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A virtual thermometer for ultrahigh-temperature-pressure experiments in a large-volume press

Matter and Radiation at Extremes 2024年第4期9卷 98-110页

作者： Bingtao Feng Longjian Xie Xuyuan Hou Shucheng Liu Luyao Chen Xinyu Zhao Chenyi Li Qiang Zhou Kuo Hu Zhaodong Liu Bingbing Liu state key laboratory of Superhard Materials Synergetic Extreme Condition User FacilityCollege of PhysicsJilin UniversityChangchun 130012China Department of Earth Sciences University College LondonLondon WC1E 6BSUnited Kingdom Earth and Planetary laboratory Carnegie Institute for ScienceWashingtonDistrict of Columbia 20015USA College of Earth Sciences Jilin UniversityChangchun 130012China

Ultrahigh-temperature-pressure experiments are crucial for understanding the physical and chemical properties of *** recent development of boron-doped diamond(BDD)heaters has made such melting experiments possible in large-volume ***,estimates of temperatures above 2600 K and of the temperature distributions inside BDD heaters are not well constrained,owing to the lack of a suitable ***,we establish a three-dimensional finite element model as a virtual thermometer to estimate the temperature and temperature field above 2600 *** advantage of this virtual thermometer over those proposed in previous studies is that it considers both alternating and direct current heating modes,the actual sizes of cell assemblies after compression,the effects of the electrode,thermocouple and anvil,and the heat dissipation by the pressure-transmitting *** virtual thermometer reproduces the power-temperature relationships of ultrahigh-temperature-pressure experiments below 2600 K at press loads of 2.8-7.9 MN(~19 to 28 GPa)within experimental *** temperatures above 2600 K predicted by our virtual thermometer are within the uncertainty of those extrapolated from power-temperature relationships below 2600 ***,our model shows that the temperature distribution inside a BDD heater(19-26 K/mm along the radial direction and<83 K/mm along the longitudinal direction)is more homogeneous than those inside conventional heaters such as graphite or LaCrO_(3) heaters(100-200 K/mm).Our study thus provides a reliable virtual thermometer for ultrahigh-temperature experiments using BDD heaters in Earth and material sciences.

关键词： virtual ultrahigh sizes

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Hierarchical vectorization for facial images

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Computational Visual Media 2024年第1期10卷 97-118页

作者： Qian Fu Linlin Liu Fei Hou Ying He School of Computer Science and Engineering Nanyang Technological University639798SingaporeSingapore Data61 Commonwealth Scientific and Industrial Research OrganisationSydney2015Australia Interdisciplinary Graduate School Nanyang Technological University and Alibaba Group639798SingaporeSingapore state key laboratory of Computer Science Institute of SoftwareChinese Academy of SciencesBeijing100190China University of Chinese Academy of Sciences Beijing100049China

The explosive growth of social media means portrait editing and retouching are in high *** portraits are commonly captured and stored as raster images,editing raster images is non-trivial and requires the user to be highly *** at developing intuitive and easy-to-use portrait editing tools,we propose a novel vectorization method that can automatically convert raster images into a 3-tier hierarchical *** base layer consists of a set of sparse diffusion curves(DCs)which characterize salient geometric features and low-frequency colors,providing a means for semantic color transfer and facial expression *** middle level encodes specular highlights and shadows as large,editable Poisson regions(PRs)and allows the user to directly adjust illumination by tuning the strength and changing the shapes of *** top level contains two types of pixel-sized PRs for high-frequency residuals and fine details such as pimples and *** train a deep generative model that can produce high-frequency residuals *** to the inherent meaning in vector primitives,editing portraits becomes easy and *** particular,our method supports color transfer,facial expression editing,highlight and shadow editing,and automatic *** quantitatively evaluate the results,we extend the commonly used FLIP metric(which measures color and feature differences between two images)to consider *** new metric,illumination-sensitive FLIP,can effectively capture salient changes in color transfer results,and is more consistent with human perception than FLIP and other quality measures for portrait *** evaluate our method on the FFHQR dataset and show it to be effective for common portrait editing tasks,such as retouching,light editing,color transfer,and expression editing.

