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Journal of Environmental Sciences 2024年第4期138卷 428-438页

作者： Jing Yang Yujie Ren Shuoyu Chen Jinsuo Lu school of Environmental and municipal engineering Xi’an University of Architecture and TechnologyXi’an 710055China

This study aimed to explore the chemical looping gasification(CLG)reaction characteristics of the metal-supported composite phosphogypsum(PG)oxygen carriers(OCs)and the thermodynamic *** FactSage 7.1 thermodynamic simulation was used to explore the oxygen release and H_(2)S removal *** experimental results showed that the syngas yield of CLG with PG-CuFe_(2)O_(4)was more than that with PG-Fe_(2)O_(3)20/CuO40 or PG-Fe_(2)O_(3)30/CuO30 OC at 1023 K when the water vapor content was ***,the maximum syngas yield of the CO selectivity was 70.3% and of the CO_(2)selectivity was 23.8%.The H_(2)/CO value was 0.78,and the highest carbon conversion efficiency was 91.9% in PG-CuFe_(2)O_(4)at the gasification temperature of 1073 *** metal-supported PG composite oxygen carrier was proved not only as an oxygen carrier to participate in the preparation of syngas but also as a catalyst to catalyze coal gasification ***,both the experimental results and FactSage 7.1 thermodynamic analysis revealed that the trapping mechanism of H_(2)S by composite OCs was as follows:CuO first lost lattice oxygen as an oxygen carrier to generate Cu_(2)O,which,in turn,reacted with H_(2)S to generate Cu_(2)*** study provided efficient guidance and reference for OC design in CLG.

关键词： Metal-supported composite phosphogypsum Reaction characteristics Thermodynamic mechanism Chemical looping gasification

Resource utilization of drinking water treatment aluminum sludge in green cementing materials: Hydration characteristics and hydration kinetics

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Journal of Environmental Sciences 2024年第10期144卷 236-248页

作者： Jing Yang Cheng Chen Shuoyu Chen Yujie Ren Jinsuo Lu school of Environmental and municipal engineering Xi’an University of Architecture and TechnologyXi’an 710055China

As a byproduct of water treatment,drinking water treatment aluminum sludge(DWTAS)has challenges related to imperfect treatment and disposal,which has caused potential harm to human health and the *** this paper,heat treatment DWTAS as a supplement cementitious material was used to prepare a green cementing *** results show that the 800℃ is considered as the optimum heat treatment temperature for ***-800℃ is fully activated after thermal decomposition to form incompletely crystallized highly activeγ-Al2O3 and active SiO_(2).The addition of DWTAS promoted the formation of ettringite and C-(A)-S-H gel,which could make up for the low early compressive strength of cementing materials to a certain *** cured for 90 days,the compressive strength of the mortar with 30% DWTAS-800℃ reached 44.86 *** dynamic process was well simulated by Krstulovi′c-Dabi′c hydration kinetics *** study provided a methodology for the fabrication of environmentally friendly and cost-effective compound cementitiousmaterials and proposed a“waste-to-resource”strategy for the sustainable management of typical solid wastes.

关键词： Drinking water treatment aluminum sludge Green cementing material Hydration characteristics Hydration kinetics

The mathematical model of kitchen smoke exhaust system in high-rise residential buildings considering the Influence of Stack effect

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Energy and Built Environment 2024年第4期5卷 580-591页

作者： Kailiang Huang Minghui Yu Xin Liu Runsheng Wang school of municipal and Environment engineering Shenyang Jianzhu UniversityShenyang100168China

In high-rise buildings with large indoor and outdoor temperature difference,neglecting the effect of stack effect in smoke exhaust shafts may cause calculation error of the fluid network *** this paper,the mathematical model of kitchen smoke exhaust system considering the influence of stack effect was put forward and it can be inserted different range hood *** with the results of six working conditions of the model without considering the stack effect,the error of the proposed model were reduced by 7.6%,4.3%,4.1%,2.8%,2.4%,and 2.1%.While the indoor and outdoor temperature difference varies from−5℃ to 49℃,the effect of stack effect on the pressure in the flue and the flow rate for each user was studied for six operating rates *** results show that under the combined effect of stack effect and flue resistance,the static pressure of the kitchen smoke exhaust system showed a low-high-low distribution,and the maximum static pressure in the flue moved toward the bottom with the increase of temperature *** flow rates exhibit a low-high-low-high distribution,with an increased flow rate in the bottom users and the largest flow rate in the top users.

