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The adsorption behavior of metals in aqueous solution by microplastics effected by UV radiation

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Journal of environmental Sciences 2020年第1期32卷 272-280页

作者： Qiongjie Wang Yong Zhang Xiaoxue Wangjin Yulai Wang Guanhua Meng Yihua Chen school of energy and environment Anhui University of Technology

Microplastics are considered as the carrier to heavy metals in the environment.But the sorption ability of microplastics influenced by photo-aging is remaining unclear.In the present study,the sorption of two kinds of metal ions(Cu^2+ and Zn^2+)in the aqueous solution by both the virgin and aged microplastics was investigated.Polyethylene terephthalate(PET)debris,one of the typical kinds of microplastics was chosen in this study.Photo-aging of microplastics in environment was simulated using UV radiation in the laboratory.Date analysis indicated that the aged microplastics had higher adsorption capacity of heavy metals than original ones.This could be related to the increased surface area and oxygen containing function appeared in the surface of aged microplastics after UV radiation.When prolonging the time of radiation,the enhanced adsorption capacities of microplastics appeared for Cu^2+ and Zn^2+.These results showed a great interaction between the aging degree of plastics and sorption capacity to heavy metals.Meanwhile,external conditions including temperature and pH value were also showed great influence to the adsorption behavior.

关键词： UV radiation Microplastics Adsorption Metal ions

energy-saving and economic analysis of passive radiative sky cooling for telecommunication base station in China

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Building Simulation 2022年第10期15卷 1775-1787页

作者： Zengkai Cui Chenyue Guo Dongliang Zhao school of energy and environment Southeast UniversityNanjing 210096China Engineering Research Center of Building Equipment Energyand EnvironmentMinistry of EducationChina

The widespread application of 4G and the rapid development of 5G technologies dramatically increase the energy consumption of telecommunication base station (TBS). Remarkably, the air conditioning system accounts for a significant part of energy consumption in TBS. In this work, passive radiative sky cooling technology has been studied to explore its application potential for TBS. We built a simulation model in DeST to investigate the effect of various envelope thermophysical properties on TBS energy saving. The main influencing factors of the radiative sky cooling on TBS energy saving have been concluded and guidance has been raised for further application. An optimized envelope design combining radiative sky cooling with appropriate heat transfer coefficients has been proposed. The energy-saving and economic analysis of the optimized envelope design at different areas shows that, except for the low heat density TBS in severe cold areas, the annual energy-saving rate is 6.77%–64.29%, and the annual total energy saving is 21.94 kWh/m2–52.74 kWh/m2. The payback period is 1.55–4.67 years, and the maximum acceptable cost limited to a 5-year payback period is $3.21/m2–$9.67/m2.

关键词： telecommunication base station radiative sky cooling energy saving economic analysis

Impact of thermal stratification on airborne transmission risk of SARS-CoV-2 in various indoor environments

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Building Simulation 2023年第7期16卷 1159-1172页

作者： Fan Liu Zhiwen Luo Hua Qian school of environment and Architecture University of Shanghai for Science and TechnologyShanghaiChina Welsh school of Architecture Cardiff UniversityCardiffUK school of energy and environment Southeast UniversityNanjingChina

There exist various vertical temperature gradients in different-type buildings.A holistic understanding of the impact of different temperature-stratified indoor environments on infection risk is necessary.In this work,the airborne transmission risk of SARS-CoV-2 in different thermally stratified indoor environments is assessed using our previously developed airborne infection risk model.Results show that the vertical temperature gradients in office building,hospital,classroom,etc.are within the range of−0.34 to 3.26℃/m.In large space such as coach station,airport terminal,and sport hall,the average temperature gradient ranges within 0.13–2.38℃/m in occupied zone(0–3 m);in ice rink with special requirements of indoor environment,the temperature gradient is higher than those in the above indoor spaces.The existence of temperature gradients causes multi-peaks of the transmission risk of SARS-CoV-2 with distancing,and our results show that in office,hospital ward and classroom,the second peak of the transmission risk is higher than 10^(−3)in most contact scenarios,while most being lower than 10^(−6)in large spaces like coach station and airport.The work is expected to provide some guidance on specific intervention policies in relation to the types of indoor environments.