关键词： face editing vectorization Poisson editing color transfer illumination editing expression editing

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Synthesis and Diameter-dependent Thermal Conductivity of InAs Nanowires

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Nano-Micro Letters 2014年第4期6卷 301-306页

作者： Pinyun Ren Xiaoli Zhu Jinyun Han Jinyou Xu Liang Ma Honglai Li Xiujuan Zhuang Hong Zhou Qinglin Zhang Minggang Xia Anlian Pan key laboratory for Micro-Nano Physics and Technology of Hunan Province State Key Laboratory of Chemo/Biosensing and Chemometrics College of Physics and Microelectronics Science Hunan University Condensed Matter Physics laboratory Center on Experimental Physics School of Science Xi’an Jiaotong University

In this work, we synthesized high-quality In As nanowires by a convenient chemical vapor deposition method,and developed a simple laser heating method to measure the thermal conductivity of a single In As nanowire in air. During the measurement, a focused laser was used to heat one end of a freely suspended nanowire, with its other end embedded into a carbon conductive adhesive. In order to obtain the thermal conductivity of In As nanowires, the heat loss in the heat transfer process was estimated, which includes the heat loss through air conduction, the heat convection, and the radiation loss. The absorption ratio of the laser power in the In As nanowire was calculated. The result shows that the thermal conductivity of In As nanowires monotonically increases from 6.4 W m-1K-1to 10.5 W m-1K-1with diameters increasing from 100 nm to 190 nm, which is ascribed to the enhanced phonon-boundary scattering.

关键词： InAs nanowires Chemical vapor deposition Thermal conductivity Phonon-boundary scattering

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Effects of connecting sequences of building blocks on reticular synthesis of covalent organic frameworks

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Nano Research 2021年第2期14卷 381-386页

作者： De-Li Ma Cheng Qian Qiao-Yan Qi Zhong-Ri Zhong Guo-Fang Jiang Xin Zhao state key lab of chemo/biosensing and chemometrics College of Chemistry and Chemical EngineeringHunan Universityf Changsha 410082China key laboratory of Synthetic and Self-Assembly Chemistry for Organic Functional Molecules Center for Excellence in Molecular SynthesisShanghai Institute of Organic ChemistryChinese Academy of Sciences345 Lingling RoadShanghai 200032China

The principle of reticular chemistry has been widely used to guide the design of crystalline porous materials such as metal organic frameworks(MOFs)and covalent organic frameworks(COFs).While in the early strategies only the symmetries of the building blocks were considered for reticular synthesis of COFs,recently a few researches on COFs with hierarchical porosities indicate that connecting sequence of building blocks also plays a crucial role in determining crystalline structures of ***,this important phenomenon has not been systematically investigated *** this article,a model system has been established to demonstrate how different connecting sequences of two C_(2v)-symmetric building blocks lead to the formation of four two-dimensional(2D)COFs with distinct framework *** verify this concept,target synthesis was conducted to produce three COFs,whose structures were confirmed by powder X-ray diffraction and pore size distribution analysis.

关键词： reticular chemistry covalent organic framework connecting sequence building block

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基于聚吡咯/蛭石/海藻纤维复合半导体材料的瞬态压阻传感器

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Science China Materials 2024年第2期67卷 580-587页

作者：王鹏真梁俊轩田维亮张克伟夏延致 state key laboratory of Bio-Fibers and Eco-Textiles Collaborative Innovation Center for Marine Biomass FibersMaterials and Textiles of Shandong ProvinceCollege of Materials Science and EngineeringInstitute of Marine Biobased MaterialsQingdao UniversityQingdao 266071China key laboratory of Chemical Engineering in South Xinjiang College of Chemistry and Chemical EngineeringTarim UniversityAlaer 843300China

电子皮肤、人机交互和健康监测等领域推动了柔性压力传感器的快速发展.然而,同时满足耐用和瞬态的需求对柔性压力传感器是一个巨大的挑战.本文开发了一种用于柔性瞬态压阻传感器的安全、耐受的聚吡咯/蛭石/海藻酸盐半导体框架.将带负电... 详细信息

