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Assessing the corrosion protection property of coatings loaded with corrosion inhibitors using the real-time atmospheric corrosion monitoring technique

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International Journal of Minerals,Metallurgy and materials 2025年第1期32卷 119-126页

作者： Xiaoxue Wang Lulu Jin Jinke Wang Rongqiao Wang Xiuchun Liu Kai Gao Jingli Sun Yong Yuan Lingwei Ma Hongchang Qian Dawei Zhang School of Energy and Power Engineering Beihang UniversityBeijing 100191China Beijing Institute of Space Long March Vehicle Beijing 100076China National materials Corrosion and Protection Data center University of Science and Technology BeijingBeijing 100083China Institute of materials intelligent Technology Liaoning Academy of MaterialsShenyang 110004China shanghai Spaceflight Precision Machinery Institute Shanghai 201600China

The atmospheric corrosion monitoring(ACM)technique has been widely employed to track the real-time corrosion behavior of metal ***,limited studies have applied ACM to the corrosion protection properties of organic *** study compared a bare epoxy coating with one containing zinc phosphate corrosion inhibitors,both applied on ACM sensors,to observe their corrosion protection properties over *** with artificial damage via scratches were exposed to immersion and alternating dry and wet environments,which allowed for monitoring galvanic corrosion currents in *** the corrosion tests,the ACM currents of the zinc phosphate/epoxy coating were considerably lower than those of the blank epoxy *** trend in ACM current variations closely matched the results obtained from regular electrochemical tests and surface *** alignment highlights the potential of the ACM technique in evaluating the corrosion protection capabilities of organic *** with the blank epoxy coating,the zinc phosphate/epoxy coating showed much-decreased ACM current values that confirmed the effective inhibition of zinc phosphate against steel corrosion beneath the damaged coating.

关键词： atmospheric corrosion monitoring technology corrosion inhibitor coating carbon steel corrosion protection

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1.56 kV/30 A vertical β-Ga2O3 Schottky barrier diodes with composite edge terminations

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Science China(Information Sciences) 2025年第2期68卷 389-390页

作者： Yitao FENG Hong ZHOU Sami ALGHAMDI Hao FANG Xiaorong ZHANG Yanbo CHEN Guotao TIAN Saud WASLY Yue HAO Jincheng ZHANG Key Lab of Wide Band Gap Semiconductor materials and devices School of MicroelectronicsXidian University center of Excellence in intelligent Engineering Systems (CEIES) King Abdulaziz University China Resources Microelectronics Limited

In recent years, large-area wide-bandgap（WBG） semiconductor materials have achieved numerous notable breakthroughs [1,2]. The ultra-WBG semiconductor β-Ga2O3,with its excellent material properties, is ideally suited for the fabrication of power devices. Moreover, it offers easily obtainable large-area substrates, with reported sizes up to 6 inches, produced through melt-grown crystal growth methods. These characteristics make β-Ga2O3highly attractive for future low-cost commercialization. Despite these advances, most research has focused on low-current and small-size diodes, with few studies addressing high-current and large-size diodes.

关键词： Schottky barrier diodes

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Influence of laser shock peening on microstructure and high-temperature oxidation resistance of Ti45Al8Nb alloy fabricated via laser melting deposition

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Transactions of Nonferrous Metals Society of China 2025年第1期35卷 157-168页

作者： Lu-lu JIANG Liang LAN Cheng-yan BAI Ru-yi XIN Shuang GAO Hao-yu WANG Bo HE Chao-yue CHEN Guo-xin LU Research center of High-Temperature Alloy Precision Forming School of Materials Science and EngineeringShanghai University of Engineering ScienceShanghai 201620China State Key Laboratory of Advanced Special Steels School of Materials Science and EngineeringShanghai UniversityShanghai 200444China School of materials Science and Engineering Shandong UniversityJinan 250061China

Laser shock peening(LSP)was used to enhance the high-temperature oxidation resistance of laser melting deposited Ti45Al8Nb *** microstructure and high-temperature oxidation behavior of the as-deposited Ti45Al8Nb alloy before and after LSP were investigated by scanning electron microscopy,X-ray diffraction,and electron backscatter *** results indicated that the rate of mass gain in the as-deposited sample after LSP exhibited a decrease when exposed to an oxidation temperature of 900℃,implying that LSP-treated samples exhibited superior oxidation resistance at high temperatures.A gradient structure with a fine-grain layer,a deformed-grain layer,and a coarse-grain layer was formed in the LSP-treated sample,which facilitated the diffusion of the Al atom during oxidation,leading to the formation of a dense Al_(2)O_(3)layer on the *** mechanism of improvement in the oxidation resistance of the as-deposited Ti45Al8Nb alloy via LSP was discussed.

