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energy & Environmental Materials 2024年第3期7卷 232-239页

作者： Fan Liu Xinghong Cai Yang Tang Wenqian Liu Qianwei Chen Peixin Dong Maowen Xu Yangyang Tan Shujuan Bao Institute for Clean energy & Advanced Materials School of Materials and EnergySouthwest University

Electrocatalytic hydrogen evolution and sulfion (S2-) recycling are promising strategies for boosting H2production and removing environmental ***,a nano-Ni-functionalized molybdenum disulfide （MoS2）nanosheet was assembled on steel mesh （Ni-MoS2/SM） for use in sulfide oxidation reaction-assisted,energy-saving *** and theoretical calculation results revealed that anchoring nano-Ni on highsurface-area slack MoS2 nanosheets not only optimized catalyst adsorption of polysulfides but also played an important role in promoting hydrogen evolution reaction kinetics by absorbing OHad,thereby greatly enhancing the catalytic performance toward sulfide oxidation reaction and hydrogen evolution ***,the Ni/MoS2-based hydrogen evolution reaction+sulfide oxidation reaction system achieved nearly 100%hydrogen production efficiency and only consumed 61%less power per kWh than the oxygen evolution reaction+hydrogen evolution reaction system,which suggested our proposed Ni-MoS2and novel hydrogen production system are promising for sustainable energy production.

关键词： hydrogen evolution reaction low energy consumption molybdenum disulfide sulfide oxidation reaction

Tetraphenylethene-based hole transporting material for highly efficient and stable perovskite solar cells

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Science China Chemistry 2024年第6期67卷 2009-2015页

作者： Peng Wang Pei Yuan Chenghao Ge Rongjun Zhao Lin Xie Yong Hua school of Materials and energy Yunnan UniversityKunming650091China

2,2,7,7-Tetrakis-(N,N-di-p-methoxyphenylamine)-9,9-spirobifluorene(Spiro-OMeTAD)has been identified as the most widely used and effective hole transporting material(HTM)in perovskite solar cells(PSCs).However,the complicated multistep synthesis and low intrinsic hole mobility of Spiro-OMe TAD limit its commercialized ***,developing highly efficient HTMs with less synthetic steps becomes increasingly ***,understanding hot carriers transfer dynamics at the interface of perovskite layer and hole transport layer is crucial for further enhancing PSCs performance towards Shockley-Queisser limit,which still lacks full investigation to ***,a new HTM based on tetraphenylethene(WP1)was successfully synthesized by a simple one-step reaction *** was found that WP1-based HTM exhibits more matched energy level,higher hole mobility and conductivity than those of the control Spiro-OMe *** femtosecond transient absorption results reveal that the transfer rate of hot holes in perovskite/WP1 sample is four times higher than that of perovskite/Spiro-OMeTAD,thereby helping enhance the device ***,the efficiency of PSCs is enhanced to 24.04%(WP1)from 22.85%(Spiro-OMeTAD).Moreover,the un-encapsulated device prepared with WP1 exhibits better long-term stability,retaining 87%of its initial PCE value after storing for 72 days under air environment,while the reference device shows76%of its initial *** work indicates that simple tetraphenylethene-based organic small molecule could be a very promising HTM candidate for highly efficient PSCs,and gives some significant insights for understanding intrinsic hot carriers transfer dynamics in device.

关键词： tetraphenylethene hole transporting material perovskite solar cells mobility hot carrier

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Optimization Control of Multi-Mode Coupling All-Wheel Drive System for Hybrid Vehicle

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Chinese Journal of Mechanical Engineering 2024年第2期37卷 340-355页

作者： Lipeng Zhang Zijian Wang Liandong Wang Changan Ren school of Vehicle and energy Yanshan UniversityQinhuangdao 066004China