电子皮肤、人机交互和健康监测等领域推动了柔性压力传感器的快速发展.然而,同时满足耐用和瞬态的需求对柔性压力传感器是一个巨大的挑战.本文开发了一种用于柔性瞬态压阻传感器的安全、耐受的聚吡咯/蛭石/海藻酸盐半导体框架.将带负电荷的蛭石纳米片插层到可生物降解的海藻酸盐织物中,进一步用高灵敏度的导电聚吡咯修饰.由此产生的多维框架实现了柔性传感器的稳定性,并且在使用寿命结束后可以在不留下电子垃圾的情况下逐渐降解.所获得的瞬态压阻传感器显示出了快速的响应时间(81/99 ms)和出色的抗疲劳性能.此外,我们开发了一种有效的机器学习模型用于人体动作识别和预测,准确率为100%.本工作为柔性瞬态电子学中有机-无机界面的设计提供了一种有前景的策略,并在基于舒适生物纤维的柔性平台中展现了广阔的应用前景.

关键词： piezoresistive sensors transient electronics machine learning tolerable hybrids

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Microstructures,corrosion behavior and mechanical properties of as-cast Mg-6Zn-2X(Fe/Cu/Ni)alloys for plugging tool applications

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International Journal of Minerals,Metallurgy and Materials 2024年第4期31卷 697-711页

作者： Baosheng Liu Jiali Wei Shaohua Zhang Yuezhong Zhang Pengpeng Wu Daqing Fang Guorui Ma School of Materials Science and Engineering Taiyuan University of Science and TechnologyTaiyuan 030024China state key laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049China Intelligent Equipment Research and Development Center Zhuhai Institute of Advanced Technology Chinese Academy of SciencesZhuhai 519080China Advanced Materials Research Institute Zhuhai Dingmei Medical Technology Co.Ltd.Zhuhai 519000China

Mg-6Zn-2X(Fe/Cu/Ni)alloys were prepared through semi-continuous casting,with the aim of identifying a degradable magnesium(Mg)alloy suitable for use in fracturing balls.A comparative analysis was conducted to assess the impacts of adding Cu and Ni,which result in finer grains and the formation of galvanic corrosion *** electronic microscopy examination revealed that precipitated phases concentrated at grain boundaries,forming a semi-continuous network structure that facilitated corrosion penetration in Mg-6Zn-2Cu and Mg-6Zn-2Ni *** corrosion was observed in Mg-6Zn-2Fe,while galvanic corrosion was identified as the primary mechanism in Mg-6Zn-2Cu and Mg-6Zn-2Ni *** the tests,the Mg-6Zn-2Ni alloy exhibited the highest corrosion rate(approximately 932.9 mm/a)due to its significant potential *** testing showed that Mg-6Zn-2Ni alloy possessed suitable ultimate compressive strength,making it a potential candidate material for degradable fracturing balls,effectively addressing the challenges of balancing strength and degradation rate in fracturing applications.

关键词： magnesium alloys microstructure micro-galvanic corrosion mechanical properties

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Microstructure Characterization of Bubbles in Gassy Soil Based on the Fractal Theory

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Journal of Ocean University of China 2024年第1期23卷 129-137页

作者： WU Chen LIN Guoqing LIU Lele LIU Tao LI Chengfeng GUO Zhenqi Shandong Provincial key laboratory of Marine Environment and Geological Engineering Ocean University of ChinaQingdao 266100China key laboratory of Gas Hydrate Ministry of Natural ResourcesQingdao Institute of Marine GeologyQingdao 266237China College of Environmental Science and Engineering Ocean University of ChinaQingdao 266100China key laboratory of Marine Environment and Ecology Ministry of EducationOcean University of ChinaQingdao 266100China Qingdao National laboratory for Marine Science and Technology Qingdao 266237China