关键词： SARS-CoV-2 temperature gradient different-type buildings transmission risk

Characterization of size-resolved effective density of atmospheric particles in an urban atmosphere in Southern China

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Journal of environmental Sciences 2024年第7期141卷 194-204页

作者： Tingting Xie Liming Cao Jinyi Zheng Peng Xuan Xiaofeng Huang Laboratory of Atmospheric Observation Supersite School of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China

Effective density(ρ_(eff))is one of the most important physical properties of atmospheric particles,providing important references in exploring the emissions and aging processes of fresh particles.In this study,a combined system of differential mobility analyzer,centrifugal particle mass analyzer,and condensation particle counter was used to periodically measure theρ_(eff)of atmospheric particles in Shenzhen from Oct.2021 to Jan.2022.Results showed that theρ_(eff)of particles with various size presented a bimodal distribution,which could be divided into main density(ρ_(m),main peak,corresponding to relatively dense particles after aging)and sub density(ρ_(s),sub peak,corresponding to fresh particles).The occurrence frequencies ofρ_(s)of particles with diameters of 50 and 80 nm were less than 20%,but were as high as about 40%of that with diameters from 120 to 350 nm.Theρ_(m)showed increasing trend with the size of particles,whileρ_(s)decreased as the increasing of the size of particles.Theρ_(eff)on pollution day varied significantly with chemical compositions.The increasing of the proportion of sulfate could promote the increasing ofρ_(eff),while black carbon and organic matter caused opposite effects,which may be related to various factors,including the difference of the material density and morphology of various chemical components.Theρ_(eff)of 50,80 and 120 nm particles decreased considerably during the new particle formation event,indicating that organic condensation was an important contributor to new particle growth.

关键词： DMA-CPMA-CPC Effective density Main/sub density Size distribution

A review on g-C_(3)N_(4)decorated with silver for photocatalytic energy conversion

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Chinese Chemical Letters 2024年第2期35卷 187-196页

作者： Ziyu Pan Wufan Ding Hanchun Chen Haodong Ji Eco-environment and Resource Efficiency Research Laboratory School of Environment and EnergyPeking University Shenzhen Graduate SchoolShenzhen 518055China

Artificial photocatalytic energy conversion is considered as the most potential strategy for solving the increasingly serious energy crisis and environmental pollution problems by directly capturing solar energy.Therefore,high efficiency photocatalyst has drawn significant research attention in recent years.Due to the excellent electronic,optical,structural,and physicochemical performances,silver-based g-C_(3)N_(4)have become promising photocatalysts.This review emphasizes the recent progresses and challenges on g-C_(3)N_(4)decorated with silver for photocatalytic energy conversion.The extensive use of g-C_(3)N_(4)decorated with silver in diverse photocatalytic reactions,including hydrogen evolution,pollutant degradation and carbon dioxide reduction,is also fully introduced.In addition,we propose the perspectives of g-C_(3)N_(4)decorated with silver on photocatalytic applications.We hope that this review will shed some light on the photocatalytic energy conversion of g-C_(3)N_(4)decorated with silver.

关键词： g-C_(3)N_(4) Silver-modified g-C_(3)N_(4) Photocatalytic energy conversion H_(2)evolution Pollutant degradation CO_(2)reduction

Activating and stabilizing the surface of anode for high-performing direct-ammonia solid oxide fuel cells

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Nano Research 2023年第2期16卷 2454-2462页

作者： Kang Xu Feng Zhu Mingyang Hou Canan Li Hua Zhang Yu Chen School of Environment and Energy South China University of TechnologyGuangzhou 510006China

Ammonia has been recognized as a promising fuel for solid oxide fuel cells(SOFCs)because of its relatively high hydrogen content and high energy density.However,the effective catalysis of ammonia on the surface of state-of-the-art anode greatly hinders the further development of direct ammonia SOFCs.In this study,we report our findings of surface activating and stabilizing of a Ni-based cermet anode for highly efficient and durable operation on ammonia fuel,achieved by a surface coating of CeO_(2)−δnanoparticles(NPs).When incorporated into a Ni-yttria-stabilized zirconia(Ni-YSZ)anode-supported single cell,the coatings demonstrate an improved electrochemical reaction activity and stability,achieving a high peak power density of 0.941 W·cm^(−2)at 700℃,and a promising stability of~60 h(degradation rate of 0.127%h^(−1)at 0.5 A·cm−2),much better than those of cells with a bare anode(~0.673 W·cm^(−2)and degradation rate of 0.294%h−1 at 0.5 A·cm^(-2)).The catalytic NPs significantly enhance the reaction activity toward the decomposition of ammonia and oxidation of hydrogen,especially at low temperatures(<700℃),as confirmed by the detailed distribution of relaxation time(DRT)analyses of the impedance spectra of the cells on NH3 fuel.

