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Methane adsorption effected by pore structure of overmature continental shale:Lower Cretaceous Shahezi Formation,Xujiaweizi Fault,Songliao Basin

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Frontiers of Earth Science 2024年第1期18卷 172-187页

作者： Pengfei ZHANG Shuangfang LU Nengwu ZHOU Zizhi LIN Xiangchun CHANG Junjian ZHANG Guo CHEN Yumao PANG Junjie WANG Hongsheng HUANG Qi ZHI College of Earth Science and Engineering Shandong University of Science and TechnologyQingdao 266590China Sanya Offshore Oil&Gas research institute Northeast Petroleum UniversitySanya 572025China School of Geoscience China University of Petroleum(East China)Qingdao 266580China College of Resources and Environment Yangtze UniversityWuhan 430100China

Overmature continental shale is commonly developed,but few studies have given insight into its pore structure and sorption *** techniques,including SEM,helium porosity and permeability,N_(2)/CO_(2)adsorption,MICP,and NMR,were used to detect the pore structure of shale from the Shahezi Formation,Xujiaweizi Fault,Songliao *** excess methane adsorption volumes were measured by the volumetric method and modeled by the Langmuir *** on the findings,the most developed pores are intraparticle pores in clay minerals,followed by the dissolution pores in feldspar,but organic pores are *** selected shales have low helium porosity(mean 1.66%)and ultralow permeability(mean 0.0498×10^(−3)μm^(2)).The pore throats are at the nanoscale,and the pore-throat size distributions are unimodal,with most less than 50 *** studied shales are characterized by the lower specific surface area(SSA)and pore volume(PV)but the larger average pore *** total SSA is contributed by the micro-and mesopores,while the PV is dominated by meso-and *** pore structures are more complex and controlled by multiple factors,such as mineral compositions and diagenesis,but organic matter is not *** maximum absolute adsorption methane volume(VL)is 0.97−3.58 cm^(3)/g(mean 1.90 cm^(3)/g),correlating well with the total SSA,SSA,and pore volume of micropores,which indicates that methane is mainly adsorbed and stored in micropores,followed by mesopores.

关键词： continental shale pore structure methane adsorption Shahezi Formation Songliao Basin

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Robust Carbon-Carbon Cleavage in Lignin to Produce Phenol and Cyclohexanone

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Chemical research in Chinese Universities 2024年第1期40卷 29-35页

作者： WANG Lulin CHENG Xiaomeng DONG Minghua LUAN Sen WU Yuxuan HAN Buxing LIU Huizhen Beijing National Laboratory for Molecular Sciences CAS Laboratory of Colloid and Interface and ThermodynamicsCAS Research/Education Center for Excellence in Molecular SciencesCenter for Carbon Neutral ChemistryInstitute of ChemistryChinese Academy of SciencesBeijing 100190P.R.China University of Chinese Academy of Sciences Beijing 100049P.R.China

The challenge of breaking 5-5'bonds in lignin,attributed to their high bonding energy,has prompted the development of a new transformation ***,an important model compound for lignin,contains these 5-5'bonds,making it crucial to devise a strategy for their cleavage in lignin *** study introduces a novel method for transforming biphenyl,involving selective hydrogenation to cyclohexylbenzene by Ni/SiO2 catalyst,followed by its oxidation to phenol and cyclohexanone through a radical *** demonstrate that the catalysts with small particles have strong catalytic activity,while there is little difference in *** reason for the high selectivity of cyclohexylbenzene is due to the limited adsorption of cyclohexylbenzene on Ni/*** work presents a fresh approach to breaking resilient C-C bonds in lignin.

