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Thermodynamic equilibrium theory-guided design and synthesis of Mg-doped LiFe_(0.4)Mn_(0.6)PO_(4)/C cathode for lithium-ion batteries

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Journal of Energy Chemistry 2024年第4期91卷 619-627页

作者： Wei Lyu Wenlong Cai Tuan Wang Xiaobo Sun Enhao Xu Jinxuan Chen Kaipeng Wu Yun Zhang college of Materials Science and Engineering Sichuan UniversityChengdu 610064SichuanChina

Mn-rich LiFe_(1-x)Mn_(x)PO_(4)(x>0.5),which combines the high operation voltage of LiMnPO_(4)with excellent rate performa nce of LiFePO4,is hindered by its sluggish kinetic ***,thermodynamic equilibrium analysis of Mn^(2+)-Fe^(2+)-Mg^(2+)-C_(2)O_(4)^(2-)-H_(2)O system is used to guide the design and preparation of insitu Mg-doped(Fe_(0.4)Mn_(0.6))_(1-x)Mg_(x)C_(2)O_(4)intermediate,which is then employed as an innovative precursor to synthesize high-performance Mg-doped LiFe_(0.4)Mn_(0.6)PO_(4).It indicates that the metal ions with a high precipitation efficiency and the stoichiometric precursors with uniform element distribution can be achieved under the optimized thermodynamic ***,accelerated Li+diffusivity and reduced charge transfer resistance originating from Mg doping are verified by various kinetic *** from the contributions of inherited homogeneous element distribution,small particle size,uniform carbon layer coating,enhanced Li+migration ability and structural stability induced by Mg doping,the Li(Fe_(0.4)Mn_(0.6))_(0.97)Mg_(0.03)PO_(4)/C exhibits splendid electrochemical performance.

关键词： (Fe_(0.4)Mn_(0.6))_(1-x)MgxC_(2)0_(4) precursors Thermodynami cequilibrium Co-precipitation Mg doping Lithium-ion batteries

Real-time Operation Optimization in Active Distribution Networks Based on Multi-agent Deep Reinforcement Learning

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Journal of Modern Power Systems and Clean Energy 2024年第3期12卷 886-899页

作者： Jie Xu Hongjun Gao Renjun Wang Junyong Liu the college of Electrical Engineering Sichuan UniversityChengduChina

The increasing integration of intermittent renewable energy sources(RESs)poses great challenges to active distribution networks(ADNs),such as frequent voltage *** paper proposes a novel ADN strategy based on multiagent deep reinforcement learning(MADRL),which harnesses the regulating function of switch state transitions for the realtime voltage regulation and loss *** deploying the calculated optimal switch topologies,the distribution network operator will dynamically adjust the distributed energy resources(DERs)to enhance the operation performance of ADNs based on the policies trained by the MADRL *** to the model-free characteristics and the generalization of deep reinforcement learning,the proposed strategy can still achieve optimization objectives even when applied to similar but unseen ***,integrating parameter sharing(PS)and prioritized experience replay(PER)mechanisms substantially improves the strategic performance and *** framework has been tested on modified IEEE 33-bus,IEEE 118-bus,and three-phase unbalanced 123-bus *** results demonstrate the significant real-time regulation capabilities of the proposed strategy.

关键词： Reconfiguration active distribution network distributed energy resource real-time control deep reinforcement learning parameter sharing scalability

Dietary sodium acetate and sodium butyrate improve high-carbohydrate diet utilization by regulating gut microbiota, liver lipid metabolism, oxidative stress, and inflammation in largemouth bass(Micropterus salmoides)

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Journal of Animal Science and Biotechnology 2024年第4期15卷 1704-1722页

作者： Qiao Liu Liangshun Cheng Maozhu Wang Lianfeng Shen Chengxian Zhang Jin Mu Yifan Hu Yihui Yang Kuo He Haoxiao Yan Liulan Zhao Song Yang college of Animal Science and Technology Sichuan Agricultural UniversityChengdu 611130SichuanChina