关键词： solid oxide fuel cells anode catalyst infiltration ammonia

Experiments on particle cluster behaviors in a fast fluidized bed

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Chinese Journal of Chemical Engineering 2017年第9期25卷 1153-1162页

作者： Dailin Chen Xuejiao Liu Ziwen Sun Wenqi Zhong Baosheng Jin school of energy & environment Southeast University

A three-dimensional(3D) fast fluidized bed with the riser of 3.0 m in height and 0.1 m in inner diameter was established to experimentally study the cluster behaviors of Geldart B particles. Five kinds of quartz sand particles(dp= 0.100, 0.139, 0.177, 0.250 and 0.375 mm and ρp= 2480 kg·m^(-3)) were respectively investigated, with the total mass of the bed material kept as 10 kg. The superficial gas velocity in the riser ranges from 2.486 to 5.594 m·s^(-1) and the solid mass flux alters from 30 to 70 kg·((m^(-2)·s))^(-1). Cluster characteristics and evolutionary processes in the different positions of the riser were captured by the cluster visualization systems and analyzed by the self-developed binary image processing. The results found four typical cluster structures in the riser,i.e., the macro stripe-shaped cluster, saddle-shaped cluster, U-shaped cluster and the micro cluster. The increasing superficial gas velocity and particle sizes result in the increasing average cluster size and the decreasing cluster time fraction, while the solid mass flux in the riser have the reverse influences on the cluster size and time fraction. Additionally, clusters in the upper region of the riser often have the larger size and time fraction than that in the lower region. All these effects of operating conditions on clusters become less obvious when particle size is less than 0.100 mm.

关键词： Gas–solid flow Cluster Fast fluidized bed Geldart B particle

Carbon capture for decarbonisation of energy-intensive industries:a comparative review of techno-economic feasibility of solid looping cycles

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Frontiers of Chemical Science and Engineering 2022年第9期16卷 1291-1317页

作者： Mónica P.S.Santos Dawid P.Hanak energy and Power School of WaterEnergy and EnvironmentCranfield UniversityBedfordshire MK430ALUK

Carbon capture and storage will play a crucial role in industrial decarbonisation.However,the current literature presents a large variability in the techno-economic feasibility of CO_(2)capture technologies.Consequently,reliable pathways for carbon capture deployment in energyintensive industries are still missing.This work provides a comprehensive review of the state-of-the-art CO_(2)capture technologies for decarbonisation of the iron and steel,cement,petroleum refining,and pulp and paper industries.Amine scrubbing was shown to be the least feasible option,resulting in the average avoided CO_(2)cost of between 62.7∈t_(CO_(2))^(-1)for the pulp and paper and 104.6∈t_(CO_(2))^(-1)for the iron and steel industry.Its average equivalent energy requirement varied between 2.7(iron and steel)and 5.1MJ_(th)·kg_(CO_(2))^(-1)(cement).Retrofits of emerging calcium looping were shown to improve the overall viability of CO_(2)capture for industrial decarbonisation.Calcium looping was shown to result in the average avoided CO_(2)cost of between 32.7(iron and steel)and 42.9(cement).Its average equivalent energy requirement varied between 2.0(iron and steel)and 3.7(pulp and paper).Such performance demonstrated the superiority of calcium looping for industrial decarbonisation.Further work should focus on standardising the techno-economic assessment of technologies for industrial decarbonisation.

关键词： industrial CO_(2)emissions CCS deployment carbonate looping net-zero industry carbon capture benchmarks

Supercritical CO_(2) Cycles for Nuclear-Powered Marine Propulsion:Preliminary Conceptual Design and Off-Design Performance Assessment

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Journal of Thermal Science 2024年第1期33卷 328-347页

作者： LI Zhaozhi SHI Mingzhu SHAO Yingjuan ZHONG Wenqi Key Laboratory of energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Using the efficient,space-saving,and flexible supercritical carbon dioxide(sCO_(2)) Brayton cycle is a promising approach for improving the performance of nuclear-powered ships.The purpose of this paper is to design and compare sCO_(2) cycle power systems suitable for nuclear-powered ships.Considering the characteristics of nuclear-powered ships,this paper uses different indicators to comprehensively evaluate the efficiency,cost,volume,and partial load performance of several nuclear-powered sCO_(2) cycles.Four load-following strategies are also designed and compared.The results show that the partial cooling cycle is most suitable for nuclear-powered ships because it offers both high thermal efficiency and low volume and cost,and can maintain relatively high thermal efficiency at partial loads.Additionally,the new load-following strategy that adjusts the turbine speed can keep the compressor away from the surge line,making the cycle more flexible and efficient compared to traditional inventory and turbine bypass strategies.

关键词： supercritical CO_(2)cycle nuclear marine propulsion off-design performance