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Spin transport of half-metal Mn_(2)X_(3) with high Curie temperature:An ideal giant magnetoresistance device from electrical and thermal drives

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Frontiers of physics 2024年第4期19卷 125-135页

作者： Bin Liu Xiaolin Zhang Jingxian Xiong Xiuyang Pang Sheng Liu Zixin Yang Qiang Yu Honggen Li Sicong Zhu Jian Wu Hubei Province key laboratory of Systems Science in Metallurgical Process The State Key Laboratory for Refractories and MetallurgyCollaborative Innovation Center for Advanced SteelsInternational Research Institute for Steel TechnologyWuhan University of Science and TechnologyWuhan 430081China key laboratory of Artificial micro-and nano-structures of Ministry of Education and school of Physical and Technology Wuhan UniversityWuhan 430072China College of Advanced Interdisciplinary Studies Nanhu Laser LaboratoryNational University of Defense TechnologyChangsha 410073China Department of Mechanical Engineering National University of SingaporeSingapore 117575Singapore i-Lab&key laboratory of nanodevices and Applications&key laboratory of nanophotonic materials and devices Suzhou Institute of Nano-Tech and NanoBionicsChinese Academy of SciencesSuzhou 215123China Institute of Optical Science and Technology School of Physics and AstronomyShanghai Jiao Tong UniversityShanghai 200240China

Currently,magnetic storage devices are encountering the problem of achieving lightweight and high integration in mobile computing devices during the information *** a result,there is a growing urgency for twodimensional half-metallic materials with a high Curie temperature(TC).This study presents a theoretical investigation of the fundamental electromagnetic properties of the monolayer hexagonal lattice of Mn_(2)X_(3)(X=S,Se,Te).Additionally,the potential application of Mn_(2)X_(3) as magneto-resistive components is *** three of them fall into the category of ferromagnetic *** particular,the Monte Carlo simulations indicate that the TC of Mn2S3 reachs 381 K,noticeably greater than room *** findings present notable advantages for the application of Mn2S3 in spintronic ***,a prominent spin filtering effect is apparent when employing non-equilibrium Green’s function simulations to examine the transport *** resulting current magnitude is approximately 2×10^(4) nA,while the peak gigantic magnetoresistance exhibits a substantial value of 8.36×10^(16)%.It is noteworthy that the device demonstrates a substantial spin Seebeck effect when the temperature differential between the electrodes is *** brief,Mn_(2)X_(3) exhibits outstanding features as a highTC half-metal,exhibiting exceptional capabilities in electrical and thermal drives spin ***,it holds great potential for usage in spintronics applications.

关键词： half-metals Mn_(2)X_(3) high Curie temperature electrical and thermal GMR

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Research progress on rolling superlubricity in solid lubricants

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Science China(Technological Sciences) 2024年第7期67卷 1980-1990页

作者： LI PanPan LI HongXuan ZHU DongXiang ZHU YongQi KANG FuYan WANG Wan ZHANG YaXin LIU XiaoHong JI Li ZHOU HuiDi CHEN JianMin State key laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Center of materials Science and optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China school of Chemical Engineering Northwest Minzu UniversityLanzhou 730030China

Superlubricity is an ideal lubrication state where friction nearly vanishes between contact interfaces. It has become one of the most important research topics and approaches owing to its significance in reducing energy consumption and preventing device failures. As an efficient and universal lubricating principle capable of achieving superlubricity, rolling lubrication has attracted widespread attention in recent years. In this review, the theoretical concept of rolling lubrication and the experimental research progress of spherical/scroll structures are summarized. The review focuses on the possibility of achieving rolling lubrication using spherical/scroll structures(such as spherical fullerenes, carbon nanotubes, and formed and constructed spherical/scroll structures). The challenges in achieving rolling lubrication are summarized, and the possibility of molecular rolling lubrication,as well as its potential applications in superlubrication, are discussed.

