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Corrugated Graphene Paper Reinforced Silicone Resin Composite for Efficient Interface Thermal Management

Chinese Journal of Polymer Science 2024年第7期42卷 1002-1014,I0010页

作者： Bo-Wen Wang Heng Zhang Qing-Xia He Hui-Tao Yu Meng-Meng Qin Wei Feng tianjin Key Laboratory of Composite and Functional Materials School of Materials Science and EngineeringTianjin UniversityTianjin300350China International engineering institute Tianjin UniversityTianjin300350China

With the rapid development of high-power-density electronic devices,interface thermal resistance has become a critical barrier for effective heat management in high-performance electronic ***,there is an urgent demand for advanced thermal interface materials(TIMs)with high cross-plane thermal conductivity and excellent compressibility to withstand increasingly complex operating *** achieve this aim,a promising strategy involves vertically arranging highly thermoconductive graphene on ***,with the currently available methods,achieving a balance between low interfacial thermal resistance,bidirectional high thermal conductivity,and large-scale production is ***,we prepared a graphene framework with continuous filler structures in in-plane and cross-plane directions by bonding corrugated graphene to planar graphene *** interface interaction between the graphene paper framework and polymer matrix was enhanced via surface functionalization to reduce the interface thermal *** resulting three-dimensional thermal framework endows the polymer composite material with a cross-plane thermal conductivity of 14.4 W·m^(-1)·K^(-1)and in-plane thermal conductivity of 130W·m^(-1)·K^(-1)when the thermal filler loading is 10.1 wt%,with a thermal conductivity enhancement per 1 wt%filler loading of 831%,outperforming various graphene structures as *** its high thermal conductivity,low contact thermal resistance,and low compressive modulus,the developed highly thermoconductive composite material demonstrates superior performance in TIM testing compared with TFLEX-700,an advanced commercial TIM,effectively solving the interfacial heat transfer issues in electronic *** novel filler structure framework also provides a solution for achieving a balance between efficient thermal management and ease of processing.

关键词： Graphene paper Vertically aligned structure Cross-plane thermal conductivity Low compressive modulus Thermal interface material

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Nanocavity enriched CuPd alloy with high selectivity for CO_(2) electroreduction toward C_(2)H_(4)

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Rare Metals 2024年第4期43卷 1513-1523页

作者： Ze-Yu Zhang Hai-Bin Wang Fei-Fei Zhang Jing-Wei Li Xin-Zhuo Hu Si-Wei Yan Yi-Ming Bai Xun Zhang Gu-Rong Shen Peng-Fei Yin Jing Yang Cun-Ku Dong Jing Mao Hui Liu Xi-Wen Du institute of New-Energy Materials School of Materials Science and EngineeringTianjin UniversityTianjin300350China

Electrocatalysis of CO_(2)reduction reaction is an effective way to convert CO_(2)into high value-added products,but the selectivity of Cu-based catalysts for C2+products needs to be improved due to the high energy barrier of C-C ***,a viable catalyst design strategy to decrease energy barrier of C-C coupling should be put ***,a nanocavity-enriched CuPd single atom alloy(CuPd SAA)catalyst is designed to promote CC coupling *** faradaic efficiency of CuPd SAA for ethylene and C_(2+)reaches 75.6%and 85.7%at-0.7 V versus reversible hydrogen electrode(RHE),*** on the results given by in situ characterization,the porous hollow structure dramatically increases the ratio of the linear-bond*CO,thus enhancing the faradaic efficiency for *** functional theory(DFT)calculation reveals that the Pd doping can regulate the electronic structure of neighboring Cu atoms to decrease the energy barrier of C-C coupling,further improving the faradaic *** work provides a new idea for designing catalyst with high selectivity for ethylene.

关键词： Adsorption configuration C-C coupling CO_(2) electrocatalysis Ethylene Single atom alloy

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Investigation of Ce/BEA as a passive NO_(x)adsorber:*** occurrences of cerium and adsorption behavior

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Journal of Rare Earths 2024年第7期42卷 1265-1271,I0003页

作者： Minghui Yu Yiying Ding Xiaojie Yu Siwei Yan Meiqing Shen Jianqiang Wang Jun Wang Gurong Shen school of Materials Science and engineering Tianjin UniversityTianjin300350China school of Chemical engineering and Technology Tianjin UniversityTianjin300350China National Rare Earth Catalysis Research institute Dongying257000China

