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Tailoring MXene Thickness and Functionalization for Enhanced Room‑Temperature Trace NO_(2) Sensing

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Nano-Micro Letters 2024年第5期16卷 71-86页

作者： Muhammad Hilal Woochul Yang Yongha Hwang Wanfeng Xie Department of Physics Dongguk UniversitySeoul 04620Republic of Korea Department of Control and Instrumentation engineering Korea UniversitySejong 30019Republic of Korea school of electronics&information University‑Industry Joint Center for Ocean Observation and Broadband CommunicationQingdao UniversityQingdao 266071China

In this study,precise control over the thickness and termination of Ti3C2TX MXene flakes is achieved to enhance their electrical properties,environmental stability,and gas-sensing performance.Utilizing a hybrid method involving high-pressure processing,stirring,and immiscible solutions,sub-100 nm MXene flake thickness is achieved within the MXene film on the Si-wafer.Functionalization control is achieved by defunctionalizing MXene at 650℃ under vacuum and H2 gas in a CVD furnace,followed by refunctionalization with iodine and bromine vaporization from a bubbler attached to the CVD.Notably,the introduction of iodine,which has a larger atomic size,lower electronegativity,reduce shielding effect,and lower hydrophilicity(contact angle:99°),profoundly affecting MXene.It improves the surface area(36.2 cm^(2) g^(-1)),oxidation stability in aqueous/ambient environments(21 days/80 days),and film conductivity(749 S m^(-1)).Additionally,it significantly enhances the gas-sensing performance,including the sensitivity(0.1119Ωppm^(-1)),response(0.2% and 23%to 50 ppb and 200 ppm NO_(2)),and response/recovery times(90/100 s).The reduced shielding effect of the–I-terminals and the metallic characteristics of MXene enhance the selectivity of I-MXene toward NO2.This approach paves the way for the development of stable and high-performance gas-sensing two-dimensional materials with promising prospects for future studies.

关键词： Controlled MXene thickness Gaseous functionalization approach Lower electronegativity functional groups Enhanced MXene stability Trace NO_(2)sensing

N:ZnO/MoS_(2)-heterostructured flexible synaptic devices enabling optoelectronic co-modulation for robust artificial visual systems

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Nano Research 2024年第3期17卷 1902-1912页

作者： Lei Xu Wenxiao Wang Yang Li Yonghui Lin Wenjing Yue Kai Qian Qinglei Guo Jeonghyun Kim Guozhen Shen school of information Science and engineering University of JinanJinan 250022China school of Microelectronics Shandong UniversityJinan 250101China Department of Electronic Convergence engineering Kwangwoon UniversitySeoul 01897Republic of Korea school of Integrated Circuits and electronics Beijing Institute of TechnologyBeijing 100081China

With the merits of non-contact,highly efficient,and parallel computing,optoelectronic synaptic devices combining sensing and memory in a single unit are promising for constructing neuromorphic computing and artificial visual chip.Based on this,a N:ZnO/MoS_(2)-heterostructured flexible optoelectronic synaptic device is developed in this work,and its capability in mimicking the synaptic behaviors is systemically investigated under the electrical and light signals.Versatile synaptic functions,including synaptic plasticity,long-term/short-term memory,and learning-forgetting-relearning property,have been achieved in this synaptic device.Further,an artificial visual memory system integrating sense and memory is emulated with the device array,and the visual memory behavior can be regulated by varying the light parameters.Moreover,the optoelectronic co-modulation behavior is verified by applying mixed electric and light signals to the array.In detail,a transient recovery property is discovered when the electric signals are applied in synergy during the decay of the light response,of which property facilitates the development of robust artificial visual systems.Furthermore,by superimposing electrical signals during the light response process,a differentiated response of the array is achieved,which can be used as a proof of concept for the color perception of the artificial visual system.

