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Journal of environmental Sciences 2024年第1期135卷 274-284页

作者： Zewen Wu Luan Zhang Hao Lin Shungui Zhou Fujian Provincial Key Laboratory of Soil environmental Health and Regulation College of Resources and EnvironmentFujian Agriculture and Forestry UniversityFuzhou 350002China school of environmental Science and Engineering Hubei Key Laboratory of Mine Environmental Pollution Control and RemediationHubei Polytechnic UniversityHuangshi 435003China Fujian Provincial Key Laboratory of Eco-Industrial Green Technology Wuyi UniversityWuyishan 354300China

This study explored the combined effects of Bacillus subtilis inoculation with biochar on the evolution of bacterial communities,antibiotic resistance genes(ARGs),and mobile genetic elements(MGEs)during the composting of chicken *** results showed that *** inoculation combined with biochar increased bacterial abundance and diversity as well as prolonged the compost thermophilic *** organic matter biodegradation and facilitated the organic waste compost humification process,reduced the proliferation of ARGs by altering the bacterial *** and Actinobacteriota were the main resistant bacteria related to ARGs and *** decrease in ARGs and MGEs was associated with the reduction in the abundance of related host *** inoculation with *** and the addition of biochar could promote nutrient transformation,reduce the increase in ARGs and MGEs,and increase the abundance of beneficial soil taxa.

关键词： Antibiotic resistance gene Bacillus subtilis Bacterial community Biochar Composting

Boron promoted Fe^(3+)/peracetic acid process for sulfamethazine degradation:Efficiency,role of boron,and identification of the reactive species

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Journal of environmental Sciences 2024年第1期135卷 72-85页

作者： Yanhong Zhang Guangbing Liu Yuzhu Xue Lichun Fu Yawei Qian Minhui Hou Xiang Li Chen Ling Ying Zhang Yuwei Pan Jiangsu Provincial Key Laboratory of environmental Engineering Jiangsu Provincial Academy of Environmental ScienceNanjing 210036China College of Biology and the Environment Nanjing Forestry UniversityNanjing 210037China school of Iron and Steel Soochow UniversitySuzhou 215000China school of the Environment Nanjing UniversityNanjing 210023China SUMEC Complete Equipment&Engineering Co. LTD.Nanjing 211500China Key Laboratory of Pollution Process and environmental Criteria Ministry of EducationCollege of Environmental Science and EngineeringNankai UniversityTianjin 300350China school of Environment Key Laboratory for Yellow River and Huai River Water Environmental and Pollution ControlMinistry of EducationHenan Key Laboratory for Environmental Pollution ControlHenan Normal UniversityXinxiang 453007China

In this work,boron(B)was used to promote Fe^(3+)/peracetic acid(Fe^(3+)/PAA)for the degradation of sulfamethazine(SMT).An SMT degradation efficiency of 9.1%was observed in the Fe^(3+)/PAA system over 60 min,which was significantly increased to 99.3%in the B/Fe^(3+)/PAA system over 10 *** B/Fe^(3+)/PAA process also exhibited superior resistance to natural substances,excellent adaptability to different harmful substances,and good removal of antibiotics in natural fresh water *** mechanism of action of boron for Fe^(3+)reduction was determined using scanning electron microscopy(SEM),X-ray photoelectron spectroscopy(XPS),Fourier transform infrared(FT-IR)spectroscopy,density functional theory(DFT)calculations,and electrochemical *** dominant role of^(·)OH was confirmed using quenching experiments,electron spin resonance(EPR)spectroscopy,and quantitative *** radicals(R-O^(·))and Fe(IV)also significantly contribute to the removal of *** calculations on the reaction between Fe^(2+)and the PAA were conducted to further determine the contribution from ^(·)OH,R-O^(·),and Fe(IV)from the perspective of thermodynamics and the reaction *** boron dosages,Fe^(3+)dosages,and initial pH values were also investigated in the B/Fe^(3+)/PAA system to study their effect of SMT removal and the production of the reactive ***(IV)production determined the k_(R-O·+Fe(IV))value suggesting that Fe(IV)may play a more important role than R-O^(·).A comparison of the results with other processes has also proved that the procedure described in this study(B/Fe^(3+)/PAA)is an effective method for the degradation of antibiotics.

