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International Journal of Minerals,Metallurgy and materials 2024年第3期31卷 508-517页

作者： Runhao Zhang Jian Yang Han Sun Wenkui Yang state key laboratory of Advanced Special Steel School of Materials Science and EngineeringShanghai UniversityShanghai 200444China

The machine learning models of multiple linear regression(MLR),support vector regression(SVR),and extreme learning ma-chine(ELM)and the proposed ELM models of online sequential ELM(OS-ELM)and OS-ELM with forgetting mechanism(FOS-ELM)are applied in the prediction of the lime utilization ratio of dephosphorization in the basic oxygen furnace steelmaking *** ELM model exhibites the best performance compared with the models of MLR and ***-ELM and FOS-ELM are applied for sequential learning and model *** optimal number of samples in validity term of the FOS-ELM model is determined to be 1500,with the smallest population mean absolute relative error(MARE)value of 0.058226 for the *** variable importance analysis reveals lime weight,initial P content,and hot metal weight as the most important variables for the lime utilization *** lime utilization ratio increases with the decrease in lime weight and the increases in the initial P content and hot metal weight.A prediction system based on FOS-ELM is applied in actual industrial production for one *** hit ratios of the predicted lime utilization ratio in the error ranges of±1%,±3%,and±5%are 61.16%,90.63%,and 94.11%,*** coefficient of determination,MARE,and root mean square error are 0.8670,0.06823,and 1.4265,*** system exhibits desirable performance for applications in actual industrial pro-duction.

关键词： basic oxygen furnace steelmaking machine learning lime utilization ratio dephosphorization online sequential extreme learning machine forgetting mechanism

Development in oxide metallurgy for improving the weldability of high -strength low-alloy steel-Combined deoxidizers and microalloying elements

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International Journal of Minerals,Metallurgy and materials 2024年第6期31卷 1263-1284页

作者： Tingting Li Jian Yang state key laboratory of Advanced Special Steel School of Materials Science and EngineeringShanghai UniversityShanghai 200444China

The mechanisms of oxide metallurgy include inducing the formation of intragranular acicular ferrite(IAF)using micron-sized inclusions and restricting the growth of prior austenite grains(PAGs)by nanosized particles during *** chaotically oriented IAF and refined PAGs inhibit crack initiation and propagation in the steel,resulting in high impact *** work summarizes the com-bined effect of deoxidizers and alloying elements,with the aim to provide a new perspective for the research and practice related to im-proving the impact toughness of the heat affected zone(HAZ)during the high heat input *** complex deoxidation with other strong deoxidants,such as Mg,Ca,Zr,and rare earth metals(REMs),can improve the toughness of the heat-affected zone(HAZ)by re-fining PAGs or increasing IAF ***,it is difficult to identify the specific phase responsible for IAF nucleation because ef-fective inclusions formed by complex deoxidation are usually *** alloying elements,such as C,Si,Al,Nb,or Cr,con-tents can impair HAZ toughness.A high C content typically increases the number of coarse carbides and decreases the potency of IAF ***,Cr,or Al addition leads to the formation of undesirable *** reduces the high-temperature stability of the ***,V,and B can enhance HAZ ***-containing precipitates present good thermal *** or V(C,N)is ef-fective in promoting IAF nucleation due to its good coherent crystallographic relationship with *** formation of the B-depleted zone around the inclusion promotes IAF *** interactions between alloying elements are complex,and the effect of adding dif-ferent alloying elements remains to be *** the future,the interactions between various alloying elements and their effects on ox-ide metallurgy,as well as the calculation of the nucleation effects of effective inclusions using first principles calculations will become the focus of

关键词： oxide metallurgy technology heat affected zone high-strength low-alloy steel intragranular acicular ferrite microalloying element

Transient Response and Ionic Dynamics in Organic Electrochemical Transistors

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Nano-Micro Letters 2024年第11期16卷 191-223页

作者： Chao Zhao Jintao Yang Wei Ma state key laboratory for Mechanical Behavior of materials Xi’an Jiaotong UniversityXi′an 710049People’s Republic of China

The rapid development of organic electrochemical transistors(OECTs)has ushered in a new era in organic electronics,distinguishing itself through its application in a variety of domains,from high-speed logic circuits to sensitive biosensors,and neuromorphic devices like artificial synapses and organic electrochemical random-access *** recent strides in enhancing OECT performance,driven by the demand for superior transient response capabilities,a comprehensive understanding of the complex interplay between charge and ion transport,alongside electron–ion interactions,as well as the optimization strategies,remains *** review aims to bridge this gap by providing a systematic overview on the fundamental working principles of OECT transient responses,emphasizing advancements in device physics and optimization *** review the critical aspect of transient ion dynamics in both volatile and non-volatile applications,as well as the impact of materials,morphology,device structure strategies on optimizing transient *** paper not only offers a detailed overview of the current state of the art,but also identifies promising avenues for future research,aiming to drive future performance advancements in diversified applications.

