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Fast thermal responsive separators toward long-life and safe lithium metal batteries

Nano Research 2024年第4期17卷 2746-2754页

作者： Pingan Li Zhifang Liu Yitong Peng Shanshan Yang Tao Meng Yunhuan Hu Yingjun Jiang Hao Sun Qi Li Xianluo Hu State Key laboratory of Materials Processing and Die and Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Lithium metal batteries(LMBs)have been extensively investigated during the past decades because of their ultrahigh energy *** the increasing demand for energy density,however,the safety issue of LMBs has become a significant *** particular,localized areas of increased temperature(namely,hotspots)may be induced and even exacerbated within LMBs by uneven current distribution,internal short circuits,or inadequate heat dissipation,which significantly sacrifices battery safety and cycle ***,we report the rational design and fabrication of a fast thermal responsive separator capable of inhibiting the growth of lithium dendrites and mitigating thermal propagation,thereby reducing the risk of thermal *** as-achieved separator comprises both an electrospun membrane using a phase change material with superior thermal-storage ability and a thermally conductive modification layer of hexagonal boron nitride nanosheets with a fast heat-transfer *** is demonstrated that such a unique integration of heat conduction and heat storage enables the functional separator with attractive abilities to mitigate hotspots and inhibit the growth of lithium dendrites upon the cycling of ***,pouch cells with the thermal-responsive separator,as well as numerical simulations,verify much enhanced safety and cycle life of *** work may offer a new conceptual design of intelligent separators that acts as a functional unit encapsulated within a single cell to boost in-situ thermal management,which will help to develop high-safety and energy-dense LMBs.

关键词： lithium metal batteries separators hotspots safety thermal management

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Coupled interactive effects of ammonia and hydrogen additions on ethylene diffusion flames: A detailed kinetic study

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science China(Technological sciences) 2024年第3期67卷 930-948页

作者： XIAO JiaYi XU TingTing SHU ZhiMei DENG QiGe ZHAO Xuan YING YaoYao LI TianJiao LIU Dong MIIT Key laboratory of Thermal Control of Electronic Equipment School of Energy and Power EngineeringNanjing University of Science and TechnologyNanjing 210094China Advanced Combustion laboratory School of Energy and Power EngineeringNanjing University of Science and TechnologyNanjing210094China

In order to create effective combustion technologies and fuels with low or no carbon emissions,the research was conducted to assess the coupled interactive effects of NH_(3) and H_(2) additions on ethylene counterflow diffusion flames from a kinetic *** effects of the NH_(3)/H_(2) combination on flame temperatures,major species,key radicals,important intermediate species,representative oxygenated species and NO_xwere *** results of the study utilizing fictitious inert NH_(3) and/or H_(2) revealed the chemical effects of the two *** was found that the NH_(3)/H_(2) coupled effects had a more effective inhibitory effect on soot precursors than the effects of corresponding sum of single NH_(3) or H_(2) *** production of soot precursors was promoted by the coupled chemical effects of NH_(3) and H_(2),but the coupled dilution and thermal effects were observed to have a greater impact,resulting in a decrease of the mole fractions of soot *** for the interaction of NH_(3) and H_(2) effects,the presence of H_(2) decreased the chemical effects of NH_(3) on the augmentation of C_(2)H_(2),A1,A2,and CH_(3)CHO mole *** NH_(3) addition alleviated the H_(2) chemical effects on increasing C_(2)H_(2),C_(3)H_(3),A1 and A2 ***,the NH_(3)chemical effects on C_(3)H_(3),OH and CH_(3)CHO were enhanced when H_(2) was *** presence of NH_(3) augmented the chemical effects of H_(2) on the growth of OH mole ***,the H_(2) chemical effects hindered the production of NO and NO_(2) in the presence of NH_(3).

