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Revisiting aluminum current collector in lithium-ion batteries:Corrosion and countermeasures

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Journal of Energy Chemistry 2024年第2期89卷 610-634,I0014页

作者： Shanglin Yang Jinyan Zhong Songmei Li Bin Li Key Laboratory of Aerospace Advanced Materials and performance of Ministry of education School of Materials Science&EngineeringBeihang UniversityBeijing 100191China

With the large-scale service of lithium-ion batteries(LIBs),their failures have attracted significant *** the decay of active materials is the primary cause for LIB failures,the degradation of auxiliary materials,such as current collector corrosion,should not be ***,it is necessary to conduct a comprehensive review in this *** this review,from the perspectives of electrochemistry and materials,we systematically summarize the corrosion behavior of aluminum cathode current collector and propose corresponding ***,the corrosion type is clarified based on the properties of passivation layers in different organic electrolyte ***,a thoroughgoing analysis is presented to examine the impact of various factors on aluminum corrosion,including lithium salts,organic solvents,water impurities,and operating ***,strategies for electrolyte and protection layer employed to suppress corrosion are discussed in *** and most importantly,we provide insights and recommendations to prevent corrosion of current collectors,facilitate the development of advanced current collectors and the implementation of next-generation high-voltage stable LIBs.

关键词： Lithium-ion battery Aluminum current collector Corrosion Electrochemical performance Electrolyte Protective layer

2:17-type SmCo permanent magnets with controllable remanence temperature coefficients via substitution of heavy rare earth elements

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Rare Metals 2024年第8期43卷 3990-3996页

作者： Jia-Yi Huang Shu-Lan Zuo Qi Zhang Hong-Yang Dai Lei Yang Jing-Hua Liu Cheng-Bao Jiang Key Laboratory of Aerospace Materials and performance(Ministry of education) School of Materials Science and EngineeringBeihang UniversityBeijing 100191China

Permanent magnets that can maintain a constant magnetic flux over a wide temperature range are highly desirable in certain applications such as precision instruments.2:17-type SmCo permanent magnets are promising for such instruments owing to their excellent high-temperature magnetic properties that can be further manipulated byadding heavy rare earth elements (HREs).

关键词： magnets permanent earth

Formation and properties of a Zr-based amorphous coating by laser cladding

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Rare Metals 2024年第4期43卷 1809-1814页

作者： Ning Zhang Ying Liu Wei Yang Shu-Jie Pang Key Laboratory of Aerospace Materials and performance(Ministry of education) School of Materials Science and EngineeringBeihang UniversityBeijing100191China

(Zr_(0.53)Al_(0.1)Ni_(0.05)Cu_(0.3)Ti_(0.02))_(99)Y_1(at%)coating with amorphous layer of about 180μm thick was prepared on a steel substrate by using laser cladding *** coating is compact and shows good metallurgical bonding with *** microstructure,microhardness and corrosion behavior along the depth from the coating surface to the substrate were *** is found that a gradient structure consisted of amorphous surface layer,amorphous-crystalline transitional layer and substrate is formed after the laser *** microhardness and corrosion behavior exhibit variation with the microstructural evolution at different depths from the coating *** microhardness and corrosion resistance in 3.5 wt%NaCl solution of the amorphous surface layer are comparable to those of the as-cast Zr-based BMG with the same composition,and higher than those of the steel substrate.

关键词： Laser cladding Amorphous coating Microstructure Hardness Corrosion resistance

Particle size dependence of the microsegregation and microstructure in the atomized Ni-based superalloy powders:Theoretical and experimental study

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Journal of Materials Science & Technology 2024年第4期171卷 54-65页

作者： Jikang Li Mingsheng Yang Yunfei Cai Yuanyuan Zhang Qingshuai Feng Jiantao Liu Tong Liu Key Laboratory of Aerospace Materials and performance(Ministry of education)school of Materials Science and Engineering Beihang UniversityBeijing 100191China Central Iron and Steel Research Institute Beijing 100081China

The microstructure and microsegregation of atomized powder,which depend on their sizes,are of great importance to the mechanical properties of the consolidated bulk ***,it is necessary to reveal the relationship between particle size and powder *** effects of particle size on the so-lidification characterization of the atomized Ni-based superalloy powders were studied via finite element *** on the simulations,a model was developed to predict the microsegregation and mi-crostructure of atomized powders with different sizes and study the influence of thermal history on the powder attributes during the atomization *** radiation heat transfer and temperature gradi-ent within the rapid solidification alloy powders were taken into account in this *** validating the accuracy of the model,the predictions of the present model were compared with the microsegregation and microstructure of the specific size powder close to the screen mesh *** results showed that mi-crostructure depended primarily on the temperature gradient within the powder,while the solidification rate had a more significant effect on the *** model predicted microstructure features in agreement with the experiment,and for microsegregation,the deviations of prediction for most ele-ments were less than 10%.This work provides a new model to precisely predict the microsegregation and microstructure of the atomized alloy powders and sets a foundation to control the powder features for various engineering applications.

