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Chinese Chemical Letters 2024年第1期35卷 310-315页

作者： Longtao Zhu Yinan Zhao Wenhao Yang Hsien-Yi Hsu Ping Peng Fang-Fang Li school of Materials science and Engineering Huazhong University of Science and TechnologyWuhan 430074China school of Energy and Environment&Department of Materials science and Engineering City University of Hong KongHong Kong 999077China

Metastable molybdenum carbide(α-MoC),as a catalyst and an excellent support for metal catalysts,has been widely used in thermo/electro-catalytic ***,the selective synthesis ofα-MoC remains a great ***,a simple one-pot synthetic strategy for the selective preparation of metastableα-MoC is proposed by electrochemical co-reduction of CO_(2)and MoO_(3)in a low-temperature eutectic molten *** synthesizedα-MoC shows a reed flower-like *** controlling the electrolysis time and monitoring the phase and morphology of the obtained products,the growth process ofα-MoC is revealed,where the carbon matrix is deposited first followed by the growth ofα-MoC from the carbon ***,by analyzing the composition of the electrolytic products,the formation mechanism forα-MoC is *** addition,through this one-pot synthetic strategy,S-dopedα-MoC is successfully *** functional theory(DFT)calculations reveal that S doping enhanced the HER performance ofα-MoC by facilitating water absorption and dissociation and weakening the bond energy of Mo-H to accelerate H *** present work not only highlights the valuable utilization of CO_(2) but also offers a new perspective on the design and controllable synthesis of metal carbides and their derivatives.

关键词： α-MoC CO_(2)electroreduction Molten salt Sulfur doping Hydrogen evolution reaction

Stable photocurrent-voltage characteristics of perovskite single crystal detectors obtained by pulsed bias

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Chinese Physics B 2024年第4期33卷 209-214页

作者：刘新陈之龙王虎张雯清董昊王鹏祥邵宇川 Laboratory of Thin Film Optics Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Center of Materials science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Key Laboratory of Materials for High-Power Laser Shanghai Institute of Optics and Fine MechanicsChinese Academy of SciencesShanghai 201800China Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China school of Microelectronics Shanghai UniversityShanghai 201899China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou 310024China

Photocurrent-voltage characterization is a crucial method for assessing key parameters in x-ray or y-ray semiconductor detectors,especially the carrier mobility lifetime ***,the high biases during photocurrent measurements tend to cause severe ion migration,which can lead to the instability and inaccuracy of the test *** the mixed electronic-ionic charac teristics,it is imperative to devise novel methods capable of precisely measuring photocurrentvoltage characteristics under high bias conditions,free from interference caused by ion *** this paper,pulsed bias is employed to explore the photocurrent-voltage characteristics of MAPbBr_(3) single *** method yields stable photocurrent-voltage characteristics at a pulsed bias of up to 30 V,proving to be effective in mitigating ion *** fitting the modified Hecht equation,we determined the mobility lifetime products of 1.0×10^(2) cm^(2)·V^(-1)for hole and 2.78×10~(-3)cm^(2)·V^(-1)for *** approach offers a promising solution for accurately measuring the transport properties of carriers in perovskite.

关键词： perovskites ion migration pulsed bias mobility lifetime product

Ethanol steam reforming over Ni/ZSM-5 nanosheet for hydrogen production

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Chinese Journal of Chemical Engineering 2024年第3期67卷 247-256页

作者： Porapak Suriya Shanshan Xu Shengzhe Ding Sarayute Chansai Yilai Jiao Joseph Hurd Daniel Lee Yuxin Zhang Christopher Hardacre Prasert Reubroycharoen Xiaolei Fan Department of Chemical Engineering School of EngineeringThe University of ManchesterManchester M139PLUnited Kingdom Program of Petrochemistry and Polymer science Faculty of ScienceChulalongkorn UniversityBangkok10330Thailand Shenyang National Laboratory for Materials science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Liaoning Academy of Materials Shenyang 110167China Center of Excellence in Catalysis for Bioenergy and Renewable Chemicals(CBRC) andDepartment of Chemical TechnologyFaculty of ScienceChulalongkorn UniversityBangkok 10330Thailand Nottingham Ningbo China Beacons of Excellence Research and Innovation Institute University of Nottingham Ningbo ChinaNingbo315100China

