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An Environment‑Tolerant Ion‑Conducting Double‑Network Composite Hydrogel for High‑Performance Flexible Electronic Devices

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Nano-Micro Letters 2024年第5期16卷 352-369页

作者： Wenchao Zhao Haifeng Zhou Wenkang Li Manlin Chen Min Zhou Long Zhao state key laboratory of Advanced Electromagnetic technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China school of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China

High-performance ion-conducting hydrogels(ICHs)are vital for developing flexible electronic ***,the robustness and ion-conducting behavior of ICHs deteriorate at extreme tempera-tures,hampering their use in soft *** resolve these issues,a method involving freeze–thawing and ionizing radiation technology is reported herein for synthesizing a novel double-network(DN)ICH based on a poly(ionic liquid)/MXene/poly(vinyl alcohol)(PMP DN ICH)*** well-designed ICH exhibits outstanding ionic conductivity(63.89 mS cm^(-1) at 25℃),excellent temperature resistance(-60–80℃),prolonged stability(30 d at ambient temperature),high oxidation resist-ance,remarkable antibacterial activity,decent mechanical performance,and ***,the ICH performs effectively in a flexible wireless strain sensor,thermal sensor,all-solid-state supercapacitor,and single-electrode triboelectric nanogenerator,thereby highlighting its viability in constructing soft electronic *** highly integrated gel structure endows these flexible electronic devices with stable,reliable signal output *** particular,the all-solid-state supercapacitor containing the PMP DN ICH electrolyte exhibits a high areal specific capacitance of 253.38 mF cm^(-2)(current density,1 mA cm^(-2))and excellent environmental *** study paves the way for the design and fabrication of high-performance mul-tifunctional/flexible ICHs for wearable sensing,energy-storage,and energy-harvesting applications.

关键词： Ionic liquids Double-network hydrogels Temperature tolerance Multifunctionality Flexible electronic devices

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FSS: algorithm and neural network accelerator for style transfer

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Science China(Information Sciences) 2024年第2期67卷 253-266页

作者： Yi LING Yujie HUANG Yujie CAI Zhaojie LI Mingyu WANG Wenhong LI Xiaoyang ZENG state key laboratory of ASIC & System Fudan University Shanghai Explore X technology Co. Ltd.

Neural networks(NNs), owing to their impressive performance, have gradually begun to dominate multimedia processing. For resource-constrained and energy-sensitive mobile devices, an efficient NN accelerator is necessary. Style transfer is an important multimedia application. However, existing arbitrary style transfer networks are complex and not well supported by current NN accelerators, limiting their application on mobile devices. Moreover, the quality of style transfer needs improvement. Thus, we design the Fast Style system(FSS), where a novel algorithm and an NN accelerator are proposed for style transfer. In FSS, we first propose a novel arbitrary style transfer algorithm, Fast Style. We propose a light network that contributes to high quality and low computational complexity and a prior mechanism to avoid retraining when the style changes. Then, we redesign an NN accelerator for Fast Style by applying two improvements to the basic NVIDIA deep learning accelerator(NVDLA) architecture. First, a flexible dat FSM and wt FSM are redesigned to enable the original data path to perform other operations(including the GRAM operation)by software programming. Moreover, statistics and judgment logic are designed to utilize the continuity of a video stream and remove the data dependency in the instance normalization, which improves the accelerator performance by 18.6%. The experimental results demonstrate that the proposed Fast Style can achieve higher quality with a lower computational cost, making it more suitable for mobile devices. The proposed NN accelerator is implemented on the Xilinx VCU118 FPGA under a 180-MHz clock. Experimental results show that the accelerator can stylize 512×512-pixel video with 20 FPS, and the measured performance reaches up to 306.07 GOPS. The ASIC implementation in TSMC 28 nm achieves about 22 FPS in the case of a 720-p video.

关键词： neural network accelerator style transfer neural network deep learning

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Photocatalytic in situ H_(2)O_(2) production and activation for enhanced ciprofloxacin degradation over CeO_(2)-Co_(3)O_(4)/g-C_(3)N_(4):key role of CeO_(2)

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Rare Metals 2024年第6期43卷 2695-2707页

作者： Hong-Jie Zhu Yi-Kai Yang Ming-Hui Li Lu-Ning Zou Hai-Tao Zhao Shandong Provincial key laboratory of Chemical Energy Storage and novel Cell technology School of Chemistry and Chemical Engin College of Ecology and Environment Anhui Normal UniversityWuhu241002China Liaocheng YiLu Advanced Materials Co. LtdLiaocheng 252000China

