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Universal design of three-dimensional porous graphene-iron based promotors for kinetically rationalized lithium-sulfur chemistry

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Journal of Energy Chemistry 2025年第1期100卷 192-200页

作者： Hua Gao Yunfeng Zhang Menglei Wang Ruoxuan Yang Shuai Feng Xuan Cao Yaping Zhang Zhongyuan Lu Yingze Song State Key Laboratory of environment-Friendly Energy Materials School of Materials and Chemistry Southwest University of Science and Technology school of Material Science and Engineering Henan University of Technology College of Chemistry and Chemical Engineering Taishan University

Lithium-sulfur （Li-S） batteries are widely deemed to be one of the most potential candidates for future secondary batteries because of their remarkable energy ***,notorious polysulfide shuttling and retarded sulfur reaction kinetics pose significant obstacles to the further application of Li-S *** rationally designed highly active electrocatalysts can facilitate polysulfide conversion,the universal and scalable synthesis strategies need to be ***,a universal synthetic strategy to construct a series of three-dimensional （3D） porous graphene-iron （3DGr-Fe） based electrocatalysts involving 3DGr-FeP,3DGr-Fe3C,and 3DGr-Fe3Se4is exploited for manipulating the Li-S redox *** has been observed that the implementation of a 3D porous Gr architecture leads to the well-designed conductive networks,while the uniformly dispersed iron nanoparticles introduce an abundance of active sites,fostering the lithium polysulfide conversion,thereby bolstering the overall electrochemical *** Li-S battery with the 3DGr-Fe based electrocatalyst exhibits remarkable capacity retention of 94.8%upon 100 times at 0.2 ***,the soft-packaged Li-S pouch cell based on such a 3DGr-Fe electrocatalyst delivers superior capacity of 1060.71 mA h g-1and guarantees for the continuous 30 min work of fan *** investigation gives comprehensive insights into the design,synthesis,and mechanism of 3DGr-Fe based electrocatalysts with high activity toward efficient and durable Li-S batteries.

关键词： Lithium-sulfur battery Universal synthesis 3D graphene-iron based promotor Electrocatalysis

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Transient receptor potential channels and calcium dysregulation: a pathogenic duo in Parkinson's disease

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Neural Regeneration Research 2025年第3期20卷 808-810页

作者： Iqira Saeed Linlin Ma Griffith Institute for Drug Discovery Griffith UniversityNathanBrisbaneQLDAustralia school of environment and Science Griffith University NathanBrisbaneQLDAustralia

Parkinson's disease(PD) has a complex and multifactorial pathophysiology. Various studies, conducted both in pre-clinical models and PD patients, have reported a link between the disruption of calcium(Ca^(2+)) homeostasis and the subsequent development of PD. Ca^(2+) regulation is crucial for neuronal survival, differentiation,exocytosis at synapses,gene transcription,and proliferation.

关键词： homeostasis clinical subsequent

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Measurements of convection electric field in the inner magnetosphere

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Science China(Technological Sciences) 2018年第12期61卷 1866-1871页

作者： LV Xin LIU WenLong school of space and environment Beihang University

In this paper, we study the characteristic of large-scale convection electric field in the inner magnetosphere, using magnetospheric multiscale(MMS) observations between L=5 and L=8 over the period from September 1, 2015 to October 31, 2016,covering almost all magnetic local time(MLT). Observations show that the DC convection electric field generally has small variations in this region. We investigate whether the convection electric field is correlated with geomagnetic indices and solar wind parameters. It is found that, among the studied parameters, solar wind electric field, z component of interplanetary magnetic field, AE and Kp indices show good correlations with the averaged convection electric field. The results in this paper provide valuable information for understanding the role of electric field on the dynamics of the inner magnetosphere.

关键词： convection electric field inner magnetosphere

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Plasma perturbations in the coexisting environment of VLF transmitter emission, lightning strokes and seismic activity

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Science China(Technological Sciences) 2018年第5期61卷 678-686页

作者： TAO Dan LIU WenLong MA YuDuan school of space and environment Beihang University

We analyzed plasma perturbations occurring in the coexisting environment of powerful VLF transmitter emission, intense lightning strokes and strong seismic activity during pregnant period. The results suggest that anomalous electron bursts with energy dispersion in the range of ~100–350 keV, forming the "wisp" signature, are due to cyclotron resonance of electrons with monochromatic waves from the powerful NWC VLF transmitters during nighttime. The intense broad band VLF emissions (up-going 0+ whistlers) are observed while the DEMETER satellite goes through the region of intense thunderstorm activities at mid-latitudes. However, the effects of intense lightning activity and pregnant earthquake have little impact on this kind of stable energy-dispersed electron structures, despite the fact that they are presumably two primary reasons for the particle precipitation in the ionosphere. The case studied here provides us a valuable opportunity to address the various sources triggering the anomalous plasma perturbations in the ionosphere.

