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Improved Multiple Feature-electrochemical Thermal Coupling Modeling of Lithium-ion Batteries at Low-temperature with Real-time Coefficient Correction

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Protection and Control of Modern Power Systems 2024年第3期9卷 157-173页

作者： Shunli Wang Haiying Gao Paul Takyi-Aninakwa Josep M.Guerrero Carlos Fernandez Qi Huang IET the school of Electric Power Inner Mongolia University of TechnologyInner Mongolia 010051China the school of Information Engineering Southwest University of Science and TechnologyMianyang 621010China southwest university of science and technology(SWUST) the Smart Energy Storage Institute the Department of Energy technology Aalborg UniversityDenmark Robert Gordon university IEEE southwest university of science and technology

Monitoring various internal parameters plays a core role in ensuring the safety of lithium-ion batteries in power supply *** also influences the sustainability effect and online state of charge *** improved multiple feature-electrochemical thermal coupling modeling method is proposed considering low-temperature performance degradation for the complete characteristic expression of multi-dimensional *** is to obtain the parameter influence mechanism with a multi-variable coupling *** optimized decoupled deviation strategy is constructed for accurate state of charge prediction with real-time correction of time-varying current and temperature *** innovative decoupling method is combined with the functional relationships of state of charge and open-circuit voltage to capture energy management ***,an adaptive equivalent-prediction model is constructed using the state-space equation and iterative feedback correction,making the proposed model adaptive to fractional *** maximum state of charge estimation errors of the proposed method are 4.57% and 0.223% under the Beijing bus dynamic stress test and dynamic stress test conditions,*** improved multiple feature-electrochemical thermal coupling modeling realizes the effective correction of the current and temperature variations with noise influencing coefficient,and provides an efficient state of charge prediction method adaptive to complex conditions.

关键词： Adaptive inner state characterization lithium-ion batteries low-temperature automatic-guided-vehicle multiple feature-electrochemical thermal coupling modeling real-time coefficient correction

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Conductive catalysis by subsurface transition metals

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National science Review 2024年第1期11卷 86-93页

作者： Xin Deng Caiyan Zheng Yangsheng Li Zeyu Zhou Jiamin Wang Yihua Ran Zhenpeng Hu Fan Yang Landong Li Frontiers science Center for New Organic Matter College of ChemistryNankai University school of Physics Nankai University school of physical science and technology Shanghai Tech University school of Materials science and Engineering Nankai University Haihe Laboratory of Sustainable Chemical Transformations

The nature of catalysis has been hotly pursued for over a century, and current research is focused on understanding active centers and their electronic structures. Herein, the concept of conductive catalysis is proposed and verified by theoretical simulations and experimental observations. Metallic systems containing buried catalytically active transitional metals and exposed catalytically inert main group metals are constructed, and the electronic interaction between them via metallic bonding is disclosed. Through the electronic interaction, the catalytic properties of subsurface transitional metals(Pd or Rh) can be transferred to outermost main group metals(Al or Mg) for several important transformations like semi-hydrogenation,Suzuki-coupling and hydroformylation. The catalytic force is conductive, in analogy with the magnetic force and electrostatic force. The traditional definition of active centers is challenged by the concept of conductive catalysis and the electronic nature of catalysis is more easily understood. It might provide new opportunities for shielding traditional active centers against poisoning or leaching and allow for precise regulation of their catalytic properties by the conductive layer.

关键词： electronic interaction conductive catalysis subsurface transition metal

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Facile synthesis of nanoparticles-stacked Co_(3)O_(4)nanoflakes with catalase-like activity for accelerating wound healing

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Regenerative Biomaterials 2024年第3期3卷 82-91页

作者： Yanan Huang Wanyi Liao Wenxuan Wang Tingting Zhang Yan Zhang Lei Lu school and Hospital of Stomatology Wenzhou Medical UniversityWenzhou 325027China sichuan Engineering Research Center for Biomimetic Synthesis of Natural Drugs School of Life Science and EngineeringSouthwest jiaotong UniversityChengdu 610031China Key Lab of Advanced technology of Materials of Education Ministry School of Materials Science and EngineeringSouthwest jiaotong UniversityChengdu 610031China school of Chemistry Southwest Jiaotong UniversityChengduSichuan 610031China

Delayed wound healing caused by excessive reactive oxygen species(Ros)remains a considerable *** recent years,metal oxide nanozymes have gained significant attention in biomedical ***,a comprehensive investigation of Co_(3)O_(4)-based nanozymes for enhancing wound healing and tissue regeneration is *** study focuses on developing a facile synthesis method to produce high-stability and costeffective Co_(3)O_(4)nanoflakes(NFs)with promising catalase(CAT)-like activity to regulate the oxidative microenvironment and accelerate wound *** closely arranged Co_(3)O_(4)nanoparticles(NPs)within the NFs structure result in a significantly larger surface area,thereby amplifying the enzymatic activity compared to commercially available Co_(3)O_(4)*** physiological conditions,itwas observed that CogO,NFs efficientlybreak down hydrogen peroxide(H_(2)O_(2))without generating harmful radicals(OH).Moreover,they exhibit excellent compatibility with various cells involved in wound healing,promoting fibroblast growth and protecting cells from oxidatives *** a ratmodel,Co_(3)O_(4) NFs facilitate both the hemostatic and proliferative phases of wound healing,consequently accelerating the ***,thepromising results of Co_(3)O_(4)NFs highlight their potential in promoting wound healing and tissue regeneration.

