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Molecular Plant 2024年第3期17卷 460-477页

作者： Fan Xu Long Wang Yingbin Li Junfeng Shi Dorothee Staiger Feng Yu state key laboratory of Chemo/Biosensing and Chemometrics College of Biologyand Hunan Key Laboratory of Plant Functional Genomics and Developmental RegulationHunanUniversityChangsha 410082P.R.China state key laboratory of Hybrid rice Hunan Agricultural Biotechnology Research InstituteHunan Academy of Agricultural SciencesChangsha 410125P.R.China rNA Biology and Molecular Physiology Faculty of BiologyBielefeld University33615 BielefeldGermany

Changes in ambient temperature profoundly affect plant growth and ***,the molecu-larbasis of plant acclimation to temperature fluctuation is of great *** this study,we discovered that GLYCINE-rICH rNA-BINDING PrOTEIN 7(GrP7)contributes to cold and heat tolerance in Arabidopsis *** found that exposure to a warm temperature rapidly induces GrP7 condensates in planta,which can be reversed by transfer to a lower *** biology and biochemical assays revealed that GrP7 undergoes liquid-liquid phase separation(LLPS)in vivo and in *** of GrP7 in the cyto-plasm contributes to the formation of stress granules that recruit rNA,along with the translation machinery component eukaryotic initiation factor 4E1(elF4E1)and the mrNA chaperones COLD SHOCK PrOTEIN 1(CSP1)and CSP3,to inhibit ***,natural variations in GrP7 affecting the residue phos-phorylated by the receptorkinase FErONIA alter its capacity to undergo LLPS and correlate with the adap-tation of some Arabidopsis accessions to a widertemperature *** together,ourfindings illustrate the role of translational control mediated by GrP7 LLPS to confer plants with temperature resilience.

关键词： fluctuating temperature glycine-rich rNA-binding protein phase separation cold shock proteins translation

Hollow Multi-shelled Structure Photoelectric Materials: Multiple Shells Bring Novel Properties

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Chemical research in Chinese Universities 2024年第3期40卷 413-427页

作者： SU Fengmei WAN Jiawei WANG Dan state key laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing 100190P.R.China University of Chinese Academy of Sciences Beijing 100049P.R.China key laboratory of Biopharmaceutical Preparation and Delivery Chinese AcademyofSciencesBeijing 100049P.R.China

Hollow multi-shelled structures(HoMSs)have made significant strides across a wide spectrum of scientific investigations since the inception of the sequential templating approach(STA)in 2009,revealing distinctive temporal-spatial ordering *** recent establishment of a mathematical model for STA has not only demystified the formation of concentration waves within the STA process but also extended its relevance to gentler solutionbased systems,thereby broadening the HoMs ***,focusing on photoelectric applications,this review first summarizes the unique temporal-spatial ordering features of ***,the greatly enhanced properties of light capture and absorption,exciton separation,and transfer are deeply ***,we conclude with a perspective on the potential challenges and burgeoning opportunities that lie ahead in the advancement of HoMs development.

关键词： Hollow multi-shelled structure Photoelectric conversion Sequential templating approach Light absorption Chargetransfer

Hollow Multishelled Structure reviving Lithium Metal Anode for High-energy-density Batteries

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Chemical research in Chinese Universities 2024年第3期40卷 428-436页

作者： WANG Haoyu WEI Peng WANG Jiangyan WANG Dan state key laboratory of Biochemical Engineering Institute of Process EngineeringChinese Academy of SciencesBeIjing 100190P.R.China University of Chinese Academy of Sciences Beijing 100049P.R.China key laboratory of Biopharmaceutical Preparation and Delivery Chinese Academy of SciencesBeijing 100190P.R.China

Due to its highest theoretical capacity and its lowest redox potential,lithium(Li)metal has been considered as the ultimate anode choice for high-energy-density rechargeable ***,its commercialization is severely hindered by its poor cyclic stability and safety *** material structure design concepts have been raised to address these failure models,wherein,hollow structure has shown great power in solving the ***,a hollow multishelled structure(HoMs)featured with two or more shells has been proved to be more efficient to improve Li metal anode than their single-shelled ***,this up-to-date review summarizes the recent progress of the application of HoMs in Li metal anode,including their adoption as Li metal host,artificial solid electrolyte interphase film,electrolyte additive,solid state electrolyte,*** offers unique advantages,such as suppressing Li dendrite growth,stabilizing electrode-electrolyte interface,and improving overall battery *** research directions are outlined,emphasizing the need for multifunctional integrated smart HoMS design and large-scale fabrication of HoMS through low-cost accurate method to further advance the commercialization of Li metal batteries.