关键词： plasma perturbation electron precipitation cyclotron resonance VLF transmitter lightning seismic activity

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Kinetic features of bursty bulk flows and dipolarization fronts

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Science China Earth Sciences 2016年第12期59卷 2463-2464页

作者： LIU WenLong school of space and environment Beihang University

Bursty bulk flows(BBFs)and dipolarization fronts(DFs)are two important phenomena responsible for the transport of energy,mass and magnetic flux from the Earth’s magnetotail to the inner magnetosphere during magnetosphere *** BBFs are defined as the high-speed flows of several hundred km/s in the central plasma sheet lasting about 10 minutes,while DFs are defined as,with much shorter time scale of several seconds,sharp increases in the northward magnetic field component in the plasma *** two phenomena

关键词： Kinetic features of bursty bulk flows and dipolarization fronts

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Controllable synthesis of biomimetic wood stem nanoporous high entropy oxides catalysts for oxygen evolution reaction

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Nano Research 2025年第1期18卷 107-117页

作者： Wei Wang Weiqi Wang Huihui Wang Xing Lu Jinwen Zhang Yunzhuo Lu school of Materials Science and Engineering Dalian Jiaotong UniversityDalian 116028China school of Intelligence and Electronic Engineering Dalian Neusoft University of InformationDalian 116023China Guangdong Key Laboratory of Materials and Equipment in Harsh Marine environment Guangzhou Maritime UniversityGuangzhou 510725China

Bubbles generated during the oxygen evolution reaction(OER)in water splitting readily adhere to the electrode surface,thereby impeding contact between the electrolyte and the active sites,thereby increasing the ***,it is imperative to elucidate the bubble release behavior and engineer electrodes that facilitate faster bubble *** this study,inspired by the wood stem of the Norway spruce,we synthesized a gradient nanoporous high-entropy oxide(GNP-HEO)electrode with a controllable pore *** GNP-HEO,featuring a well-controlled gradient in pore size,is achieved through a straightforward strategy combining selective laser melting with selective phase *** unique gradient nanoporous structure not only facilitates bubble release but also diminishes the bubble shielding effect in OER,thereby enhancing electrocatalytic *** affect interaction of Al,Co,Cr,Fe,and Ni,coupled with the gradient nanoporous structure,yields exceptional OER performance,evidenced by an overpotential of 250 mV at a current density of 50 mA/cm^(2) and a Tafel slope of 38.0 mV/dec in 1 M *** functional theory calculations confirm that the GNPHEO adheres to the adsorbate evolution mechanism reaction pathway and exhibits significant *** work highlights a promising approach for the design and synthesis of high-performance OER electrocatalysts.

关键词： oxygen evolution reaction high-entropy oxides selective phase dis-solution selective laser melting gradient nanoporous

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Satellite remote sensing reveals overwhelming recovery of forest from disturbances in Asia

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Atmospheric and Oceanic Science Letters 2025年第1期18卷 46-51页

作者： Yiying Zhu Hesong Wang Anzhi Zhang school of Ecology and Nature Conservation Beijing Forestry UniversityBeijingChina Key Laboratory of Regional Climate and environment for Temperate East Asia Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina College of Forestry and Landscape Architecture Xinjiang Agricultural UniversityUrumqiChina

Forest ecosystems play key roles in mitigating human-induced climate change through enhanced carbon uptake;however,frequently occurring climate extremes and human activities have considerably threatened the stability of *** the same time,detailed accounts of disturbances and forest responses are not yet well quantified in *** study employed the Breaks For Additive Seasonal and Trend method-an abrupt-change detection method-to analyze the Enhanced Vegetation Index time series in East Asia,South Asia,and Southeast *** approach allowed us to detect forest disturbance and quantify the resilience after *** showed that 20%of forests experienced disturbance with an increasing trend from 2000 to 2022,and Southeast Asian countries were more severely affected by ***,95%of forests had robust resilience and could recover from disturbance within a few *** resilience of forests suffering from greater magnitude of disturbance tended to be stronger than forests with lower disturbance *** summary,this study investigated the resilience of forests across the low and middle latitudes of Asia over the past two *** authors found that most forests exhibited good resilience after disturbance and about two-thirds had recovered to a better state in *** findings of this study underscore the complex relationship between disturbance and resilience,contributing to comprehension of forest resilience through satellite remote sensing.

