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The Mass Assembly History for Galaxies with MaNGA

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Research in Astronomy and Astrophysics 2024年第3期24卷 58-69页

作者： Xue Ge Hong-Tao Wang Cheng-Long Lei Yun-Jun Guo Yi-Long Jiang Xiao-Xiao Cao school of Physics and Information engineering Jiangsu Second Normal University jiangsu Province engineering Research Center of Basic Education Big Data Application Jiangsu Second Normal University Key Laboratory of Modern Astronomy and Astrophysics Nanjing UniversityMinistry of Education school of Science Langfang Normal University

How galaxies assemble masses through their own star formation or interaction with the external environment is still an important topic in the field of galaxy formation and *** use Value Added Catalogs with galaxy features that are spatially and temporally resolved from Sloan Digital Sky Survey Data Release 17 to investigate the mass growth histories of early-type galaxies(ETGs)and late-type galaxies(LTGs).We find that the mass growth of ETGs is earlier than that of LTGs for massive galaxies(M_(*)>10^(10)M_⊙),while low-mass(M_(*)≤10^(10)M_⊙)ETGs have statistically similar mass assembly histories as low-mass *** stellar metallicity of all massive galaxies shows a negative gradient and basically does not change with ***,in low-mass galaxies,the stellar metallicity gradient of elliptical galaxies is negative,and the stellar metallicity gradient of lenticular and spiral galaxies evolves from positive to *** are not all in a high-density environment,but exhibit mass *** the tidal strength increases,the star formation rate of low-mass ETGs rapidly *** results support a picture where massive galaxies exhibit inside-out quenching mode,while low-mass galaxies show outside-in quenching *** effects play an important role in regulating the mass assembly histories of low-mass ETGs.

关键词： Galaxy evolution-galaxies star formation-Galaxy formation

A Review on engineering Design for Enhancing Interfacial Contact in Solid-State Lithium–Sulfur Batteries

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Nano-Micro Letters 2024年第4期16卷 219-252页

作者： Bingxin Qi Xinyue Hong Ying Jiang Jing Shi Mingrui Zhang Wen Yan Chao Lai school of Chemistry and Materials Science Jiangsu Normal UniversityXuzhou 221116JiangsuPeople’s Republic of China

The utilization of solid-state electrolytes(SSEs)presents a promising solution to the issues of safety concern and shuttle effect in Li–S batteries,which has garnered significant interest ***,the high interfacial impedances existing between the SSEs and the electrodes(both lithium anodes and sulfur cathodes)hinder the charge transfer and intensify the uneven deposition of lithium,which ultimately result in insufficient capacity utilization and poor cycling ***,the reduction of interfacial resistance between SSEs and electrodes is of paramount importance in the pursuit of efficacious solid-state *** this review,we focus on the experimental strategies employed to enhance the interfacial contact between SSEs and electrodes,and summarize recent progresses of their applications in solidstate Li–S ***,the challenges and perspectives of rational interfacial design in practical solid-state Li–S batteries are outlined as *** expect that this review will provide new insights into the further technique development and practical applications of solid-state lithium batteries.

关键词： Solid-state lithium–sulfur batteries Solid-state electrolytes Electrode/electrolyte interface Interfacial engineering Enhancing interfacial contact

Thioacetamide Additive Homogenizing Zn Deposition Revealed by In Situ Digital Holography for Advanced Zn Ion Batteries

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Nano-Micro Letters 2024年第6期16卷 261-275页

作者： Kaixin Ren Min Li Qinghong Wang Baohua Liu Chuang Sun Boyu Yuan Chao Lai Lifang Jiao Chao Wang school of Chemistry and Materials Science Jiangsu Normal UniversityXuzhou 221116JiangsuPeople’s Republic of China jiangsu Key Laboratory of Advanced Laser Materials and Devices School ofPhysics and Electronic EngineeringJiangsu Normal UniversityXuzhou 221116JiangsuPeople’s Republic of China Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Nankai University300071 TianjinPeople’s Republic of China