关键词： Organic electrochemical transistors Transient response Ion dynamics Electronic dynamics Volatility and non-volatility

Multiplexed manipulation of orbital angular momentum and wavelength in metasurfaces based on arbitrary complex-amplitude control

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Light(Science & Applications) 2024年第5期13卷 930-940页

作者： Guoli He Yaqin Zheng Changda Zhou Siyang Li Zhonghong Shi Yanhui Deng Zhang-Kai Zhou state key laboratory of Optoelectronic materials and Technologies School of PhysicsSun Yat-sen UniversityGuangzhou 510275China

Due to its unbounded and orthogonal modes,the orbital angular momentum(OAM)is regarded as a key optical degree of freedom(DoF)for future information processing with ultra-high capacity and *** the manipulation of OAM based on metasurfaces has brought about great achievements in various fields,such manipulation currently remains at single-DoF level,which means the multiplexed manipulation of OAM with other optical DoFs is still lacking,greatly hampering the application of OAM beams and advancement of *** order to overcome this challenge,we propose the idea of multiplexed coherent pixel(MCP)for *** approach enables the manipulation of arbitrary complex-amplitude under incident lights of both plane and OAM waves,on the basis of which we have realized the multiplexed DoF control of OAM and *** a result,the MCP method expands the types of incident lights which can be simultaneously responded by metasurfaces,enriches the information processing capability of metasurfaces,and creates applications of information encryption and OAM *** findings not only provide means for the design of high-security and high-capacity metasurfaces,but also raise the control and application level of OAM,offering great potential for multifunctional nanophotonic devices in the future.

关键词： momentum offering overcome

The Effect of Blending Ratio on the Structure and Properties of the PPR/PS In situ Fiber Reinforced System Prepared by Multi-Flow Vibration Injection Molding

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Chinese Journal of Polymer Science 2024年第6期42卷 851-863页

作者： Yan-Jiang Li Meng-Long Hu Jun-Wen Zhang Qiang Fu Jie Zhang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu610065China

To enhance the mechanical properties of polypropylene random copolymer(PPR),polystyrene(PS)with four different contents were added to the PPR matrix through melt ***,using the Multi-Flow Vibration Injection Molding(MFVIM)technology,PPR/PS in situ microfiber composites(MFC)with different blending ratios were *** results indicated that blending ratio had a great impact on the phase morphology and crystal structure of MFVIM samples,which was different from those of conventional injection molding(CIM)*** ultrafine fibers could be formed under the shear field and could absorb the PPR molecular chains to form hybrid shish-kebab ***,the PPR matrix could also form shish-kebab structures under the effect of strong *** the PS content reached 20%,under the combined action of PS in situ microfibers and highly oriented crystal structure,the tensile strength and Young’s modulus of the sample were obviously improved and the impact strength remained at a relatively high *** a strong and tough balanced PPR based material was *** results provide valuable insights for expanding the industrial and daily-life applications of PPR and show promising development prospects.

关键词： PPR MFVIM In situ microfibers Shearfield Hybrid shish-kebab structures

Review and prospects on the low-voltage Na_(2)Ti_(3)O_(7) anode materials for sodium-ion batteries

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Journal of Energy Chemistry 2024年第1期88卷 446-460,I0011页

作者： Jun Dong Yalong Jiang Ruxing Wang Qiulong Wei Qinyou An Xiaoxing Zhang Hubei key laboratory for High-efficiency Utilization of Solar Energy and Operation Control of Energy Storage System Hubei University of TechnologyWuhan 430068HubeiChina state key laboratory of New Textile materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200HubeiChina Xiamen key laboratory of High-Performance Metals and materials College of MaterialsXiamen UniversityXiamen 361005FujianChina state key laboratory of Advanced Technology for materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070HubeiChina