关键词： NH_(3)/H_(2)addition kinetic analysis coupled interactive effects chemical effects

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Optimal and robust control of population transfer in asymmetric quantum-dot molecules

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Chinese Physics B 2024年第2期33卷 353-359页

作者：郭裕马松山束传存 Hunan Provincial Key laboratory of Flexible Electronic Materials Genome Engineering School of Physics and Electronic ScienceChangsha University of Science and TechnologyChangsha 410114China Hunan Key laboratory of Nanophotonics and Devices School of PhysicsCentral South UniversityChangsha 410083China

We present an optimal and robust quantum control method for efficient population transfer in asymmetric double quantum-dot *** derive a long-duration control scheme that allows for highly efficient population transfer by accurately controlling the amplitude of a narrow-bandwidth *** overcome fluctuations in control field parameters,we employ a frequency-domain quantum optimal control theory method to optimize the spectral phase of a single pulse with broad bandwidth while preserving the spectral *** is shown that this spectral-phase-only optimization approach can successfully identify robust and optimal control fields,leading to efficient population transfer to the target state while concurrently suppressing population transfer to undesired *** method demonstrates resilience to fluctuations in control field parameters,making it a promising approach for reliable and efficient population transfer in practical applications.

关键词： population transfer quantum optimal control theory quantum-dot molecules

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Enhancing electromagnetic wave absorption with core‐shell structured SiO_(2)@MXene@MoS_(2)nanospheres

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Carbon Energy 2024年第8期6卷 90-104页

作者： Xuewen Jiang Qian Wang Limeng Song Hongxia Lu Hongliang Xu Gang Shao Hailong Wang Rui Zhang Changan Wang Bingbing Fan school of Material science and Engineering Zhengzhou UniversityZhengzhouHenanChina Henan Key laboratory of Aeronautical Materials and Application Technology School of Material Science and EngineeringZhengzhou University of AeronauticsZhengzhouHenanChina school of Materials science and Engineering Tsinghua UniversityBeijingChina

Material composition and structural design are important factors influencing the electromagnetic wave(EMW)absorption performance of *** alleviate the impedance mismatch attributed to the high dielectric constant of Ti_(3)C_(2)T_(x)MXene,we have successfully synthesized core‐shell structured SiO_(2)@MXene@MoS_(2)*** architecture,comprising SiO_(2)as the core,MXene as the intermediate layer,and MoS_(2)as the outer shell,is achieved through an electrostatic self‐assembly method combined with a hydrothermal *** complex core‐shell structure not only provides a variety of loss mechanisms that effectively dissipate electromagnetic energy but also prevents self‐aggregation of MXene and MoS_(2)***,the synergistic combination of SiO_(2)and MoS_(2)with highly conductive MXene enables the suitable dielectric constant of the composites,ensuring optimal impedance ***,the core‐shell structured SiO_(2)@MXene@MoS_(2)nanospheres exhibit excellent EMW absorption performance,featuring a remarkable minimum reflection loss(RL_(min))of−52.11 dB(2.4 mm).It is noteworthy that these nanospheres achieve an ultra‐wide effective absorption bandwidth(EAB)of 6.72 *** work provides a novel approach for designing and synthesizing high‐performance EMW absorbers characterized by“wide bandwidth and strong reflection loss.”

关键词： core‐shell structure electromagnetic wave absorption multiloss mechanism SiO_(2)@MXene@MoS_(2)

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Forced boiling of nonazeotropic immiscible mixture in a supercapillary microchannel array for ultra-high heat flux removal with chip junction temperature below 85℃

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science China(Technological sciences) 2024年第5期67卷 1364-1380页

作者： SUN Bo BAO YuChen TIAN Tong LI Ji school of Engineering science University of Chinese Academy of SciencesBeijing100049China laboratory of Advanced Thermal Management Technologies School of Engineering ScienceUniversity of Chinese Academy of SciencesBeijing100049China