Zinc ion batteries are considered as potential energy storage devices due to their advantages of low-cost,high-safety,and high theoretical ***,dendrite growth and chemical corrosion occurring on Zn anode limit their *** problems can be tackled through the optimization of the ***,the screening of electrolyte additives using normal electrochemical methods is time-consuming and ***,a fast and simple method based on the digital holography is *** can realize the in situ monitoring of electrode/electrolyte interface and provide direct information concerning ion concentration evolution of the diffusion *** is effective and time-saving in estimating the homogeneity of the deposition layer and predicting the tendency of dendrite growth,thus able to value the applicability of electrolyte *** feasibility of this method is further validated by the forecast and evaluation of thioacetamide *** on systematic characterization,it is proved that the introduction of thioacetamide can not only regulate the interficial ion flux to induce dendrite-free Zn deposition,but also construct adsorption molecule layers to inhibit side reactions of Zn *** easy to operate,capable of in situ observation,and able to endure harsh conditions,digital holography method will be a promising approach for the interfacial investigation of other battery systems.

关键词： Digital holographic microscopy In situ observation Electrode/electrolyte interface Zn dendrites Screening electrolyte additives

Enhancing action discrimination via category-specific frame clustering for weakly-supervised temporal action localization

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Frontiers of Information Technology & Electronic engineering 2024年第6期25卷 809-823页

作者： Huifen XIA Yongzhao ZHAN Honglin LIU Xiaopeng REN school of Computer Science and Communication engineering Jiangsu UniversityZhenjiang 212013China jiangsu engineering Research Center of Big Data Ubiquitous Perception and Intelligent Agricultural Applications Zhenjiang 212013China Changzhou Vocational Institute of mechatronic Technology Changzhou 213164China

Temporal action localization (TAL) is a task of detecting the start and end timestamps of action instances and classifying them in an untrimmed video. As the number of action categories per video increases, existing weakly-supervised TAL (W-TAL) methods with only video-level labels cannot provide sufficient supervision. Single-frame supervision has attracted the interest of researchers. Existing paradigms model single-frame annotations from the perspective of video snippet sequences, neglect action discrimination of annotated frames, and do not pay sufficient attention to their correlations in the same category. Considering a category, the annotated frames exhibit distinctive appearance characteristics or clear action ***, a novel method to enhance action discrimination via category-specific frame clustering for W-TAL is proposed. Specifically,the K-means clustering algorithm is employed to aggregate the annotated discriminative frames of the same category, which are regarded as exemplars to exhibit the characteristics of the action category. Then, the class activation scores are obtained by calculating the similarities between a frame and exemplars of various categories. Category-specific representation modeling can provide complimentary guidance to snippet sequence modeling in the mainline. As a result, a convex combination fusion mechanism is presented for annotated frames and snippet sequences to enhance the consistency properties of action discrimination,which can generate a robust class activation sequence for precise action classification and localization. Due to the supplementary guidance of action discriminative enhancement for video snippet sequences, our method outperforms existing single-frame annotation based methods. Experiments conducted on three datasets (THUMOS14, GTEA, and BEOID) show that our method achieves high localization performance compared with state-of-the-art methods.

关键词： Weakly supervised Temporal action localization Single-frame annotation Category-specific Action discrimination

Synthesis of carbon dots with predictable photoluminescence by the aid of machine learning

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Nano Research 2024年第3期17卷 1984-1989页

作者： Chenyu Xing Gaoyu Chen Xia Zhu Jiakun An Jianchun Bao Xuan Wang Xiuqing Zhou Xiuli Du Xiangxing Xu jiangsu Key Laboratory of Biofunctional Materials Jiangsu Key Laboratory of New Power BatteriesSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023China school of Mathematical Sciences Nanjing Normal UniversityNanjing 210023China State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210093China

Carbon dots(CDs)have wide application potentials in optoelectronic devices,biology,medicine,chemical sensors,and quantum techniques due to their excellent fluorescent ***,synthesis of CDs with controllable spectrum is challenging because of the diversity of the CD components and *** this report,machine learning(ML)algorithms were applied to help the synthesis of CDs with predictable photoluminescence(PL)under the excitation wavelengths of 365 and 532 *** combination of precursors was used as the *** PL peaks of the strongest intensity(λ_(s))and the longest wavelength(λ_(l))were used as target *** six investigated ML models,the random forest(RF)model showed outstanding)performance in the prediction of the PL peaks.

