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Liquid metal as an efficient protective layer for lithium metal anodes in all-solid-state batteries

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Carbon Energy 2024年第7期6卷 219-229页

作者： Shiqiang Zhou Mengrui Li Peike Wang Lukuan Cheng Lina Chen Yan Huang Boxuan Cao Suzhu Yu Qingju Liu Jun Wei Shenzhen Key Laboratory of Flexible Printed Electronics technology Harbin Institute of TechnologyShenzhenChina school of Materials science and Engineering Harbin Institute of TechnologyShenzhenChina State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbinChina Yunnan Key Laboratory for Micro/nano Materials and technology School of Materials and EnergyYunnan UniversityKunmingChina

Lithium metal batteries with inorganic solid-state electrolytes have emerged as strong and attractive candidates for electrochemical energy storage devices because of their high-energy content and ***,inherent challenges of deleterious lithium dendrite growth and poor interfacial stability hinder their commercial ***,we report a liquid metal-coated lithium metal(LM@Li)anode strategy to improve the contact between lithium metal and a Li6PS5Cl inorganic *** LM@Li symmetric cell shows over 1000 h of stable lithium plating/stripping cycles at 2mA cm^(-2) and a significantly higher critical current density of 9.8 mAcm^(-2) at 25°*** addition,a full battery assembled with a high-capacity composite LiNbO3@-LiNi_(0.7)Co_(0.2)Mn_(0.1)O_(2)(LNO@NCM721)cathode shows stable cycling *** and computational results have demonstrated that dendrite growth tolerance and physical contact in solid-state batteries can be reinforced by using LM interlayers for interfacial modification.

关键词： all-solid-state batteries interface engineering liquid metals lithium metal anodes

Mitigation of Optical Multipath Interference Algorithms in IM-DD Transmission System

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China Communications 2024年第4期21卷 1-9页

作者： Huo Jiahao Zhu Jin Zhu Zuqing Zhang Xiaoying Liu Shaonan Tao Jianlong Wei Huangfu school of Computer and Communication Engineering University of Science and Technology BeijingBeijing 100083China school of Information science and technology University of Science and Technology of ChinaHefei 230026China

This paper aimed to propose two algorithms,DA-M and RF-M,of reducing the impact of multipath interference(MPI)on intensity modulation direct detection(IM-DD)systems,particularly for four-level pulse amplitude modulation(PAM4)***-M reduced the fluctuation by averaging the signal in blocks,RF-M estimated MPI by subtracting the decision value of the corresponding block from the mean value of a signal block,and then generated interference-reduced samples by subtracting the interference signal from the product of the corresponding MPI estimate and then weighting *** paper firstly proposed to separate the signal before decision-making into multiple blocks,which significantly reduced the complexity of DA-M and *** results showed that the MPI noise of 28 GBaud IMDD system under the linewidths of 1e5 Hz,1e6 Hz and 10e6 Hz can be effectively alleviated.

关键词： IM-DD multipath interference PAM4

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Step-edge-guided nucleation and growth mode transition of α-Ga_(2)O_(3) heteroepitaxy on vicinal sapphire

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Chinese Physics B 2024年第8期33卷 397-403页

作者：郝景刚张彦芳张贻俊徐科韩根全叶建东 Test&Analysis Platform Suzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China school of Electronic science and Engineering Nanjing UniversityNanjing 210023China Wuxi Institute of technology Wuxi 214121China school of Microelectronics Xidian UniversityXi'an 710071China Suzhou National Laboratory for Materials science Jiangsu Institute of Advanced SemiconductorsSuzhou 215123China