关键词： High-rise residential buildings Kitchen ventilation Central exhaust system Buoyancy-driven ventilation Ventilation mathematical model

Resistance-capacitance model of the capillary heat exchanger in subway tunnels

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Energy and Built Environment 2024年第1期5卷 1-8页

作者： Zhen Tong Hao Wu Yiming Guan Yongming Ji Songtao Hu school of Environmental and municipal engineering Qingdao University of TechnologyQingdao 266033China

The subway operation generates a large amount of waste heat,which will lead to a disruption of the underground thermal *** remove the heat,a ground source heat pump system adopting capillary net as the front-end heat exchanger can be built in the tunnels to recycle the waste heat and use it for building *** simulation method was used to analyze the heat transfer process in the tunnel and the surrounding *** existing simulation method usually takes a long time for calculation and can not be used for a real-time regulation of the *** on the concept of thermoelectric analogy,a resistance-capacitance(RC)model was proposed for rapid prediction and analysis on the heat transfer of the capillary net in subway *** annual thermal response in the tunnel was analyzed,and the influence of the tunnel air temperature and the capillary inlet water temperature was examined using this *** maximum heat transfer flux of the capillary in summer(release heat)and in winter(extract heat)was 55.27 W/m 2 and 38.33 W/m 2,*** effect of capillary inlet water temperature was more remarkable than that of the tunnel air temperature on the capillary heat exchange process.

关键词： Subway tunnel Heat pump Capillary heat exchanger Resistance-capacitance model

The optimization research on the coupled of active and passive energy supplying in public institutions in China

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Energy and Built Environment 2024年第2期5卷 288-299页

作者： Shui Yu Xueyan Liu Jianghui Yang Fuhong Han Jiashuai Wei school of municipal and Environmental engineering Shenyang Jianzhu UniversityShenyang 110168China

The building sector is one of the largest energy user and carbon emitters *** increase the utilization rate of renewable energy and reduce carbon dioxide emissions,the optimal technical scheme of active public institutions and coupled utilization of renewable energy is *** this study,the energy consumption of three types of public institutions in various regions of China was simulated by using DeST building energy consumption software,combined with energy conversion efficiency and data released by the National Bureau of Statistics,and the total energy demand and total energy supply of public institutions were predicted using the load density *** on the coupling mechanism of the MARKAL model,the optimal proportion of renewable energy in the energy supply of public buildings in different regions is *** the study of the number of public institutions in various regions of China,energy consumption characteristics,construction area,and other related data,the reverse energy flow method is creatively proposed,and the active and renewable energy coupling algorithm from the energy demand side of public institutions to the energy supply side is *** results show that the central region has the highest utilization rate of renewable energy in the public sector,reaching 36.18%.The use of renewable energy in public buildings in hot summer and warm winter zones decreased to 35.08%,and it was 12.82% in cold *** 2025,the proportion of renewable energy resources in China is expected to reach 29.2%.The energy coupling model and algorithm constructed in this paper can provide a basis for the coupling macro configuration of renewable energy in public institutions in China.

