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Emerging probing perspective of two-dimensional materials physics:terahertz emission spectroscopy

Light(Science & Applications) 2024年第7期13卷 1278-1298页

作者： Yifei Wu Yuqi Wang Di Bao Xiaonan Deng Simian Zhang Lin Yu-chun Shengxian Ke Jianing Liu Yingjie Liu Zeli Wang Pingren Ham Andrew Hanna Jiaming Pan Xinyue Hu Zhengcao Li Ji Zhou Chen Wang state key laboratory of New ceramics and fine processing Key Laboratory of Advanced Materials of Ministry of EducationSchool of Materials Science and EngineeringTsinghua University100084 BeijingChina Beijing advanced Innovation Center for Integrated Circuits 100084 BeijingChina

Terahertz(THz)emission spectroscopy(TES)has emerged as a highly effective and versatile technique for investigating the photoelectric properties of diverse materials and nonlinear physical processes in the past few ***,research on two-dimensional(2D)materials has experienced substantial growth due to their atomically thin structures,exceptional mechanical and optoelectronic properties,and the potential for applications in flexible electronics,sensing,and ***,these materials offer advantages such as tunable bandgap,high carrier mobility,wideband optical absorption,and relatively short carrier *** applying TES to investigate the 2D materials,their interfaces and heterostructures,rich information about the interplay among photons,charges,phonons and spins can be unfolded,which provides fundamental understanding for future *** it is timely to review the nonlinear processes underlying THz emission in 2D materials including optical rectification,photon-drag,high-order harmonic generation and spin-to-charge conversion,showcasing the rich diversity of the TES employed to unravel the complex nature of these *** applications based on THz emissions,such as THz lasers,ultrafast imaging and biosensors,are also *** further,we analyzed the unique advantages of spintronic terahertz emitters and the future technological advancements in the development of new THz generation mechanisms leading to advanced THz sources characterized by wide bandwidth,high power and integration,suitable for industrial and commercial *** continuous advancement and integration of TES with the study of 2D materials and heterostructures promise to revolutionize research in different areas,including basic materials physics,novel optoelectronic devices,and chips for post-Moore’s era.

关键词： optoelectronic versatile exceptional

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Grain size refinement of additive manufactured Ce-TZP ceramics by coupled two-step pre-sintering and HIP

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Journal of advanced ceramics 2024年第5期13卷 621-629页

作者： Ruoshi Zhao Hongbing Yang Xintong Liu Hezhen Li Chang-An Wang Jing Ma Yanhao Dong state key Lab of New ceramics and fine processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

Ceria-stabilized tetragonal zirconia polycrystal(Ce-TZP)has exceptional fracture toughness and flaw tolerance due to facile t‒m phase transformation ***,its wider-range applications are limited by its relatively low strength due to its large grain size and low transformation stress,which results in yield-like ***,we combined additive manufacturing(AM),pressureless two-step sintering,and hot isostatic pressing(HIP),and addressed the challenging grain size refinement problem in *** successfully produced dense ultrafine-grained Ce-TZP ceramics with an average grain size below 500 nm,a three-point bending strength above 800 MPa,and a single-edge-notch-beam fracture toughness in the range of 11‒12 MPa·m^(1/2).The critical roles of processing design,mixed Ce valences,and ***-stabilization of tetragonal polymorphs were *** work offers insights and strategies for the future development of stronger and tougher Ce-TZP ceramics that can compete with tetragonal yttria-stabilized zirconia in various applications,including additive manufacturing.

关键词： zirconia additive manufacturing(AM) two-step sintering hot isostatic pressing(HIP) grain size refinement

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3D-shaped 3D-continuously graphene cellulose(3D^(2)GC)architecture

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Nano Research 2024年第7期17卷 6695-6699页

作者： Abdelrahman Brakat Hongwei Zhu state key Lab of New ceramics and fine processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