关键词： Boron Peracetic acid Sulfamethazine DFT Reactive species

Long-term changes in radial growth of seven tree species in the mixed broadleaf-Korean pine forest in Northeast China:Are deciduous trees favored by climate change?

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Journal of forestry Research 2024年第5期35卷 63-77页

作者： Xiufang Gong Danyang Yuan Liangjun Zhu Zongshan Li Xiaochun Wang National Engineering Laboratory for Applied Technology of forestry and Ecology in South China College of Life Science and TechnologyCentral South University of Forestry and TechnologyChangsha 410004People’s Republic of China Center for Ecological Research and Key Laboratory of Sustainable Forest Ecosystem Management-Ministry of Education School of ForestryNortheast Forestry UniversityHarbin 150040People’s Republic of China State Key Laboratory of Urban and Regional Ecology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085People’s Republic of China

The role of the temperate mixed broadleaf-Korean pine forest(BKF)in global biogeochemical cycles will depend on how the tree species community responds to climate;however,species-specific responses and vulner-abilities of common trees in BKF to extreme climates are poorly *** we used dendrochronological meth-ods to assess radial growth of seven main tree species(Pinus koraiensis,Picea jezoensis,Abies nephrolepis,Fraxinus mandshurica,Phellodendron amurense,Quercus mongolica,and Ulmus davidiana)in an old-growth BKF in response to climate changes in the Xiaoxing’an Mountains and to improve predictions of changes in the tree species *** in most months and winter precipita-tion significantly negatively affected growth of *** and ***,but positively impacted growth of *** and the broadleaf species,especially ***-rica and *** and relative humidity in June significantly positively impacted the growth of most tree *** positive effect of the temperature during the previous non-growing season(PNG)on growth of *** and *** strengthened significantly with rapid warming around 1981,while the impact of PNG temperature on the growth of *** and *** changed from significantly negative to weakly negative or positive at this *** negative response of radial growth of *** and *** to precipitation during the growing season gradually weakened,and the negative response to PNG precipitation was *** the studied species,*** was the most resistant to drought,and *** recovered the best after extreme *** davidiana,*** and *** were more resistant to extreme cold than the other *** warming generally exacerbated the opposite growth patterns of conifer(decline)and broadleaf(increase)*** broadleaf tree species in the old-growth BKF probably will gradually become dominan

关键词： Tree rings Extreme climate Resistance and recovery Broad-leaved and Korean pine mixed forest

Nanocarbon catalysts with co-active S−P−C sites enhance metal-free direct oxidation of alcohols

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SusMat 2024年第5期4卷 202-215页

作者： Juan Meng Huidong Liu Jianing Xu Yuhan Lou Haixin Sun Bo Jiang Yongzhuang Liu Hengfei Qin Shuo Dou Haipeng Yu Key Laboratory of Bio-Based Material Science and Technology of Ministry of Education Northeast Forestry UniversityHarbinChina school of Resources and environmental Engineering Jiangsu University of TechnologyChangzhouChina school of Urban Construction Changzhou UniversityChangzhouChina College of Chemistry Chemical Engineering and Resource UtilizationNortheast Forestry UniversityHarbinChina

In this study,a sulfur–phosphorus co-doped nanocarbon(SPC)catalyst was syn-thesized using a straightforward one-step colloidal carbonization method and demonstrated high performance in the metal-free direct oxidation of alcohols to *** metal-free SPC catalyst showed exceptional efficiency,achiev-ing a conversion rate of 90%for benzyl alcohol and a selectivity of 94%toward benzaldehyde within only 1 h at 130◦***,it displays exceptional cycle stability and a high turnover frequency(17.1×10-3 mol g-1 h-1).Theoretical analysis suggested that the catalyst’s superior performance is attributed to the presence of unsaturated edge defects and S-P-moieties,which increase the density of states at the Fermi level,lower the band gap energy,and promote electron ***,the doping introduces cooperative co-active S-P-C sites,facilitating a synergistic multisite catalytic effect that lowers the energy *** findings represent a significant advancement in the field of metal-free direct alcohol oxidation.