关键词： Hollow multishelled structure Lithium metal anode Solid electrolyte interphase Coulombic efficiency Cyclic stability

Enzyme-driven Nanorobots Walking Along Predesigned Tracks on the DNA Origami for Cargo Transport and Catalysis

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Chemical research in Chinese Universities 2024年第2期40卷 333-342页

作者： NIE Cunpeng MA Tianran CHEN Tingting CHU Xia state key laboratory of Chemo/Bio-Sensing and Chemometrics College of Chemistry and Chemical EngineeringHunan UniversityChangsha410082P.R.China

In molecular engineering,designing and synthesizing molecular machines with capable of performing complex tasks,remains a formidable *** is an excellent candidate for building molecular robots because it is highly ***,we present an artificial nanorobot,in which a DNA cube serves as the inert‘body’,and nucleic acid catalysts based on an enzymatic nicking reaction act as the‘legs’for *** nanorobot can execute a series of actions,such as‘start’,‘turn’,and‘stop’when it walks along a predefined *** performance could be confirmed and monitored by using an atomic force microscope(AFM)and fluorescence *** by biological machines,we artificially designed a series of specialized tasks that combined walking with control of cargo transport and ***-time fluorescence kinetics curves provide monitoring signals for cargo transport and catalytic *** work can enrich the toolbox of DNA machinery and has great potential for engineering molecular nanofactories.

关键词： DNA origami DNA nanorobot Controlled cargo transport DNAzyme catalysis

Uncovering the largest negative carbon isotope excursion in Earth history

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Science China Earth Sciences 2024年第3期67卷 885-889页

作者： Chao LI Haiyang WANG state key laboratory of Oil and Gas reservoir Geology and Exploitation Chengdu University of TechnologyChengdu 610059China Institute of Sedimentary Geology Chengdu University of TechnologyChengdu 610059China key laboratory of Deep-time Geography and Environment reconstruction and Applications of Ministry of Natural resources Chengdu University of TechnologyChengdu 610059China International Center for Sedimentary Geochemistry and Biogeochemistry research Chengdu University of TechnologyChengdu 610059China state key laboratory of Biogeology and Environmental Geology China University of GeosciencesWuhan 430074China

The carbon cycle plays a pivotal role in regulating Earth’s surface environment through atmospheric-oceanic acid-base and redox processes, functioning as the engine driving the evolution of our planet’s surface. A deep understanding of the carbon cycle’s evolution is thus essential for our understanding of the evolution of our planet’s habitability.

关键词： carbon planet evolution

Imaging of human parafoveal area with large field of view in adaptive optics line scanning ophthalmoscope

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Journal of Innovative Optical Health Sciences 2024年第6期17卷 41-51页

作者： Wen Kong Yiwei Chen Guohua Shi Yi He Department of Biomedical Engineering University of Science and Technology of ChinaHefei 230041P.R.China Jiangsu key laboratory of Medical Optics Suzhou Institute of Biomedical Engineering and TechnologyChinese Academy of SciencesSuzhou 215163P.R.China Center for Excellence in Brain Science and Intelligence Technology Chinese Academy of SciencesShanghai 200031P.R.China key laboratory of Myopia of state Health Ministry and Key Laboratory of Visual Impairment and Restoration of ShanghaiShanghai 200003P.R.China

The parafoveal area,with its high concentration of photoreceptors andfine retinal capillaries,is crucial for central vision and often exhibits early signs of pathological *** current adaptive optics scanning laser ophthalmoscope(AOSLO)provides an excellent tool to acquire accurate and detailed information about the parafoveal area with cellular ***,limited by the scanning speed of two-dimensional scanning,thefield of view(FOV)in the AOSLO system was usually less than or equal to 2,and the stitching for the parafoveal area required dozens of images,which was time-consuming and ***,almost half of patients are unable to obtain stitched images because of their *** solve this problem,we integrate AO technology with the line-scan imaging method to build an adaptive optics line scanning ophthalmoscope(AOLSO)system with a larger *** the AOLSO,afocal spherical mirrors in pairs are nonplanar arranged and the distance and angle between optical elements are optimized to minimize the aberrations,two cylinder lenses are orthogonally placed before the imaging sensor to stretch the point spread function(PSF)for su±ciently digitizing light *** human retinal images show the whole parafoveal area with 55FOV,60 Hz frame rate and cellular *** advantage of the 5FOV of the AOLSO,only 9 frames of the retina are captured with several minutes to stitch a montage image with an FOV of 99,in which photoreceptor counting is performed within approximately 5*** AOLSO system not only provides cellular resolution but also has the capability to capture the parafoveal region in a single frame,which offers great potential for noninvasive studying of the parafoveal area.