Due to its low cost and natural abundance of sodium,Na-ion batteries(NIBs)are promising candidates for large-scale energy storage *** development of ultralow voltage anode materials is of great significance in improving the energy density of ***-voltage anode materials,however,are severely lacking in *** all the reported insertion oxides anodes,the Na_(2)Ti_(3)O_(7) has the lowest operating voltage(an average potential of 0.3 V ***^(+)/Na)and is less likely to deposit sodium,which has excellent potential for achieving NIBs with high energy densities and high *** significant progress has been made,achieving Na_(2)Ti_(3)O_(7) electrodes with excellent performance remains a severe *** paper systematically summarizes and discusses the physicochemical properties and synthesis methods of Na_(2)Ti_(3)O_(7).Then,the sodium storage mechanisms,key issues and challenges,and the optimization strategies for the electrochemical performance of Na_(2)Ti_(3)O_(7) are classified and further ***,remaining challenges and future research directions on the Na_(2)Ti_(3)O_(7) anode are *** review offers insights into the design of high-energy and high-safety NIBs.

关键词： Sodium-ion batteries Low-voltage anode materials Na_(2)Ti_(3)O_(7) Electrochemical performances Electrochemical mechanism

Highly responsive broadband Si-based MoSphototransistor on high-k dielectric

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Science China(Information Sciences) 2024年

作者： Ali IMRAN Xin HE Jiwei LIU Qinghai ZHU Muhammad SULAMAN Fei XUE Mingsheng XU Deren YANG Beijing key Lab of Nanophotonics and Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of Technology ZJU-Hangzhou Global Scientific and Technological Innovation Centre College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University School of materials Science and Engineering State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University

The demand for photodetectors and image sensors has grown exponentially in the past decade in biomedical, security surveillance, robotics, automotive, quality control, image recognition, and military applications, due to their superior quality, broadband detection, lower noise, and economic viability. Here,we report a MoS2channel-based phototransistor over an HfO2/n-Si substrate isolated by an h BN layer. The high photoresponse is achieved through the integration of the photoconduction, photogating, and mobility enhancement process by utilizing excellent features of MoS2, HfO2/Si, and h BN. The capacitive coupling of the photogenerated carriers by high-k dielectric HfO2leads to modulation of MoS2Fermi level due to electrostatic doping. Furthermore, the MoS2also contributes to the photogeneration of carriers due to its semiconducting nature, leading to additional photocurrent. Ultimately, the combination of photogating,photoconduction, and swift carrier extraction with remarkable mobility of 11.65 cm2·V-1·s-1results in high responsivity, external quantum efficiency, and detectivity of 4.5×108A·W-1, 0.72×106, and 6.20×1016Jones at 266 nm illumination, respectively. The device also demonstrates broadband photoresponse from 266–1000 nm wavelengths. The high responsivity distinguishes the potential of our device for the future of optoelectronics and broadband image sensing applications.

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3D printing encouraging desired in-situ polypyrrole seed-polymerization for ultra-high energy density supercapacitors

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Journal of Energy Chemistry 2024年第8期95卷 117-125,I0004页

作者： Tiantian Zhou Shangwen Ling Shuxian Sun Ruoxin Yuan Ziqin Wu Mengyuan Fu Hanna He Xiaolong Li Chuhong Zhang state key laboratory of Polymer materials Engineering Polymer Research InstituteSichuan UniversityChengdu 610065SichuanChina

The tireless pursuit of supercapacitors with high energy density entails the parallel advancement of wellsuited electrode materials and elaborately engineered ***(PPy)emerges as an exceedingly conductive polymer and a prospective pseudocapacitive materials for supercapacitors,yet the inferior cyclic stability and unpredictable polymerization patterns severely impede its real-world ***,for the first time,an innovative seed-induced in-situ polymerization assisted 3D printing strategy is proposed to fabricate PPy-reduced graphene oxide/poly(vinylidene difluoride-cohexafluoropropylene)(PVDF-HFP)(PPy-rGO/PH)electrodes with controllable polymerization behavior and exceptional areal mass *** preferred active sites uniformly pre-planted on the 3D-printed graphene substrates serve as reliable seeds to induce efficient polypyrrole deposition,achieving an impressive mass loading of 185.6 mg cm^(-2)(particularly 79.2 mg cm^(-2)for polypyrrole)and a superior areal capacitance of 25.2 F cm^(-2)at 2 mA cm^(-2)for a 12-layer *** agreement with theses appealing features,an unprecedented areal energy density of 1.47 mW h cm^(-2)for a symmetrical device is registered,a rarely achieved value for other PPy/rGO-based *** work highlights a promising route to preparing high energy density energy storage modules for real-world applications.