关键词： alcohol oxidation reaction carbon catalysts electronic structures

Effect of coir geotextile and geocell on ephemeral gully erosion in the Mollisol region of Northeast China

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Journal of Arid Land 2024年第4期16卷 518-530页

作者： QIN Xijin SUN Yiqiu ZHANG Yan GUAN Yinghui WU Hailong WANG Xinyu WANG Guangyu school of Soil and Water Conservation Beijing Forestry UniversityBeijing 100083China Tianjin Eco-environmental Protection Design&Research Institute Tianjin 300042China College of environmental Science and Safety Engineering Tianjin University of TechnologyTianjin 300384China Faculty of forestry University of British Columbia2424 Main MallVancouver BC V6T 1Z4Canada

The unique geomorphological features and farming methods in the Mollisol region of Northeast China increase water catchment flow and aggravate the erosion of ephemeral gully(EG).Vegetation suffers from rain erosion and damage during the growth stage,which brings serious problems to the restoration of grass in the early ***,effects of coir geotextile and geocell on EG erosion under four confluence intensities were researched in this *** of the simulated water discharge erosion test showed that when the confluence strength was less than 30 L/min,geocell and coir geotextile had a good effect on controlling EG erosion,and sediment yield of geocell and coir geotextile was reduced by 25.95%–37.82%and 73.73%–88.96%,***,when confluence intensity increased to 40 L/min,protective effect of coir geotextile decreased,and sediment yield rate increased sharply by 189.03%.When confluence intensity increased to 50 L/min,the protective effect of coir geotextile was *** the other hand,geocell showed that the greater the flow rate,the better the protective *** addition,with the increase in confluence intensity,erosion pattern of coir geotextile developed from sheet erosion to intermittent fall and then to completion of main rill,and the protective effect was gradually *** contrast,the protective effect of EG under geocell was gradually enhanced from the continuous rill to the intermittent rill and finally to the intermittent *** study shows that coir geotextile and geocell can prevent EG erosion,and the effect of geocell is better than that of coir geotextile on the surface of EG.

关键词： geocell coir geotextile ephemeral gully confluence intensity erosion control

The variation of DOM during long distance water transport by the China South to North Water Diversion Scheme and impact on drinking water treatment

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Frontiers of environmental Science & Engineering 2024年第5期18卷 85-100页

作者： Hankun Yang Yujuan Li Hongyu Liu Nigel J.D.Graham Xue Wu Jiawei Hou Mengjie Liu Wenyu Wang Wenzheng Yu State Key Laboratory of environmental Aquatic Chemistry Key Laboratory of Drinking Water Science and TechnologyResearch Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing100085China school of Environment and Municipal Engineering Qingdao Technological UniversityQingdao266033China Colleges of forestry Northeast Forestry UniversityHarbin150006China Department of Civil and environmental Engineering Imperial College LondonSouth Kensington CampusLondonSW7 2AZUK school of Chemistry and Chemical Engineering Beijing Institute of TechnologyBeijing100081China State Key Laboratory of Separation Membrane Processes School of Environment Science and EngineeringTiangong UniversityTianjin300387China

In this study,samples were taken from three locations,upstream to downstream,along the central route project of the China South to North Water Diversion(SNWD)scheme in summer and *** were used to reveal the variations of dissolved organic matter(DOM)during the water transfer process,and the effects of these variations on drinking water treatment and disinfection by-products formation potential(DBPs-FP).The results showed that polysaccharides accumulate in summer and reduce in winter with flow distance,which has an important effect on the overall properties of DOM,as well as on the performance of coagulation,ultrafiltration,and the formation of *** substances,and their hydrophilic content,also increased in summer and decreased in winter with flow *** contrast,the concentration of small organic substances(MW≤1000 Da)increased in both summer and winter with flow distance,which affected both nanofiltration(NF)membrane fouling and *** results provide a useful case study of spatial and temporal changes in raw water DOM during long distance water transfer and their impact on the treatment and quality of drinking water from the SNWD.