关键词： carbon dots(CDs) synthesis photoluminescence(PL) machine learning(ML) PL prediction

Catalytic asymmetric(3+3)cycloaddition between different 2-indolylmethanols

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Science China Chemistry 2024年第8期67卷 2629-2636页

作者： Tianzhen Li Sijia Liu Shufang Wu Qi Cheng Qun Chen Yinchun Jiao Yuchen Zhang Feng Shi school of Petrochemical engineering School of Materials ScienceEngineeringChangzhou UniversityChangzhou 213164China Research Center of Chiral Functional Heterocycles School of Chemistry and Materials ScienceJiangsu Normal UniversityXuzhou 221116China school of Chemistry and Chemical engineering Hunan University of Science and TechnologyXiangtan 411201China school of Chemistry and Chemical engineering Henan Normal UniversityXinxiang 453007China

The catalytic asymmetric(3+3)cycloaddition between different 2-indolylmethanols has been established,in which a series of chiral indole-fused six-membered heterocycles were constructed in high yields with excellent *** work not only has established the first catalytic asymmetric cycloaddition between different 2-indolylmethanols but also provided a powerful strategy for constructing enantioenriched indole-fused six-membered ***,biological evaluation discovered some products with promising antitumor ***,theoretical calculations performed on the reaction pathway and activation mode provide an in-depth understanding of this catalytic asymmetric(3+3)cycloaddition among different 2-indolylmethanols,which will advance the understanding of the chemistry of indolylmethanols.

关键词： asymmetric organocatalysis chiral phosphoric acid cycloaddition enantioselectivity 2-indolylmethanol

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Sustainable production of high-energy-density jet fuel via cycloaddition reactions

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Journal of Energy Chemistry 2024年第8期95卷 712-722,I0016页

作者： Yan-Cheng Hu Yingying Zhao Ning Li Jing-Pei Cao school of Chemical engineering and Technology China University of Mining and TechnologyXuzhou 221116JiangsuChina school of Education Science Jiangsu Normal UniversityXuzhou 221116JiangsuChina CAS Key Laboratory of Science and Technology on Applied Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023LiaoningChina

Developing an energy supply-chain based on renewable biomass holds great potential to build a low carbon ***-energy-density(HED)jet fuel,featuring unique fused/strained cycloalkanes,is of great significance for volume-limited military aircrafts,as their high density and combustion heat can extend flight duration and increase the ***,the exploration of biomass-based routes towards HED fuel has drawn much attention over the past *** reaction features rapid construction of various carbocycles in an atom-and step-economical *** elegant strategy has been widely applied in the manufacture of sustainable HED *** we carefully summarize the progress achieved in this fascinating area and the review is categorized by the cycloaddition patterns including[4+2],[2+2],[4+4],and[2+1]***,the energy densities of the as-prepared biofuels and petroleumbased fuels(conventional Jet-A and advanced JP-10)are also *** review will provide important insights into rational design of new HED fuel with different ring-types/sizes and inspire the chemists to turn those literature studies into practical applications in military field.