In this study,a structure-optimized two-phase microchannel heat sink with sintered submicron nucleation sites was developed and *** copper-based microchannels had a rectangular cross-section with an equivalent hydraulic diameter of 222μ*** subcooled flow boiling characteristics were comprehensively compared between pure HFE-7100 and a non-azeotropic,immiscible binary mixture of HFE-7100 and water,considering heating areas of 1 and 5 cm^(2).The total heating power input to the test section were 100–1500 and 250–3000 W for a 1 and 5 cm^(2)heat source,respectively,with a flow rate ranging from 50 to150 L/*** to pure HFE-7100,the non-azeotropic immiscible binary mixture of HFE-7100/water in the sintered porous microchannels exhibited a much higher overall heat transfer coefficient and lower power *** maintain the junction temperature of a high power electronic chip below 85℃,the proposed supercapillary microchannel heat sink could effectively dissipate the heat flux of 1275 W/cm^(2)over 1 cm^(2)heat source and 500 W/cm^(2)over 5 cm^(2)heat *** addition,the volume ratio of the binary mixture strongly influence the two-phase flow heat transfer *** optimal volume ratio exist in terms of the thermal resistance–pumping power minimization(HFE-7100:water=2:8 is recommended in this study).The findings of this investigation on the flow boiling properties of non-azeotropic immiscible mixtures help fill a gap in the related field.

关键词： microchannel sintered powder coating submicron nucleation cavities nonazeotropic immiscible ultra-high heat flux

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Deadline-Constrained and Cost-Effective Multi-Workflow Scheduling with Uncertainty in Cloud Control Systems

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Journal of Systems science & Complexity 2024年第5期37卷 1861-1886页

作者： YE Lingjuan YANG Liwen XIA Yuanqing ZHAN Yufeng ZHAO Xinchao school of science Beijing University of Posts and Telecommunications Key laboratory of Mathematics and Information Networks Beijing University of Posts and Telecommunications Ministry of Education school of Automation Nanjing University of Information Science and Technology school of Automation Beijing Institute of Technology

In cloud control systems, generating an efficient and economical workflow scheduling strategy for deadline-constrained workflow applications, especially in uncertain multi-workflow dynamic scheduling processes, is a crucial challenge. To optimize the total cost of workflow scheduling, the authors propose a cost-driven heuristic scheduling algorithm F-MWSA which consists of two phases:Fuzzy deadline distribution and fuzzy task scheduling. In the fuzzy deadline distribution phase, a new workflow deadline distribution strategy with fuzziness is designed to obtain the sub-deadline constraint of each task. The fuzzy task scheduling phase focuses on a cost-effective strategy to assign tasks to cloud resources, reducing multi-workflow scheduling costs. Performance evaluations on five real-world workflows demonstrate that the proposed F-MWSA outperforms the baseline policy in terms of total cost, success ratio, resource utilization, and makespan.

关键词： Cloud computing cost-effective deadline constraint multi-workflow scheduling uncertainty

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Effects of content and particle size of TiH2 powders on the energy output rules of RDX composite explosives

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Defence Technology（防务技术） 2024年第2期32卷 297-308页

作者： Hao Wang Yangfan Cheng Shoujun Zhu Zihan Li Zhaowu Shen school of Chemical Engineering Anhui University of Science and TechnologyHuainan 232001China Anhui Engineering laboratory of Explosive Materials and Technology Anhui University of Science and TechnologyHuainan 232001China school of Engineering science University of Science and Technology of ChinaHefei 230027China

In order to improve the detonation characteristics of RDX,a RDX-based composite explosive with TiH_(2)powders was *** effects of content and particle size of TiH_(2)powders on thermal safety,shock wave parameters and thermal damage effects of RDX-based composite explosive were studied with the C80 microcalorimeter,air blast experiment system and colorimetric thermometry *** results showed that TiH_(2)powders could enhance the thermal stability of RDX-based composite explosive and increase its ultimate decomposition *** content and particle size of TiH_(2)powders also had significant effects on the thermal safety,detonation velocity,shock wave parameters,fireball temperature and duration of RDX-based composite ***,the differences of TiH_(2)and Ti powders on the detonation energy output rules of RDX-based composite explosives were also compared,showing that TiH_(2)powders had better influences on improving the explosion power and thermal damage effect of RDX-based composite explosives than Ti powders,for the participation of free H_(2)released by TiH_(2)powders in the detonation ***_(2)powders have important research values as a novel energetic additive in the field of military composite explosives.