关键词： Particle size Solidification microstructure Microsegregation Numerical simulation

Considerations for exerkine research focusing on the response to exercise training

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Journal of Sport and Health Science 2024年第2期13卷 130-132页

作者： Ian A.J.Darragh Brendan Egan school of Health and human performance Dublin City UniversityGlasnevinDublin D09 V209Ireland Florida Institute for human and Machine Cognition PensacolaFL 32502USA

García-Hermoso and colleagues1 recently published a systematic literature review and meta-analysis on exercise training-induced changes in exerkine concentrations in type 2diabetes mellitus patients,providing a contemporary view on how exerkines respond to exercise *** review prompted us to highlight 2 additional considerations that should be taken into account when studying the response of exerkines to exercise ***,whether exerkines can exhibit discordant responses to acute exercise compared to exercise training,and secondly,the need to consider the residual effects of the most recent exercise bout.

关键词： acute exercise prompt

In situ formation of multiple catalysts for enhancing the hydrogen storage of MgH_(2) by adding porous Ni_(3)ZnC_(0.7)/Ni loaded carbon nanotubes microspheres

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Journal of Magnesium and Alloys 2024年第3期12卷 1227-1238页

作者： Bing Zhang Xiubo Xie Yukun Wang Chuanxin Hou Xueqin Sun Yuping Zhang Xiaoyang Yang Ronghai Yu Wei Du school of Environmental and Material Engineering Yantai UniversityNo.30 Qingquan RoadYantai 264005China Key Laboratory of Aerospace Materials and performance(Ministry of education)school of Materials Science and Engineering Beihang UniversityNo.37 Xueyuan RoadBeijing 100191China

MgH_(2) is considered one of the most promising hydrogen storage materials because of its safety,high efficiency,high hydrogen storage quantity and low cost *** some shortcomings are still existed:high operating temperature and poor hydrogen absorption dynamics,which limit its *** Ni_(3)ZnC_(0.7)/Ni loaded carbon nanotubes microspheres(NZC/Ni@CNT)is prepared by facile filtration and calcination *** the different amount of NZC/Ni@CNT(2.5,5.0 and 7.5 wt%)is added to the MgH_(2) by ball *** the three samples with different amount of NZC/Ni@CNT(2.5,5.0 and 7.5 wt%),the MgH_(2)-5 wt%NZC/Ni@CNT composite exhibits the best hydrogen storage *** testing,the MgH_(2)-5 wt%NZC/Ni@CNT begins to release hydrogen at around 110℃ and hydrogen absorption capacity reaches 2.34 wt%H_(2) at 80℃ within 60 ***,the composite can release about 5.36 wt%H_(2) at 300℃.In addition,hydrogen absorption and desorption activation energies of the MgH_(2)-5 wt%NZC/Ni@CNT composite are reduced to 37.28 and 84.22 KJ/mol H_(2),*** in situ generated Mg_(2)NiH_(4)/Mg_(2)Ni can serve as a"hydrogen pump"that plays the main role in providing more activation sites and hydrogen diffusion channels which promotes H_(2) dissociation during hydrogen absorption *** addition,the evenly dispersed Zn and MgZn2 in Mg and MgH_(2) could provide sites for Mg/MgH_(2) nucleation and hydrogen diffusion *** attempt clearly proved that the bimetallic carbide Ni_(3)ZnC_(0.7) is a effective additive for the hydrogen storage performances modification of MgH_(2),and the facile synthesis of the Ni_(3)ZnC_(0.7)/Ni@CNT can provide directions of better designing high performance carbide catalysts for improving MgH_(2).

关键词： Mg-based hydrogen storage material Ni_(3)ZnC_(0.7)/Ni@CNT particles Ni loaded carbon nanotubes Multiple catalysts.

Controllable CPL response driven by achiral UV-photosensitive dichroic dye through cholesteric liquid crystals

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Science China Chemistry 2024年第4期67卷 1250-1255页

作者： Yihan Chen Yang Li Hang Li Lulu Li Yiwu Quan Yixiang Cheng State Key Laboratory of Analytical Chemistry for Life Science School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Key Laboratory of High-performance Polymer Material and Technology of Ministry of education School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China school of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China

Versatile stimuli-responsive circularly polarized luminescent(CPL)materials have potential applications in information storage,security encryption,and intelligent *** this study,the Z/E isomerization of ultraviolet(UV)-photosensitive achiralα-cyanostilbene derivative was used as an achiral dichroic dye(Switch)to drive the controllable CPL-active response in cholesteric liquid crystals(CLCs).Under irradiation by 365 nm UV light,the resulting CLCs-Z-Switch underwent a Z-to-E configuration isomerization as CLCs-E-Switch,accompanied by a decrease in its dichroic order parameter(SFvalue)from 0.15to *** the quantum yield(QY)of CLCs-E-Switch increased from 8.1%(CLCs-Z-Switch)to 16.8%,the corresponding glumvalues of CPL emission decreased from+0.55/-0.57 to+0.37/-0.39 due to a decrease in the order of helical arrangement of E-Switch in E7 *** study enables photosensitive CLCs-Switch to be applied for optical information storage devices.