关键词： TiAl alloy laser melting deposition laser shock peening additive manufacturing oxidation resistance

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Recent progress on stability and applications of flexible perovskite photodetectors

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Journal of Semiconductors 2025年第1期46卷 5-19页

作者： Ying Hu Qianpeng Zhang Junchao Han Xinxin Lian Hualiang Lv Yu Pei Siqing Shen Yongli Liang Hao Hu Meng Chen Xiaoliang Mo Junhao Chu State Key Laboratory of Photovoltaic Science and Technology Shanghai Frontiers Science Research Base of Intelligent Optoelectronics and PerceptionDepartment of Materials ScienceInstitute of OptoelectronicsFudan UniversityShanghai 200433China Advanced Silicon Technology Co. Ltd.Shanghai 201616China

Flexible photodetectors have garnered significant attention by virtue of their potential applications in environmental monitoring,wearable healthcare,imaging sensing,and portable optical *** stand out as particularly promising materials for photodetectors,offering exceptional optoelectronic properties,tunable band gaps,low-temperature solution processing,and notable mechanical *** this review,we explore the latest progress in flexible perovskite photodetectors,emphasizing the strategies developed for photoactive materials and device structures to enhance optoelectronic performance and ***,we discuss typical applications of these devices and offer insights into future directions and potential applications.

关键词： perovskite flexible photodetector stability versatile applications

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Double[5]carbohelicene:facile synthesis,chiroptical properties,isomerization study,and lasing application

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Science China Chemistry 2025年第1期68卷 233-240页

作者： Peipei Liu Yantong Li Meng-Xiang Wu Hao Kang Xiao-Li Zhao Lin Xu Linlin Liu Xiaodong Li Junfeng Fang Zhiwei Fang Ya Cheng Hai-Bo Yang Huakang Yu Xueliang Shi State Key Laboratory of Petroleum Molecular&Process Engineering Shanghai Key Laboratory of Green Chemistry and Chemical ProcessesSchool of Chemistry and Molecular EngineeringEast China Normal UniversityShanghai 200062China School of Physics and Optoelectronics South China University of TechnologyGuangzhou 510640China School of Physics and Electronic Science Engineering Research Center of Nanophotonics&Advanced InstrumentMinistry of EducationEast China Normal UniversityShanghai 200241China State Key Laboratory of Precision Spectroscopy School of Physics and Electronic ScienceEast China Normal UniversityShanghai 200241China Institute of Polymer Optoelectronic materials&devices State Key Laboratory of Luminescent Materials&DevicesSouth China University of TechnologyGuangzhou 510640China

Double carbohelicenes have attracted considerable attention due to their aesthetic structures,distinctπ-conjugation extension,inherent chirality,and intriguing optical and electronic ***,the concise de novo synthesis of a new double[5]carbohelicene 1 together with its chiroptical properties,isomerization process and lasing application is presented.1 was synthesized by a simple protocol involving the formation of a 6,6′-bipentacene as the key *** is worth noting that1 existed as two diastereomers 1-PP/MM and 1-PM,which were successfully isolated and unambiguously confirmed by Xray *** optical resolution of the racemic 1-PP/MM was successfully achieved by chiral-phase highperformance liquid chromatography(HPLC),and 1-PP and 1-MM were characterized by circular ***,it was found that 1-PP/MM could be completely isomerized to 1-PM upon heating,and the detailed thermodynamics and kinetics of the isomerization process were systematically investigated.1-PM exhibited deep-red luminescence with emission maximum at 723 nm and fluorescence quantum yield as high as 32.95%.Consequently,we can showcase the lasing application of 1-PM by doping with epoxy resin to assemble a bottle microlaser spontaneously,which the lasing wavelength is 796.6 nm at a threshold of 0.8 m J cm^(-2).We believe that our studies,including the facile synthesis methodology,detailed isomerization studies,and lasing application,will shed some light on the design and synthesis of novel carbohelical systems with more functions.