In the endeavor to develop three-dimensional(3D)-architected sophisticated hierarchical structures,the synergy between inplane and out-of-plane interactions at interfaces offers new *** interplay,governed by van der Waals(vdW)interfacial nanoarchitectonics,facilitates the design of efficient thermally conductive *** work delves into the kinetics underlying a dual-templating strategy,seamlessly integrating two-dimensional(2D)-graphene sheets with one-dimensional(1D)-cellulose chains at heterointerfaces,thereby transforming into 3D-shaped and 3D-continuously anisotropic structures,termed as(3D^(2)GC)***,we designed and fabricated an anisotropic graphene cellulose scaffold(GCS)employing a nickel *** as-grown GCS replicates the 3D-shaped and configuration of the *** 3D-continuously interconnected fibrous-porous network of the GCS,combined with its anisotropic thermal properties(λ_(axial)/λ_(radial)),not only is promising for advanced thermal technologies but also offers advantages in cost-effectiveness and eco-effectiveness.

关键词： two-dimensional(2D)-graphene one-dimensional(1D)-cellulose heterointerface anisotropic three-dimensional(3D)-architecture

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Interfacial Oxygen Octahedral Coupling-Driven Robust Ferroelectricity in Epitaxial Na_(0.5)Bi_(0.5)TiO_(3)Thin Films

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Research 2024年第2期2023卷 149-157页

作者： Haojie Han Qinghua Zhang Wei Li Yiqun Liu Jiasheng Guo Yue Wang Qian Li Lin Gu Ce-Wen Nan Jing Ma state key laboratory of New ceramics and fine processing Schoolof Materials Science and EngineeringTsinghua UniversityBeijing 100084China Beijing National laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China

The oxygen octahedral rotation(OOR)forms fundamental atomic distortions and symmetries in perovskite oxides and definitely determines their properties and ***,epitaxial strain and interfacial structural coupling engineering have been developed to modulate the OOR patterns and explore novel properties,but it is difficult to distinguish the 2 ***,different symmetries are induced in Na_(0.5)Bi_(0.5)TiO_(3)(NBT)epitaxial films by interfacial oxygen octahedral coupling rather than epitaxial *** NBT film grown on the Nb:SrTiO_(3)substrate exhibits a paraelectric tetragonal phase,while with La_(0.5)Sr_(0.5)MnO_(3)as a buffer layer,a monoclinic phase and robust ferroelectricity are obtained,with a remanent polarization of 42μC cm^(-2)and a breakdown strength of 7.89 MV cm^(-1),which are the highest record among NBT-based ***,the interfacial oxygen octahedral coupling effect is demonstrated to propagate to the entire thickness of the film,suggesting an intriguing long-range *** work provides a deep insight into understanding the structure modulation in perovskite heterostructures and an important avenue for achieving unique functionalities.

关键词： effect. interfacial coupling

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Control of interfacial reaction and defect formation in Gd/Bi_(2)Te_(2.7)Se_(0.3)composites with excellent thermoelectric and magnetocaloric properties

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Chinese Physics B 2024年第8期33卷 474-481页

作者：薛天畅魏平刘承姗李龙舟朱婉婷聂晓蕾赵文俞 state key laboratory of advanced Technology for Materials Synthesis and processing Wuhan University of TechnologyWuhan 430070China

The method to combine thermoelectric(TE)and magnetocaloric(MC)cooling techniques lies in developing a new material that simultaneously possesses a large TE and good MC cooling *** this work,using n-type Bi_(2)Te_(2.7)Se_(0.3)(BTS)as the TE base material and Gd as the second-phase MC material,Gd/BTS composites were prepared by the spark plasma sintering *** the composites,interfacial reaction between Gd and BTS was identified,resulting in the formation of Gd Te,which has a large impact on the electron concentration through the adjustment of defect *** MC/TE composite containing 2.5 wt%Gd exhibited a ZT value of 0.6 at 300 K,essentially retaining the original TE performance,while all the composites largely maintained the excellent MC performance of *** work provides a potential pathway to achieving high performance in MC/TE composites.