关键词： Long-distance water transfer The China South to North Water Diversion Scheme Coagulation Membrane filtration Disinfection by-products

Effect of catalyst diesel particulate filter aging and catalyst loadings on particulate emission characteristics from a diesel vehicle

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Journal of environmental Sciences 2024年第2期136卷 35-44页

作者： Yunhua Zhang Diming Lou Piqiang Tan Zhiyuan Hu Liang Fang school of Automotive studies Tongji UniversityShanghai 201804China

In this study,the effect of new and used catalyzed diesel particulate filter(CDPF)with different catalyst loadings on the particulate emissions including the particle mass(PM),particle number(PN),particle size distribution(PSD)and geometric mean diameter(GMD)from a diesel vehicle were investigated based on a heavy chassis *** showed that more than 97.9%of the PN and 95.4%of the PM were reduced by the CDPF,and the reduction efficiency was enhanced by the catalyst *** using the CDPF,the PSD transformed from bimodal to trimodal with the peak shifting towards smaller particle size,more nucleation mode particles were reduced compared with accumulation mode ones,but the reduction effect on the accumulation mode particles was more significantly influenced by the catalyst ***,the CDPF increased the accumulation mode particles proportion,producing a larger *** the used CDPF,its reduction effect on the particulate emissions enhanced,especially for the PM in accumulation *** PSD returned to bimodal,but the peak at accumulation mode began to be higher than that at nucleation mode,illustrating that more nucleation mode particles was *** aging of the CDPF resulted in greater effect on the PN-based PSD than that of PM-based PSD,but the effect of catalyst loading on the PN and PM emission factors was *** used CDPF further increased the GMD,and the effect of catalyst loading on the GMD was strengthened,a higher catalyst loading led to a reduction in the GMD.

关键词： Catalyzed diesel particulate filter (CDPF) Catalyst loading Aging Particle Particle size distribution Geometric mean diameter

Clean,but not green:Emission assessment,forecast modelling and policy solutions for plastic microbeads from personal care products in India

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Emerging Contaminants 2024年第3期10卷 124-133页

作者： Riya Kumbukattu Alex Thomas Maes Suja Purushothaman Devipriya school of environmental studies Cochin University of Science and Technology682022India GRID-Arendal Teaterplassen 34836ArendalNorway

Intentionally added plastic microbeads in personal care products(PCP)are an underestimated source of *** microbeads are added as fillers,to increase product volume or aesthetics and allegedly have the purpose of cleansing and *** assess and forecast microbead emissions in India,this study analysed 45 items from four different categories of personal care products:face wash,face scrub,shower gel and body scrub available in the Indian market and determined microbead abundance,size,colour,shape and polymer ***,an emission estimation and time-seriesbased forecast for 2030 was done using ARIMA(0,2,0)for individual categories and *** results indicate that 45.00%of the products contained irregular or smooth microplastics,with Polyethylene being the dominant polymer,followed by Polypropylene,Polystyrene,Polyurethane and Polycaprolactone.A significant number of products(23.33%)contained cellulose microbeads,with ambiguity regarding their *** identified microbeads were mainly irregular in shape and granular in texture,especially ***/transparent colour dominated the identified microbeads,followed by blue,pink,yellow,red and *** 1.34%of the total product contained plastic microbeads,with 5.04%and 0.04%being the highest and lowest percentages *** average size of microbeads was found to be 640.74 mm,452.45 mm,556.66 mm and 606.30 mm in different *** overall annual emission estimation was 3.51×10^(19)(highest),2.14×10^(18)(lowest)and 1.37×10^(19)(average)in 2021 and forecasted to be 4.12×10^(19)(highest),2.52×10^(18)(lowest)and 1.611019(average)in *** exorbitantly high value is due to India's significant population,globalisation,inefficient wastewater efficiency,growing economy and disposable income.A lack of policies and adequate regulations further add to *** study emphasises and recommends the development of stringent policies and other well-tailored mitig