关键词： flexible synaptic device synaptic plasticity optoelectronic synapse robust visual memory optoelectronic co-modulation artificial visual system

Varifocal occlusion in an optical see-through near-eye display with a single phase-only liquid crystal on silicon

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Photonics Research 2024年第4期12卷 833-853页

作者： WOONGSEOB HAN JAE-WON LEE JUNG-YEOP SHIN MYEONG-HO CHOI HAK-RIN KIM JAE-HYEUNG PARK Department of Electrical and Computer engineering Inha University100 Inha-roMichuhol-guIncheon 22212Republic of Korea school of Electronic and Electrical engineering Kyungpook National University80 Daehak-roBuk-guDaegu 41566Republic of Korea school of electronics engineering Kyungpook National University80 Daehak-roBuk-guDaegu 41566Republic of Korea Department of information and Communication engineering Inha University100 Inha-roMichuhol-guIncheon 22212Republic of Korea

We propose a near-eye display optics system that supports three-dimensional mutual occlusion.By exploiting the polarization-control properties of a phase-only liquid crystal on silicon (LCoS),we achieve real see-through scene masking as well as virtual digital scene imaging using a single LCoS.Dynamic depth control of the real scene mask and virtual digital image is also achieved by using a focus tunable lens (FTL) pair of opposite curvatures.The proposed configuration using a single LCoS and opposite curvature FTL pair enables the self-alignment of the mask and image at an arbitrary depth without distorting the see-through view of the real scene.We verified the feasibility of the proposed optics using two optical benchtop setups:one with two off-the-shelf FTLs for continuous depth control,and the other with a single Pancharatnam–Berry phase-type FTL for the improved form factor.

关键词： optics crystal phase

Advances in advanced solution-synthesis-based structural materials for tactile sensors and their intelligent applications

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InfoMat 2024年第1期6卷 31-64页

作者： Hongsen Niu Ning Li Eun-Seoung Kim Young Kee Shin Nam-Young Kim Guozhen Shen Yang Li school of information Science and engineering University of JinanJinanthe People's Republic of China RFIC Centre Department of Electronics EngineeringKwangwoon UniversitySeoulRepublic of Korea Department of Molecular Medicine and Biopharmaceutical Sciences Seoul National UniversitySeoulRepublic of Korea school of Integrated Circuits and electronics Beijing Institute of TechnologyBeijingthe People's Republic of China school of Microelectronics Shandong UniversityJinanthe People's Republic of China

Intelligent applications,with tactile sensors at their core,represent significant advancement in the field of artificial intelligence.However,achieving perception abilities in tactile sensors that match or exceed human skin remains a formidable challenge.Consequently,the design and implementation of hierarchical structural materials are considered the optimal solution to this challenge.In contrast to conventional methods,such as complicated lithography and three-dimensional printing,the cost-effective and scalable nature of advanced solution-synthesis methods makes them ideal for preparing diverse tactile sensors with hierarchical structural materials.However,the process and applicability of advanced solution synthesis methods have yet to form a seamless system.Accordingly,the development and intellectualization of tactile sensors based on advanced solution synthesis methods are still in their early stages,and require a comprehensive and systematic review to usher in progress.This study delves into the advantages and disadvantages of various advanced solution synthesis methods,providing detailed insights.Furthermore,the positive effects of hierarchical structural materials constructed using these methods in tactile sensors and their intelligent applications are also discussed in depth.Finally,the challenges and future opportunities faced by this emerging field are summarized.

关键词： aqueous phase reduction artificial intelligence hydrothermal growth in situ polymerization tactile sensor

Surface Patterning of Metal Zinc Electrode with an In‑Region Zincophilic Interface for High‑Rate and Long‑Cycle‑Life Zinc Metal Anode

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Nano-Micro Letters 2024年第6期16卷 192-209页

作者： Tian Wang Qiao Xi Kai Yao Yuhang Liu Hao Fu Venkata Siva Kavarthapu Jun Kyu Lee Shaocong Tang Dina Fattakhova‑Rohlfing Wei Ai Jae Su Yu Department of electronics and information Convergence engineering Institute for Wearable Convergence ElectronicsKyung Hee UniversityYongin‑siGyeonggi‑do 17104Republic of Korea Frontiers Science Center for Flexible electronics(FSCFE)and Shaanxi Institute of Flexible electronics(SIFE) Northwestern Polytechnical University(NPU)127 West Youyi RoadXi’an 710072People’s Republic of China Institute of Energy and Climate Research:Materials Synthesis and Processing(IEK‑1) Forschungszentrum Julich GmbH52425 JulichGermany school of Chemical engineering Sungkyunkwan University2066 Seobu‑RoJangan‑GuSuwon‑siGyeonggi‑doRepublic of Korea