关键词： Adaptive optics line scanning retinal imaging system parafoveal capillary vasculature.

Integrating Neighborhood Geographic Distribution and Social Structure Influence for Social Media User Geolocation

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Computer Modeling in Engineering & Sciences 2024年第9期140卷 2513-2532页

作者： Meng Zhang Xiangyang Luo Ningbo Huang key laboratory of Cyberspace Situation Awareness of Henan Province Zhengzhou450001China state key laboratory of Mathematical Engineering and Advanced Computing Zhengzhou450001China

Geolocating social media users aims to discover the real geographical locations of users from their publicly available data,which can support online location-based applications such as disaster alerts and local content *** relationship-based methods represent a classical approach for geolocating social ***,geographically proximate relationships are sparse and challenging to discern within social networks,thereby affecting the accuracy of user *** address this challenge,we propose user geolocation methods that integrate neighborhood geographical distribution and social structure influence(NGSI)to improve geolocation ***,we propose a method for evaluating the homophily of locations based on the k-order neighbor-hood geographic distribution(k-NGD)similarity among *** are notable differences in the distribution of k-NGD similarity between location-proximate and non-location-proximate *** this distinction,we filter out non-location-proximate social relationships to enhance location homophily in the social *** better utilize the location-proximate relationships in social networks,we propose a graph neural network algorithm based on the social structure *** algorithm enables us to perform a weighted aggregation of the information of users’multi-hop neighborhood,thereby mitigating the over-smoothing problem of user features and improving user geolocation *** results on real social media dataset demonstrate that the neighborhood geographical distribution similarity metric can effectively filter out non-location-proximate social ***,compared with 7 existing social relationship-based user positioning methods,our proposed method can achieve multi-granularity user geolocation and improve the accuracy by 4.84%to 13.28%.

关键词： User geolocation social media neighborhood geographic distribution structure influence

The late Early-Paleozoic granitic magmatism in Northwestern Fujian, China: constraints on intraplate orogeny in the South China block

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Acta Geochimica 2024年第1期43卷 134-149页

作者： WanLi Gao ZongXiu Wang Institute of Geomechanics Chinese Academy of Geological ScienceBeijing 100081People’s Republic of China key laboratory of Paleomagnetism and Tectonic reconstruction of Ministry of Natural resources Beijing 100081People’s Republic of China

The Early Paleozoic tectono-thermal event was a significant orogenic activity during the Phanerozoic era,which had a profound impact on the early crust of the South China Block(SCB) and established the foundation for later tectonic *** Wuyi-Yunkai orogenic belt in Southeastern China was extensively exposed to Early Paleozoic magmatism,the genetic mechanism of which remains *** shed light on this issue,detailed petrological,geochemical,and zircon U-Pb-Hf isotopic studies were carried out on two granitoids,namely the Yuntongshan pluton and the Gaoqiao pluton,identified in the central *** U-Pb chronology of the Yuntongshan and Gaoqiao bodies yielded ages of437±4 Ma(MSWD=2.2) and 404±2 Ma(MSWD=12),respectively,indicating that they were emplaced during the Early Silurian and Early Devonian *** granitoids are primarily composed of biotite-granite and biotite-monzonitic-granites,with high concentrations of S_(i)O_(2)(73.59-75.91 wt%),K_(2)O+Na_(2)O(8.31-8.73wt%),and low contents of MgO,CaO,Cr,*** are classified as high-K calc-alkaline and weakly metaluminous-strongly peraluminous S-type *** granitoids are enriched in light rare earth elements(LrEEs) and large ion lithophile elements(LILEs) and depleted in heavy rare earth elements(HrEEs) and high field strength elements(HFSEs) with arc *** εHf(t) values of-3.3 to-15.4 with two-stage Hf model ages ranging from 2829 to 1644 Ma,combined with the presence of Neoproterozoic inherited zircons,suggest that the primary magma of these granitoids was derived from the partial melting of Neoproterozoic crust with a Paleoproterozoic crustal model *** findings,combined with the spatio-temporal distribution of regional magmatism,reveal that the late Early-Paleozoic granitoids formed in the intraplate orogenic background originating from the subduction of the proto-Tethys Ocean and proto-Pacific Ocean around the margin of the east Gondwana supercontinent.