关键词： spherical/scroll structure rolling lubrication superlubricity fullerene

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Gas diffusion in catalyst layer of flow cell for CO_(2) electroreduction toward C_(2+) products

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nano Research 2024年第3期17卷 1101-1106页

作者： Xiqing Wang Qin Chen Yajiao Zhou Yao Tan Ye Wang Hongmei Li Yu Chen Mahmoud Sayed Ramadan A.Geioushy Nageh K.Allam Junwei Fu Yifei Sun Min Liu hunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics and ElectronicsCentral South UniversityChangsha 410083China school of energy and Power Engineering Beihang UniversityBeijing 100191China school of materials Science and Engineering Zhengzhou UniversityZhengzhou 450002China Central Metallurgical Research and Development Institute(CMRDI) P.O.Box 87Helwan 11421CairoEgypt energy materials laboratory School of Sciences and EngineeringThe American University in CairoNew Cairo 11835Egypt Research Center for Advanced energy and Carbon Neutrality Beihang UniversityBeijing 100191China

The use of gas diffusion electrode(GDE)based flow cell can realize industrial-scale CO_(2) reduction reactions(CO_(2)RRs).Controlling local CO_(2) and CO intermediate diffusion plays a key role in CO_(2)RR toward multi-carbon(C_(2+))*** this work,local CO_(2) and CO intermediate diffusion through the catalyst layer(CL)was investigated for improving CO_(2)RR toward C_(2+)*** gas permeability tests and finite element simulation results indicated CL can balance the CO_(2) gas diffusion and residence time of the CO intermediate,leading to a sufficient CO concentration with a suitable CO_(2)/H_(2)O supply for high C_(2+)*** a result,an excellent selectivity of C_(2+)products~79%at a high current density of 400 mA·cm^(-2) could be obtained on the optimal 500 nm Cu CL(Cu500).This work provides a new insight into the optimization of CO_(2)/H_(2)O supply and local CO concentration by controlling CL for C_(2+)products in CO_(2)RR flow cell.

关键词： gas diffusion electrode CO_(2)reduction Cu mass transfer C_(2)product

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Metamaterial terahertz device with temperature regulation function that can achieve perfect absorption and complete reflection conversion of ultrawideband

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Communications in Theoretical physics 2024年第7期76卷 125-135页

作者： Hao Sun Zao Yi Can Ma Shubo Cheng Bin Tang Qingdong Zeng Sohail Ahmad school of Mathematics and Science Joint Laboratory for Extreme Conditions Matter Properties State Key Laboratory of Environment-Friendly Energy Materials Tianfu Institute of Research and InnovationSouthwest University of Science and Technology Department of Oncology Sichuan Science City Hospital school of Chemistry and Chemical Engineering Jishou University school of physics and Optoelectronic Engineering Yangtze University school of microelectronics and Control Engineering Changzhou University school of physics and Electronic Information Engineering Hubei Engineering University Institute of physics Bahauddin Zakariya University

The field of terahertz devices is important in terahertz technology. However, most of the current devices have limited functionality and poor performance. To improve device performance and achieve multifunctionality, we designed a terahertz device based on a combination of VO2and metamaterials. This device can be tuned using the phase-transition characteristics of VO2, which is included in the triple-layer structure of the device, along with SiO2and Au. The terahertz device exhibits various advantageous features, including broadband coverage, high absorption capability, dynamic tunability, simple structural design, polarization insensitivity, and incidentangle insensitivity. The simulation results showed that by controlling the temperature, the terahertz device achieved a thermal modulation range of spectral absorption from 0 to 0.99. At 313 K, the device exhibited complete reflection of terahertz waves. As the temperature increased,the absorption rate also increased. When the temperature reached 353 K, the device absorption rate exceeded 97.7% in the range of 5–8.55 THz. This study used the effective medium theory to elucidate the correlation between conductivity and temperature during the phase transition of VO2. Simultaneously, the variation in device performance was further elucidated by analyzing and depicting the intensity distribution of the electric field on the device surface at different temperatures. Furthermore, the impact of various structural parameters on device performance was examined, offering valuable insights and suggestions for selecting suitable parameter values in real-world applications. These characteristics render the device highly promising for applications in stealth technology, energy harvesting, modulation, and other related fields, thus showcasing its significant potential.