Controlling the epitaxial growth mode of semiconductor layers is crucial for optimizing material properties and device *** this work,the growth mode ofα-Ga_(2)O_(3) heteroepitaxial layers was modulated by tuning miscut angles(θ)from 0°to 7°off the(1010)direction of sapphire(0002)*** flat sapphire surfaces,the growth undergoes a typical three-dimensional(3D)growth mode due to the random nucleation on wide substrate terraces,as evidenced by the hillock morphology and high dislocation *** the miscut angle increases toθ=5°,the terrace width of sapphire substrate is comparable to the distance between neighboring nuclei,and consequently,the nucleation is guided by terrace edges,which energetically facilitates the growth mode transition into the desirable two-dimensional(2D)coherent ***,the mean surface roughness decreases to only 0.62 nm,accompanied by a significant reduction in screw and edge dislocations to 0.16×10^(7) cm^(-2)and 3.58×10^(9) cm^(-2),***,the further increment of miscut angles toθ=7°shrink the terrace width less than nucleation distance,and the step-bunching growth mode is *** this circumstance,the misfit strain is released in the initial growth stage,resulting in surface morphology degradation and increased dislocation densities.

关键词： growth mode miscut angle crystalline quality surface morphology

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Sulfur vacancies and heterogeneous interfaces promote high performance sodium storage of bimetallic chalcogenide hollow nanospheres

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Journal of Energy Chemistry 2024年第8期95卷 596-610,I0013页

作者： Shiyue Cao Xiaoting Xu Qiming Liu Huijuan Zhu Ting Hu Key Laboratory of Artificial Micro-and nano-structures of Ministry of Education School of Physics and TechnologyWuhan UniversityWuhan 430072HubeiChina

Transition metal sulfides have high theoretical capacities and are considered as potential anode materials for sodium-ion ***,due to low inherent conductivity and significant volume expansion,the electrochemical performance is greatly *** this study,a nickel/manganese sulfide material(Ni_(0.96)S_(x)/MnS_(y)-NC)with adjustable sulfur vacancies and heterogeneous hollow spheres was prepared using a simple *** introduction of a concentration-adjustable sulfur vacancy enables the generation of a heterogeneous interface between bimetallic sulfide and sulfur *** interface collectively creates an internal electric field,improving the mobility of electrons and ions,increasing the number of electrochemically active sites,and further optimizing the performance of Na~+*** direction of electron flow is confirmed by Density functional theory(DFT)*** hollow nano-spherical material provides a buffer for expansion,facilitating rapid transfer *** innovative discovery involves the interaction between the ether-based electrolyte and copper foil,leading to the formation of Cu_9S_5,which grafts the active material and copper current collector,reinforcing mechanical *** results in a new heterostructure of Cu_9S_5 with Ni_(0.96)S_(x)/MnS_(y),contributing to the stabilization of structural integrity for long-cycle ***,Ni_(0.96)S_(x)/MnS_(y)-NC exhibits excellent electrochemical properties following our modification *** stability performance,Ni0_(.96)S_(x)/MnS_(y)-NC demonstrates an average decay rate of 0.00944%after 10,000 cycles at an extremely high current density of 10000 mA g^(-1),A full cell with a high capacity of 304.2 mA h g^(-1)was also successfully assembled by using Na_(3)V_(2)(PO_(4))_(3)/C as the *** study explores a novel strategy for interface/vacancy co-modification in the fabrication of high-performance sodium-ion batteries electrode.

关键词： Sulfur vacancies Heterogeneous interface Interactions Sodium ion batteries

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Adaptive neural network control of a 2-DOF helicopter system considering input constraints and global prescribed performance

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science China(Information sciences) 2024年第7期67卷 224-239页

作者： Zhijia ZHAO Jiale WU Zhijie LIU We HE C.L.Philip CHEN school of Mechanical and Electrical Engineering Guangzhou University school of Intelligence science and technology and Key Laboratory of Intelligent Bionic Unmanned Systems of Ministry of Education University of Science and Technology Beijing school of Computer science and Engineering South China University of Technology Pazhou Lab

In this study, an adaptive neural network(NN) control is proposed for nonlinear two-degree-offreedom(2-DOF) helicopter systems considering the input constraints and global prescribed ***, radial basis function NN(RBFNN) is employed to estimate the unknown dynamics of the helicopter system. Second, a smooth nonaffine function is exploited to approximate and address nonlinear constraint functions. Subsequently, a new prescribed function is proposed, and an original constrained error is transformed into an equivalent unconstrained error using the error transformation and barrier function transformation methods. The analysis of the established Lyapunov function proves that the controlled system is globally uniformly bounded. Finally, the simulation and experimental results on a constructed Quanser's test platform verify the rationality and feasibility of the proposed control.