关键词： circularly polarized luminescent photosensitive dichroic dye cholesteric liquid crystals chiral induction

Biomimetic soft robotic wrist with 3-DOF motion and stiffness tunability based on ring-reinforced pneumatic actuators and a particle jamming joint

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Science China(Technological Sciences) 2024年第3期67卷 774-790页

作者： HU TeTe LU XinJiang YI Jian WANG YuHui XU Du State Key Laboratory of Precision Manufacturing for Extreme Service performance School of Mechanical and Electrical EngineeringCentral South UniversityChangsha 410083China

The human wrist, a complex articulation of skeletal muscles and two-carpal rows, substantially contributes to improvements in maneuverability by agilely performing three-degree-of-freedom(3-DOF) orienting tasks and regulating stiffness according to variations in interaction forces. However, few soft robotic wrists simultaneously demonstrate dexterous 3-DOF motion and variable stiffness;in addition, they do not fully consider a soft-rigid hybrid structure of integrated muscles and two carpal *** this study, we developed a soft-rigid hybrid structure to design a biomimetic soft robotic wrist(BSRW) that is capable of rotating in the x and y directions, twisting around the z-axis, and possessing stiffness-tunable capacity. To actuate the BSRW, a lightweight soft-ring-reinforced bellows-type pneumatic actuator(SRBPA) with large axial, linear deformation(η_(lcmax)=70.6%,η_(lemax)=54.3%) and small radial expansion(η_(demax)=3.7%) is designed to mimic the motion of skeletal muscles. To represent the function of two-carpal rows, a compact particle-jamming joint(PJJ) that combines particles with a membrane-covered ballsocket mechanism is developed to achieve various 3-DOF motions and high axial load-carrying capacity(>60 N). By varying the jamming pressure, the stiffness of the PJJ can be adjusted. Finally, a centrally positioned PJJ and six independently actuated SRBPAs, which are in an inclined and antagonistic arrangement, are sandwiched between two rigid plates to form a flexible,stable, and compact BSRW. Such a structure enables the BSRW to have a dexterous 3-DOF motion, high load-carrying ability,and stiffness tunability. Experimental analysis verify 3-DOF motion of BSRW, producing force of 29.6 N and 36 N and torque of2.2 Nm in corresponding rotations. Moreover, the range of rotational angle and stiffness-tuning properties of BSRW are studied by applying jamming pressure to the PJJ. Finally, a system combining a BSRW and a soft enclosing gripper is proposed to demo

关键词： pneumatic soft actuators particle jamming robotic wrist soft robotics stiffness-tunable

The anti-inflammatory effects of exercise on autoimmune diseases:A 20-year systematic review

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Journal of Sport and Health Science 2024年第3期13卷 353-367,I0001页

作者： Beibei Luo Dao Xiang Xiaorong Ji Xuan Chen Rui Li Shuxin Zhang Yujun Meng David C.Nieman Peijie Chen school of Exercise and Health Shanghai University of SportShanghai 200438China Shanghai Key Laboratory of human performance Shanghai University of SportShanghai 200438China Department of Diving and Hyperbaric Medicine Naval Medical CenterShanghai 200433China National Key Laboratory of Immunity and Inflammation Naval Medical UniversityShanghai 200433China human performance Laboratory Appalachian State UniversityNorth Carolina Research CampusKannapolisNC 28081USA Research Institute for Doping Control Shanghai University of SportShanghai 200438China

Background:The anti-inflammatory effect of exercise may be an underlying factor in improving several autoimmune *** aim of this systematic review was to examine the evidence on the role of exercise training in mitigating inflammation in adolescents and adults with autoimmune ***:PubMed,Web of Science,and Embase databases were systematically reviewed for related studies published between January 1,2003,and August 31,*** randomized and non-randomized controlled trials of exercise interventions with autoimmune disease study participants that evaluated inflammation-related biomarkers were *** quality of evidence was assessed using the Tool for the assEssment of Study qualiTy and reporting in EXercise scale and Cochrane bias risk ***:A total of 14,565 records were *** screening the titles,abstracts,and full texts,87 were eligible for the systematic *** studies were conducted in 25 different countries and included a total of 2779 participants(patients with autoimmune disease,in exercise or control groups).Overall,the evidence suggests that inflammation-related markers such as C-reactive protein,interleukin 6,and tumor necrosis factor a were reduced by regular exercise *** exercise interventions combined with multiple exercise modes were associated with greater ***:Regular exercise training by patients with autoimmune disease exerts an anti-inflammatory *** systematic review provides support for the promotion and development of clinical exercise intervention programs for patients with autoimmune *** patients with autoimmune disease can safely adopt moderate exercise training protocols,but changes in inflammation biomarkers will be modest at *** exercise interventions are ineffective or even modestly but transiently pro-inflammatory.

关键词： Autoimmune diseases Cytokines Inflammation Physical activity Training