The undesirable dendrite growth induced by non-planar zinc(Zn)deposition and low Coulombic efficiency resulting from severe side reactions have been long-standing challenges for metallic Zn anodes and substantially impede the practical application of rechargeable aqueous Zn metal batteries(ZMBs).Herein,we present a strategy for achieving a high-rate and long-cycle-life Zn metal anode by patterning Zn foil surfaces and endowing a Zn-Indium(Zn-In)interface in the microchannels.The accumulation of electrons in the microchannel and the zincophilicity of the Zn-In interface promote preferential heteroepitaxial Zn deposition in the microchannel region and enhance the tolerance of the electrode at high current densities.Meanwhile,electron aggregation accelerates the dissolution of non-(002)plane Zn atoms on the array surface,thereby directing the subsequent homoepitaxial Zn deposition on the array surface.Consequently,the planar dendrite-free Zn deposition and long-term cycling stability are achieved(5,050 h at 10.0 mA cm^(−2) and 27,000 cycles at 20.0 mA cm^(−2)).Furthermore,a Zn/I_(2) full cell assembled by pairing with such an anode can maintain good stability for 3,500 cycles at 5.0 C,demonstrating the application potential of the as-prepared ZnIn anode for high-performance aqueous ZMBs.

关键词： Zn metal anode Surface patterning Directional Zn deposition Aqueous Zn-I_(2)batteries

Recent advances in halide perovskite memristors:From materials to applications

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Frontiers of physics 2024年第2期19卷 73-104页

作者： Sixian Liu Jianmin Zeng Qilai Chen Gang Liu Department of Micro/Nano electronics School of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai 200240China aerospace Science&Industry Shenzhen(Group)Co.Ltd. Shenzhen 518000China

With the emergence of the Internet of Things(IoT)and the rapid growth of big data generated by edge devices,there has been a growing need for electronic devices that are capable of processing and transmitting data at low power and high speeds.Traditional Complementary Metal-Oxide-Semiconductor(CMOS)devices are nonvolatile and often limited by their ability for certain IoT applications due to their unnecessary power consumption for data movement in von Neuman architecture-based systems.This has led to a surge in research and development efforts aimed at creating innovative electronic components and systems that can overcome these shortcomings and meet the evolving needs of the information era,which share features such as improved energy efficiency,higher processing speeds,and increased functionality.Memristors are a novel type of electronic device that has the potential to break down the barrier between storage and computing.By storing data and processing information within the same device,memristors can minimize the need for data movement,which allows for faster processing speeds and reduced energy consumption.To further improve the energy efficiency and reliability of memristors,there has been a growing trend toward diversifying the selection of dielectric materials used in memristors.Halide perovskites(HPs)have unique electrical and optical properties,including ion migration,charge trapping effect caused by intrinsic defects,excellent optical absorption efficiency,and high charge mobility,which makes them highly promising in applications of memristors.In this paper,we provide a comprehensive overview of the recent development in resistive switching behaviors of HPs and the underlying mechanisms.Furthermore,we summarize the diverse range of HPs,their respective performance metrics,as well as their applications in various fields.Finally,we critically evaluate the current bottlenecks and possible opportunities in the future research of HP memristors.

关键词： halide perovskite memristor mechanism neuromorphic computing non-volatile memory

Exploring Antarctic subglacial lakes with RECoverable Autonomous Sonde(RECAS): Design and first field tests

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Science China Technological Sciences 2024年第6期67卷 1866-1878页

作者： SUN YouHong PAVEL Talalay LI YuanSheng YU HaiBin WANG DongLiang LI GuoPing XU LiPing GONG Da WANG JiXin WANG JianHua WANG Ting ZHANG Nan WANG ZhiGang CHEN YanJi LIU YunChen LI YaZhou PENG ShiLin SHI JianGuang AN ChunLei GE Qun XU Jing NI XiaoKang CUI QiFeng JIANG Qiang MIKHAIL Sysoev Yang Yang WANG RuSheng WEI XianZhe WANG Yu ZHU TianXin DENG ZhiPeng ALEXEY Markov LI Bing FAN XiaoPeng Polar Research Center Jilin University school of engineering and Technology China University of Geosciences Polar Research Institute of China College of electronics and information Hangzhou Dianzi University aerospace System engineering Shanghai Nanjing Institute of Astronomical Optics & Technology National Astronomical ObservatoriesChinese Academy of Sciences National Ocean Technology Center