关键词： Public institutions Energy demand Energy supply Active and renewable energy coupling ratio Energy conversion efficiency

Nonlinear constitutive models of rock structural plane and their applications

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Journal of Rock Mechanics and Geotechnical engineering 2024年第3期16卷 790-806页

作者： Wenlin Feng Shuangjian Niu Chunsheng Qiao Dujian Zou school of Civil and Environmental engineering Harbin Institute of TechnologyShenzhenChina Shenzhen municipal engineering Corporation Shenzhen518000China school of Civil engineering Beijing Jiaotong UniversityBeijing100044China

Structural planes play an important role in controlling the stability of rock engineering,and the influence of structural planes should be considered in the design and construction process of rock *** this paper,mechanical properties,constitutive theory,and numerical application of structural plane are studied by a combination method of laboratory tests,theoretical derivation,and program *** test results reveal the change laws of various mechanical parameters under different roughness and normal *** the pre-peak stage,a non-stationary model of shear stiffness is established,and threedimensional empirical prediction models for initial shear stiffness and residual stage roughness are *** nonlinear constitutive models are established based on elasto-plastic mechanics,and the algorithms of the models are developed based on the return mapping *** to a large number of statistical analysis results,empirical prediction models are proposed for model parameters expressed by structural plane characteristic ***,the discrete element method(DEM)is chosen to embed the constitutive models for practical *** running programs of the constitutive models have been compiled into the discrete element model *** comparison results between the proposed model and the Mohr-Coulomb slip model show that the proposed model can better describe nonlinear changes at different stages,and the predicted shear strength,peak strain and shear stiffness are closer to the test *** research results of the paper are conducive to the accurate evaluation of structural plane in rock engineering.

关键词： Structural plane engineering stability Roughness Normal stress Elasto-plastic constitutive model Discrete element method

Evaluation of Compatibilizers for Improving Compatibility between Waste Vegetable Oil and Aged Asphalt

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1278-1286页

作者： WANG Yanghui DING Yongjie LI Danli CAO Zhilong SUN Guoqiang MEI Zijun Department of Road and Urban Railway engineering Beijing University of TechnologyBeijing 100124China school of Civil engineering Chongqing Jiaotong UniversityChongqing 400074China Shanghai municipal engineering Design Instit Shanghai 230031China

Modifying agents 2,2-Bis(4-glycidyloxyphenyl)propane(2BPE)and dibutyl phthalate(DBP)were selected to enhance the *** using molecular simulation software(Materials Studio,MS),nine systems were constructed,including molecular models of aged asphalt and WVO monomers with 2BPE and/or *** solubility parameters,Flory-Huggins parameters,and interaction energies of these systems were calculated to determine the impact of 2BPE and DBP on the compatibility of WVO and aged *** showed that the addition of 2BPE and DBP reduced the difference in the solubility parameters between WVO and aged asphalt,thus improving the compatibility between WVO and aged ***,using a combination of 2BPE and DBP in both aged asphalt and rejuvenator was found to be more effective than using either 2BPE or DBP ***,it was determined that evaluating the compatibility of WVO and aged asphalt using Van der Waals potential and non-bonding energy as evaluation indicators was more accurate than using electrostatic potential energy.

关键词： road engineering aged asphalt compatibility molecular dynamics solubility parameter Flory-Huggins parameter

Preparation of crab-shell-based N,O co-doped graded porous carbon for supercapacitors using the confined nanospace deposition

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Waste Disposal and Sustainable Energy 2024年第2期6卷 173-183页

作者： Yiming Li Zhihao Yu Mengyan Guo Ming Zhang Jian Xiong Yina Qiao Rui Zhang Xuebin Lu school of Environmental Science and engineering Tianjin UniversityTianjin 30000China school of Ecology and Environment Tibet UniversityLhasa 850000China school of Environment and Safety engineering North University of ChinaTaiyuan 030051China school of Environmental and municipal engineering Tianjin Chengjian UniversityTianjin 300384China

Biomass-based carbon materials with hierarchical porous structures have attracted attention for their ability to provide more channels and shorten ion transport ***,we developed a simple method based on confined nanospace ***-ing high-temperature treatment,the mesoporous silica layer wrapped around the outside of the crab shells acted as a closed nanospace and effectively suppressed the severe deformation of the crab shell structure by shrinking *** prepared carbon material has a layered porous structure with abundant and stable N and O co-doping(N 7.32%,O 3.69%).The specific capacitance of the three-electrode system was 134.3 F/g at a current density of 0.5 A/g in a 6 mol/L KOH electrolyte,and the assembled aqueous symmetric supercapacitors exhibited an excellent cycling stability of 98.81%even after 5000 cycles.