关键词： Lignin 5-5'Bond Ni/SiO_(2) Phenol

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Pathology of pain and its implications for therapeutic interventions

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Signal Transduction and Targeted Therapy 2024年第7期9卷 2851-2899页

作者： Bo Cao Qixuan Xu Yajiao Shi Ruiyang Zhao Hanghang Li Jie Zheng Fengyu Liu You Wan Bo Wei Department of General Surgery First Medical CenterChinese PLA General HospitalBeijing 100853China Medical School of Chinese PLA Beijing 100853China Neuroscience research institute and Department of Neurobiology School of Basic Medical SciencesKey Laboratory for NeuroscienceMinistry of Education/National Health CommissionPeking UniversityBeijing 100191China

Pain is estimated to affect more than 20%of the global population,imposing incalculable health and economic *** pain management is crucial for individuals suffering from ***,the current methods for pain assessment and treatment fall short of clinical *** from advances in neuroscience and biotechnology,the neuronal circuits and molecular mechanisms critically involved in pain modulation have been *** research achievements have incited progress in identifying new diagnostic and therapeutic *** this review,we first introduce fundamental knowledge about pain,setting the stage for the subsequent *** review next delves into the molecular mechanisms underlying pain disorders,including gene mutation,epigenetic modification,posttranslational modification,inflammasome,signaling pathways and *** better present a comprehensive view of pain research,two prominent issues,sexual dimorphism and pain comorbidities,are discussed in detail based on current *** status quo of pain evaluation and manipulation is summarized.A series of improved and innovative pain management strategies,such as gene therapy,monoclonal antibody,brain-computer interface and microbial intervention,are making strides towards clinical *** highlight existing limitations and future directions for enhancing the quality of preclinical and clinical *** to decipher the complexities of pain pathology will be instrumental in translating scientific discoveries into clinical practice,thereby improving pain management from bench to bedside.

关键词： pain thereby summarized

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Heat source recognition sensor mimicking the thermosensation function of human skin

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The Innovation 2024年第5期5卷 84-90,83页

作者： Wenting Sun Pengxiang Zhang Xinyi Lin Yupeng Wang Shuaihua Wang Bin Yang Zijian Zheng Weishu Liu Department of Materials Science and Engineering Southern University and Science and TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Functional Oxide Materials and Devices Southern University of Science and TechnologyShenzhen 518055China School of Fashion and Textiles The Hong Kong Polytechnic UniversityHong Kong SARChina Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityHong Kong SAR 999077China research institute for Intelligent Wearable Systems(RI-IWEAR) The Hong Kong Polytechnic UniversityHong Kong SAR 999077China research institute for Smart Energy(RISE) The Hong Kong Polytechnic UniversityHong Kong SAR 999077China

The human skin maintains a comfortable and healthy somatosensory state by sensing different aspects of the thermal environment,including temperature value,heat source,energy level,and ***,state-of-the-art thermosensors only measure basic temperature values,not the full range of the thermosensation function of human ***,we propose a heat source recognition(hsr)sensor of poly(butyl acrylate)-lithium bis(n-fluoroalkylsulfonyl)imide(PBA-Li:nFSI;n=1,3,5),which enables response to temperature,pressure,and proximity stimulus signals based on the relaxation behavior of the ionic gel and distinguished between different types of heat sources(i.e.,radiation,convection,and conduction).The hsr sensor was integrated into a prosthetic limb covered by an e-skin with isothermal regulation,and experiments with a robot showed that it could achieve human-like thermosensation function,recognizing multidimensional information about thermal environments,such as temperature value,comfort level,and heat source *** work deeply mimics the human body’s thermosensation function and provides a reliable solution for the development of bionic e-skin for intelligent robots and prosthetics.

关键词： robot function source

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Multi-scale physics-informed neural networks for solving high Reynolds number boundary layer flows based on matched asymptotic expansions

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Theoretical & Applied Mechanics Letters 2024年第2期14卷 76-81页

作者： Jianlin Huang Rundi Qiu Jingzhu Wang Yiwei Wang Key Laboratory for Mechanics in Fluid Solid Coupling Systems Institute of MechanicsChinese Academy of SciencesBeijing 100190China School of Future Technology University of Chinese Academy of SciencesBeijing 100049China School of Engineering Science University of Chinese Academy of SciencesBeijing 100049China Guangdong Aerospace research Academy Guangzhou 511458China

Multi-scale system remains a classical scientific problem in fluid dynamics,biology,*** the present study,a scheme of multi-scale Physics-informed neural networks is proposed to solve the boundary layer flow at high Reynolds numbers without any *** flow is divided into several regions with different scales based on Prandtl's boundary *** regions are solved with governing equations in different *** method of matched asymptotic expansions is used to make the flow field continuously.A flow on a semi infinite flat plate at a high Reynolds number is considered a multi-scale problem because the boundary layer scale is much smaller than the outer flow *** results are compared with the reference numerical solutions,which show that the msPINNs can solve the multi-scale problem of the boundary layer in high Reynolds number *** scheme can be developed for more multi-scale problems in the future.