Ce/BEA has great potential as a passive NO_(x)absorber(PNA)to reduce the NO_(x)emissions during the cold start phase especially in diesel engine for its high resistance to CO and suitable NO_(x)desorption temperature ***,as a novel material,its physical and chemical properties still remain *** this work,Ce/BEA was synthesized by ion-exchange method to identify the active species in NO_(x)adsorption,compared with aggregated Ce species in Ce/SiAlO_(x) prepared by impregnation method.X-ray diffraction(XRD),high resolution-transmission electron microscopy(HR-TEM)and aberration-corrected-scanning transmission electron microscopy(AC-STEM)were performed to confirm the isolated single atom formation of Ce species in Ce/***-vis diffraction reflection spectra(DRS)and X-ray photoelectron spectroscopy(XPS)were conducted to find the difference of chemical environment between the isolated Ce species and aggregated *** performance evaluation and temperature programmed reduction of hydrogen(H_(2)-TPR)results show the high NO_(x)storage capacity and active oxygen species quantity in Ce/*** is also found that the main NO_(x)adsorption species are Ce^(4+)-O^(∗)rather than Ce^(3+).NO_(x)-diffuse reflectance infrared Fourier transform spectroscopy(NO_(x)-DRIFTS)confirms that the bidentate nitrite species are the critical NO_(x)adsorption intermediates and the conception of NO_(x)adsorption and desorption processes is proposed.

关键词： Passive NO_(x)absorber Ce/BEA Isolated Ce species Rare earths

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Investigation of Ce/BEA as a passive NO_(x)adsorber:*** aging deactivation mechanism

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Journal of Rare Earths 2024年第8期42卷 1524-1530,I0004页

作者： Yiying Ding Minghui Yu Xiaojie Yu Meiqing Shen Jianqiang Wang Jun Wang Gurong Shen school of Chemical engineering and Technology Tianjin UniversityTianjin300350China school of Materials Science and engineering Tianjin UniversityTianjin300350China National Rare Earth Catalysis Research institute Dongying257000China

Ce/BEA has the potential to be applied as a novel passive NO_(x)absorber(PNA)in the after-treatment of vehicles due to its considerable NO_(x)storage ***,as a vehicle exhaust after-treatment material,it must withstand the test of long-term hydrothermal *** work examined the deactivation mechanism of Ce/BEA during hydrothermal aging.3.0 wt%Ce/BEA was prepared using the ionexchange method,and then subjected to hydrothermal treatment at 650℃with 10%H_(2)O for 1-12 h to obtain samples with different aging *** comparison,the H-BEA support was aged under the same ***-Emmett-Teller(BET)method,X-ray diffraction(XRD),NH_(3)temperature programmed reduction(NH_(3)-TPD),^(27)Al MAS nuclear magnetic resonance(^(27)Al MAS NMR),H_(2)temperature programmed reduction(H_(2)-TPR),and high resolution-transmission electron microscopy(HR-TEM)were performed to characterize the changes in PNA performance,structure,Ce species,and *** HR-TEM and H_(2)-TPR results show that CeO_(x)particles appear after hydrothermal aging,which results from the detachment and aggregation of active Ce *** on the^(27)Al MAS NMR results,we conclude that BEA zeolite dealumination leads to the loss of acidic sites and the transformation of active Ce species on the acidic sites into the less active CeO_(x).This is the primary reason for the hydrothermal aging deactivation of Ce/BEA.

关键词： Passive NO_(x)adsorber Ce/BEA Hydrothermal aging CeO_(x) Dealumination Rare earths

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Edge dislocation-induced strains break the limit of PtNi alloys in boosting Pt mass activity for efficient alkaline hydrogen evolution

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Nano Research 2024年第6期17卷 4711-4719页

作者： Miao Zhou Yao Zhao Zhanwei Liu Xueru Zhao Enzuo Liu Liyang Xiao Pengfei Yin Cunku Dong Hui Liu Xiwen Du Jing Yang New Energy Materials institute School of Materials Science and EngineeringTianjin UniversityTianjin 300072China school of Aerospace engineering Beijing Institute of TechnologyBeijing 100081China Chemistry Division Brookhaven National LaboratoryUptonNew York 11973USA Advanced Metallic Materials institute School of Materials Science and EngineeringTianjin UniversityTianjin 300072China