关键词： Late Early-Paleozoic Granites Intraplate orogeny Cathysian block Zircon U-Pb-Hf Isotopic composition

Vanadium(V) Complexes Containing Unsymmetrical N-Heterocyclic Carbene Ligands: Highly Efficient Synthesis and Catalytic Behavior towards Ethylene/Propylene Copolymerization

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Chinese Journal of Polymer Science 2024年第1期42卷 32-41,I0006页

作者： Yi-Cong Wang Hui Zhat Pei-Yi Cheng Shu Zhang Xiang-Wei Liu Yi-Xian Wu state key laboratory of Chemical resource Engineering Beijing University of Chemical TechnologyBejing 100029China

The highly efficient method has been developed for the synthesis of NHC·VOCl_(3) containing symmetrical or unsymmetrical Nheterocyclic carbene(NHC) ligands by the transmetallation reaction of NHC·AgCl with VOCl_(3).The total isolated yield of VOCl_(3)[1,3-(2,4,6-Me_(3)C_(6)H_(2))_(2)(NCH=)_(2)C:](V4') reached 86% by transmetallation reaction,which is much higher than that(48%) by direct coordination *** methodology has also been used to synthesize the novel vanadium complexes containing unsymmetrical NHC ligands of VOCl_(3)[PhCH_(2)NCH=CHNr)C:](V5',r=2,4,6-Me_(3)C_(6)H_(2);V6',r=2,4-Me_(2)-6-Ph-C_(6)H_(2);V7',r=2,6-^(i)Pr_(2)-C_(6)H_(3)) with high yield,which could not be obtained by direct coordination *** catalytic activity and copolymerization ability would be improved by introducing unsymmetrical NHC ligands due to their less steric bulky *** vanadium complex V5' containing unsymmetrical NHC ligand exhibits higher catalytic activity(3.7×10^(5)g_(copolymer)·mol^(-1) of V·h^(-1)) than that of V4' containing symmetrical NHC ***,the higher propylene incorporation ratio(45.6 mol%) in the copolymers of ethylene with propylene could be obtained by using V5' than that(39.9%) by using V4'.The results would provide a highly efficient strategy for the synthesis of early transition metal complexes containing versitile NHC ligands,affording the catalyst with both high catalytic activity and copolymerization ability for the synthesis of high performance polyolefin elastomers.

关键词： Vanadium complex N-heterocyclic carbene ligand Transmetallation reaction Copolymerization of ethylene with propylene

Effects of physical properties of supercritical water on heat transfer characteristics of single particle within a particle cluster Author links open overlay panel

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Particuology 2024年第8期91卷 291-302页

作者： Xiaoyu Li Bowei Zhang Huibo Wang Hui Jin state key laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an710049China

The complex physical properties of supercritical water(SCW)make the heat transfer characteristics of particles within a particle cluster *** heat transfer characteristics of single particle within a particle cluster in SCW,influenced by surrounding particles,have not been effectively *** numerical simulations were conducted to investigate the heat transfer characteristics of particle clusters in SCW under different *** results were compared and analyzed with those from constant property *** was found that reynolds number(re)and the void fraction of particle cluster have no special effects on the variation trends of Nusselt number(Nu)for the focused ***,the particle temperature had a significant effect on the variation trends of *** effect of re on the heat transfer rate exponent(η)of the focused particle can be divided into two zones:a significant effect zone and a non-significant effect *** effect of void fraction onηin the non-significant effect zone was *** the non-significant effect zone,ηdecreased with the increasing particle *** the significant effect zone,the variation trends ofηbecame more *** fundamental reason for this series of phenomena is the changes in distribution of physical properties.A model forηwas developed for the non-significant effect *** model can filter out the effects of re and certain particle cluster spatial configurations,and it demonstrates good predictive performance.

关键词： Supercritical water Particle cluster Heat transfer characteristics Heat transfer rate exponent Physical properties correction