关键词： RDX Hydrogen storage alloy Air blast After-burn reaction Colorimetric thermometry

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Ultrafast micro/nano-manufacturing of metastable materials for energy

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National science Review 2024年第4期11卷 283-298页

作者： Xiaoya Cui Yanchang Liu Yanan Chen school of Materials science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology(Ministry of Education) and Tianjin Key Laboratory of Composite and Functional MaterialsTianjin University Ministry of Education Key laboratory of Protein sciences School of Life SciencesTsinghua University

The structural engineering of metastable nanomaterials with abundant defects has attracted much attention in energy-related fields. The high-temperature shock(HTS) technique, as a rapidly developing and advanced synthesis strategy, offers significant potential for the rational design and fabrication of high-quality nanocatalysts in an ultrafast, scalable, controllable and eco-friendly way. In this review, we provide an overview of various metastable micro-and nanomaterials synthesized via HTS, including single metallic and bimetallic nanostructures, high entropy alloys, metal compounds(e.g. metal oxides) and carbon nanomaterials. Note that HTS provides a new research dimension for nanostructures, i.e. kinetic modulation. Furthermore, we summarize the application of HTS—as supporting films for transmission electron microscopy grids—in the structural engineering of 2D materials, which is vital for the direct imaging of metastable materials. Finally, we discuss the potential future applications of high-throughput and liquid-phase HTS strategies for non-equilibrium micro/nano-manufacturing beyond energy-related *** is believed that this emerging research field will bring new opportunities to the development of nanoscience and nanotechnology in both fundamental and practical aspects.

关键词： high-temperature shock technique defect engineering metastable phase kinetic modulation non-equilibrium micro/nano-manufacturing

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A Distributed Self-Tallying Electronic Voting System Using the Smart Contract

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Chinese Journal of Electronics 2024年第4期33卷 1063-1076页

作者： Jingyu YAO Bo YANG Tao WANG Wenzheng ZHANG school of Computer science Shaanxi Normal University State Key laboratory of Integrated Services Networks Xidian University science and Technology on Communication Security laboratory

For electronic voting(e-voting) with a trusted authority, the ballots may be discarded or tampered, so it is attractive to eliminate the dependence on the trusted party. An e-voting protocol, where the final voting result can be calculated by any entity, is known as self-tallying e-voting protocol. To the best of our knowledge, addressing both abortive issue and adaptive issue simultaneously is still an open problem in self-tallying e-voting *** Ethereum blockchain with cryptographic technologies, we present a decentralized self-tallying e-voting protocol. We solve the above problem efficiently by utilizing optimized Group Encryption Scheme and standard Exponential El Gamal Cryptosystem. We use zero-knowledge proof and homomorphic encryption to protect votes' secrecy and achieve self-tallying. All ballots can be verified by anyone and the final voting result can be calculated by any entity. In addition, using the paradigm of score voting and “1-out-of-k” proof, our e-voting system is suitable for a wide range of application scenarios. Experiments show that our protocol is more competitive and more suitable for large-scale voting.

关键词： Electronic voting systems Smart contracts Blockchains Cryptocurrency Electronic voting Homomorphic encryption Standards

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Two sandwich-type uranyl-containing polytungstates catalyze aerobic synthesis of benzimidazoles

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Rare Metals 2024年第3期43卷 1316-1322页

作者： Yu-Feng Liu Qi-Long Hu Xue-Jiao Chen Ke Li Pei Luo Guo-Ping Yang school of Chemistry and Material science Jiangxi Province Key Laboratory of Synthetic ChemistryJiangxi Key Laboratory for Mass Spectrometry and InstrumentationEast China University of TechnologyNanchang330013China school of Environmental science and Engineering Southern University of Science and TechnologyShenzhen518055China

Diversified synthetic strategies are extremely important for the structural diversity of uranium-containing polyoxometalates(U-POMs)and their functional ***,two sandwich-type U-POMs were reported,which are Na_(5.6)K_(6.4)[(UO_(2))(H_(2)O)(TeW_(9)O_(33))]_(2)·21H_(2)O(UTeW_(9))and Na_(8.9)K_(2.7)H_(1.19)[K_(0.79)(UO_(2))_(2.21)(PW_(9)O_(34))_(2)]·12H_(2)O(UPW_9)using in-situ strategy and lacunary precursor strategy,***_9 shows a typical Keggin-typeopen or half-sandwich configuration.

关键词： configuration expansion sandwich

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