关键词： Physics-informed neural networks(PINNs) Multi-scale Fluid dynamics Boundary layer

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Design and Performance Analysis of HMDV Dynamic Inertial Suspension Based on Active Disturbance Rejection Control

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Computer Modeling in Engineering & Sciences 2024年第8期140卷 1485-1506页

作者： Xiaofeng Yang Wei Wang Yujie Shen Changning Liu Tianyi Zhang School of Automotive and Traffic Engineering Jiangsu UniversityZhenjiang212013China Automotive Engineering research institute Jiangsu UniversityZhenjiang212013China Chongqing Key Laboratory of Urban Rail Transit System Integration and Control Chongqing400074China State Key Laboratory of Advanced Design and Manufacturing Technology for Vehicle Hunan universityChangsha410082China

This paper addresses the impact of vertical vibration negative effects,unbalanced radial forces generated by the static eccentricity of the hub motor,and road excitation on the suspension performance of Hub Motor Driven Vehicle(HMDV).A dynamic inertial suspension based on Active Disturbance Rejection Control(ADRC)is proposed,combining the vertical dynamic characteristics of dynamic inertial suspension with the features of ADRC,which distinguishes between internal and external disturbances and arranges the transition ***,a simulation model of the static eccentricity of the hub motor is established to simulate the unbalanced radial electromagnetic force generated under static eccentricity.A quarter-vehicle model of an HMDV with a controllable dynamic inertial suspension is then ***,the passive suspension model is studied under different grades of road excitation,and the impact mechanism of suspension performance at speeds of 0–20 m/s is ***,the three main components within the ADRC controller are designed for the second-order controlled system,and optimization algorithms are used to optimize its internal ***,the performance of the traditional passive suspension,the PID-based controllable dynamic inertial suspension,and the ADRC-based controllable dynamic inertial suspension are analyzed under different road *** results show that,under sinusoidal road input,the ADRC-based controllable dynamic inertial suspension exhibits a 52.3%reduction in the low-frequency resonance peak in the vehicle body acceleration gain diagram compared to the traditional passive suspension,with significant performance optimization in the high-frequency *** random road input,the ADRC-based controllable dynamic inertial suspension achieves a 29.53%reduction in the root mean square value of vehicle body acceleration and a 14.87%reduction in dynamic tire *** indicates that the designed controllable dynamic inertia

关键词： HMDV static eccentricity ADRC dynamic inertial suspension road excitation

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A Study of 10 Rotating Radio Transients Using Parkes Radio Telescope

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research in Astronomy and Astrophysics 2024年第4期24卷 114-123页

作者： Xinhui Ren Jingbo Wang Wenming Yan Jintao Xie Shuangqiang Wang Yirong Wen Yong Xia Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China University of Chinese Academy of Sciences Beijing 100049China institute of Optoelectronic Technology Lishui UniversityLishui 323000China Xinjiang Key Laboratory of Radio Astrophysics Urumqi 830011China research Center for Intelligent Computing Platforms Zhejiang LaboratoryHangzhou 311100China