关键词： Microplastic beads Time-series forecast Policy solutions Emission estimation Personal care products

A novel electro-Fenton hybrid system for enhancing the interception of volatile organic compounds in membrane distillation desalination

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Journal of environmental Sciences 2024年第4期138卷 189-199页

作者： Hongxin Liu Kuiling Li Kunpeng Wang Zhiyong Wang Zimou Liu Sichao Zhu Dan Qu Yu Zhang Jun Wang State Key Laboratory of environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China State Key Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua UniversityBeijing 100084China school of Chemical and environmental Engineering Beijing CampusChina University of Mining and TechnologyBeijing 100083China Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China

Membrane distillation(MD)is a promising alternative desalination technology,but the hydrophobic membrane cannot intercept volatile organic compounds(VOCs),resulting in aggravation in the quality of *** term of this,electro-Fenton(EF)was coupled with sweeping gas membrane distillation(SGMD)in a more efficient way to construct an advanced oxidation barrier at the gas-liquid interface,so that the VOCs could be trapped in this layer to guarantee the water quality of the *** the so-called EF-MD process,an interfacial interception barrier containing hydroxyl radical formed on the hydrophobic membrane *** contributed to the high phenol rejection of 90.2% with the permeate phenol concentration lower than 1.50 mg/*** interceptions can be achieved in a wide temperature range,even though the permeate flux of phenol was also *** EF-MD system was robust to high salinity and could electrochemically regenerate ferrous ions,which endowed the long-term stability of the *** novel EF-MD configuration proposed a valuable strategy to intercept VOCs in MD and will broaden the application of MD in hypersaline wastewater treatment.

关键词： Membrane distillation VOC interception Interfacial oxidation Electro-Fenton Hypersaline wastewater

Performance and mechanism of La-Fe metal-organic framework as a highly efficient adsorbent for fluoride removal from mine water

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Journal of environmental Sciences 2024年第5期139卷 245-257页

作者： Chaomin Jia Jianbing Wang Huijiao Wang Sichao Zhu Xiaohui Zhang Yuxiang Wang school of Chemical&environmental Engineering China University of Mining&Technology-BeijingBeijing 100083China Beijing Polytechnic Beijing 100176China Chinese Society for Urban studies Beijing 100835China

Water fluoride pollution has caused non-negligible harm to the environment and humans,and thus it is crucial to find a suitable treatment *** this study,La-Fe@PTA adsorbent was synthesized for the defluoridation of mine *** results showed that the optimum conditions for defluoridation by La-Fe@PTA were p H close to 7.0,the initial F-concentration of 10 mg/L,the dosage of 0.5 g/L and the adsorption time of 240 *** with SO_4^(2-),Cl^(-),NO_(3)^(-),Ca^(2+)and Mg^(2+),CO_(3)^(2-)and HCO_(3)^(-)presented severer inhibition on fluoride uptake by La-Fe@*** adsorption process fits well with the pseudo-second-order kinetic model and Freundlich model,and the maximum adsorption capacity of Langmuir model was 95 mg/***-bed adsorption results indicated that fluoride in practical fluorinated mine water could be effectively removed from 3.6 mg/L to less than 1.5 mg/L within130 bed volume(BV)by using 1.5 g La-Fe@***,the adsorbent still had good adsorption capacity after regeneration,which confirms the great application potential of La-Fe@PTA as a fluoride ion *** mechanism analysis showed that La-Fe@PTA adsorption of fluorine ions is a physicochemical reaction driven by electrostatic attraction and ion exchange.

关键词： Adsorption La-Fe@PTA Fluoride ion Mine water Mechanism