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Interactions of phenol and benzaldehyde in electrocatalytic upgrading process

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Chinese Chemical Letters 2024年第2期35卷 464-468页

作者： Lan Liang Chuanbin Wang Xukai Lu Yunan Sun Beibei Yan Ning Li Guanyi Chen Li'an Hou school of Environmental Science and engineering Tianjin Key Lab of Biomass/Wastes UtilizationTianjin UniversityTianjin 300350China school of Mechanical engineering Tianjin University of CommerceTianjin 300134China Georgia Tech Shenzhen institute Tianjin UniversityShenzhen 518071China High Tech Inst Beijing Beijing 100085China

Biomass pyrolysis oil can be improved effectively by electrocatalytic hydrogenation(ECH).However,the unclear interactions among different components lead to low bio-oil upgrading efficiency in the conversion ***,benzaldehyde and phenol,as common compounds in bio-oil,were chosen as model *** interactions between the two components were explored in the ECH process by combining experiments and theoretical *** showed that phenol could accelerate the conversion of benzaldehyde in the *** selectivity of benzyl alcohol was increased from 60.9%of unadded phenol to 99.1%with 30 mmol/L phenol concentration at 5 *** inhibited the ECH of *** the presence of benzaldehyde,the conversion rate of phenol was below 10.0%with no cyclohexanone and cyclohexanol formation at 5 *** density functional theory(DFT)calculations revealed that the phenol could promote the adsorption of benzaldehyde and facilitate the targeted conversion of benzaldehyde on the active site by lowering the reaction energy *** research on the interaction between phenol and benzaldehyde in the ECH provides a theoretical basis for the application of ECH in practical bio-oil upgrading.

关键词： Interaction Bio-oil Electrocatalytic hydrogenation Phenol Benzaldehyde

A perspective to ammonia-hydrogen energy industry in China

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Science China Chemistry 2024年第6期67卷 1765-1775页

作者： Baoshun Zhang Wangyang Ji Jiewei Zhu Baian Shen Menghao Lv Bin Zhang Tihu Wang Yifu Yu Department of Chemistry Institute of Molecular PlusSchool of ScienceTianjin UniversityTianjin300072China tianjin University-Asia Silicon Joint Research Center of Ammonia-Hydrogen New Energy Asia Silicon(Qinghai)Co.Ltd.Xining810007China Department of Catalysis Science and engineering School of Chemical Engineering and TechnologyTianjin UniversityTianjin300072China

1 *** meet the 1.5℃ climate goal in our planet,the world is making a hard work for decarbonization[1-5].Constructing a clean energy system based on green energy is considered as the most promising way to achieve the ... 详细信息

关键词： ammonia planet energy

Nacre-inspired MXene-based film for highly sensitive piezoresistive sensing over a broad sensing range

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Bio-Design and Manufacturing 2024年第4期7卷 463-475页

作者： Gaofeng Wang Lingxian Meng Xinyi Ji Xuying Liu Jiajie Liang Shuiren Liu school of Materials Science and engineering Zhengzhou UniversityZhengzhou 450001China school of Materials Science and engineering National Institute for Advanced MaterialsNankai UniversityTianjin 300350China

As the main component of wearable electronic equipment,flexible pressure sensors have attracted wide attention due to their excellent sensitivity and their promise with respect to applications in health monitoring,electronic skin,and human-computer ***,it remains a significant challenge to achieve epidermal sensing over a wide sensing range,with short response/recovery time and featuring seamless conformability to the skin *** is critical since the capture of minute electrophysiological signals is important for health care *** this paper,we report the preparation of a nacre-like MXene/sodium carboxymethyl cellulose(CMC)nanocomposite film with a“brick-and-mortar”interior structure using a vacuum-induced self-assembly *** synergistic behavior of the MXene“brick”and flexible CMC“mortar”contributes to attenuating interlamellar self-stacking and creates numerous variable conductive pathways on the sensing *** resulted in a high sensitivity over a broad pressure range(i.e.,0.03-22.37 kPa:162.13 kPa^(-1);22.37-135.71 kPa:127.88 kPa^(-1);135.71-286.49 kPa:100.58 kPa^(-1)).This sensor also has a low detection limit(0.85 Pa),short response/recovery time(8.58 ms/34.34 ms),and good stability(2000 cycles).Furthermore,we deployed pressure sensors to distinguish among tiny particles,various physiological signals of the human body,space arrays,robot motion monitoring,and other related applications to demonstrate their feasibility for a variety of health and motion monitoring use cases.