Rotating Radio Transients(RRATs)are a relatively new subclass of pulsars that emit detectable radio bursts *** analyzed 10 RRATs observed using the Parkes telescope,with eight of these observed via the ultra-wide-bandwidth low-frequency(UWL)*** measured the burst rate and produced integrated profiles spanning multiple frequency bands for three *** also conducted a spectral analysis on both integrated pulses and individual pulses of three *** of their integrated pulses follow a simple power law,consistent with the known range of pulsar spectral *** average spectral indices of single pulses are-0.9,-1.2,and-1.0 respectively,which are within the known range of pulsar spectral ***,we find that the spreads of single-pulse spectral indices for these RRATs(ranging from-3.5 to+0.5)are narrower compared to what has been observed in other ***,the average spectral index and scatter of single pulses are both relatively *** the remaining five RRATs observed at the UWL receiver,we also provide the upper limits on fluence and flux *** addition,we obtain the timing solution of PSR *** analysis shows that PSRs J1919+1745,J1709-43,and J1649-4653 are potentially nulling pulsars or weak pulsars with sparse strong pulses.

关键词： (stars:)pulsars:general stars:neutron stars:individual(PSRs J1919+1745.1909+0641,0628+0909)

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Erratum to“The power of many brains:Catalyzing neuropsychiatric discovery through open neuroimaging data and large-scale collaboration”[Sci Bull 2024;69:1536-1555]

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Science Bulletin 2024年第17期69卷 2793-2793页

作者： Bin Lu Xiao Chen Francisco Xavier Castellanos Paul MThompson Xi-Nian Zuo Yu-Feng Zang Chao-Gan Yan CAS Key Laboratory of Behavioral Science Institute of PsychologyBeijing 100101China Department of Psychology University of Chinese Academy of SciencesBeijing 100101China Department of Child and Adolescent Psychiatry NYU Grossman School of MedicineNew York 10016USA Nathan Kline institute for Psychiatric research Orangeburg 10962USA Imaging Genetics Center Mark&Mary Stevens Institute for Neuroimaging&InformaticsKeck School of MedicineUniversity of Southern CaliforniaLos Angeles 90033USA Developmental Population Neuroscience research Center IDG/McGovern Institute for Brain ResearchBeijing Normal UniversityBeijing 100875China National Basic Science Data Center Beijing 100190China Centre for Cognition and Brain Disorders The Affiliated Hospital of Hangzhou Normal UniversityHangzhou 310004China institute of Psychological Science Hangzhou Normal UniversityHangzhou 310030China Zhejiang Key Laboratory for research in Assessment of Cognitive Impairment Hangzhou 311121China International Big-Data Center for Depression research Institute of PsychologyChinese Academy of SciencesBeijing 100101China Magnetic Resonance Imaging research Center Institute of PsychologyChinese Academy of SciencesBeijing 100101China

The publisher regrets to note that reference citation errors have occurred in panels b,c,e-l in Fig 2 and the sentence“However,the literature reports both decreased and increased intra-network functional connections among patients with depression[115,116].”The publisher would like to apologise for any inconvenience *** neuroimaging findings in major depressive disorder.(a)Decreased intra-DMN FC is observed in recurrent MDD patients[35].(b)Eight-week antidepressant treatment reduce extensive large-scale functional networks[107].(c)Reduced global and local efficiency(Eglob/Eloc)are revealed in MDD patients[108].(d)Structural variations of the cortex and subcortical nuclei are found in ENIGMA-MDD studies[82].(e)Accelerated brain aging based on functional MRI is observed in MDD patients[114].(f)Accelerated brain aging based on structural MRI is observed in MDD patients[115].(g)Two subtypes of MDD can be identified through DMN FC[127].(h)A significant schizophrenia PRS by MDD interaction for rostral anterior cingulate cortex thickness is found in the UK Biobank dataset[215].(i)Stability of the four MDD subtypes based on FC[126].(j)The two subtypes of MDD exhibit distinct patterns of FC within and between SMS,DMN,and subcortical structures[130].(k)Performance of the functional connectivity-based classifiers across two multicenter datasets[135].(l)Salient brain regions that serve as important classification features for the graph convolutional network-based classifier[136].Brain-PAD:brain-predicted age difference;DAN:dorsal attention network;DMN:default mode network;FC:functional connectivity;FEDN:first-episode and drug-naïve;FPN:frontoparietal network;GCN:graph convolutional neural network;HC:healthy control;linear-SVM:linear support vector machine;MDD:major depressive disorder;mddrest:REST-meta-MDD dataset;NC:normal control;RACC:rostral anterior cingulate cortex;PRS:polygenic risk score;psymri:PsyMRI dataset;rbf-SVM:radial basis function support vector