关键词： Forest ecosystem Enhanced vegetation index Breaks for additive seasonal and trend method Disturbance Resilience

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Reconstructing the flux-rope topology using the FOTE method

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Science China(Technological Sciences) 2019年第1期62卷 144-150页

作者： CHEN ZuZheng FU HuiShan WANG TieYan CAO Dong PENG FangZheng YANG Jian XU Yin school of space and environment Beihang UniversityBeijing 100083China

With high-resolution data of the Magnetospheric Multiscale(MMS) mission, we observe a magnetic flux rope(MFR) in the Earth's magnetosheath. This MFR, showing a clear bipolar variation of the magnetic field in the normal component to local current sheet, contains a strong core field. We use the FOTE method to reconstruct the topology of this MFR and find it is consistent with previous expectation. For the first time, the spiral field and core field of the MFR are both revealed from the FOTE method. Comparing topologies reconstructed at different times, we suggest that the axis of the MFR rotates about 88° at different spatial location. Shape and size of the normal projection to axis vary with the spatial location as well. Inside the MFR, a significant increase of plasma density from 40 to 80 cm^(-3), a sharp decrease of ion temperature from 200 to 50 eV, an enhancement of cold ions and a series of filamentary currents are found.

关键词： magnetic flux rope First-Order Taylor Expansion (FOTE)method reconstructing three-dimensional topology

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Gene therapy for spinal muscular atrophy:perspectives on the possibility of optimizing SMN1 delivery to correct all neurological and systemic perturbations

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Neural Regeneration Research 2025年第7期20卷 2011-2012页

作者： Sharon J.Brown Rafael J.Yáñez-Muñoz Heidi R.Fuller school of Pharmacy and Bioengineering Keele UniversityKeeleUK Wolfson Center for Inherited Neuromuscular Disease TORCH BuildingRJAH Orthopaedic HospitalOswestryUK *** Center of Gene and Cell TherapyDepartment of Biological SciencesSchool of Life Sciences and the EnvironmentRoyal Holloway University of LondonEghamUK

Spinal muscular atrophy(SMA)is a genetic condition that results in selective lower motor neuron loss with concomitant muscle weakness and *** genetic cause of SMA was understood in 1995 when loss or impairment of the survival motor neuron 1(SMN1)gene was identified as the main contributing factor(Lefebvre et al.,1995).This,in combination with the discovery that humans have a“back-up”gene,SMN2,which can produce low levels(approximately 10%)of the full-length functional SMN protein,has led to the generation of SMA-specific gene *** was traditionally classified according to age of symptom onset and developmental milestones achieved,with life expectancy and severity varying between ***,SMN2 copy number is used as a proxy for the prediction of disease severity,with higher SMN2 copy number typically being associated with reduced severity of SMA,although this relationship is not absolute:some individuals with low SMN2 copy number have less severe SMA phenotypes and vice ***,the etiology of SMA is further complicated by other factors,such as non-typical nucleotide variants and SMN2-independent modifiers of disease severity.

关键词： atrophy traditionally absolute

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PM10 emissions from industrial coal-fired chain-grate boilers

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Frontiers of environmental Science & Engineering 2017年第6期11卷 171-178页

作者： Xinghua Li Junzan Han Lei Duan school of space and environment Beihang University Beijing 100191 China school of environment Tsinghua University Beijing 100084 China

Industrial coal-fired boiler is an important air pollutant emission source in China. The chain-grate boiler is the most extensively used type of industrial coal-fired boiler. An electrical low-pressure impactor, and a Dekati？ Low Pressure Impactor were applied to determine mass and number size distributions of PM10 at the inlet and the outlet of the particulate emission control devices at six coalfired chain-grate boilers. The mass size distribution of PM10 generated from coal-fired chain-grate boilers generally displays a bimodal distribution that contains a submicron mode and a coarse mode. The PM in the submicron mode for burning with raw coal contributes to 33% ± 10 % of PM10 emissions, much higher than those for pulverized boilers. And the PM in the submicron mode for burning with briquette contributes up to 86 % of PM10 emissions. Multiclones and scrubbers are not efficient for controlling PM10 emission. Their average collection efficiencies for sub-micron particle and super-micron particle are 34% and 78%, respectively. Operating conditions of industrial steam boilers have influence on PM generation. Peak of the submicron mode during normal operation period is larger than the start-up period.

关键词： Coal-fired chain-grate boiler PM10 Size distribution Particulate emission control devices Size-dependent collection efficiency

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