The microscopic characterization of isolated bubbles in gassy soil plays an important role in the macroscopic physical properties of sediments and is a key factor in the study of geological hazards in gas-bearing *** on the box-counting method and the pore fractal features in porous media,a fractal model of bubble microstructure parameters in gassy soil under different gas con-tents and vertical load conditions is established by using an industrial X-ray CT scanning *** results show that the fractal di-mension of bubbles in the sample is correlated with the volume fraction of bubbles,and it is also restricted by the vertical *** three-dimensional fractal dimension of the sample is about 1 larger than the average two-dimensional fractal dimension of all the slices from the same *** uniform porous media fractal model is used to test the equivalent diameter,and the results show that the variation of the measured pore diameter ratio is jointly restricted by the volume fraction and the vertical *** addition,the measured self-similarity interval of the bubble area distribution is tested by the porous media fractal capillary bundle model,and the fitting curve of measured pore area ratio in a small loading range is obtained in this paper.

关键词： gassy soil bubble microstructure parameters fractal dimension vertical load

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一种实现单层MoS_(2)光致发光显著增强的有效缺陷工程策略

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Science China Materials 2024年第7期67卷 2232-2238页

作者：陈荧黄卓睿刘华伟喻国粮张金鼎徐哲元陈明星李东马超黄明朱小莉陈舒拉蒋英潘安练 key laboratory for Micro-Nano Physics and Technology of Hunan Province Hunan Institute of Optoelectronic IntegrationSchool of Physics and ElectronicsCollege of Materials Science and EngineeringHunan UniversityChangsha 410082China School of Physics and Electronics Hunan Normal UniversityChangsha 410081China state key laboratory of Powder Metallurgy Central South UniversityChangsha 410083China

二维过渡金属硫族化合物(TMDCs)材料被认为是拓展摩尔定律的极具前景的候选材料.然而,该材料的低光致发光效率严重限制了其实际应用,其本质源于材料制备中不可避免引入的缺陷.在本文中,我们报道了一种Sr掺杂单层MoS_(2)的有效缺陷工程策... 详细信息

二维过渡金属硫族化合物(TMDCs)材料被认为是拓展摩尔定律的极具前景的候选材料.然而,该材料的低光致发光效率严重限制了其实际应用,其本质源于材料制备中不可避免引入的缺陷.在本文中,我们报道了一种Sr掺杂单层MoS_(2)的有效缺陷工程策略,该策略在实验上通过简便的化学气相沉积(CVD)一步法成功实现.所制备的具有亚毫米(~324μm)级的大尺寸样品的光致发光可实现高达两个数量级的增强,并伴随着载流子寿命的显著增强.这一现象主要归因于Sr掺杂后MoS_(2)体系中其三激子向激子转换.与此同时,掺杂样品的辐射质量和稳定性也显著提升.第一性原理计算进一步阐明了其调控机制,即在MoS_(2)中引入适当互补缺陷能级与其自身的缺陷能级协同,从而可调节其载流子组分,以实现光致发光的显著增强.此外,我们的缺陷工程策略也适用于其他掺杂剂,如钙掺杂剂.我们的工作报告了一种可以显著提升单层MoS_(2)的荧光性能的有效缺陷工程策略,这为设计和调控二维TMDCs的光电特性提供一种极具前途的方法.

关键词： MoS_(2) substitutional doping photoluminescence in-tensity enhancement first-principles calculations

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Salinity fronts shape spatial patterns in zooplankton distribution in Hangzhou Bay

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Acta Oceanologica Sinica 2024年第6期43卷 96-106页

作者： Yepeng Xu Yiqi Wang Lin Zhan Yijun Ou Kangning Jia Ming Mao Xuyu Zhu Zhibing Jiang Yuanli Zhu Wei Huang Ping Du Jiangning Zeng Lu Shou Feng Zhou key laboratory of Marine Ecosystem Dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China key laboratory of Nearshore Engineering Environment and Ecological Security of Zhejiang Province Hangzhou 310012China state key laboratory of Satellite Ocean Environment Dynamics Ministry of Natural ResourcesHangzhou 310012China Nantong Marine Environmental Monitoring Center Ministry of Natural ResourcesNantong 226002China key laboratory of Ocean Space Resource Management Technology Ministry of Natural ResourcesHangzhou 310012China Observation and Research Station of Marine Ecosystem in the Yangtze River Delta Ministry of Natural ResourcesZhoushan 316021China