Compared to reforming reactions using hydrocarbons,ethanol steam reforming(ESR)is a sustainable alternative for hydrogen(H_(2))production since ethanol can be produced sustainably using *** work explores the catalyst design strategies for preparing the Ni supported on ZSM-5 zeolite catalysts to promote ***,two-dimensional ZSM-5 nanosheet and conventional ZSM-5 crystal were used as the catalyst carriers and two synthesis strategies,i.e.,in situ encapsulation and wet impregnation method,were employed to prepare the *** on the comparative characterization of the catalysts and comparative catalytic assessments,it was found that the combination of the in situ encapsulation synthesis and the ZSM-5 nanosheet carrier was the effective strategy to develop catalysts for promoting H_(2) production via ESR due to the improved mass transfer(through the 2-D structure of ZSM-5 nanosheet)and formation of confined small Ni nanoparticles(resulted via the in situ encapsulation synthesis).In addition,the resulting ZSM-5 nanosheet supported Ni catalyst also showed high Ni dispersion and high accessibility to Ni sites by the reactants,being able to improve the activity and stability of catalysts and suppress metal sintering and coking during ESR at high reaction ***,the Ni supported on ZSM-5 nanosheet catalyst prepared by encapsulation showed the stable performance with~88% ethanol conversion and~65% H_(2) yield achieved during a 48-h longevity test at 550-C.

关键词： ZSM-5 nanosheet In situ encapsulation Ni catalyst Ethanol steam reforming Hydrogen production

Structural integration of solar desalination system

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science China Materials 2024年第6期67卷 2039-2041页

作者： Diling Yang Hao Zhang Hongbo Zeng school of Materials and Environmental Engineering Hunan University of HumanitiesScience and TechnologyLoudi 417000China Department of Chemical and Materials Engineering University of AlbertaEdmontonAlberta T6G 1H9Canada

As population grow and climate change place significant water stress on numerous regions,the demand for efficient and environmentally friendly water resource solutions becomes increasingly *** address this challenge,desalination technology has received much attention and is widely employed,with a recent emphasis on solar-powered solutions driven by the global push for carbon neutrality.

关键词： neutral system integration

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Exact satisfiability and phase transition analysis of the regular(k,d)-CNF formula

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Frontiers of Computer science 2024年第1期18卷 263-265页

作者： Guoxia NIE Daoyun XU Xi WANG Zaijun ZHANG College of Computer science and Technology Guizhou UniversityGuiyang 550025China school of Mathematics and Statistics Qiannan Normal University for NationalitiesDuyun 558000China Key Laboratory of Industrial Automation and Machine Vision of Qiannan Duyun 558000China

1Introduction The satisfiability(SAT)problem has been considered the"seed"of other NP-complete *** regular partial exact(k,d)-SAT problem is an important extension of the SAT *** any(k,d)-CNF formula with a variable set V,V'is a proper subset of V,the problem involves determining whether a truth assignment set on V'exists such that only a literal in each clause is *** V'=V,it is a regular exact(k,d)-SAT ***,both experimental verifications and theoretical analyses of k-SAT problem have shown that the ratioα(clause constraint density)of the number of clauses m to the number of variables n is an important parameter affecting the satisfiability of the formula[1].However,the regular(k,d)-SAT problem has the same clause constraint density d/k.