关键词： Co_(3)O_(4) nanoflake nanozyxygen species wound healing

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Furan-derived Schiff base covalent adaptable thermosets with recyclability and anti-flammability

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Green Chemical Engineering 2024年第3期5卷 364-373页

作者： Ping Zhang Shuyu Jia Ruishi Xie Lin Chen Ying Xiong State Key Laboratory of Environment-friendly Energy Materials School of Materials Science and EngineeringSouthwest University of Science and TechnologyMianyang621010China

Conventional thermosetting polymers,mostly derived from nonrenewable petroleum resources,are not reprocessable and recyclable due to their highly cross-linked three-dimensional networks and face the disadvantage of high *** solve these issues,in this study,we synthesized a novel Schiff base covalent adaptable thermoset from a furan-derived tri-aldehyde monomer(TMFP)and a furan-derived di-amine monomer(DFDA).The as-prepared TMFP-DFDA-Vitrimer exhibited superior anti-flammability with a high limiting oxygen index(LOI)of 35.0%and a UL-94 V-0 rating,which was attributed to the excellent charring ***,TMFPDFDA-Vitrimer could also be conveniently recycled by chemical decomposition under a mixed hydrochloric acid/tetrahydrofuran(HCl/THF)*** recycling for 5 times,the thermal,mechanical,and flame retardant properties of the recycled TMFP-DFDA-Vitrimer retained almost unchanged compared to the original *** work provides a prime instance to develop advanced thermosetting polymers from abundant furan-based compounds.

关键词： Furan-based compounds Vitrimer Recyclability Flame retardancy

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A low-cost and high-strength basalt/carbon fiber reinforced polymer improved by imitating tree-root micro/nano aramid short fiber

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Chinese Journal of Aeronautics 2024年第10期37卷 526-538页

作者： Guangming YANG Yanan LYU Fei CHENG Jiaxin HE Shihao ZUO Wenyi HUANG Yunsen HU Xiaozhi HU Xi CHEN Shock and Vibration of Engineering Materials and Structures Key Lab of Sichuan Province Southwest University of Science and TechnologyMianyang 621010China Engineering Research Center of Biomass Materials Ministry of EducationSouthwest University of Science and TechnologyMianyang 621010China school of Materials and Chemistry Southwest University of Science and TechnologyMianyang 621010China Institute of Automation Chinese Academy of SciencesBeijing 100190China school of Artificial Intelligence University of Chinese Academy of SciencesBeijing 100101China school of Mechanical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China Department of Mechanical Engineering University of Western AustraliaPerth 6009Australia

The high-strength Basalt Carbon Fiber Reinforced Polymer(BCFRP)composites had been manufactured by guiding Imitating Tree-root Micro/Nano Aramid Short Fiber(ITMNASF)into the interlayer of Basalt Fiber(BF)and Carbon Fiber(CF)plies to form thin interleaving,and various mass proportions of IT-MNASF were designed to discuss the reinforcing effect on the BCFRP heterogeneous *** results of three points bending tests showed that flexural strength and energy absorption of 4wt%IT-MNASF reinforced BCFRP heterogeneous composites had been improved by 32.4%and 134.4%respectively compared with that of unreinforced *** 4wt%IT-MNASF reinforced BCFRP specimens showed both a greater strength and a lower cost(reduced by 31%around)than that of plain CFRP composites.X-ray micro-computed tomography scanning results exhibited that the delamination-dominated failure of plain BCFRP composites was changed into multi-layer BF and CF fabrics *** reinforcing mechanism revealed that the introduced IT-MNASF could construct quasi-vertical fiber bridging,and it was used as"mechanical claws"to grasp adjacent fiber layers for creating a stronger mechanical interlocking,and this effectively improved resin-rich region and interfacial transition region at the *** simple and effective IT-MNASF interleaving technique was very successful in low-cost and high-strength development of BCFRP heterogeneous composites.