The all-wheel drive(AWD)hybrid system is a research focus on high-performance new energy vehicles that can meet the demands of dynamic performance and passing *** optimization of the power and economy of hybrid vehicles becomes an issue.A unique multi-mode coupling(MMC)AWD hybrid system is presented to realize the distributed and centralized driving of the front and rear axles to achieve vectored distribution and full utilization of the system power between the axles of *** on the parameters of the benchmarking model of a hybrid vehicle,the best model-predictive control-based energy management strategy is ***,the drive system model was built after the analysis of the MMC-AWD’s drive ***,three fundamental strategies were established to address power distribution adjustment and battery SOC maintenance when the SOC changed,which was followed by the design of a road driving force ***,the energy consumption rate in the average time domain was processed before designing the minimum fuel consumption controller based on the equivalent fuel consumption ***,the advantage of the MMC-AWD was confirmed by comparison with the dynamic performance and economy of the BYD Song PLUS *** findings indicate that,in comparison to the comparative hybrid system at road adhesion coefficients of 0.8 and 0.6,the MMC-AWD’s capacity to accelerate increases by 5.26%and 7.92%,*** the road adhesion coefficient is 0.8,0.6,and 0.4,the maximum climbing ability increases by 14.22%,12.88%,and 4.55%,*** a result,the dynamic performance is greatly enhanced,and the fuel savings rate per 100 km of mileage reaches 12.06%,which is also very *** proposed control strategies for the new hybrid AWD vehicle can optimize the power and economy simultaneously.

关键词： Hybrid vehicle All-wheel drive Multi-mode coupling energy management Model predictive control

Microwave-assisted pyrolysis of plastics for aviation oil production:energy and economic analyses

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Frontiers of Chemical Science and Engineering 2024年第7期18卷 141-153页

作者： Sichen Fan Yifan Liu Yaning Zhang Wenke Zhao Chunbao Xu school of energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China school of energy and Environment City University of Hong KongHong Kong SARChina

Microwave-assisted pyrolysis is an effective method for recycling plastic wastes into oils that can be used for aviation fuels. In this study, energy and economic analyses of aviation oil production from microwave-assisted pyrolysis of polystyrene were performed. The total energy efficiency, recovered energy efficiency, unitary cost, unitary energy economic cost, relative cost difference, and energy economic factor were detailed. And the effects of microwave power, pyrolysis temperature, microwave absorbent loading, and microwave absorbent type on these parameters were covered. It was found that pyrolysis temperature has the most significant effect on the unitary cost and unitary energy economic cost of aviation oil, and-microwave absorbent type has a significant influence on energy economic factor during the whole microwave-assisted pyrolysis process. The optimum reaction conditions at the tonnage system for pyrolysis of 1 t polystyrene were microwave power of 650 W, pyrolysis temperature of 460 ℃, and silicon carbide (microwave absorbent) at a loading of 2 t (twice than feedstock loading). At these optimal conditions, the total energy efficiency, recovered energy efficiency, unitary cost, unitary energy economic cost, relative cost difference, and energy economic factor were 62.78%, 96.51%, 3.21 × 10^(4) yuan·t^(-1), 779 yuan·GJ^(-1), 1.49, and 71.02%, respectively.

关键词： energy analysis economic analysis microwave-assisted pyrolysis polystyrene aviation oil

From longan peel waste to energy storage: Porous activated carbon as a cathode matrix for advanced Li/Na-selenium batteries

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Progress in Natural Science:Materials International 2024年第2期34卷 329-337页

作者： Mustafa Khan Suxia Yan Mujahid Ali Faisal Mahmood Yang Zheng Xiaohui Song Guochun Li Junfeng Liu Yong Wang Institute for energy Research Jiangsu University school of energy and Power Engineering Jiangsu University school of Materials Science and Engineering Hefei University of Technology

This paper explores the potential of Longan peel waste（LPw） as a sustainable and cost-effective matrix for selenium-based cathodes in Li-Se and Na-Se *** activation,we created LP2—a designation for the carbon precursor derived from LPw,activated at a 1:2 ratio of carbonized LPw to *** nomenclature,where'LP' stands for 'Longan peel' and '2' reflects the optimization of this ratio,led to a hierarchical porous structure with an average pore size of 3.0307 nm and a significant BET surface area of 111.9386 m2g-1Selenium was incorporated into the LP2matrix using a simple melt diffusion technique,yielding the composite Se@*** Li-Se batteries,Se@LP2exhibited an initial discharge capacity of 1033.75 mAh g-1at *** a 1C rate,the composite demonstrated a capacity retention of 301.14 mAh g-1after 550 cycles and 380.91 mAh g-1after 100 ***,for Na-Se batteries,the composite showcased a capacity retention of 347.18 mAh g-1after 100 cycles *** findings underscore LP2's potential as a viable and efficient matrix for selenium-based cathodes,revealing promising prospects for the advancement of highly efficient Li-Se and Na-Se batteries.