Conducting scientific drilling on subglacial lakes and obtaining samples of subglacial lake water holds great significance in unraveling the formation and evolution of Antarctic subglacial lakes and early Earth's life forms. Despite various approaches to access and directly sample subglacial water and sediments, clean access and exploration of subglacial lakes remain challenging.To address this concern, Jilin university has developed the RECoverable Autonomous Sonde(RECAS) prototype. This technology enables sampling and in-situ detection of subglacial lake water while being isolated from the surface, thus minimizing the risk of pollution. Laboratory tests, including downward and upward drilling, long-running, remote-control, and cold-environment assessments, were conducted to validate the sonde's principle and functionality. During the 38th Chinese National Antarctic Research Expedition, CHINARE(2021–2022 season), the RECAS prototype underwent testing on the flank region of D?lk glacier, 10 km from Zhongshan Station in Antarctica. Three boreholes with depths of 200.3, 183.2, and 133.5 m were successfully drilled, with the refrozen meltwater sealing the boreholes during the process. Approximately 600 mL of melted water samples were collected from each hole. Throughout the drilling tests, all systems of the RECAS prototype performed within the expected ranges.

关键词： subglacial lake thermal drilling water sampling Antarctic autonomous sonde

Cooperative Anti-Jamming and Interference Mitigation for UAV Networks: A Local Altruistic Game Approach

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China Communications 2024年第2期21卷 183-196页

作者： Yueyue Su Nan Qi Zanqi Huang Rugui Yao Luliang Jia College of Electronic information engineering Nanjing University of Aeronautics and AstronauticsNanjing 211106China National Mobile Communications Research Laboratory Southeast UniversityNanjing 210096China school of electronics and information Northwestern Polytechnical UniversityXi’an 710072China school of Space information Space Engineering UniversityBeijing 101416China

To improve the anti-jamming and interference mitigation ability of the UAV-aided communication systems, this paper investigates the channel selection optimization problem in face of both internal mutual interference and external malicious jamming. A cooperative anti-jamming and interference mitigation method based on local altruistic is proposed to optimize UAVs’ channel selection. Specifically, a Stackelberg game is modeled to formulate the confrontation relationship between UAVs and the jammer. A local altruistic game is modeled with each UAV considering the utilities of both itself and other UAVs. A distributed cooperative anti-jamming and interference mitigation algorithm is proposed to obtain the Stackelberg equilibrium. Finally, the convergence of the proposed algorithm and the impact of the transmission power on the system loss value are analyzed, and the anti-jamming performance of the proposed algorithm can be improved by around 64% compared with the existing algorithms.

关键词： channel selection cooperative antijamming and interference mitigation local altruistic game Stackelberg game unmanned aerial vehicle(UAV)

Improving path planning efficiency for underwater gravity-aided navigation based on a new depth sorting fast search algorithm

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Defence Technology（防务技术） 2024年第2期32卷 285-296页

作者： Xiaocong Zhou Wei Zheng Zhaowei Li Panlong Wu Yongjin Sun school of Automation Nanjing University of Science and TechnologyNanjing210094China China Academy of aerospace Science and Innovation Beijing100176China Qian Xuesen Laboratory of Space Technology China Academy of Space TechnologyBeijing100094China school of electronics and information engineering Harbin Institute of TechnologyHarbin150001China

This study focuses on the improvement of path planning efficiency for underwater gravity-aided navigation.Firstly,a Depth Sorting Fast Search(DSFS)algorithm was proposed to improve the planning speed of the Quick Rapidly-exploring Random Trees*(Q-RRT*)algorithm.A cost inequality relationship between an ancestor and its descendants was derived,and the ancestors were filtered accordingly.Secondly,the underwater gravity-aided navigation path planning system was designed based on the DSFS algorithm,taking into account the fitness,safety,and asymptotic optimality of the routes,according to the gravity suitability distribution of the navigation space.Finally,experimental comparisons of the computing performance of the ChooseParent procedure,the Rewire procedure,and the combination of the two procedures for Q-RRT*and DSFS were conducted under the same planning environment and parameter conditions,respectively.The results showed that the computational efficiency of the DSFS algorithm was improved by about 1.2 times compared with the Q-RRT*algorithm while ensuring correct computational results.

关键词： Depth Sorting Fast Search algorithm Underwater gravity-aided navigation Path planning efficiency Quick Rapidly-exploring Random Trees*(QRRT*)