关键词： complete reflection perfect absorption smart device temperature regulation terahertz ultrawideband

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Wearable multichannel-active pressurized pulse sensing platform Yunlong

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microsystems & nanoengineering 2024年第3期10卷 283-292页

作者： Zhao Qingxia Sun Shixuan Mei Libo Gao Xikuan Zhang Zekun Yang Xueli Nan Haiyan Zhang Chenyang Xue Junyang Li Pen-Tung Sah Institute of micro-nano Science and Technology Xiamen University361102 XiamenChina Discipline of Intelligent Instrument and Equipment Xiamen University361102 XiamenChina Department of Electronic Engineering Ocean University of China266000 QingdaoChina school of Automation and Software Engineering Shanxi University030006 TaiyuanChina Innovation laboratory for Sciences and Technologies of energy materials of Fujian Province(IKKEM) 361005 XiamenChina key laboratory of Instrumentation Science and Dynamic Measurement Ministry of Education North University of China030051 TaiyuanChina Science and Technology on Vacuum Technology and physics laboratory Lanzhou Institute of PhysicsChinese Academy of Space Technology730000 LanzhouChina

With the modernization of traditional Chinese medicine(TCM),creating devices to digitalize aspects of pulse diagnosis has proved to be *** currently available pulse detection devices usually rely on external pressure devices,which are either bulky or poorly integrated,hindering their practical *** this work,we propose an innovative wearable active pressure three-channel pulse monitoring device based on TCM pulse diagnosis *** combines a flexible pressure sensor array,flexible airbag array,active pressure control unit,advanced machine learning approach,and a companion mobile application for human–computer *** to the high sensitivity(460.1 kPa^(−1)),high linearity(R^(2)>0.999)and flexibility of the flexible pressure sensors,the device can accurately simulate finger pressure to collect pulse waves(Cun,Guan,and Chi)at different external pressures on the *** addition,by measuring the change in pulse wave amplitude at different pressures,an individual’s blood pressure status can be successfully *** enables truly wearable,actively pressurized,continuous wireless dynamic monitoring of wrist pulse *** innovative and integrated design of this pulse monitoring platform could provide a new paradigm for digitizing aspects of TCM and other smart healthcare systems.

关键词： pulse diagnosis enable

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Interface optimization and defects suppression via Na F introduction enable efficient flexible Sb_(2)Se_(3) thin-film solar cells

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Journal of energy Chemistry 2024年第3期90卷 165-175,I0006页

作者： Mingdong Chen Muhammad Ishaq Donglou Ren Hongli Ma Zhenghua Su Ping Fan David Le Coq Xianghua Zhang Guangxing Liang Shuo Chen Shenzhen key laboratory of Advanced Thin Films and Applications Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060GuangdongChina State key laboratory of Featured Metal materials and Life-cycle Safety for Composite Structures MOE Key Laboratory of New Processing Technology for Nonferrous Metals and MaterialsSchool of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004GuangxiChina CNRS ISCR(Institut des Sciences Chimiques de Rennes)UMR 6226Universitéde RennesRennes F-35000France

Sb_(2)Se_(3) with unique one-dimensional(1D) crystal structure exhibits exceptional deformation tolerance,demonstrating great application potential in flexible ***,the power conversion efficiency(PCE) of flexible Sb_(2)Se_(3) photovoltaic devices is temporarily limited by the complicated intrinsic defects and the undesirable contact ***,a high-quality Sb_(2)Se_(3) absorber layer with large crystal grains and benign [hkl] growth orientation can be first prepared on a Mo foil *** NaF intermediate layer is introduced between Mo and Sb_(2)Se_(3),which can further optimize the growth of Sb_(2)Se_(3)thin ***,positive Na ion diffusion enables it to dramatically lower barrier height at the back contact interface and passivate harmful defects at both bulk and *** a result,the champion substrate structured Mo-foil/Mo/NaF/Sb_(2)Se_(3)/CdS/ITO/Ag flexible thin-film solar cell delivers an obviously higher efficiency of 8.03% and a record open-circuit voltage(V_(OC)) of 0.492 *** flexible Sb_(2)Se_(3) device also exhibits excellent stability and flexibility to stand large bending radius and multiple bending times,as well as superior weak light photo-response with derived efficiency of 12.60%.This work presents an effective strategy to enhance the flexible Sb_(2)Se_(3) device performance and expand its potential photovoltaic applications.