关键词： thermo-electro-magnetic energy conversion materials interfacial reaction thermoelectric performance magnetic entropy change

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Exceptional electrostrain with minimal hysteresis and superior temperature stability under low electric field in KNN-based lead-free piezoceramics

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Journal of advanced ceramics 2024年第3期13卷 364-372页

作者： Huan Liu Yijin Hao Ziqi Yang Tianyi Feng Bin Su Xin Zhang Mengping Xue Bo-Ping Zhang Jing-Feng Li Beijing Municipal key laboratory of New Energy Materials and Technologies School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China state key laboratory of New ceramics and fine processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

Over the past two decades,(K_(0.5)Na_(0.5))NbO_(3)(KNN)-based lead-free piezoelectric ceramics have made significant ***,attaining a high electrostrain with remarkable temperature stability and minimal hysteresis under low electric fields has remained a significant *** address this long-standing issue,we have employed a collaborative approach that combines defect engineering,phase engineering,and relaxation *** LKNNS-6BZH ceramic,when sintered at T_(sint)=1170℃,demonstrates an impressive electrostrain with a d_(33) value of 0.276%and 1379 pm·V^(-1)under 20 kV·cm^(-1),which is comparable to or even surpasses that of other lead-free and Pb(Zr,Ti)O_(3)***,the electrostrain performance of this ceramic remains stable up to a temperature of 125℃,with the lowest hysteresis observed at 9.73%under 40 kV·cm^(-1).These excellent overall performances are attributed to the presence of defect dipoles involving V′_(A)-V∙∙_(O) and B′_(Nb)-V∙∙O,the coexistence of R-O-T multiphase,and the tuning of the trade-off between long-range ordering and local *** work provides a lead-free alternative for piezoelectric actuators and a paradigm for designing piezoelectric materials with outstanding comprehensive performance under low electric fields.

关键词： lead-free piezoelectric ceramics temperature stability electrostrain potassium sodium niobate low hysteresis

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Effect of Molecular Weight on Thermoelectric Performance of P3HT Analogues with 2-Propoxyethyl Side Chains

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Journal of Wuhan University of Technology(Materials Science) 2024年第2期39卷 268-281页

作者：董得福 WANG Wei ZHAN Chun LI Chenglong ZHOU Qisheng 肖生强 state key laboratory of advanced Technology for Materials Synthesis and processing Wuhan University of TechnologyWuhan 430070China

By replacing hexyl chains in poly(3-hexylthiophene)(P3HT)with 2-propoxyethyls,four poly(3-(2-propoxyethyl)thiophene)(P3POET)homopolymers with comparable polydispersity indexes(PDI)and regioregularities were prepared herein in addition with step increment of about 7 kDa on numberaverage molecular weight(M_(n))from around 11 to 32 kDa(accordingly denoted as P11k,P18k,P25k,and P32k).When doped in film by FeCl_(3)at the optimized conditions,the maximum power factor(PF_(max))increases greatly from 4.3μW·m^(-1)·K^(-2)for P11k to 8.8μW·m^(-1)·K^(-2)for P18k,and further to 9.7μW·m^(-1)·K^(-2)for P25k,followed by a slight decrease to 9.2μW·m^(-1)·K^(-2)for *** close Seebeck coefficients(S)at PF_(max)are observed in these doped polymer films due to their consistent frontier orbital energy levels and Fermi *** main contribution to this PF_(max)evolution thus comes from the corresponding conductivities(σ).Theσvariation of the doped films can be rationally correlated with their microstructure evolution.

关键词： conjugated polymer molecular weight microstructure thermoelectric performance

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Microstructure Regulation and Combustion Performance Optimization of PVDF/Al Composite Powder by Non-covalent Functionalized Graphenes

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 904-911页

作者：易卓然 DENG Haoyuan QIN Mei 孙一 LUO Guoqiang state key laboratory of advanced Technology for Materials Synthesis and processing Wuhan University of TechnologyWuhan 430070China

Graphene prepared by non-covalent modification of sulfonated poly(ether-ether-ketone)(SPG)was combined with polyvinylidene fluoride(PVDF)/Al to improve the PVDF/Al thermal conductivity while reducing the effect of the thermal resistance at the graphene-polymer *** regulation rule of SPG with different contents on the energy release of fluorine-containing system was *** the content of SPG is 4%,the peak pressure and rise rate of SPG/PVDF/Al composite powder during ignition reach the maximum of 4845.28 kPa and 8683.58 kPa/*** the content of SPG is 5%,the PVDF/Al composite powder is completely coated by SPG,and the calorific value of the material reachs the maximum of 29.094 kJ/*** the design and micro-control of the composite powder,the calorific value of the material can be effectively improved,but the improvement of the mass release rate still depends on the graphene content and surface modification state.