The abused ciprofloxacin antibiotics have caused significant environmental *** oxidative degradation of ciprofloxacin exhibits promising efficacy,it often entails excessive energy ***,it is necessary to explore an effective and ecologically sustainable degradation ***,we demonstrated that g-C_(3)N_(4) decorated with the coordinated CeO_(2)and Co_(3)O_(4)(CeO_(2)-Co_(3)O_(4)/CN)exhibited effective ciprofloxacin photodegradation via in situ H_(2)O_(2) production and activation *** indicate that the introduced CeO_(2) enhances the transference of photogenerated electrons to O_(2) by adjusting the oxygen vacancy of photocatalyst,thereby increasing the generation of superoxide radicals,which in turn generate H_(2)O_(2),resulting in a 22.4-fold increase in H_(2)O_(2) generation over g-C_(3)N_(4).Moreover,the in situ H_(2)O_(2)generation facilitated by CeO_(2) is confirmed to be essential for ciprofloxacin degradation via CeO_(2)-Co_(3)O_(4)/CN,as it provides enough oxidant for Co_(3)O_(4) to activate into hydroxyl radicals for the pollutants ***,CeO_(2)-Co_(3)O_(4)/CN achieves a ciprofloxacin degradation ratio of 97.7%within 80 *** study introduces a novel approach that combines H_(2)O_(2) generation and activation,offering an innovative perspective for achieving clean and efficient purification of antibiotic-contaminated water.

关键词： CeO_(2) In situ H_(2)O_(2)generation Ciprofloxacin degradation Photocatalyst

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From Topological Nodal-Line Semimetals to Quantum Spin Hall Insulators in Tetragonal SnX Monolayers(X=F,Cl,Br,I)

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Chinese Physics Letters 2024年第6期41卷 98-111页

作者：朱晔赵宝薛阳徐玮徐文婷杨中芹 state key laboratory of Surface Physics Key Laboratory of Computational Physical Sciences(MOE)and Department of PhysicsFudan UniversityShanghai 200433China Shandong key laboratory of Optical Communication Science and technology School of Physics Science and Information TechnologyLiaocheng UniversityLiaocheng 252059China school of Physics East China University of Science and TechnologyShanghai 200237China Shanghai Qi Zhi Institute Shanghai 200030China

Two-dimensional(2D)topological materials have recently garnered significant interest due to their profound physical properties and promising applications for future quantum *** various topological states within one type of materials is,however,seldom *** on first-principles calculations and tightbinding models,we investigate topological electronic states in a novel family of 2D halogenated tetragonal stanene(T-SnX,X=F,Cl,Br,I).All the four monolayers are found to be unusual topological nodal-line semimetals(NLSs),protected by a glide mirror *** spin-orbit coupling(SOC)is turned on,T-SnF and TSnCl are still ascertained as topological NLSs due to the remaining band inversion,primarily composed of Sn pxy orbitals,while T-Sn Br and T-SnI become quantum spin Hall *** phase transition is ascribed to moving up in energy of Sn s orbitals and increasing of SOC *** topology origin in the materials is uniformly rationalized through elementary band *** robust and diverse topological states found in the 2D T-SnX monolayers position them as an excellent material platform for development of innovative topological electronics.

关键词： topological metals quantum

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An evolutionary multiobjective method based on dominance and decomposition for feature selection in classification

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Science China(Information Sciences) 2024年第2期67卷 5-19页

作者： Jing LIANG Yuyang ZHANG Ke CHEN Boyang QU Kunjie YU Caitong YUE Ponnuthurai Nagaratnam SUGANTHAN school of Electrical and Information Engineering Zhengzhou University state key laboratory of Intelligent Agricultural Power Equipment school of Electrical Engineering and Automation Henan Institute of Technology school of Electronics and Information Zhongyuan University of Technology KINDI Center for Computing Research College of EngineeringQatar University

Feature selection in classification can be considered a multiobjective problem with the objectives of increasing classification accuracy and decreasing the size of the selected feature subset. Dominance-based and decomposition-based multiobjective evolutionary algorithms(MOEAs) have been extensively used to address the feature selection problem due to their strong global search capability. However, most of them face the problem of not effectively balancing convergence and diversity during the evolutionary process. In addressing the aforementioned issue, this study proposes a unified evolutionary framework that combines two search forms of dominance and decomposition. The advantages of the two search methods assist one another in escaping the local optimum and inclining toward a balance of convergence and diversity. Specifically, an improved environmental selection strategy based on the distributions of individuals in the objective space is presented to avoid duplicate feature subsets. Furthermore, a novel knowledge transfer mechanism that considers evolutionary characteristics is developed, allowing for the effective implementation of positive knowledge transfer between dominance-based and decomposition-based feature selection methods. The experimental results demonstrate that the proposed algorithm can evolve feature subsets with good convergence and diversity in a shorter time compared with 9 state-of-the-art feature selection methods on 20 classification problems.