Creating lattice defects and alloying to produce strain effect in Pt-based bimetallic alloys are both effective methods to optimize the crystal and electronic structure and improve the electrocatalytic ***,the principles that govern the alkaline hydrogen evolution reaction(HER)performance remain unclear,which is detrimental to the rational design of efficient Pt-based ***,PtNi alloys with different Pt/Ni ratios and edge dislocations were synthesized,and the effects of Pt/Ni composition and edge dislocations on the alkaline HER electrocatalytic activity of PtNi alloys were systematically *** experimental and theoretical investigations reveal that tuning Pt/Ni ratio results in only 1.1 times enhancements in Pt mass activity,whereas edge dislocations-induced extra tensile strain on Ni site and compressive strain on Pt site further boost the alkaline HER intrinsic activity at all Pt/Ni ***,the introduction of edge dislocations in PtNi alloys could break the limit of alloying in boosting Pt mass activity and result in up to 13.7-fold enhancement,in the case that Pt and Ni contents are nearly identical and thus edge dislocation density reaches the *** mechanism studies demonstrate that the edge dislocation strategy could make a breakthrough in facilitating water dissociation kinetics of PtNi alloys.

关键词： edge dislocations PtNi composition strain effects water dissociation hydrogen evolution reaction

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Digital Twin Modeling Enabled Machine Tool Intelligence:A Review

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Chinese Journal of Mechanical engineering 2024年第2期37卷 29-54页

作者： Lei Zhang Jianhua Liu Cunbo Zhuang school of Mechanical engineering Tianjin University of CommerceTianjin 300134China Laboratory of Digital Manufacturing School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 10081China

Machine tools,often referred to as the“mother machines”of the manufacturing industry,are crucial in developing smart manufacturing and are increasingly becoming more *** twin technology can promote machine tool intelligence and has attracted considerable research ***,there is a lack of clear and systematic analyses on how the digital twin technology enables machine tool ***,digital twin modeling was identified as an enabling technology for machine tool intelligence based on a comparative study of the characteristics of machine tool intelligence and digital *** review then delves into state-of-the-art digital twin modelingenabled machine tool intelligence,examining it from the aspects of data-based modeling and mechanism-data dual-driven ***,it highlights three bottleneck issues facing the *** these problems,the architecture of a digital twin machine tool(DTMT)is proposed,and three key technologies are expounded in detail:Data perception and fusion technology,mechanism-data-knowledge hybrid-driven digital twin modeling and virtual-real synchronization technology,and dynamic optimization and collaborative control technology for multilevel ***,future research directions for the DTMT are *** work can provide a foundation basis for the research and implementation of digital-twin modeling-enabled machine tool intelligence,making it significant for developing intelligent machine tools.

关键词： Machine tool Digital twin Smart manufacturing Synchronization

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Parking choice behaviour analysis of rural residents based on the latent variable random forest model

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Transportation Safety and Environment 2024年第3期6卷 167-180页

作者： Minqing Zhu Bo Zhao Hongjun Cui Sheng Yao Feng Xu school of Architecture and art Design Hebei University of TechnologyTianjin 300130China school of Civil and Transportation engineering Hebei University of TechnologyTianjin 300401China

The imbalance of rural parking supply and demand has a great impact on traffic congestion and environmental pollution,which has attracted the attention of many scholars as well as ***,most of the current research on parking choice focuses on urban business and residential areas rather than on rural parking choice behaviour,and focuses on the analysis of observable factors,ignoring the internal relationship with potential *** study considers the heterogeneity of individuals and uses the random forest(RF)algorithm to construct a model of rural residents’willingness to choose parking with both latent and explicit variables,to explore how much and in what ways individual characteristics and parking characteristics affect rural residents’parking choices,and to explore parking planning programmes and strategies that are truly applicable to rural *** results of the study suggest that the safety and convenience of the parking environment are key factors influencing the parking choice behaviour of rural residents,and can greatly improve the predictive accuracy of the parking willingness *** comparison,it is found that the application of the RF algorithm is also significantly better than the logit model in terms of prediction effect,indicating that there is a nonlinear effect among the factors influencing the parking choice behaviour of rural residents and that the RF model with the addition of latent variables provides a better explanatory ability for the study of the parking choice behaviour of rural residents.