关键词： Sb_(2)Se_(3) Flexible solar cells NaF intermediate layer Interface optimization Defects suppression

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Phase reconfiguration of heterogeneous CoFeS/CoNiS nanoparticles for superior battery-type supercapacitors

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Journal of energy Chemistry 2024年第9期96卷 217-225页

作者： Lina Ma Fan Li Min Zhou Jidong Dong Hao Luo Wei Zhang Wenchao Zhao Xinliang Li Zaixing Jiang Yudong Huang College of Chemistrynd Chemical Engineering Qingdao UniversityQingdao 266071ShandongChina school of materials Sciencend Engineering Xiamen University of TechnologyXiamen 361024FujianChina Co-Innovation Center of Efficient Processingnd Utilization of Forest Resources College of Materials Sciencend EngineeringNanjing Forestry UniversityNanjing 210037JiangusChina key laboratory of Material physics Ministry of EducationSchool of Physicsnd MicroelectronicsZhengzhou UniversityZhengzhou 450052HenanChina MIIT key laboratory of Critical materials Technology for New energy Conversionnd Storage State Key Laboratory of Urban Water Resourcend EnvironmentSchool of Chemistrynd Chemical EngineeringHarbin Institute of TechnologyHarbin 150001HeilongjiangChina Material Sciencend Engineering College Northeast Forestry UniversityHarbin 150040HeilongjiangChina

Developing advanced battery-type materials with abundant active sites,high conductivity,versatile morphologies,and hierarchically porous structures is crucial for realizing high-quality hybrid ***,heterogeneous FeS@NiS is synthesized by cationic Co doping via surface-structure *** density functional theory(DFT)theoretical calculations are firstly performed to predict the advantages of Co dopant by improving the OH^(−)adsorption properties and adjusting electronic structure,benefiting ions/electron *** dynamic surface evolution is further explored which demonstrates that CoFeS@CoNiS could be quickly reconstructed to Ni(Co)Fe_(2)O_(4)during the charging process,while the unstable structure of the amorphous Ni(Co)Fe_(2)O_(4)results in partial conversion to Ni/Co/FeOOH at high potentials,which contributes to the more reactive active site and good structural ***,the free-standing electrode reveals excellent electrochemical performance with a superior capacity(335.6 mA h g^(−1),2684 F g^(−1))at 3 A g^(−1).Furthermore,the as-fabricated device shows a quality energy density of 78.1 W h kg^(−1)at a power density of 750 W kg^(−1)and excellent cycle life of 92.1%capacitance retention after 5000 *** work offers a facile strategy to construct versatile morphological structures using electrochemical activation and holds promising applications in energy-related fields.

关键词： In-situ reconfiguration Heterogeneous design Battery-type supercapacitors Superior performance Sulphide

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Numerical studies for plasmas of a linear plasma device HIT-PSI with geometry modified SOLPS-ITER

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Chinese physics B 2024年第3期33卷 503-508页

作者：王敏聂秋月黄韬王晓钢张彦杰 school of physics Harbin Institute of TechnologyHarbin 150001China school of Electrical Engineering and Automation Harbin Institute of TechnologyHarbin 150001China laboratory for Space Environment and Physical Sciences Harbin Institute of TechnologyHarbin 150001China MOE (Ministry of Education) key laboratory of materials Modification by Laser Ionand Electron BeamsSchool of PhysicsDalian Institute of TechnologyDalian 116024China

The HIT-PSI is a linear plasma device built for physically simulating the high heat flux environment of future reactor divertors to test/develop advanced target plate *** this study,the geometry-modified SOLPS-ITER program is employed to examine the effects of the magnetic field strength and neutral pressure in the device on the heat flux experienced by the target plate of the HIT-PSI *** findings of the numerical simulation indicate a positive correlation between the magnetic field strength and the heat flux ***,there is a negative correlation observed between the heat flux density and the neutral *** the magnetic field strength at the axis exceeds 1 tesla and the neutral pressure falls below 10 Pa,the HIT-PSI has the capability to attain a heat flux of 10 MW·m-2 at the target *** simulation results offer a valuable point of reference for subsequent experiments at HIT-PSI.