关键词： evolutionary algorithms feature selection multiobjective optimization knowledge transfer classification

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Evolution of anomalous Hall effect in ferromagnetic Weyl semimetal Nb_(x)Zr_(1-x)Co_(2)Sn

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Chinese Physics B 2024年第8期33卷 491-496页

作者：陈博文沈冰 Center for Neutron Science and technology Guangdong Provincial Key Laboratory of Magnetoelectric Physics and DevicesSchool of PhysicsSun Yat-Sen UniversityGuangzhou 510275China state key laboratory of Optoelectronic Materials and Technologies Sun Yat-Sen UniversityGuangzhou 510275China

Magnetic topological semimetal can host various topological non-trivial states leading to exotic novel transport *** we report the systematic magneto-transport studies on the Heusler alloy Nb_(x)Zr_(1-x)Co_(2)Sn considered as a ferromagnetic(FM)Weyl *** cusp anomaly of temperature-dependent resistivity and large isotropic negative magneto-resistivity(MR)emerge around the FM transition consistent with the theoretical half-metallic *** prominent anomalous Hall effect(AHE)has the same behavior with the applied field along various crystal *** Nb doping introduces more disorder resulting in the enhancement of the upturn for the temperature-dependent resistivity in low *** Nb doping,the AHE exhibits systemic evolution with the Fermi level *** the doping level of x=0.25,the AHE mainly originates from the intrinsic contribution related to non-trivial topological Weyl states.

关键词： anomalous Hall effect magnetic Weyl semimetal ferromagnetism

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A dual-function selection system enables positive selection of multigene CRISPR mutants and negative selection of Cas9-free progeny in Arabidopsis

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aBIOTECH 2024年第2期5卷 140-150页

作者： Feng-Zhu Wang Ying Bao Zhenxiang Li Xiangyu Xiong Jian-Feng Li state key laboratory of Biocontrol Guangdong Provincial Key Laboratory of Plant ResourcesSchool of Life SciencesSun Yat-sen UniversityGuangzhou 510275China

The CRISPR/Cas9 technology revolutionizes targeted gene knockout in diverse organisms including ***,screening edited alleles,particularly those with multiplex editing,from herbicide-or antibiotic-resistant transgenic plants and segregating out the Cas9 transgene represent two laborious *** solutions to facilitate these processes rely on different selection ***,by taking advantage of the opposite functions of a D-amino acid oxidase(DAO)in detoxifying D-serine and in metabolizing non-toxic D-valine to a cytotoxic product,we develop a DAO-based selection system that simultaneously enables the enrichment of multigene edited alleles and elimination of Cas9-containing progeny in Arabidopsis *** five DAOs tested in Escherichia coli,the one encoded by Trigonopsis variabilis(TvDAO)could confer slightly stronger D-serine resistance than other *** expression of TvDAO in Arabidopsis allowed a clear distinction between transgenic and nontransgenic plants in both D-serine-conditioned positive selection and D-valine-conditioned negative *** a proof of concept,we combined CRISPR-induced single-strand annealing repair of a dead TvDAO with D-serine-based positive selection to help identify transgenic plants with multiplex editing,where D-serine-resistant plants exhibited considerably higher co-editing frequencies at three endogenous target genes than those selected by ***,D-valine-based negative selection successfully removed Cas9 and TvDAO transgenes from the survival offspring carrying inherited ***,this work provides a novel strategy to ease CRISPR mutant identification and Cas9 transgene elimination using a single selection marker,which promises more efficient and simplified multiplex CRISPR editing in plants.

关键词： CRISPR Genome editing D-amino acid oxidase Cas9-free Selection marker

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Multifunctional 2-(2-hydroxyphenyl)benzoxazoles: Ready synthesis,mechanochromism, fluorescence imaging, and OLEDs

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Chinese Chemical Letters 2024年第10期35卷 249-253页

作者： Kangmin Wang Liqiu Wan Jingyu Wang Chunlin Zhou Ke Yang Liang Zhou Bijin Li Chongqing key laboratory of Natural Product Synthesis and Drug Research School of Pharmaceutical Sciences Chongqing University state key laboratory of Rare Earth Resource Utilization Changchun Institute of Applied Chemistry Chinese Academy of Sciences Jiangsu key laboratory of Advanced Catalytic Materials & technology School of Petrochemical Engineering Changzhou University