关键词： Basalt carbon fiber reinforced polymer Micro/nano aramid fiber Fiber bridging Strength improvement Low-cost substitution

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Structure,electronic,and nonlinear optical properties of superalkaline M_(3)O(M=Li,Na)doped cyclo[18]carbon

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Chinese Physics B 2024年第2期33卷 311-317页

作者：刘晓东卢其亮罗其全 school of Physics and Material science Anhui UniversityHefei 230601China Institute of physical science and Information technology Anhui UniversityHefei 230601China Department of Chemical Physics University of Science and Technology of ChinaHefei 230026China

Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic *** have low ionization *** a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer *** this paper,the geometry,bonding properties,electronic structure,absorption spectrum,and nonlinear optical(NLO)properties of superalkaline M_(3)O(M=Li,Na)-doped cyclo[18]carbon were studied by using density functional theory.M_(3)O and the C_(18) rings are not *** C_(18) ring still exhibits alternating long and short *** charge transfer between M_(3)O and C_(18) forms stable[M_(3)O]+[C_(18)]-ionic complexes.C_(18)M_(3)O(M=Li,Na)shows striking optical nonlinearity,i.e.,their first-and second-order hyperpolarizability(βvec andγ||)increase considerably atλ=1907 nm and 1460 nm.

关键词： superalkaline doped cyclocarbon structure and electronic properties nonlinear optical properties density functional theory(DFT)

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Microfluidic preparation of surfactant-free ultrafine DAAF with tunable particle size for insensitive initiator explosives

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Defence technology（防务技术） 2024年第9期39卷 42-52页

作者： Bo Yang Rui Li Wei Cao Si-min He Jincan Zhu Qi Wu Heng Ding Jin Chen Weimiao Wang Zhiqiang Qiao Xiaodong Li Guangcheng Yang Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900China southwest university of science and technology Mianyang 621010China school of Chemical Engineering Nanjing University of Science and TechnologyNanjing 210094China

High purity and ultrafine DAAF(u-DAAF)is an emerging insensitive charge in *** there are many ways to obtain u-DAAF,developing a preparation method with stable operation,accurate control,good quality consistency,equipment miniaturization,and minimum manpower is an inevitable requirement to adapt to the current social technology development *** reported is the microfluidic preparation of u-DAAF with tunable particle size by a passive swirling *** the guidance of recrystallization growth kinetics and mixing behavior of fluids in the swirling microreactor,the key parameters(liquid flow rate,explosive concentration and crystallization temperature)were screened and optimized through screening *** the condition that no surfactant is added and only experimental parameters are controlled,the particle size of recrystallized DAAF can be adjusted from 98 nm to 785 nm,and the corresponding specific surface area is 8.45 m^(2)·g^(-1)to 1.33 m^(2)·g^(-1).In addition,the preparation method has good batch stability,high yield(90.8%-92.6%)and high purity(99.0%-99.4%),indicating a high practical application *** explosion derived flyer initiation tests demonstrate that the u-DAAF shows an initiation sensitivity much lower than that of the raw DAAF,and comparable to that of the refined DAAF by conventional spraying crystallization *** study provides an efficient method to fabricate u-DAAF with narrow particle size distribution and high reproducibility as well as a theoretical reference for fabrication of other ultrafine explosives.

关键词： Microfluidic preparation Screening crystallization conditions Narrow particle size distribution Low initiation sensitivity Ultrafine DAAF

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The B-site ordering in RFe_(0.5)Cr_(0.5)O_(3)ceramics and its effect on magnetic properties

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Chinese Physics B 2024年第10期33卷 434-441页

作者： Li Hou Lei Shi Liping Yang Yiqiang Liu Zhitao Li Lanxiang Meng school of Materials science and Engineering Anyang Institute of TechnologyAnyang 455000China Hefei National Laboratory for physical sciences at Microscale University of Science and Technology of ChinaHefei 230026China

To insight into the B-site ordering in RFe_(0.5)Cr_(0.5)O_(3)ceramics,a series of RFe_(0.5)Cr_(0.5)O_(3)ceramics(R=La,Y,Lu)were synthesized by the sol-gel method,and the structural and magnetic properties were systemically *** using the Rietveld refinement of all samples,it is found that the structural distortion is increased as the R ionic radius decreases,leading to the weakened interactions between Fe/Cr ***,the Fe and Cr are arranged in disorder in LaFe_(0.5)Cr_(0.5)O_(3),but partially ordered in YFe_(0.5)Cr_(0.5)O_(3)and LuFe_(0.5)Cr_(0.5)O_(3),showing an increasing trend of the proportion of ordered domains with the decrease of R ionic *** fitting the temperature-dependent magnetizations,it is identified that the magnetization reversal(MR)in disorder LaFe_(0.5)Cr_(0.5)O_(3)is resulted from the competition between the moments of Cr and Fe *** the partially ordered YFe_(0.5)Cr_(0.5)O_(3)and LuFe_(0.5)Cr_(0.5)O_(3)ceramics,because of the presence of Fe-O-Cr networks in the ordered domains whose moment is antiparallel to that of Fe-O-Fe and Cr-O-Cr in the disordered domains,the compensation temperature T_(comp)of MR is increased by nearly 50 *** results suggest that the changing of R-site ions could be used very effectively to modify the Fe-O-Cr ordering,apart from the structural distortion,which has a direct effect on the magnetic exchange interactions in RFe_(0.5)Cr_(0.5)O_(3)*** at values of composition where ordered domains are expected to be larger in number as compared to disordered domains and with a weaker structural distortion,one can expect a higher transition temperature Tcomp,providing a different view for adjustment of the magnetic properties of RFe_(0.5)Cr_(0.5)O_(3)ceramics for practical applications.