关键词： Supercapacitor Confined nanospace deposition Biomass-based carbon materials Crab shell

Measurement and analysis of airtightness safeguard measures for typical ultra-low energy buildings

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Energy and Built Environment 2024年第3期5卷 348-363页

作者： Yongming Ji Lin Duanmu Songtao Hu school of Environmental and municipal engineering Qingdao University of TechnologyQingdaoShandong Province 266033China school of Civil engineering Dalian University of TechnologyDalianLiaoning Province 116024China

Zero-energy buildings constitute an effective means of reducing urban carbon *** airtightness,a typical characteristic of zero-energy building,is closely related to the building’s air infiltration and has a signifi-cant impact on the performance of the building envelope,indoor air quality,building energy consumption,and efficient operation of air-conditioning ***,thus far,systematic developments in high-airtightness assurance technologies remain *** existing studies have tested the airtightness of buildings and typical building components;however,in-depth analyses into the formation of infiltration have not been ***-fore,for realizing zero-energy buildings,ensuring airtightness is an urgent problem that needs to be ***,in this study,based on several building airtightness measurement studies,the typical air leakage paths in buildings were summarized,and the causes of typical air leakage components in buildings were further analysed by tracing construction ***,targeted measures for airtightness in buildings were estab-lished and applied to practical ***,the resulting improved building airtightness was measured and the results show that the airtightness of the measured ultra-low energy consumption buildings ranges from 0.13 h^(−1)to 0.57 h^(−1),with a mean value of 0.32 h^(−1).The effectiveness of the airtightness safeguard measures was *** study serves as a basis for the assumption of the air leakage path distribution when simulating building air infiltration and also provides a design reference for improving the construction technologies and airtightness of buildings.

关键词： Carbon neutrality Airtightness Safeguard measures Ultra-low energy buildings

Effects of operating conditions on iron(hydr)oxides evolution and ciprofloxacin degradation in potassium ferrate-ozone stepwise oxidation system

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Journal of Environmental Sciences 2024年第1期135卷 367-378页

作者： Xiaochen Li Yifan Wang Ning Wang Mei Li Maomao Bai Jingtao Xu Hongbo Wang school of municipal and Environmental engineering Shandong Jianzhu UniversityJinan 250101China Resources and Environment Innovation Institute Shandong Jianzhu UniversityJinan 250101China

In this study,a stepwise oxidation system of potassium ferrate(K_(2)FeO_(4))combined with ozone(O+3)was used to degrade ciprofloxacin(CIP).The effects of pH and pre-oxidation time of K_(2)FeO_(4) on the evolution of K_(2)FeO_(4) reduction products(iron(hydr)oxides)and CIP degradation were *** was found that in addition to its own oxidation capacity,K_(2)FeO_(4) can also influence the treatment effect of CIP by changing the catalyst *** presence of iron(hydr)oxides effectively enhanced the mineralization rate of CIP by catalyzing *** pH value can influence the content and types of the components with catalytic ozonation effect in iron(hydr)*** K_(2)FeO_(4) pre-oxidation stage can produce more iron(hydr)oxides with catalytic components for subsequent ozonation,but the evolution of iron(hydr)oxides components was influenced by O_(3) *** can also avoid the waste of oxidation capacity owing to the oxidation of iron(hydr)oxides by O_(3) and free *** intermediate degradation products were identified by Fourier transform ion cyclotron resonance mass spectrometry(FT-ICR-MS).Besides,the degradation pathways were *** the degradation products of CIP,the product with broken quinolone ring structure only appeared in the stepwise oxidation system.

关键词： Potassium ferrate reduction products Catalytic ozonation Ciprofloxacin Potassium ferrate pre-oxidation time