关键词： formula constraint exact

Current therapies for osteoarthritis and prospects of CRISPR-based genome,epigenome,and RNA editing in osteoarthritis treatment

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Journal of Genetics and Genomics 2024年第2期51卷 159-183页

作者： Yuxi Chen Xiao Luo Rui Kang Kaixin Cui Jianping Ou Xiya Zhang Puping Liang MOE Key Laboratory of Gene Function and Regulation State Key Laboratory of BiocontrolSchool of Life SciencesSun Yat-sen UniversityGuangzhouGuangdong 510275China Center for Reproductive Medicine The Third Affiliated Hospital of Sun Yat-sen UniversitySun Yat-sen UniversityGuangzhouGuangdong 510630China

Osteoarthritis(OA)is one of the most common degenerative joint diseases worldwide,causing pain,disability,and decreased quality of *** balance between regeneration and inflammation-induced degradation results in multiple etiologies and complex pathogenesis of ***,there is a lack of effective therapeutic strategies for OA *** the development of CRISPR-based genome,epigenome,and RNA editing tools,OA treatment has been improved by targeting genetic risk factors,activating chondrogenic elements,and modulating inflammatory *** by cell therapy and in vivo delivery vectors,genome,epigenome,and RNA editing tools may provide a promising approach for personalized OA *** review summarizes CRISPR-based genome,epigenome,and RNA editing tools that can be applied to the treatment of OA and provides insights into the development of CRISPR-based therapeutics for OA ***,in-depth evaluations of the efficacy and safety of these tools in human OA treatment are needed.

关键词： Osteoarthritis Genome editing Epigenone editing RNA editing

Service Migration Algorithm Based on Markov Decision Process with Multiple Service Types and Multiple System Factors

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Chinese Journal of Electronics 2024年

作者： Anhua MA Su PAN Weiwei ZHOU Broadband Wireless Communication College Nanjing University of Posts and Telecommunications school of Computer science and Technology Nanjing Tech University

This paper proposes a Markov decision process based service migration algorithm to satisfy quality of service(Qo S) requirements when the terminals leave the original server. Services were divided into real-time services and non-real-time services, each type of them has different requirements on transmission bandwidth and latency,which were considered in the revenue function. Different values were assigned to the weight coefficients of QoS parameters for different service types in the revenue and cost functions so as to distinguish the differences between the two service types. The overall revenue was used for migration decisions, rather than fixed threshold or instant revenue. The Markov decision process was used to maximize the overall revenue of the system. Simulation results show that the proposed algorithm obtained more revenue compared with the existing works.

关键词：

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电池衰减诊断及状态评估研究进展

science China Materials 2024年第4期67卷 1014-1041页

作者：袁君秦之理黄海坤甘兴栋王子为杨毅琛刘书江文安毕闯李白海孙成华 school of Materials and Energy University of Electronic Science and Technology of China Yangtze Delta Region Institute(Huzhou) University of Electronic Science and Technology of China school of Computer science and Engineering University of Electronic Science and Technology of China Power Research Institute of State Grid Shaanxi Electric Power Company Limited Department of Chemistry and Biotechnology Swinburne University of Technology

锂离子电池(LIB)广泛应用于储能及动力输出等领域.准确预测电池的健康状态对于优化性能、降低运营费用和防止电池故障等方面具有重要的意义.本文对预测LIB的荷电状态(SOC)、健康状态(SOH)和剩余使用寿命(RUL)方面的最新发展进行了全面回... 详细信息

锂离子电池(LIB)广泛应用于储能及动力输出等领域.准确预测电池的健康状态对于优化性能、降低运营费用和防止电池故障等方面具有重要的意义.本文对预测LIB的荷电状态(SOC)、健康状态(SOH)和剩余使用寿命(RUL)方面的最新发展进行了全面回顾,重点关注机器学习技术方面的研究进展,深入分析了LIB的退化机制及其基本理论,评估了各种传统方法及机器学习技术在预测SOC,SOH和RUL方面的优势和限制.此外,还探讨了电动汽车动力电池在实际应用中面临的挑战,特别是性能退化问题.最后提出了对LIB未来研究方向有价值的见解.尽管机器学习方法在提高预测SOC,SOH和RUL准确性方面具有巨大潜力,但在实际应用中仍然有许多技术和实际障碍需要克服.