关键词： RFe_(0.5)Cr_(0.5)O_(3)ceramics structural distortion B-site ordering magnetization reversal

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Investigation on the roles of equilibrium toroidal rotation during edge-localized mode mitigated by resonant magnetic perturbations

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Plasma science and technology 2024年第1期26卷 16-33页

作者：董良康陈少永牟茂淋罗杨秦晨晨唐昌建 College of Physics Sichuan UniversityChengdu 610064People’s Republic of China Key Laboratory of High Energy Density Physics and technology of Ministry of Education Sichuan UniversityChengdu 610064People’s Republic of China Institute of Fusion science School of Physical Science and TechnologySouthwest Jiaotong UniversityChengdu 610031People’s Republic of China

The effects of equilibrium toroidal rotation during edge-localized mode(ELM)mitigated by resonant magnetic perturbation(RMP)are studied with the experimental equilibria of the EAST tokamak based on the four-field model in the BOUT++*** the two main parameters to determine the toroidal rotation profiles,the rotation shear and magnitudes were separately scanned to investigate their roles in the impact of RMPs on peeling-ballooning(P-B)*** one hand,the results show that strong toroidal rotation shear is favorable for the enhancement of the self-generated E×B shearing ratewith RMPs,leading to significant ELM mitigation with RMP in the stronger toroidal rotation shear *** the other hand,toroidal rotation magnitudes may affect ELM mitigation by changing the penetration of the RMPs,more precisely the resonant *** can lead to a reduction in the pedestal energy loss by enhancing the multimode coupling in the turbulence transport *** shielding effects on RMPs increase with the toroidal rotation magnitude,leading to the enhancement of the multimode coupling with RMPs to be significantly ***,the reduction in pedestal energy loss by RMPs decreased with the rotation *** brief,the results show that toroidal rotation plays a dual role in ELM mitigation with RMP by changing the shielding effects of plasma by rotation magnitude and affectingby rotation *** the high toroidal rotation region,toroidal rotation shear is usually strong and hence plays a dominant role in the influence of RMP on P-B modes,whereas in the low rotation region,toroidal rotation shear is weak and has negligible impact on P-B modes,and the rotation magnitude plays a dominant role in the influence of RMPs on the P-B modes by changing the field ***,the dual role of toroidal rotation leads to stronger ELM mitigation with RMP,which may be achieved both in the low toroidal rotation region and the relatively high rotation regi

关键词： edge-localized mode peeling–ballooning modes resonant magnetic perturbation toroidal rotation plasma response tokamak

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Heterogeneous Task Allocation Model and Algorithm for Intelligent Connected Vehicles

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Computers, Materials & Continua 2024年第9期80卷 4281-4302页

作者： Neng Wan Guangping Zeng Xianwei Zhou school of Computer and Communication Engineering University of Science and Technology BeijingBeijing100083China school of Mechanical and Transportation Southwest Forestry UniversityKunming650224China

With the development of vehicles towards intelligence and connectivity,vehicular data is diversifying and growing dramatically.A task allocation model and algorithm for heterogeneous Intelligent Connected Vehicle(ICV)applications are proposed for the dispersed computing network composed of heterogeneous task vehicles and Network Computing Points(NCPs).Considering the amount of task data and the idle resources of NCPs,a computing resource scheduling model for NCPs is *** the heterogeneous task execution delay threshold as a constraint,the optimization problem is described as the problem of maximizing the utilization of computing resources by *** proposed problem is proven to be NP-hard by using the method of reduction to a 0-1 knapsack problem.A many-to-many matching algorithm based on resource preferences is *** algorithm first establishes the mutual preference lists based on the adaptability of the task requirements and the resources provided by *** enables the filtering out of un-schedulable NCPs in the initial stage of matching,reducing the solution space *** solve the matching problem between ICVs and NCPs,a new manyto-many matching algorithm is proposed to obtain a unique and stable optimal matching *** simulation results demonstrate that the proposed scheme can improve the resource utilization of NCPs by an average of 9.6%compared to the reference scheme,and the total performance can be improved by up to 15.9%.

关键词： Task allocation intelligent connected vehicles dispersed computing matching algorithm

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