关键词： rural residents parking choice random forest(RF) latent variable SEM-RF model

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Reconfigurable mechanism-based metamaterials for ternary-coded elastic wave polarizers and programmable refraction control

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Applied Mathematics and Mechanics(English Edition) 2024年第7期45卷 1225-1242页

作者： Zhou HU Zhibo WEI Yan CHEN Rui ZHU school of Aerospace engineering Beijing Institute of TechnologyBeijing100081China school of Mechanical engineering Tianjin UniversityTianjin300350China Key Laboratory of Mechanism Theory and Equipment Design of Ministry of Education Tianjin UniversityTianjin300350China

Elastic metamaterials with unusual elastic properties offer unprecedented ways to modulate the polarization and propagation of elastic ***,most of them rely on the resonant structural components,and thus are frequency-dependent and ***,we present a reconfigurable 2D mechanism-based metamaterial which possesses transformable and frequency-independent elastic *** on the proposed mechanism-based metamaterial,interesting functionalities,such as ternarycoded elastic wave polarizer and programmable refraction,are ***,unique ternary-coded polarizers,with 1-trit polarization filtering and 2-trit polarization separating of longitudinal and transverse waves,are first ***,the strong anisotropy of the proposed metamaterial is harnessed to realize positive-negative bi-refraction,only-positive refraction,and only-negative ***,the wave functions with detailed microstructures are numerically verified.

关键词： elastic metamaterial elastic wave reconfigurable design zero mode ternary code programmable refraction

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Editable semiconductor photo-electrodes for sustainable ammonia synthesis

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Nano Research 2024年第4期17卷 3107-3112页

作者： Ning Lan Kun Du Erling Zhao Wei Zhao Tao Ling Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of Education Institute of New-EnergySchool of Materials Science and EngineeringTianjin UniversityTianjin 300072China school of Materials Science and engineering Tianjin Chengjian UniversityTianjin 300384China

Powered by an inexhaustible supply of solar energy,photoelectrochemical(PEC)nitrogen reduction reaction(NRR)provides an ideal solution for the synthesis of green ammonia(NH_(3)).Although great efforts have been made in the past decades,there are still significant challenges in increasing the NH_(3) yields of the PEC-NRR *** addition to the issues of low activity and selectivity similar to electrochemical NRR,the progress of PEC-NRR is also impeded by the limited increase in NH_(3) yields as the electrode is ***,we propose an editable electrode design strategy that parallels unit photo-electrodes to achieve a linear increase in NH_(3) yields with electrode active *** demonstrate that the editable electrode design strategy minimizes the electrode charge transfer resistance,allowing more photo-generated carriers to reach the electrode surface and promote the catalytic *** believe that this editable electrode design strategy provides an avenue to achieve sustainable PEC NH_(3) production.

关键词： editable electrode photoelectrochemical nitrogen reduction reaction parallel electrode ZnSe

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Influence of Incomplete Soil Plugs on Bearing Capacities of Bucket Foundations in Clay

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China Ocean engineering 2024年第1期38卷 144-155页

作者： LI Hui-shan LIU Run YANG Xu LIAN Ji-jian State Key Laboratory of Hydraulic engineering Intelligent Construction and Operation Tianjin UniversityTianjin 300072China school of Civil engineering Tianjin UniversityTianjin 300072China institute of Marine Energy and Intelligent Construction Tianjin University of TechnologyTianjin 300384China

Due to the uneven seabed and heaving of soil during pumping,incomplete soil plugs may occur during the installation of bucket foundations,and the impacts on the bearing capacities of bucket foundations need to be *** this paper,the contact ratio(the ratio of the top diameter of the soil plug to the diameter of the bucket)and the soil plug ratio(the ratio of the soil heave height to the skirt height)are defined to describe the shape and size of the incomplete soil ***,finite element models are established to investigate the bearing capacities of bucket foundations with incomplete soil plugs and the influences of the contact ratios,and the soil plug ratios on the bearing capacities are *** results show that the vertical bearing capacity of bucket foundations in homogeneous soil continuously improves with the increase of the contact ***,in normally consolidated soil,the vertical bearing capacity barely changes when the contact ratio is smaller than 0.75,while the bearing capacity suddenly increases when the contact ratio increases to 1 due to the change of failure *** contact ratio hardly affects the horizontal bearing capacity of bucket ***,the moment bearing capacity improves with the increase of the contact ratio for small aspect ratios,but hardly varies with increasing contact ratio for aspect ratios larger than ***,the reduction coefficient method is proposed based on this analysis to calculate the bearing capacities of bucket foundations considering the influence of incomplete soil *** comparison results show that the proposed reduction coefficient method can be used to evaluate the influences of incomplete soil plug on the bearing capacities of bucket foundations.

关键词： bucket foundation incomplete soil plug uniaxial bearing capacity contact ratio soil plug ratio

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