Triphenylamine(TPA)-containing 2-(2-hydroxyphenyl)benzoxazoles(2a-2c) have been synthesized via a highly efficient rhodium-catalyzed C–H/C–H cross-coupling reaction. Compound 2a is a novel mechanofluorochromic material with blue-shifted mechanochromic properties. Compounds 2b and 2c presented opposite mechanochromic trends. For 2b, the enol-form emission enhanced, and the ketoform emission blue-shift after grinding. In contrast, 2c exhibited the weak enol-form emission disappeared and the keto-form emission slightly red-shift after grinding treatments. The estrone-containing2b-based water-dispersed nanoparticles(NPs) exhibit apparent dual-emission and were applied for fluorescence images. In addition, bis(TPA)-containing 2c-based devices exhibit dual-emission with good performance and a singlet exciton yield of 92%, which breaks through the theoretical upper limit of 25%in conventional fluorescent OLEDs. This is one of the highest exciton utilization values recorded for the ESIPT molecules with a dual emission system.

关键词： 2-(2′-Hydroxyphenyl)benzoxazoles Fluorescence images Mechanochromism OLEDs Rhodium-catalyzed

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Computational Experiments for Complex Social Systems:Experiment Design and Generative Explanation

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IEEE/CAA Journal of Automatica Sinica 2024年第4期11卷 1022-1038页

作者： Xiao Xue Deyu Zhou Xiangning Yu Gang Wang Juanjuan Li Xia Xie Lizhen Cui Fei-Yue Wang the school of Computer software College of Intelligence and ComputingTianjin UniversityTianjin 300350China the school of software and the Joint SDUNTU Centre for Artificial Intelligence Research(C-FAIR) Shandong UniversityJinan 250101China the Information school Xi’an University of Financial and EconomicsXi’an 710100China the state key laboratory of Multimodal Artificial Intelligence Systems Institute of AutomationChinese Academy of SciencesBeijing 100190China Hainan University Haikou 570228China the state key laboratory for Management and Control of Complex Systems Institute of AutomationChinese Academy of SciencesBeijing 1001901China

Powered by advanced information technology,more and more complex systems are exhibiting characteristics of the cyber-physical-social systems(CPSS).In this context,computational experiments method has emerged as a novel approach for the design,analysis,management,control,and integration of CPSS,which can realize the causal analysis of complex systems by means of“algorithmization”of“counterfactuals”.However,because CPSS involve human and social factors(e.g.,autonomy,initiative,and sociality),it is difficult for traditional design of experiment(DOE)methods to achieve the generative explanation of system *** address this challenge,this paper proposes an integrated approach to the design of computational experiments,incorporating three key modules:1)Descriptive module:Determining the influencing factors and response variables of the system by means of the modeling of an artificial society;2)Interpretative module:Selecting factorial experimental design solution to identify the relationship between influencing factors and macro phenomena;3)Predictive module:Building a meta-model that is equivalent to artificial society to explore its operating ***,a case study of crowd-sourcing platforms is presented to illustrate the application process and effectiveness of the proposed approach,which can reveal the social impact of algorithmic behavior on“rider race”.

关键词： Agent-based modeling computational experiments cyber-physical-social systems(CPSS) generative deduction generative experiments meta model

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Adaptive Bistable Stochastic Resonance Based Weak Signal Reception in Additive Laplacian Noise

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China Communications 2024年第1期21卷 228-241页

作者： Jin Liu Zan Li Qiguang Miao Li Yang school of Computer Science and technology Xidian UniversityXi’an 710071China state key laboratory of Integrated Services Networks Xidian UniversityXi’an 710071China

Weak signal reception is a very important and challenging problem for communication systems especially in the presence of non-Gaussian noise,and in which case the performance of optimal linear correlated receiver degrades *** at this,a novel uncorrelated reception scheme based on adaptive bistable stochastic resonance(ABSR)for a weak signal in additive Laplacian noise is *** analyzing the key issue that the quantitative cooperative resonance matching relationship between the characteristics of the noisy signal and the nonlinear bistable system,an analytical expression of the bistable system parameters is *** this basis,by means of bistable system parameters self-adaptive adjustment,the counterintuitive stochastic resonance(SR)phenomenon can be easily generated at which the random noise is changed into a benefit to assist signal ***,it is demonstrated that approximately 8dB bit error ratio(BER)performance improvement for the ABSR-based uncorrelated receiver when compared with the traditional uncorrelated receiver at low signal to noise ratio(SNR)conditions varying from-30dB to-5dB.

关键词： adaptive bistable stochastic resonance additive Laplacian noise low signal to noise ratio uncorrelated reception scheme weak signal reception

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