薛万云槐文信 state key laboratory of water resources and hydropower engineering science Wuhan University

The effect of vegetation on the flow structure and the dispersion in a 180 o curved open channel is studied. The Micro ADV is used to measure the flow velocities both in the vegetation cases and the non-vegetation case. It is shown that the velocities in the vegetation area are much smaller than those in the non-vegetation area and a large velocity gradient is generated between the vegetation area and the non-vegetation area. The transverse and longitudinal dispersion coefficients are analyzed based on the experimental data by using the modified N- zone models. It is shown that the effect of the vegetation on the transverse dispersion coefficient is small, involving only changes of a small magnitude, however, since the primary velocities become much more inhomogeneous with the presence of the vegetation, the longitudinal dispersion coefficients are much larger than those in the non-vegetation case.

关键词： vegetation curved open channel flow velocity transverse dispersion coefficient longitudinal dispersion coefficient

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