关键词： Hierarchical porous structure Li/Na-Se batteries Longan peel waste Melt diffusion technique Selenium-based cathode

Supercritical CO_(2) Cycles for Nuclear-Powered Marine Propulsion:Preliminary Conceptual Design and Off-Design Performance Assessment

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Journal of Thermal Science 2024年第1期33卷 328-347页

作者： LI Zhaozhi SHI Mingzhu SHAO Yingjuan ZHONG Wenqi Key Laboratory of energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Using the efficient,space-saving,and flexible supercritical carbon dioxide(sCO_(2)) Brayton cycle is a promising approach for improving the performance of nuclear-powered *** purpose of this paper is to design and compare sCO_(2) cycle power systems suitable for nuclear-powered *** the characteristics of nuclear-powered ships,this paper uses different indicators to comprehensively evaluate the efficiency,cost,volume,and partial load performance of several nuclear-powered sCO_(2) *** load-following strategies are also designed and *** results show that the partial cooling cycle is most suitable for nuclear-powered ships because it offers both high thermal efficiency and low volume and cost,and can maintain relatively high thermal efficiency at partial ***,the new load-following strategy that adjusts the turbine speed can keep the compressor away from the surge line,making the cycle more flexible and efficient compared to traditional inventory and turbine bypass strategies.

关键词： supercritical CO_(2)cycle nuclear marine propulsion off-design performance

Design of acceleration control schedule for adaptive cycle engine based on direct simulation model

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Chinese Journal of Aeronautics 2024年第6期37卷 307-318页

作者： Keran SONG Linyuan JIA Yuchun CHEN Tian TAN school of Power and energy Northwestern Polytechnical UniversityXi’an 710072China

To design the optimum acceleration control schedule for the Adaptive Cycle Engine(ACE)in the full flight envelope,this paper establishes a direct simulation model of the ACE transient *** this model,geometric parameters are used to replace the component state *** corresponding relationship between geometric parameters and component state parameters is determined by sensitivity *** geometric variables are controlled when the geometric adjustment speed exceeds the limit,and at the same time the corresponding component state parameters are *** gradient optimization algorism is used to optimize the ground acceleration process of ACE,and the control schedule in terms of operating point of compression components and corrected acceleration rate is used as the full-envelope acceleration control schedule based on the similarity *** acceleration control schedules of the triple-bypass mode and the double-bypass mode are designed in this *** acceleration processes under various flight conditions are simulated using the acceleration control *** with the acceleration process with the linear geometric adjustment schedule,the acceleration performance of ACE is improved by the acceleration control schedule,with the impulse of the acceleration process of the triple-bypass mode being increased by 8.7%-12.3% and the impulse of the double-bypass mode acceleration process being increased by 11.8%-14.1%.

关键词： Adaptive Cycle Engine(ACE) Direct simulation method Acceleration Control schedule Full flight envelope

Novel data-driven sparse polynomial chaos and analysis of covariance for aerodynamics of compressor cascades with dependent geometric uncertainties

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Chinese Journal of Aeronautics 2024年第6期37卷 89-108页

作者： Zhengtao GUO Wuli CHU Haoguang ZHANG Tianyuan JI school of Power and energy Northwestern Polytechnical UniversityXi’an 710072China