Background Adequate level of carbohydrates in aquafeeds help to conserve protein and reduce cost. However, studies have indicated that high-carbohydrate(HC) diet disrupt the homeostasis of the gut–liver axis in largemouth bass, resulting in decreased intestinal acetate and butyrate *** Herein, we had concepted a set of feeding experiment to assess the effects of dietary sodium acetate(SA) and sodium butyrate(SB) on liver health and the intestinal microbiota in largemouth bass fed an HC diet. The experimental design comprised 5 isonitrogenous and isolipidic diets, including LC(9% starch), HC(18% starch), HCSA(18% starch;2 g/kg SA), HCSB(18% starch;2 g/kg SB), and HCSASB(18% starch;1 g/kg SA + 1 g/kg SB). Juvenile largemouth bass with an initial body weight of 7.00 ± 0.20 g were fed on these diets for 56 *** We found that dietary SA and SB reduced hepatic triglyceride accumulation by activating autophagy(ATG101, LC3B and TFEB), promoting lipolysis(CPT1α, HSL and AMPKα), and inhibiting adipogenesis(FAS, ACCA, SCD1 and PPARγ). In addition, SA and SB decreased oxidative stress in the liver(CAT, GPX1α and SOD1) by activating the Keap1-Nrf2 pathway. Meanwhile, SA and SB alleviated HC-induced inflammation by downregulating the expression of pro-inflammatory factors(IL-1β, COX2 and Hepcidin1) through the NF-κB pathway. Importantly, SA and SB increased the abundance of bacteria that produced acetic acid and butyrate(Clostridium_sensu_stricto_1). Combined with the KEGG analysis, the results showed that SA and SB enriched carbohydrate metabolism and amino acid metabolism pathways, thereby improving the utilization of carbohydrates. Pearson correlation analysis indicated that growth performance was closely related to hepatic lipid deposition, autophagy, antioxidant capacity, inflammation, and intestinal microbial *** In conclusion, dietary SA and SB can reduce hepatic lipid deposition;and alleviate oxidative stress and inflammation in largemout

关键词： High carbohydrate diet Intestinal microbiota Largemouth bass Lipid deposition Sodium acetate Sodium butyrate

Efficient privacy-preserving federated learning under dishonest-majority setting

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Science China(Information Sciences) 2024年第5期67卷 323-324页

作者： Yinbin MIAO Da KUANG Xinghua LI Tao LENG Ximeng LIU Jianfeng MA School of Cyber Engineering Xidian University Intelligent Policing Key Laboratory of sichuan Province Sichuan Police College Institute of Information Engineering Chinese Academy of Sciences School of Cyber Security University of Chinese Academy of Sciences Key Laboratory of Information Security of Network Systems Fuzhou University

Federated learning(FL) is an emerging distributed learning paradigm that solves the problem of isolated data by jointly learning the global model through distributed ***, recent studies have shown that FL may not always guarantee sufficient privacy preservation, this is mainly because the model parameters(e.g., weights or gradients)may leak sensitive information to malicious adversaries.

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Low-energy inelastic electron scattering from carbon monoxide:Excitation and de-excitation of the X^(1)Σ^(+),a^(3)Π,a'^(3)∑^(+),A^(1)Π,d^(3)Δ,e^(3)∑^(-),I^(1)∑^(-)and D^(1)Δelectronic states

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Chinese Physics B 2024年第4期33卷 444-450页

作者：卫鹏宇黄朝文程新路张红 Institute of Atomic and Molecular Physics Sichuan UniversityChengdu 610065China college of Physics Sichuan UniversityChengdu 610065China

Cross-sections for electronic excitation and de-excitation among the ground state and lowest-lying seven electronic excited states of carbon monoxide(CO)by low-energy electron impact are computed using the R-matrix *** excitation cross-sections from the ground state to the electronic states a^(3)Π,a'^(3)Σ^(+)+and A^(1)Πagree with previous experimental and theoretical *** addition,the cross-sections for the I^(1)Σ^(+)-and D^(1)Δstates of CO,which will cascade to CO a'^(3)Σ^(+)+and A^(1)Πstates,are ***,in contrast to the typical increase in electronic excitation cross-sections with collision energy,the de-excitation cross-sections show a negative trend with increasing energy.

关键词： electron-CO collision electronic excitation cross-sections R-matrix method

Arbitrary skin metallization by pencil-writing inspired solid-ink rubbing for advanced energy storage and harvesting

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Journal of Energy Chemistry 2024年第1期88卷 592-602,I0013页

作者： Yonghan Zhou Zhongfeng Ji Wenrui Cai Xuewei He Ruiying Bao Xuewei Fu Wei Yang Yu Wang college of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu 610065SichuanChina

The development of a durable metallic coating on diverse substrates is both intriguing and challenging,particularly in the research of metal-conductive materials for applications such as batteries,soft electronics,and ***,by learning from the pencil-writing process,a facile solid-ink rubbing technology(SIR-tech)is invented to address the above *** solid-ink is exampled by rational combination of liquid metal and graphite *** harnessing the synergistic effects between rubbing and adhesion,controllable metallic skin is successfully formed onto metals,woods,ceramics,and plastics without limitation in size and ***,outperforming pure liquid-metal coating,the composite metallic skin by SIR-tech is very robust due to the self-lamination of graphite nanoplate exfoliated by liquid-metal *** critical factors controlling the structures-properties of the composite metallic skin have been systematically investigated as *** applications,the SIR-tech is demonstrated to fabricate high-performance composite current collectors for next-generation batteries without traditional metal ***,advanced skin-electrodes are further demonstrated for stable triboelectricity generation even under temperature fluctuation from-196 to 120℃.This facile and highly-flexible SIR-tech may work as a powerful platform for the studies on functional coatings by liquid metals and beyond.