关键词： HIT-PSI heat flux linear plasma SOLPS-ITER device

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Simultaneously optimizing exciton diffusion length and nonradiative energy loss in organic solar cells via ternary strategy

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Science China Chemistry 2024年第9期67卷 3004-3011页

作者： Huanxiang Jiang Hao Lu Zezhou Liang Yonghai Li Guangliu Ran Chenyu Han Yuqiang Liu Hongxiang Li Xichang Bao Zhishan Bo College of Textiles and Clothing State Key Laboratory of Bio-fibers and Eco-textiles Qingdao University key laboratory for Physical Electronics and devices of the Ministry of Education & Shaanxi Key Lab of Photonic Technique for InformationSchool of Electronics Science & Engineering Faculty of Electronic and Information Engineering Xi'an Jiaotong University Qingdao Institute of Bioenergy and Bioprocess Technology Chinese Academy of Sciences laboratory of Solar energy Shandong Energy Institute Department of physics and Applied Optics Beijing Area Major laboratory Center for Advanced Quantum Studies Beijing Normal University College of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University

Significant nonradiative energy loss and short exciton diffusion length in organic solar cells(OSCs) are two major obstacles to achieving state-of-the-art efficiencies. It is crucial to conduct a study on the intensive mechanism and improvement strategies for future breakthroughs in the efficiency of OSCs. In this work, nonradiative energy loss and exciton diffusion length are optimized simultaneously by incorporating a guest acceptor(LA15) to construct ternary OSC(D18:L8-BO:LA15). Firstly, LA15 exhibits excellent compatibility with the host acceptor L8-BO, and effectively improves the fluorescence quantum efficiency(FLQY),resulting in suppressed non-radiative energy loss. Moreover, LA15 effectively prolongs the fluorescent lifetime of the acceptor phase from 0.85 to 1.12 ns, leading to larger exciton diffusion length, which is beneficial for reducing geminate ***, the addition of LA15 optimizes the crystallinity of the active layer with amplified charge transport capacity. As a result,the optimized D18:L8-BO:LA15 device achieves ultralow nonradiative energy loss of 0.18 e V and improved fill factor(FF) with high efficiency up to 19.13%. These results highlight the crucial roles of regulating FLQYand exciton lifetime in achieving highefficiency OSCs.

关键词： organic solar cells nonradiative energy loss exciton lifetime exciton diffusion length

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Ta_(2)NiSe_(5)/GaN范德华异质结用于具有超高响应性和耐恶劣环境的紫外光电探测器

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Science China materials 2024年第3期67卷 863-870页

作者：雷剑鹏郑涛吴望龙郑照强郑筌升王小周肖文波李京波杨孟孟 Jiangxi Engineering laboratory for optoelectronics Testing Technology Nanchang Hangkong UniversityNanchang 330063China Guangdong Provincial key laboratory of Chip and Integration Technology School of Semiconductor Science and TechnologySouth China Normal UniversityFoshan 528225China school of materials and energy Guangdong University of TechnologyGuangzhou 510006China Department of Applied physics School of Physics and ElectronicsHunan UniversityChangsha 410082China College of Optical Science and Engineering Zhejiang UniversityHangzhou 310027China

氮化镓由于其直接带隙、固有的紫外吸收和高击穿电压引起了人们对其在紫外光电探测领域的极大研究兴趣.在本工作中,我们成功地将新型三元硫族化合物Ta_(2)NiSe_(5)与非故意掺杂的GaN堆叠,形成了具有典型I型能带排列的混合维度的Ta_(2)Ni... 详细信息

氮化镓由于其直接带隙、固有的紫外吸收和高击穿电压引起了人们对其在紫外光电探测领域的极大研究兴趣.在本工作中,我们成功地将新型三元硫族化合物Ta_(2)NiSe_(5)与非故意掺杂的GaN堆叠,形成了具有典型I型能带排列的混合维度的Ta_(2)NiSe_(5)/GaN(2D/3D)范德瓦尔斯异质结构.该异质结构表现出优异的紫外探测性能(光开关比为10~7,响应度为1.22×10^(4)A W^(-1)).此外,在365 nm的光照和4 V的偏压下,探测度提高至1.3×10^(16)Jones,并表现出1.22/31.6 ms的快速响应速率.值得注意的是,该器件还具有优异的稳定性、可重复性和抗恶劣环境条件(包括高温和酸性条件)的耐受性.得益于光电探测器的高响应度、探测度和光开关比,我们成功地将该异质结构器件集成到紫外光通信中,证明了Ta_(2)NiSe_(5)/GaN光电探测器在信息传输中有着优异的应用前景.

关键词： GaN Ta_(2)NiSe_(5) heterojunction UV photodetector super-high responsivity harsh environment-resistant

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