Polynomial Chaos Expansion(PCE)has gained significant popularity among engineers across various engineering disciplines for uncertainty ***,traditional PCE suffers from two major ***,the orthogonality of polynomial basis functions holds only for independent input variables,limiting the model’s ability to propagate uncertainty in dependent ***,PCE encounters the"curse of dimensionality"due to the high computational cost of training the model with numerous polynomial *** practical manufacturing,compressor blades are subject to machining precision limitations,leading to deviations from their ideal geometric *** deviations require a large number of geometric parameters to describe,and exhibit significant *** efficiently quantify the impact of high-dimensional dependent geometric deviations on the aerodynamic performance of compressor blades,this paper firstly introduces a novel approach called Data-driven Sparse PCE(DSPCE).The proposed method addresses the aforementioned challenges by employing a decorrelation algorithm to directly create multivariate basis functions,accommodating both independent and dependent random ***,the method utilizes an iterative Diffeomorphic Modulation under Observable Response Preserving Homotopy regression algorithm to solve the unknown coefficients,achieving model sparsity while maintaining fitting ***,the study investigates the simultaneous effects of seven dependent geometric deviations on the aerodynamics of a high subsonic compressor cascade by using the DSPCE method proposed and sensitivity analysis of *** joint distribution of the dependent geometric deviations is determined using Quantile-Quantile plots and normal copula functions based on finite measurement *** results demonstrate that the correlations between geometric deviations significantly impact the variance of aerodynamic performance and the flow ***,

关键词： Data-driven sparse polyno-mial chaos Analysis of covariance Dependent uncertainty Aerodynamic performance Compressor cascade

An uncertainty investigation for liner impedance eduction methods

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Chinese Journal of Aeronautics 2024年第3期37卷 49-59页

作者： Weihao SHI Xiaodong JING school of energy and Power Engineering Beihang UniversityBeijing 100191China

Impedance eduction methods have been developed for decades to meet the increasing need for high-quality impedance data in the design and optimization of acoustic *** this end,it is important to fully investigate the uncertainty problem,to which only limited attention has been devoted so *** paper considers the possibility of acoustically-induced structural vibration as a nonnegligible uncertainty or error source in impedance eduction *** the frequency moves away from the resonant frequency,with the increase in the value of cavity reactance,the acoustic particle velocity inside liner orifices possibly decreases to the extent comparable to the vibration velocity of liner facing ***,the acoustically-induced vibration,although generally being weak except at the inherent structural frequencies,may considerably affect the impedance eduction results near the anti-resonant frequency where the liner has poor *** demonstrate the effect of structural vibration,the vibration velocity of liner facing sheet is estimated from the experimentally educed admittance of the liner samples whose orifices are sealed with ***,a three-dimensional numerical model is set up,in which normal particle velocity is introduced over the solid portion of liner facing sheet to imitate structural vibration,rather than directly solving the acoustic-structural coupling *** shown by the results,the vibration of liner facing sheet,whose velocity is as small as estimated by the experiment,can result in anomalous deviation of the educed impedance from the impedance model near the anti-resonant *** trend that the anomalous deviation varies with frequency is numerically captured.

关键词： Impedance eduction Uncertainty analysis Acoustically-induced structural vibration Anti-resonant frequency Perforated liner

Experimental study on combustion characteristics of supersonic combustor based on alternating-wedge strut

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Chinese Journal of Aeronautics 2024年第5期37卷 214-227页

作者： Jie LI Wenyan SONG Yuhang WANG school of Power energy Northwestern Polytechnical UniversityXi’an 710129China

Acetone Planar Lase-Induced Fluorescence(PLIF)and OH-PLIF were employed to capture the fuel distribution and OH distribution downstream for the supersonic combustor based on the alternating-wedge *** combustion establishment process and combustion mode in the combustor under different fuel injection methods and different equivalence ratios were *** with the kerosene-PLIF and OH-PLIF results in the cavity combustor,a comparative analysis was conducted to understand the combustion characteristics and combustion modes between the alternating-wedge strut-based combustor and the cavity-based *** results show that the combustor is in weak combustion mode in the case of low equivalence ratio,and the combustor is in intensive combustion mode in the case of high equivalence *** lower limit of the equivalence ratio of the combustor to maintain the intensive combustion mode varies based on different fuel injection *** OH distribution under reacting condition has a strong correlation with the fuel distribution under non-reacting *** OH fluorescence signal near the injector is weaker when the fuel distribution is more *** injector position located at the base of the strut rear has better mixing performance,enabling the combustor to be in intensive combustion mode at a lower equivalence *** combustion reaction in the alternating-wedge strut-based combustor is not necessarily dominated by mass transfer due to the mixing enhancement and premixed zone downstream of strut,while the combustion reaction process in the cavity-based combustor is mainly influenced by mass transfer.

关键词： Supersonic combustor Alternating-wedge strut Cavity PLIF Fuel injection Fuel distribution Combustion characteristics Combustion mode