关键词： Microadhesion guided technology Skin metallization by solid-ink rubbing Liquid metal composites Composite current collector Batteries and triboelectric nanogenerators

Coordination structure regulation in non-flammable electrolyte enabling high voltage lithium electrochemistry

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Journal of Energy Chemistry 2024年第9期96卷 282-290页

作者： Zhiwen Deng Ye Jia Yan Deng Changhaoyue Xu Xuemei Zhang Qiujie He Jianan Peng Hao Wu Wenlong Cai college of Materials Science and Engineering Sichuan UniversityChengdu 610064SichuanChina Engineering Research Center of Alternative Energy Materials and Devices Sichuan UniversityChengdu 610064SichuanChina

High-voltage battery systems bring significant increases in energy density but are also accompanied by fast degradation of electrochemical performance and serious safety ***,Li^(+)coordination structure regulation was conducted to formulate a non-flammable electrolyte,which consists of 1.5 M lithium bis(fluor sulfonyl)imide(LiFSI)in triethyl phosphate and methyl 2,2,2-trifluoromethyl carbonate(FEMC).The renamed TEP-FEMC-FEC(TFF)electrolyte exhibits an FSI^(−)-dominated solvation structure contributed by the weakly-solvating ability of *** generated inorganic-rich interfacial layers are conducive to stabilizing the phase transition of high-voltage cathodes while suppressing the dendritic growth on lithium metal or co-intercalation behavior in graphite *** TFF electrolyte enables LiCoO_(2)||Li batteries to achieve capacity maintenance over 79%after 400 cycles with high-rate of 5 C at an ultra-high voltage of 4.6 V,and an outstanding capacity exceeding 100 mA h g^(−1)even at a super-high current density of 20 ***,the Ah-level LiCoO_(2)||graphite pouch cells also exhibit high capacity retention and satisfactory safety performance even under fast *** work provides a novel research direction for the pursuit of high energy density non-flammable electrolytes.

关键词： Non-flammable Solvation structure High-voltage Lithium batteries

Mid-infrared computational temporal ghost imaging

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Light(Science & Applications) 2024年第6期13卷 1088-1097页

作者： Han Wu Bo Hu Lu Chen Fei Peng Zinan Wang Goery Genty Houkun Liang college of Electronics and Information Engineering Sichuan UniversityChengduSichuan610064China college of Electrical Engineering Sichuan UniversityChengduSichuan610064China Key Lab of Optical Fiber Sensing&Communications University of Electronic Science&Technology of ChinaChengduSichuan611731China Laboratory of Photonics Tampere UniversityFI-33014TampereFinland

Ghost imaging in the time domain allows for reconstructing fast temporal objects using a slow *** technique involves correlating random or pre-programmed probing temporal intensity patterns with the integrated signal measured after modulation by the temporal ***,the implementation of temporal ghost imaging necessitates ultrafast detectors or modulators for measuring or pre-programming the probing intensity patterns,which are not available in all spectral regions especially in the mid-infrared ***,we demonstrate a frequency downconversion temporal ghost imaging scheme that enables to extend the operation regime to arbitrary wavelengths regions where fast modulators and detectors are not *** approach modulates a signal with temporal intensity patterns in the near-infrared and transfers the patterns to an idler via difference-frequency generation in a nonlinear crystal at a wavelength where the temporal object can be *** a proof-of-concept,we demonstrate computational temporal ghost imaging in the mid-infrared with operating wavelength that can be tuned from 3.2 to 4.3μ*** scheme is flexible and can be extended to other *** results introduce new possibilities for scan-free pump-probe imaging and the study of ultrafast dynamics in spectral regions where ultrafast modulation or detection is challenging such as the mid-infrared and THz regions.

关键词： ghost Ghost scheme

Image Recognition Model of Fraudulent Websites Based on Image Leader Decision and Inception-V3 Transfer Learning

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China Communications 2024年第1期21卷 215-227页

作者： Shengli Zhou Cheng Xu Rui Xu Weijie Ding Chao Chen Xiaoyang Xu Information Department of Zhejiang police college Hangzhou 310053China Hangzhou Dianzi University Hangzhou 310018China Big Data Laboratory of Zhejiang police college Hangzhou 310053China Hangzhou Public Security Bureau Hangzhou 310002China

The fraudulent website image is a vital information carrier for telecom *** efficient and precise recognition of fraudulent website images is critical to combating and dealing with fraudulent *** research on image recognition of fraudulent websites is mainly carried out at the level of image feature extraction and similarity study,which have such disadvantages as difficulty in obtaining image data,insufficient image analysis,and single identification *** study develops a model based on the entropy method for image leader decision and Inception-v3 transfer learning to address these *** data processing part of the model uses a breadth search crawler to capture the image ***,the information in the images is evaluated with the entropy method,image weights are assigned,and the image leader is *** model training and prediction,the transfer learning of the Inception-v3 model is introduced into image recognition of fraudulent *** selected image leaders to train the model,multiple types of fraudulent websites are identified with high *** experiment proves that this model has a superior accuracy in recognizing images on fraudulent websites compared to other current models.

关键词： fraudulent website image leaders telecom fraud transfer learning