Ocean fronts play important roles in nutrient transport and in the shaping ecological *** zones in small bays are typically small in scale,have a complex structure,and they are spatially and temporally variable,but there are limited data on how biological communities respond to this *** Bay,a mediumsized estuary in China,is an ideal place in which to study the response of plankton to small-scale ocean fronts,because three water masses(Qiantang River Diluted Water,Changjiang River Diluted Water,and the East China Sea current) converge here and form dynamic salinity fronts throughout the *** investigate zooplankton communities,and temperature,salinity and chlorophyll a(Chl a) in Hangzhou Bay in June(wet perio d) and December(dry period) of 2022 and examine the dominant environmental factors that affect zooplankton community spatial *** then match the spatial distributions of zooplankton communities with those of salinity fronts.S alinity is the most important explanatory variable to affect zooplankton community spatial variability during both wet and dry periods,in that it contributes>60% of the variability in community ***,the spatial distributions of zooplankton match well with salinity *** December,with weaker Qiantang River Diluted Water and a stronger secondary Changjiang River Plume,zooplankton communities occur in moderate salinity(MS,salinity range 15.6±2.2) and high salinity(HS,22.4±1.7) regions,and their ecological boundaries closely match the Qiantang River Diluted Water *** June,different zooplankton communities occur in low salinity(LS,3.9±1.0),MS(11.7±3.6) and HS(21.3±1.9) *** the LS region occurs abnormally in the central bay rather than its apex because of the anomalous influence of rising and falling tides during the sampling perio d,the ecological boundaries still match salinity ***-salinity or brackish-water zooplankter taxa are relatively more abunda

关键词： zooplankton spatial distribution salinity fronts Hangzhou Bay

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Flexible bidirectional self-powered photodetector with significantly reduced volume and accelerated response speed based on hydrogel and lift-off GaN-based nanowires

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Fundamental Research 2024年第2期4卷 369-378页

作者： Min Jiang Yukun Zhao Penghui Zheng Jianya Zhang Wenxian Yang Min Zhou Yuanyuan Wu Renjun Pei Shulong Lu key lab of Nanodevices and Applications Suzhou Institute of Nano-Tech and Nano-Bionics(SINANO)Chinese Academy of Sciences(CAS)Suzhou 215123China School of Nano-Tech and Nano-Bionics University of Science and Technology of ChinaHefei 230026China CAS key laboratory of Nano-Bio Interface Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China Nanchang Research Institute Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesNanchang 330200China

Due to the wide range of potential applications for next-generation multi-functional devices,the flexible selfpowered photodetector(PD)with polarity-switchable behavior is essential but very challenging to be ***,a wearable bidirectional self-powered PD based on detached(Al,Ga)N and(In,Ga)N nanowires has been proposed and demonstrated *** from the photovoltage-competing dynamics across(Al,Ga)N and(In,Ga)N nanowire photoelectrodes,such PD can generate the positive(33.3 mA W−1)and negative(-0.019 mA W−1)photo-responsivity under ultraviolet(UV)and visible illumination,respectively,leading to the bidirectional photocurrent *** to the introduction of quasi solid-state hydrogel,the PD can work without the liquid-electrolyte,thus remarkably reducing the volume from about 482 cm3 to only 0.18 ***,the use of hydrogel is found to enhance response speed in the UV range by reducing the response time for more than 95%,which is mainly attributed to the increased open circuit potential and reduced ion transport *** the GaN connecting segment is pretty thin,the piezoelectric charges generated by stress are proposed to have only a limited effect on the photocurrent ***,both the stable on-off switching characteristics and photocurrent densities can still be achieved after being bent 400 *** an excellent flexibility,this work creates opportunities for technological applications of bidirectional photocurrent PDs in flexible optoelectronic devices,e.g.,wearable intelligent sensors.

关键词： Flexible photodetector Bidirectional photocurrent Lift-off GaN-based nanowires Hydrogel Self-powered device

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