关键词： High-energy-density fuel Biomass-based chemicals Cycloaddition Cycloalkanes Catalysis

An improved lightweight network based on deep learning for grape recognition in unstructured environments

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Information Processing in Agriculture 2024年第2期11卷 202-216页

作者： Bingpiao Liu Yunzhi Zhang Jinhai Wang Lufeng Luo Qinghua Lu Huiling Wei Wenbo Zhu school of mechatronic engineering and Automation Foshan UniversityFoshan 528000China

In unstructured environments,dense grape fruit growth and the presence of occlusion cause difficult recognition problems,which will seriously affect the performance of grape picking *** address these problems,this study improves the YOLOx-Tiny model and proposes a new grape detection model,YOLOX-RA,which can quickly and accurately identify densely growing and occluded grape *** proposed YOLOX-RA model uses a 3×3 convolutional layer with a step size of 2 to replace the focal layer to reduce the computational *** CBS layer in the ResBlock_Body module of the second,third,and fourth layers of the backbone layer is removed,and the CSPLayer module is replaced by the ResBlock-M module to speed up the *** auxiliary network(AlNet)with the remaining network blocks was added after the ResBlock-M module to improve the detection *** depth-separable convolutions(DsC)are used in the neck module layer to replace the normal convolution to reduce the computational *** evaluated the detection performance of SSD,YOLOv4 SSD,YOLOv4-Tiny,YOLO-Grape,YOLOv5-X,YOLOX-Tiny,and YOLOX-RA on a grape test *** results show that the YOLOX-RA model has the best detection performance,achieving 88.75%mAP,a recognition speed of 84.88 FPS,and model size of 17.53 *** can accurately detect densely grown and shaded grape bunches,which can effectively improve the performance of the grape picking robot.

关键词： YOLOX Grape recognition Depthwise separable convolution Res Block-M AINet

Manipulating d-d orbital hybridization induced by Mo-doped Co_(9)S_(8) nanorod arrays for high-efficiency water electrolysis

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Journal of Energy Chemistry 2024年第6期93卷 592-600,I0015页

作者： Xue Zhou Jing Li Guangyao Zhou Weiran Huang Yucan Zhang Jun Yang Huan Pang Mingyi Zhang Dongmei Sun Yawen Tang Lin Xu jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Centre of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing 210023JiangsuChina 'College of Science Jinling Institute of TechnologyNanjing 211169JiangsuChina State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Nanjing IPE Institute of Green Manufacturing Industry Nanjing 211100JiangsuChina school of Chemistry and Chemical engineering Yangzhou UniversityYangzhou 225009JiangsuChina Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of EducationSchool of Physics and Electronic EngineeringHarbin Normal UniversityHarbin 150025HeilongjiangChina

Precisely refining the electronic structure of electrocatalysts represents a powerful approach to further optimize the electrocatalytic ***,we demonstrate an ingenious d-d orbital hybridization concept to construct Mo-doped Co_(9)S_(8) nanorod arrays aligned on carbon cloth(CC)substrate(abbreviated as Mo-Co_(9)S_(8)@CC hereafter)as a high-efficiency bifunctional electrocatalyst toward water *** has experimentally and theoretically validated that the 4d-3d orbital coupling between Mo dopant and Co site can effectively optimize the H_(2)O activation energy and lower H^(*)adsorption energy barrier,thereby leading to enhanced hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)*** to the unique electronic and geometrical advantages,the optimized Mo-Co_(9)S_(8)@CC with appropriate Mo content exhibits outstanding bifunctional performance in alkaline solution,with the overpotentials of 75 and 234 mV for the delivery of a current density of 10 mA cm^(-2),small Tafel slopes of 53.8 and 39.9 mV dec~(-1)and long-term stabilities for at least 32 and 30 h for HER and OER,*** impressively,a water splitting electrolylzer assembled by the self-supported Mo-Co_(9)S_(8)@CC electrode requires a low cell voltage of 1.53 V at 10 mA cm^(-2)and shows excellent stability and splendid reversibility,demonstrating a huge potential for affordable and scalable electrochemical H_(2) *** innovational orbital hybridization strategy for electronic regulation herein provides an inspirable avenue for developing progressive electrocatalysts toward new energy systems.

关键词： d-d orbital hybridization Transition metal sulfides Nanorods arrays Water electrolysis