关键词： energetic materials PVDF/Al composites graphene modification energy release combustion

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Spontaneous anchoring Cl into α-Co（OH）2 as efficient and stable oxygen reduction electrocatalysts for seawater battery

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Rare Metals 2024年第7期43卷 3074-3083页

作者： Wang Zheng Xue-Rong Zheng Qi Lu Yan-Hui Cao Yang Wang Hai-Peng Fu Jin-Feng Zhang Yi-Da Deng Wen-Bin Hu School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin University state key laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan University key laboratory of Electromagnetic processing of Materials Ministry of EducationNortheastern University

Seawater battery is an advanced energy storage system that enables conversion of chemical energy to electricity by consuming metals,dissolved oxygen and seawater in anode,cathode and electrolyte,***,the oxygen reduction reaction（ORR） activity and stability of electrocatalysts can be easily deactivated due to the severe Cl-permeation and corrosion in seawater ***,we developed a structural buffer engineering strategy by spontaneously anchoring Cl-into α-Co（OH）2as efficient and stable ORR electrocatalysts,in which the ultrathin α-Co（OH）2nanosheets were synthesized using an ultrafast solution high-temperature shock（SHTS） *** large lattice space（～ 0.8 nm） of layered α-Co（OH）2ensured the spontaneously penetration of Cl-into the lattice structure and replaced part of OH-to form α-Co（OH）*** continuous leaching and compensating of saturated Cl in α-Co（OH）2-xClxcould enhance the Cl-corrosion resistance and modulate electronic structure of Co metallic sites,thus improving the ORR electrocatalytic activity and stability in seawater *** α-Co（OH）2-xClxseawater batteries display superior onset and half-wave potentials of 0.71 and 0.66 V,respectively,which are much better than the counterparts of α-Co（OH）2and of β-Co（OH）2with no Cl-penetrating and no buffer *** α-Co（OH）2-xClx-based seawater batteries display stable open-circuit potential of 1.69 V and outstanding specific capacity of 1345 mAh·g-1.

关键词： Seawater battery Oxygen reduction electrocatalyst Solution high-temperature shock Structural buffer engineering

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Engineering neuroregenerative microenvironment via aligned hydrogel-assisted magnetic stimulation for complete spinal cord injury repair

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Engineered Regeneration 2024年第2期5卷 139-152页

作者： Chun-Yi Yang Zhe Meng Zhijun He Pengchao Ma Zhaohui Hou Kunkoo Kim Jingsong Lu Kaiyuan Yang Guihuai Wang Xiumei Wang state key laboratory of New ceramics and fine processing Key Laboratory of Advanced Materials of Ministry of EducationSchool of Materials Science and EngineeringTsinghua UniversityBeijing 100084China Department of Neurosurgery Beijing Tsinghua Changgung HospitalSchool of Clinical MedicineTsinghua UniversityBeijing102218China

Utilizing biomaterials in tissue engineering has shown considerable promise for tissue regeneration,particularly through delivering multimodel cell-regulatory signals,including the material-related signals and extrinsic *** this research,we developed a magnetic-responsive aligned nanofiber fibrin hydrogel(MAFG),integrating the structured alignment of nanofibers and the pliability of fibrin hydrogel with an external magnetic *** design aimed to enhance the regenerative response in spinal cord injury treatment.A medium-strength magnetic field,aligned with the spinal cord,was applied to aid motor function recovery in rats with spinal cord *** use of MAFG in this context not only intensified the effect of the magnetic field but also encouraged the activation and differentiation of native neural stem ***,this method effectively steered macrophage polarization towards a beneficial M2 phenotype,addressing immune dysregulation at the injury *** parallel application of magnetic field stimulation through MAFG in a spinal cord injury model contributed to the concurrent promotion of neurogenesis,angiogenesis,and immunomodulation,resulting in marked improvement in motor function in *** investigation underscores the therapeutic potential of magnetic field stimulation and highlights how aligning this stimulation with the spinal cord can significantly enhance the regenerative milieu at the injury site.

关键词： Angiogenesis Neurogenesis Immunomodulation Magnetic-responsive hydrogel Magnetic stimulation

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