关键词： cortex network scale

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Temporal and Spectral Characteristics of Persistent Emission and Special Bursts of Magnetar SGR J1935+2154 Based on Insight-HXMT

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research in Astronomy and Astrophysics 2024年第6期24卷 225-233页

作者： Xue-Feng Lu Li-Ming Song Ming-Yu Ge Shuang-Nan Zhang Jin-Lu Qu Ce Cai Cong-Zhan Liu Cheng-Kui Li Yu-Cong Fu Ying-Chen Xu Key Laboratory of Particle Astrophysics Institute of High Energy PhysicsBeijing 100049China University of Chinese Academy of Sciences Chinese Academy of SciencesBeijing 100049China College of Physics and Hebei Key Laboratory of Photophysics research and Application Hebei Normal UniversityShijiazhuang 050024China Department of Astronomy Beijing Normal UniversityBeijing 100875China

In October 2022,the magnetar SGR J1935+2154 entered the active outburst *** the episode,the InsightHXMT satellite carried out a long observation that lasted for 20 *** than 300 bursts were detected,and a certain amount of persistent radiation signals were also *** paper mainly introduces the results of persistent radiation profile folding and period search based on Insight-HXMT *** the same time,the burst phase distribution characteristics,spectral lag results of burst,the spectral characteristics of zero-lag bursts and the time-resolved spectral evolution characteristics of high-flux bursts are *** found that there is no significant delay feature during different energy bands for the bursts of SGR J1935+*** observed zero-lag burst does not have a unique *** time-resolved spectrum of the individual burst has consistent spectral types and spectral parameters at different time periods of the *** also find that the burst number phase distribution and the burst photon phase distribution have the same tendency to concentrate in specific regions of the persistent emission profile.

关键词： radiation mechanisms:general dense matter magnetic fields

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Synergistic effects of peroxydisulfate on UV/O_(3) process for tetracycline degradation:Mechanism and pathways

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Chinese Chemical Letters 2024年第10期35卷 408-413页

作者： Fengrui Yang Debing Wang Xinying Zhang Jie Zhang Zhichao Wu Qiaoying Wang State Key Laboratory of Pollution Control and Resource Reuse Shanghai Institute of Pollution Control and Ecological SecuritySchool of Environmental Science and EngineeringTongji UniversityShanghai 200092China Fujian Provincial Engineering research Center of Rural Waste Recycling Technology College of Environment&Safety EngineeringFuzhou University.Fuzhou 350108China

Tetracycline(TC)as a typical emerging pollutant is becoming a serious threat to the environment and human health.A combined advanced oxidation technology of UV/Ozone(O_(3))/peroxydisulfate(PDS)process was developed to explore an efficient and economic treatment process of TC in ***,the reactive sites and transformation pathways of TC were explored and the toxicity of the intermediates was quantified with a quantitative structure-activity relationship(QSAR)*** degradation performance of TC was substantially enhanced in UV/O_(3)/PDS process with a kobsof 0.0949 min-1,which was 2.3 times higher than UV/O_(3)and 3.2 times than sole *** results demonstrated that there was a superior synergistic effect of PDS on UV/O_(3)processes for the degradation of *** paramagnetic resonance(EPR)analysis and quenching experiments show that·OH,SO_(4)·-,O_(2)·-and1O_(2)all contributed to TC degradation in the UV/O_(3)/PDS process and exhibited a synergistic effect,which inhibited the generation of harmful *** addition,the UV/O_(3)/PDS system can effectively degrade TC in a wide range of substrate concentrations and pH,and also showed excellent adaptability to various concentrations of anions(Cl-and HCO_(3)-).This study proves the feasibility of UV/O_(3)/PDS process for treating TC contaminated wastewater with complicated water matrix.

关键词： UV/ozonation/peroxydisulfate Synergistic effect Tetracycline Degradation Wastewater

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