关键词： 3D printing Seed-induced polymerization Supercapacitor Polypyrrole High energy density

In-situ formation of nitrogen doped microporous carbon nanospheres derived from polystyrene as lubricant additives for anti-wear and friction reduction

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Friction 2024年第3期12卷 439-451页

作者： Yixin WANG Qi LU Huijie XIE Shujuan LIU Qian YE Feng ZHOU Weimin LIU state key laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi'an 710072China state key laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

This study presents a nitrogen-doped microporous carbon nanospheres(N@MCNs)prepared by a facile polymerization–carbonization process using low-cost *** N element in situ introduces polystyrene(PS)nanospheres via emulsion polymerization of styrene with cyanuric chloride as crosslinking agent,and then carbonization obtains N@*** as-prepared carbon nanospheres possess the complete spherical structure and adjustable nitrogen amount by controlling the relative proportion of tetrachloromethane and cyanuric *** friction performance of N@MCNs as lubricating oil additives was surveyed utilizing the friction experiment of ball-disc *** results showed that N@MCNs exhibit superb reduction performance of friction and *** the addition of N@MCNs was 0.06 wt%,the friction coefficient of PAO-10 decreased from 0.188 to 0.105,and the wear volume reduced by 94.4%.The width and depth of wear marks of N@MCNs decreased by 49.2% and 94.5%,*** carrying capacity of load was rocketed from 100 to 400 N *** the analysis of the lubrication mechanism,the result manifested that the prepared N@MCNs enter clearance of the friction pair,transform the sliding friction into the mixed friction of sliding and rolling,and repair the contact surface through the repair ***,the tribochemical reaction between nanoparticles and friction pairs forms a protective film containing nitride and metal oxides,which can avert direct contact with the matrix and improve the tribological *** experiment showed that nitrogen-doped polystyrene-based carbon nanospheres prepared by in-situ doping are the promising materials for wear resistance and reducing *** preparing method can be ulteriorly expanded to multi-element co-permeable *** and boron co-doped carbon nanospheres(B,N@MCNs)were prepared by mixed carbonization of N-enriched PS and boric acid,and exhibited high load carrying capacity and good tribolog

关键词： lubricant additives hypercrosslinked polystyrene carbon nanospheres friction reduction anti-wear

Self-assembled aerogel sheet electrodes of thermocells for low-grade heat harvest

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Science China Chemistry 2024年第5期67卷 1672-1679页

作者： Ziwei Mo Shouhao Wei Daibin Xie Kaihua Zhu Hongxiong Li Xin Lu Lirong Liang Chunyu Du Zhuoxin Liu Guangming Chen College of materials Science and Engineering Shenzhen UniversityShenzhen 518055China state key laboratory of Polymer materials Engineering Sichuan UniversityChengdu 610065China

Efficiently harvesting low-grade heat is crucial for sustainable energy management. Thermocells(TECs), inducing heat-toelectricity conversion via the thermogalvanic effect, have thus drawn tremendous attention in recent years. This study introduces a self-assembly approach for fabricating aerogel sheet electrodes(ASEs) tailored for TECs. The crafted ASEs retain a remarkable porous architecture with approximately 95% porosity, even with their slimmed-down thickness. Results reveal that the electrode composition has minimal influence on the thermopower of TECs. Notably, the porous ASE with tunned composition demonstrates an optimal effective surface area for the thermogalvanic effect, resulting in enhanced output current density. This balances the desirable traits of electrode compactness with abundant redox active sites, positioning it favorably against conventional bulky electrode designs. The TECs utilizing the optimized ASE achieve a peak output power of 22.10 μW cm^(-2)under a temperature difference of 30 K. Furthermore, a tubular TEC device is readily assembled and specially designed for harvesting heat energy from hot fluids. These findings underscore the potential of composite electrodes in the realm of low-grade heat harvest, paving the way for broader applications in sustainable energy solutions.

关键词： thermocells low-grade heat harvest energy conversion composite electrodes

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