关键词： Flexible pressure sensor MXene Bioinspired Physiological signals Interlayer spacing

Energy budget of cold and hot gas-solid fluidized beds through CFD-DEM simulations

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Particuology 2024年第6期89卷 153-171页

作者： Lei Bi Yunpeng Jiao Chunjiang Liu Jianhua Chen Wei Ge school of Chemical engineering and Technology Tianjin UniversityTianjin 300072China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing100190China school of Chemical engineering University of Chinese Academy of SciencesBeijing 100049China

Direct energy budget is carried out for both cold and hot flow in gas–solid fluidization ***,the energy paths are proposed from thermodynamic *** consumption means total power input to the specific system,and it can be decomposed into energy retention and energy *** retention is the variation of accumulated mechanical energy in the system,and energy dissipation is the energy converted to heat by irreversible *** based on the Computational Fluid Dynamics-Discrete Element Method(CFD-DEM)framework,different energy terms are quantified from the specific flow elements of fluid cells and particles as well as their interactions with the *** order to clarify the energy budget,it is important to identify which system is studied:the particle-fluid system or the particle *** the cold flow,the total energy consumption of the particle sub-system can well indicate the onset of bubbling and turbulent,while the variation of local energy consumption terms can reflect the evolution of heterogeneous *** the hot flow,different heat transfer mechanisms are analyzed and the solver is modified to reproduce the experimental *** impact of the heat transfer mechanisms and heat production on energy consumption is also *** proposed budget method has proven to be energy-conservative and easy to conduct,and it is hopeful to be applied to other multiphase flow systems.

关键词： Energy budget Gas-solid fluidization CFD-DEM Regime transition Heat transfer mechanism

Regulatable Orthotropic 3D Hybrid Continuous Carbon Networks for Efficient Bi-Directional Thermal Conduction

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Nano-Micro Letters 2024年第10期16卷 136-148页

作者： Huitao Yu Lianqiang Peng Can Chen Mengmeng Qin Wei Feng school of Materials Science and engineering Tianjin Key Laboratory of Composite and Functional MaterialsTianjin UniversityTianjin 300350People's Republic of China

Vertically oriented carbon structures constructed from low-dimen-sional carbon materials are ideal frameworks for high-performance thermal inter-face materials(TIMs).However,improving the interfacial heat-transfer efficiency of vertically oriented carbon structures is a challenging ***,an orthotropic three-dimensional(3D)hybrid carbon network(VSCG)is fabricated by depositing vertically aligned carbon nanotubes(VACNTs)on the surface of a horizontally oriented graphene film(HOGF).The interfacial interaction between the VACNTs and HOGF is then optimized through an annealing *** regulating the orientation structure of the VACNTs and filling the VSCG with polydimethylsi-loxane(PDMS),VSCG/PDMS composites with excellent 3D thermal conductive properties are *** highest in-plane and through-plane thermal conduc-tivities of the composites are 113.61 and 24.37 W m^(-1)K^(-1),*** high contact area of HOGF and good compressibility of VACNTs imbue the VSCG/PDMS composite with low thermal *** addition,the interfacial heat-transfer efficiency of VSCG/PDMS composite in the TIM performance was improved by 71.3%compared to that of a state-of-the-art thermal *** new structural design can potentially realize high-performance TIMs that meet the need for high thermal conductivity and low contact thermal resistance in interfacial heat-transfer processes.

关键词： Orthotropic continuous structures Hybrid carbon networks Carbon/polymer composites Thermal interface materials

Improvement of maximum power point tracking in photovoltaic arrays in different environments using hybrid algorithms

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Optoelectronics Letters 2024年第1期20卷 28-34页

作者： ZHANG Jiuchao REN Guangjun XUE Yuming XIA Dan WANG Jiangchao HU Zhaoshuo institute of New Energy Intelligence Equipment School of Integrated Circuit Science and EngineeringTianjin University of TechnologyTianjin 300384China

When the photovoltaic(PV)system is generating PV power,the partial shading(PS)condition will cause multiple peaks in the power-voltage curve,and changes in light intensity and ambient temperature will cause the curve to *** maximum power point tracking(MPPT)methods,such as the incremental conductance(INC)method,have the problem of being trapped in the local optimal *** optimization algorithms,such as particle swarm optimization(PSO),have problems with oscillation and low tracking efficiency near the global maximum power point(GMPP).As a result,a hybrid algorithm CS-INC based on the cuckoo search(CS)algorithm and the perturb and observe(P&O)approach is proposed in this *** light intensity remains constant,the light intensity changes in steps,and the partial shade scenario are *** results show that the MPPT improves accuracy,speed,and stability.