关键词： adaptive NN control 2-DOF helicopter global prescribed performance input constraints

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Journal of Computer science & technology 2024年第1期39卷 63-81页

作者：陈章玉华宇左鹏飞孙园园郭云程 Wuhan National Laboratory for Optoelectronics School of Computer Science and TechnologyHuazhong University of Science and TechnologyWuhan 430074China

Image bitmaps,i.e.,data containing pixels and visual perception,have been widely used in emerging applica-tions for pixel operations while consuming lots of memory space and *** with legacy DRAM(dynamic ran-dom access memory),non-volatile memories(NVMs)are suitable for bitmap storage due to the salient features of high density and intrinsic ***,writing NVMs suffers from higher energy consumption and latency compared with read *** precise or approximate compression schemes in NVM controllers show limited performance for bitmaps due to the irregular data patterns and variance in *** observe the pixel-level similarity when writing bitmaps due to the analogous contents in adjacent *** exploiting the pixel-level similarity,we propose SimCom,an approximate similarity-aware compression scheme in the NVM module controller,to efficiently compress data for each write access *** idea behind SimCom is to compress continuous similar words into the pairs of base words with *** storage costs for small runs are further mitigated by reusing the least significant bits of base *** adaptively selects an appropriate compression mode for various bitmap formats,thus achieving an efficient trade-off be-tween quality and memory *** implement SimCom on GEM5/zsim with NVMain and evaluate the perfor-mance with real-world image/video *** results demonstrate the efficacy and efficiency of our SimCom with an efficient quality-performance trade-off.

关键词： approximate computing data compression memory architecture non-volatile memory

Highly Sensitive Ammonia Gas Sensors at Room Temperature Based on the Catalytic Mechanism of N,C Coordinated Ni Single-Atom Active Center

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nano-Micro Letters 2024年第12期16卷 515-531页

作者： Wenjing Quan Jia Shi Min Zeng Wen Lv Xiyu Chen Chao Fan Yongwei Zhang Zhou Liu Xiaolu Huang Jianhua Yang Nantao Hu Tao Wang Zhi Yang National Key Laboratory of Advanced Micro and nano Manufacture technology Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Department of Micro/nano Electronics School of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Shanghai Key Laboratory of Intelligent Sensing and Detection technology School of Mechanical and Power EngineeringEast China University of Science and TechnologyShanghai 200237People’s Republic of China

Significant challenges are posed by the limitations of gas sensing mechanisms for trace-level detection of ammonia(NH3).In this study,we propose to exploit single-atom catalytic activation and targeted adsorption properties to achieve highly sensitive and selective NH3 gas ***,Ni singleatom active sites based on N,C coordination(Ni-N-C)were interfacially confined on the surface of two-dimensional(2D)MXene nanosheets(Ni-N-C/Ti_(3)C_(2)Tx),and a fully flexible gas sensor(MNPE-Ni-N-C/Ti_(3)C_(2)Tx)was *** sensor demonstrates a remarkable response value to 5 ppm NH3(27.3%),excellent selectivity for NH3,and a low theoretical detection limit of 12.1 *** analysis by density functional calculation reveals that the Ni single-atom center with N,C coordination exhibits specific targeted adsorption properties for ***,its catalytic activation effect effectively reduces the Gibbs free energy of the sensing elemental reaction,while its electronic structure promotes the spill-over effect of reactive oxygen species at the gas-solid *** sensor has a dual-channel sensing mechanism of both chemical and electronic sensitization,which facilitates efficient electron transfer to the 2D MXene conductive network,resulting in the formation of the NH3 gas molecule sensing ***,the passivation of MXene edge defects by a conjugated hydrogen bond network enhances the long-term stability of MXene-based electrodes under high humidity *** work achieves highly sensitive room-temperature NH3 gas detection based on the catalytic mechanism of Ni single-atom active center with N,C coordination,which provides a novel gas sensing mechanism for room-temperature trace gas detection research.