关键词：锂离子电池剩余使用寿命状态评估机器学习技术健康状态动力输出运营费用退化机制

Control of temperature dependent viscosity for manufacturing of Bi-doped active fiber

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International Journal of Extreme Manufacturing 2024年第3期6卷 522-530页

作者： Rui Duan Jingfei Chen Hao Ke Tianxia Wei Ke Zhang Xueliang Li Xu Feng Qiuju Zheng Zhixue He Jianrong Qiu Shifeng Zhou State Key Laboratory of Luminescent Materials and Devices School of Materials Science and EngineeringSouth China University of TechnologyGuangzhou 510640People’s Republic of China Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and DevicesGuangzhou 510640People’s Republic of China school of Materials science and Engineering Qilu University of TechnologyJinanPeople’s Republic of China Peng Cheng Laboratory Shenzhen 518000People’s Republic of China College of Optical science and Engineering State Key Laboratory of Modern Optical InstrumentationZhejiang UniversityHangzhou 310027People’s Republic of China

Bi-activated photonic materials are promising for various applications in high-capacity telecommunication,tunable laser,and advanced bioimaging and *** various Bi-doped material candidates have been explored,manufacturing of Bi heavily doped fiber with excellent optical activity remains a long-standing ***,a novel viscosity evolutional behavior mediated strategy for manufacturing of Bi-doped active fiber with high dopant solubility is *** intrinsic relation among the evolution of Bi,reaction temperature and viscosity of the glass system is ***,the effective avenue to prevent the undesired deactivation of Bi during fiber drawing by tuning the temperature dependent viscosity evolution is *** applying the strategy,for the first time we demonstrate the success in fabrication of heavily doped Bi active ***,the principal fiber amplifier device is constructed and broadband optical signal amplification is *** findings indicate the effectiveness of the proposed temperature dependent viscosity mediated strategy for developing novel photonic active fiber,and they also demonstrate the great potential for application in the next-generation high-capacity telecommunication system.

关键词： infrared luminescence active fiber optical amplification

Swimmer with submerged SiO_(2)/Al/LiNbO_(3) surface acoustic wave propulsion system

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Biomimetic Intelligence & Robotics 2024年第2期4卷 71-77页

作者： Deqing Kong Ryo Tanimura Fang Wang Kailiang Zhang Minoru Kuribayashi Kurosawa Manabu Aoyagi Department of Engineering Muroran Institute of TechnologyMuroran 050-8585Japan Tianjin Key Laboratory of Film Electronic and Communication Devices School of Integrated Circuit Science and EngineeringTianjin University of TechnologyTianjin 300384China school of Engineering Tokyo Institute of TechnologyYokohama 226-8501Japan

Acoustic propulsion system presents a novel underwater propulsion approach in small scale *** study introduces a submerged surface acoustic wave(SAW)propulsion system based on the SiO_(2)/Al/LiNbO_(3) *** 19.25 MHz,the SAW propulsion system is proposed and investigated by the propulsion force calculation,PIV measurements and propulsion measurements.3.3 mN propulsion force is measured at 27.6 V_(pp).To evaluate the miniature swimmer,the SAW propulsion systems with multiple frequencies are *** 2.2 W,the submerged SAW propulsion system at 38.45 MHz demonstrates 0.83 mN/mm^(2) propulsion *** 96.13 MHz and 24 V_(pp),the movements of miniature swimmer with a fully submerged SAW propulsion system are recorded and analyzed to a maximum of 177 mm/*** of miniaturization,high power density,and simple structure,the SAW propulsion system can be expected for some microrobot applications,such as underwater drone,pipelinerobotand intravascularrobot.

关键词： Acoustofluidics Surface acoustic wave Swimmer Underwater propulsion system