关键词： power maximum optimization

Tuning the band gap of the CIGS solar buffer layer Cd_(1-x)Zn_(x)S(x=0—1) to achieve high efficiency

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Optoelectronics Letters 2024年第2期20卷 100-106页

作者： TAN Zhiyuan XUE Yuming DAI Hongli WANG Luoxin HU Xiaofeng BAI Xin institute of New Energy Intelligence Equipment School of Integrated Circuit Science and EngineeringTianjin University of TechnologyTianjin 300384China

To evaluate the impact of zinc sulfate(ZnSO_(4)) concentration on the structural properties of the films,Cd_(1-x)Zn_(x)S thin films were formed on glass substrates using chemical bath deposition(CBD) in this *** effect of ZnSO_(4) precursor concentration on the surface morphology,optical properties,and morphological structure of the Cd_(1-x)Zn_(x)S films was *** study the impact of zinc doping content on the performance metrics of Cu(In_(1-x)Ga_(x))Se_(2)(CIGS)cells in the experimental group and to improve the buffer layer thickness,simulations were run using one-dimensional solar cell capacitance simulator(SCAPS-1D) software.

关键词： CIGS (x) layer

Theoretical study on the stability of nanobubbles and its verification in molecular dynamics simulation

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Particuology 2024年第4期87卷 99-105页

作者： Sheng Mi Chaofeng Hou Wei Ge school of Chemical engineering and Technology Tianjin UniversityTianjin300072China State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing.100190China school of Chemical engineering University of Chinese Academy of SciencesBeijing100049China

The stability of vapor nanobubbles in bulk liquid was investigated theoretically and the critical bubble size was derived from macroscale thermodynamic equations,below which the system destabilizes with sharp drop in *** critical size was quantitatively verified in molecular dynamic simulation using the Lennard-Jones model of argon,where stronger attraction between the molecules at lower density is found to contribute most to the drop of system pressure and,as the Laplace pressure on the curved bubble interface fails to balance the pressure difference across the interface,the bubbles become *** theoretical model could be extended to other systems where reliable equations of state and interfacial tension are available.

关键词： Nanobubble Stability Phase diagram Critical size

Swimmer with submerged SiO_(2)/Al/LiNbO_(3) surface acoustic wave propulsion system

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Biomimetic Intelligence & Robotics 2024年第2期4卷 71-77页

作者： Deqing Kong Ryo Tanimura Fang Wang Kailiang Zhang Minoru Kuribayashi Kurosawa Manabu Aoyagi Department of engineering Muroran Institute of TechnologyMuroran 050-8585Japan tianjin Key Laboratory of Film Electronic and Communication Devices School of Integrated Circuit Science and EngineeringTianjin University of TechnologyTianjin 300384China school of engineering Tokyo Institute of TechnologyYokohama 226-8501Japan

Acoustic propulsion system presents a novel underwater propulsion approach in small scale *** study introduces a submerged surface acoustic wave(SAW)propulsion system based on the SiO_(2)/Al/LiNbO_(3) *** 19.25 MHz,the SAW propulsion system is proposed and investigated by the propulsion force calculation,PIV measurements and propulsion measurements.3.3 mN propulsion force is measured at 27.6 V_(pp).To evaluate the miniature swimmer,the SAW propulsion systems with multiple frequencies are *** 2.2 W,the submerged SAW propulsion system at 38.45 MHz demonstrates 0.83 mN/mm^(2) propulsion *** 96.13 MHz and 24 V_(pp),the movements of miniature swimmer with a fully submerged SAW propulsion system are recorded and analyzed to a maximum of 177 mm/*** of miniaturization,high power density,and simple structure,the SAW propulsion system can be expected for some microrobot applications,such as underwater drone,pipelinerobotand intravascularrobot.

关键词： Acoustofluidics Surface acoustic wave Swimmer Underwater propulsion system