关键词： Gas sensor Single atom Catalytic activation Targeted adsorption End-sealing passivation

Simultaneously enhancing erosion and compression resistance:designing AlCoCrFeNi high-entropy alloy strengthened Ag-based contacts

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Rare Metals 2024年第9期43卷 4476-4492页

作者： Xiao-Yang Xue Zhe Wang Hui-Ling Nie Zhao Yuan Jun Wang Chang-Hu Xu Kai Wen Cong-Hao Yu school of Materials science and Engineering Xi’an Polytechnic University school of Physics Xi’an Jiaotong University Key Laboratory of Pulsed Power technology School of Electrical and Electronic EngineeringHuazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and technology School of Electrical and Electronic EngineeringHuazhong University of Science and Technology

Designing microstructures and unveiling dynamic erosion mechanisms remain important challenges for Ag-based contacts. To simultaneously enhance erosion and compression resistance, an Al Co Cr Fe Ni high-entropy alloy(HEA) is introduced into Ag-based materials to fabricate novel Ag-HEA contacts with island-and skeletonrestricted microstructures. The arc erosion experimental results reveal that the skeleton-restricted HEA microstructure is the key factor in reducing the hill and crater morphologies of the contact surface, effectively delaying material transfer between the movable and stationary contacts. The molten bridge evolution and compressive deformation behavior of Ag-HEA contacts with various microstructures are investigated using molecular dynamics(MD) simulations. MD results indicate that the constraint of Ag atom diffusion in the molten pool and the involvement of HEA atoms in the molten bridge are the primary mechanisms for improving erosion resistance. The skeleton-restricted HEA microstructure reduces the total energy and structural stability of the molten bridge system and promotes its fracture and disintegration. Moreover, the synergistic effect of the twin and Lomerz–Cottrell lock structures can hinder dislocation glide, generating dispersed and small-area stacking faults in the Ag matrix and mitigating the concentration of shear strains. Thus, the skeleton-restricted HEA microstructure contributes positively to compression resistance. This study presents a novel approach to designing Ag-based contacts.

关键词： Arc erosion Electrical contact materials High entropy alloys Microstructures Molecular dynamics

Accumulated-state-error-based event-triggered sampling scheme and its application to H∞ control of sampled-data systems

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science China(Information sciences) 2024年第6期67卷 328-341页

作者： Xian-Ming ZHANG Qing-Long HAN Bao-Lin ZHANG Xiaohua GE Dawei ZHANG school of science Computingand Engineering TechnologiesSwinburne University of Technology College of Automation and Electronic Engineering Qingdao University of Science & Technology school of Mathematics Shandong University

This paper is concerned with event-triggered H∞control of sampled-data systems. Its novelties lie in three aspects:（i） A novel accumulated-state-error-based event-triggered scheme is introduced by comparing the integral of the state error from tk to t with the system state sampled at tk. This condition works well due to the fact that the so-called Zeno behaviour does not occur.（ii） A novel Lyapunov functional is constructed to establish a criterion to ensure some certain H∞performance of the closed-loop system. This Lyapunov functional is dependent on the integral of the state error involved in the event-triggered scheme.（iii） Under the event-triggered sampling scheme, suitable state-feedback controllers can be designed rather than be given a priori. Moreover, a self-triggered implementation of the proposed event-triggered sampling scheme is presented as well. Finally, a batch reactor model and an inverted pendulum system are given to demonstrate the effectiveness of the proposed method.

关键词： event-triggered sampling self-triggered implementation $H_\infty$ control looped-functional