关键词： double carbohelicene optical resolution organic laser isomerization X-ray diffraction

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Anomalous open orbits in Hofstadter spectrum of Chern insulator

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Science China(Physics,Mechanics & Astronomy) 2025年第3期68卷 139-144页

作者： Haijiao Ji Peng Zhou Noah F.Q.Yuan Hua Jiang Haiwen Liu X.C.Xie center for Advanced Quantum Studies Department of PhysicsBeijing Normal UniversityBeijing100875China Tsung-Dao Lee Institute Shanghai Jiao Tong UniversityShanghai201210China Department of Mathematics UC BerkeleyBerkeley94720USA Institute for Nanoelectronic devices and Quantum Computing Fudan UniversityShanghai200433China International center for Quantum materials School of PhysicsPeking UniversityBeijing100871China Hefei National Laboratory Hefei230088China

The nontrivial band topology of Chern insulator can enrich the content of its Hofstadter butterfly spectra,which is closely related to recent experiments in twisted bilayer graphene and cold atom *** investigate the Hofstadter spectrum for various models of Chern insulators under a rational fluxφ_(0)/q,hereφ_(0)=h/e and q being an *** find the number of splitting subbands is|q-C|with C denoting the Chern number of parent ***,anomalous open-orbital subbands with Chern numbers q-1 and-q-1 emerge unexpectedly,which are beyond the parameter window(-q/2,q/2)of the Diophantine equation studied by Thouless-Kohmoto-Nightingale-den Nijs[***.49,405(1982)].The emergence of anomalous open orbits can be traced by analyzing the evolution of the Hofstadter spectrum,identifying as a new type of topological phase *** novel findings not only pinpoint the peculiar Hofstadter spectrum of Chern insulator,but also provide routes to study exotic characteristics beyond the Landau level physics.

关键词： Hofstadter spectrum topological phase transition open orbit

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Enhancing performance of fullerene-based organic electrochemical transistors via side-chain engineering

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Nano Research 2025年第2期18卷 905-912页

作者： Wenxin Fang Zijie Li Chengdong Wang Xiaowei Zhao Junyu Li Gang Ye Fengwei Huo Li Qiu Yanxi Zhang Wei Huang Institute of Flexible Electronics(IFE Future Technologies)Xiamen UniversityXiamen 361005China Yunnan Key Laboratory of Electromagnetic materials and devices National Center for International Research on Photoelectric and Energy MaterialsSchool of Materials and EnergyYunnan UniversityKunming 650091China Sinopec shanghai Research Institute of Petrochemical Technology Shanghai 201028China Key Laboratory for the Green Preparation and Application of Functional materials Hubei Key Laboratory of Polymer MaterialsSchool of Materials Science and EngineeringHubei UniversityWuhan 430062China Key Laboratory of Flexible Electronics(KLOFE)&Institute of Advanced materials(IAM) Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing Tech University(NanjingTech)Nanjing 211800China Frontiers Science center for Flexible Electronics MIIT Key Laboratory of Flexible Electronics(KLoFE)Northwestern Polytechnical UniversityXi'an 710072China

The performance of organic electrochemical transistors(OECTs)relies on the interaction between organic semiconductors and ***,hydrophilic ethylene glycol(EG)side chains are incorporated into organic semiconductors to improve the channel’s capacity to absorb ***,the EG substituted organic semiconductors tend to swell when immersed in aqueous electrolytes and exhibit microstructural changes induced by dopant *** our research,we introduce an alkyl spacer to create distance between the fullerene and EG *** approach is designed to reduce the negative effects of swelling and balance the ion and electron *** conducted an analysis of OECTs using four fullerene derivatives:no alkyl spacer,butyl,hexyl,and octyl *** OECTs based on fullerene derivatives with butyl and hexyl spacers exhibit enhanced transconductance(g_(m)=11.8 and 19.4 mS)compared to the ones without alkyl *** has also been observed that the butyl and hexyl spacers lead to a more than tenfold increase in volumetric *** increasing the alkyl spacer(octyl group)leads to no transistor *** study uncovers the relationship between alkyl spacers and the performance of OECTs based on fullerene *** will serve as a guideline for designing n-type small molecules for ***,we showcased the potential of utilizing OECTs based on these fullerene derivatives in cation sensing,which is promising for developing sweat sensors.

关键词： organic electrochemical transistors fullerene derivatives ethylene glycol side chains ion and electron conduction

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Experimental Investigation of Possibility of Simultaneously Monitoring Lung Perfusion/Cardiomotility and Ventilation via Thoracic Impedance Measurement

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Journal of shanghai Jiaotong university(Science) 2025年第1期30卷 81-90页

作者： BAI Zicuan MA Yicin KONG Zhibin XUE Shan School of Electronic Information and Electrical Engineering Shanghai Jiao Tong UniversityShanghai200240China shanghai Engineering Research center for intelligent Diagnosis and Treatment Instrument Shanghai200240China The Sixth People’s Hospital Shanghai Jiao Tong University School of MedicineShanghai200235China Renji Hospital Shanghai Jiao Tong University School of MedicineShanghai200127China

Impedance pneumography has a significant advantage for continuous and noninvasive monitoring of respiration,compared with conventional flowmeter-based ventilation measurement *** thoracic impedance is sensitive to pulmonary ventilation,it is also sensitive to physiological activities such as blood flow and cardiomotility,in addition,body movement/*** paper explores the possibility of simultaneously monitoring pulmonary ventilation,blood circulation and cardiomotility by bioimpedance ***,blood perfusion and cardiomotility signals are extracted using the wavelet method from thoracic impedance data measured in breath-holding and tidal breathing statuses,to investigate signal strength and their *** research provides a foundation for the development of bedside devices to monitor various physiological activities.

关键词： impedance pneumography respiration blood perfusion cardiomotility wavelet analysis

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Research progress of lignin-derived materials in lithium/sodium ion batteries

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Green Energy & Environment 2025年第2期10卷 322-344页

作者： Jingke Zhang Hengxue Xiang Zhiwei Cao Shichao Wang Meifang Zhu Institute of Hybrid materials National Center of International Research for Hybrid Materials TechnologyNational Base of International Science&Technology CooperationCollege of Materials Science and EngineeringQingdao UniversityQingdao266071China State Key Laboratory for Modification of Chemical Fibers and Polymer materials College of Materials Science and EngineeringDonghua UniversityShanghai201620China

With the increase of energy consumption,the shortage of fossil resource,and the aggravation of environmental pollution,the development of cost-effective and environmental friendly bio-based energy storage devices has become an urgent *** the second most abundant natural polymer found in nature,lignin is mainly produced as the by-product of paper pulping and bio-refining *** possesses several inherent advantages,such as low-cost,high carbon content,abundant functional groups,and bio-renewable,making it an attractive candidate for the rechargeable battery ***,there has been a surge of research interest in utilizing lignin or lignin-based carbon materials as the components of lithium-ion(LIBs)or sodium-ion batteries(SIBs),including the electrode,binder,separator,and *** review provides a comprehensive overview on the research progress of lignin-derived materials used in LIBs/SIBs,especially the application of lignin-based carbons as the anodes of LIBs/*** preparation methods and properties of lignin-derived materials with different dimensions are systemically discussed,which emphasizes on the relationship between the chemical/physical structures of lignin-derived materials and the performances of LIBs/*** current challenges and future prospects of lignin-derived materials in energy storage devices are also proposed.

关键词： Lignin-based carbons Lithium battery Sodium battery Chemical structure evolution

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Light-activated tautomeric transition enhanced buried heterointerface for highly efficient and ultraviolet robust perovskite solar cells

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Science China Chemistry 2025年第2期68卷 723-732页

作者： Sheng Jiang Shaobing Xiong Shuaifei Mao Yefan Zhang Dongyang Zhao Xiaomeng You Vladimir Gaishun Dmitry Kovalenk Qinye Bao School of Physics and Electronic Science East China Normal UniversityShanghai 200241China shanghai Frontiers Science Research Base of intelligent Optoelectronics and Perception Institute of OptoelectronicsFudan UniversityShanghai 200433China Institute of Functional Nano&Soft materials(FUNSOM) Soochow UniversitySuzhou 215123China shanghai Key Laboratory of Magnetic Resonance East China Normal UniversityShanghai 200241China Collaborative Innovation center of Extreme Optics Shanxi UniversityTaiyuan 030006China Department of Physics and Information Technologies Francisk Skorina Gomel State UniversityGomel 246028Belarus

The buried heterointerface of perovskite solar cells(PSCs)suffers from serious nonradiative recombination and ultraviolet(UV)light stress,relentlessly limiting further increase in their power conversion efficiency and operational ***,we develop an emerging strategy of incorporating a thin UV-activated tautomeric transition layer onto underlying charge transport layer and then depositing perovskite layer to construct an efficient hole-selective buried *** is revealed that the UV-activated tautomeric transition interlayer not only improves upper perovskite crystallinity,diminishes thermionic loss for collecting hole and passivates defect site at such buried contact that significantly promote charge transport and suppress nonradiative recombination,but also effectively protects adjacent perovskite from UV degradation through“UV sunscreen”*** a result,we report a remarkably enhanced efficiency of 24.76%compared to 22.02%of the control *** importantly,the achieved high-efficiency PSC features excellent resistance against UV radiation at 365 nm of 100 and 850 mW cm^(−2),which are approximately 21 and 184 times of UV flux(4.6 mW cm^(−2))under AM 1.5G solar *** work provides a promising approach of strengthening buried heterointerface for simultaneous realization of highly efficient and UV robust PSCs.

关键词： buried heterointerface energetics nonradiative recombination ultraviolet resistance perovskite solar cell

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